Using a quantum theory for an ensemble of three-level atoms (lambda) placed in an optical cavity abd driven by electromagnetic fields, we show that the long-lived spin associated with the ground state sublevels can be squeezed. Two kinds of squeezing are obtained: self-spin squeezing, when the input fields are coherent states and the atomic ensemble exhibit a large non-linearity; squeezing transfer, when one of the incoming fields is squeezed.
The interaction of classical and quantized electromagnetic fields with an ensemble of atoms in an optical cavity is considered. Four fields drive a double-lambda level scheme in the atoms, consisting of a pair of lambda systems sharing the same set of lower levels. Two of the fields produce maximum coherence, rho12 = -1/2, between the ground state sublevels 1 and 2. This pumping scheme involves equal intensity fields that are resonant with both the one and two-photon transitions of the lambda system. There is no steady-state absorption of these fields, implying that the fields induce a type el…
In this paper, we study the interaction between a moving $Λ$-type three-level atom and a single-mode cavity field in the presence of intensity-dependent atom-field coupling. After obtaining the state vector of the entire system explicitly, we study the nonclassical features of the system such as quantum entanglement, position-momentum entropic squeezing, quadrature squeezing and sub-Poissonian statistics. According to the obtained numerical results we illustrate that the squeezed period, the duration of entropy squeezing and the maximal squeezing can be controlled by choosing the appropriate n…
We study the multipartite correlations of the multi-atom dark states, which are characterized by the atomic squeezing beyond the pairwise entanglement. It is shown that, in the photon storage process with atomic ensemble via electromagnetically induced transparency (EIT) mechanism, the atomic squeezing and the pairwise entanglement can be created by adiabatically manipulating the Rabi frequency of the classical light field on the atomic ensemble. We also consider the sudden death for the atomic squeezing and the pairwise entanglement under various decoherence channels. An optimal time for gene…
Squeezing of atomic resonance fluorescence is shown to be optimized by a properly designed environment, which can be realized by a quasi-resonant cavity. Optimal squeezing is achieved if the atomic coherence is maximized, corresponding to a pure atomic quantum state. The atomic-state purification is achieved by the backaction of the cavity field on the atom, which increases the atomic coherence and decreases the atomic excitation. For realistic cavities, the coupling of the atom to the cavity field yields a purity of the atomic state of more than 99%. The fragility of squeezing against dephasi…
We show that the sensitivity of an atomic clock can be enhanced below the shot-noise level by initially squeezing, and then measuring in output, the population of a single atomic level. This can simplify current experimental protocols which requires squeezing of the relative number of particles of the two populated states. We finally study, as a specific application, the clock sensitivity obtained with a single mode quantum non-demolition measurement.
We investigate the possibility to perform a Quantum Non Demolition measurement of the collective alignment of an atomic ensemble in the case of a $F\geq 1$ spin. We compare the case of purely vectorial and purely tensorial Hamiltonians and show how to achieve conditional squeezing or entanglement of atomic alignment components.
We study relations between bosonic quadrature squeezing and atomic spin squeezing, and find that the latter reduces to the former in the limit of a large number of atoms for even and odd states. We demonstrate this reduction by treating even and odd spin coherent states, for which analytical solutions are readily obtained, and prove that even spin coherent states always exhibit spin squeezing, whereas odd spin coherent states do not, analogous to the squeezing characteristic of even and odd bosonic coherent states. Finally, we examine the squeezing transfer between photons and atoms via the Di…
We consider squeezing of one component of the collective spin vector of an atomic ensemble inside an optical cavity. The atoms interact with a cavity mode, and the squeezing is obtained by probing the state of the light field that is transmitted through the cavity. Starting from the stochastic master equation, we derive the time evolution of the state of the atoms and the cavity field, and we compute expectation values and variances of the atomic spin components and the quadratures of the cavity mode. The performance of the setup is compared to spin squeezing of atoms by probing of a light fie…
When linearly polarized light propagates through a medium in which elliptically polarized light would undergo self-rotation, squeezed vacuum can appear in the orthogonal polarization. A simple relationship between self-rotation and the degree of vacuum squeezing is developed. Taking into account absorption, we find the optimum conditions for squeezing in any medium that can produce self-rotation. We then find analytic expressions for the amount of vacuum squeezing produced by an atomic vapor when light is near-resonant with a transition between various low-angular-momentum states. Finally, we …
Recent years have witnessed revolutionary improvement in the production, manipulation, characterization and quantification of multiatom (multiqubit) states - because of their promising applications in high precision atomic clocks, atomic interferrometry, quantum metrology and quantum information protocols. In the characterization and quantification of non-classical atomic correlations, two concepts namely, spin squeezing and quantum entanglement emerge. While spin squeezing originates from the uncertainty relation between atomic collective angular momentum operators, entanglement is a peculiar…
We propose an efficient method for controlled generation of field squeezing with cold atomic clouds trapped close to a superconducting transmission line resonator. It is shown that, based on the coherent strong magnetic coupling between the collective atomic spins and microwave fields in the transmission line resonator, two-mode or single mode field squeezed states can be generated through coherent control on the dynamics of the system. The degree of squeezing and preparing time can be directly controlled through tuning the external classical fields. This protocol may offer a promising platfor…
We discuss the theory and experimental considerations of a quantum feedback scheme for producing deterministically reproducible spin squeezing. Continuous nondemolition atom number measurement from monitoring a probe field conditionally squeezes the sample. Simultaneous feedback of the measurement results controls the quantum state such that the squeezing becomes unconditional. We find that for very strong cavity coupling and a limited number of atoms, the theoretical squeezing approaches the Heisenberg limit. Strong squeezing will still be produced at weaker coupling and even in free space (t…
In this paper, we investigate theoretically the quantum state transfer in a laser driven hybrid optomechanical cavity with two Duffing-like anharmonic movable end mirrors containing an ensemble of identical two-level trapped atoms. The quantum state transfer from the Bogoliubov modes of the two anharmonic oscillators to the atomic mode results in the atomic quadrature squeezing beyond the standard quantum limit of 3 dB which can be controlled by both the optomechanical and atom-field coupling strengths. Interestingly, the generated atomic squeezing can be made robust against the noise sources …
We provide a framework for understanding recent experiments on squeezing of a collective atomic pseudo-spin, induced by a homodyne measurement on off-resonant probe light interrogating the atoms. The detection of light decimates the atomic state distribution and we discuss the conditions under which the resulting reduced quantum fluctuations are metrologically relevant. In particular, we consider a dual probe scheme which benefits from a cancelation of classical common mode noise sources such that quantum fluctuations from light and atoms are the main contributions to the detected signal.
We propose and analyze a simple method to squeeze dynamically and unconditionally the collective spin of a dilute atomic ensemble by interaction with a driven mode of an optical resonator, as recently demonstrated [I. D. L., M. H. S., and V. V., Phys. Rev. Lett. 104, 073602 (2010)]. We show that substantial squeezing can be achieved in the regime of strong collective ensemble-resonator coupling. The squeezing is ultimately limited either by photon emission into free space or by the curvature of the Bloch sphere. We derive both limits and show where each prevails.
We propose schemes for the unconditional preparation of a two-mode squeezed state of effective bosonic modes realized in a pair of atomic ensembles interacting collectively with optical cavity and laser fields. The scheme uses Raman transitions between stable atomic ground states and under ideal conditions produces pure entangled states in the steady state. The scheme works both for ensembles confined within a single cavity and for ensembles confined in separate, cascaded cavities.
We show that an ensemble of identical d-level atoms can be efficiently described by d-1 collective oscillator degrees of freedom in the vicinity of a product state with all atoms in the same, but otherwise arbitrary single-particle state. We apply our description to two different kinds of spin squeezing: (i) when each spin-F atom is individually squeezed without creating interatomic entanglement and (ii) when a particular collective atomic oscillator mode is squeezed via quantum non-demolition (QND) measurement and feedback. When combined in sequence, the order of the two methods is relevant i…
The compatibility of cavity-generated spin-squeezed atomic states with atom-interferometric sensors that require freely falling atoms is demonstrated. An ensemble of $500,000$ spin-squeezed atoms in a high-finesse optical cavity with near-uniform atom-cavity coupling is prepared, released into free space, recaptured in the cavity, and probed. Up to $\sim$10 dB of metrologically-relevant squeezing is retrieved for 700 microsecond free-fall times, and decaying levels of squeezing are realized for up to 3 millisecond free-fall times. The degradation of squeezing results from loss of atom-cavity c…
We propose an efficient scheme for realizing squeezing for both an atomic ensemble and a cavity field via adiabatic evolution of the dark state of the atom-cavity system. Controlled symmetry breaking of the Hamiltonian ensures a unique dark state for the total system, in which the atomic system or cavity mode is squeezed depending upon the choice of the detunings. Since the generation of the atomic squeezed state requires neither the cavity mode nor the atomic system to be excited, the decoherence effects are effectively suppressed. The scheme is insensitive to the uncertainty in the atomic nu…
Entangled many body systems have recently attracted significant attention in various contexts. Among them, spin squeezed atoms and ions have raised interest in the field of precision measurements, as they allow to overcome quantum noise of uncorrelated particles. Precise quantum state engineering is also required as a resource for quantum computation, and spin squeezing can be used to create multi-partite entangled states. Two-mode spin squeezed systems have been used for elementary quantum communication protocols. Until now spin squeezing has been always achieved via generation of entanglemen…
Planar squeezed states, i.e. quantum states which are squeezed in two orthogonal spin components, have recently attracted attention due to their applications in atomic interferometry and quantum information [Q. Y. He et al, New J. Phys. 14, 093012 (2012)]. While canonical variables such as quadratures of the radiation field can be squeezed in at most one component, simultaneous squeezing in two orthogonal spin components can be achieved due to the angular momentum commutation relations. We present a novel scheme for planar squeezing via quantum non-demolition (QND) measurements in spin-1 syste…
We propose a scheme for the generation of strong mechanical squeezing beyond 3dB in hybrid atom-optomechanical systems in the highly unresolved sideband (HURSB) regime where the decay rate of cavity is much larger than the frequency of the mechanical oscillator. The system is formed by two two-level atomic ensembles and an optomechanical system with cavity driven by two lasers with different amplitudes. In the HURSB regime, the squeezing of the movable mirror can not be larger than 3dB if no atomic ensemble or only one atomic ensemble is put into the optomechanical system. However, if two atom…
This dissertation studies spin squeezing, entanglement and decoherence in large ensembles of cold, trapped alkali atoms with hyperfine spin f interacting with optical fields. Restricting the state of each atom to a qutrit embedded in the 2f+1 dimensional hyperfine spin enables us to efficiently model the coherent and dissipative dynamics of the ensemble. This formalism also allows us to explore the effects of local control on the internal hyperfine spins of the atoms. State preparation using such control increases the entangling power of the atom-light interface for f>1/2. Subsequent control o…
It has been shown elsewhere that two spatially separated atoms can jointly absorb one photon, whose frequency is equal to the sum of the transition frequencies of the two atoms. We describe this process in the presence of an ensemble of many two-level atoms, and show that it can be used to generate spin squeezing and entanglement. This resonant collective process allows to create a sizeable squeezing already at the single-photon limit. It represents a novel way for generating manybody spin-spin interactions, yielding a two-axis twisting-like interaction among the spins, which is very effcient …
In this paper we consider a system of two two-level atoms interacting with a single-mode quantized electromagnetic field in a lossless resonant cavity via $l$-photon-transition mechanism. The field and the atoms are initially prepared in the coherent state and the excited atomic states, respectively. For this system we investigate the entropy squeezing, the atomic variances, the von Neumann entropy and the atomic inversions for the single-atom case. We show that the more the number of the parties in the system the less the amounts of the nonclassical effects exhibited in the entropy squeezing.…
Two well-known mechanisms, one-axis twisting (OAT) and two-axis countertwisting (TACT), generate spinsqueezed states dynamically. The latter provides better spin squeezing (SS) but has not been demonstrated as the form of its interaction does not occur naturally in known physical systems. Several proposals for realizing effective TACT transformed from OAT require stringent experimental conditions in order to overcome the resulting nonstationary (oscillating) SS and continuously varying mean spin directions. This work presents a simple scheme that solves both problems by freezing SS at an optim…
To establish an applicable system for advanced quantum information processing between light and atoms, we have demonstrated the quantum non-demolition (QND) measurement with a collective spin of cold ytterbium atoms (171Yb), and observed 1.8 (-1.5, +2.4) dB spin squeezing. Since a 171Yb atom has only a nuclear spin of 1/2 in the ground state, the system is the simplest spin ensemble and robust against decoherence. We used very short pulses with the width of 100 ns, so the interaction time became much shorter than the decoherence time, which is important for multi-step quantum information proce…
Deterministic light-induced spin squeezing in an atomic gas is limited by photon shot noise or, equivalently, by atomic state information escaping with the light field mediating the effective atom-atom interaction. We show theoretically that the performance of cavity spin squeezing [M.H. Schleier-Smith, I.D. Leroux, and V. Vuletić, Phys. Rev. A 81, 021804(R) (2010)] can be substantially improved by erasing the light-atom entanglement, and propose several methods for doing so. Accounting for light scattering into free space, quantum erasure improves the scaling of cavity squeezing from S^(-1/2)…
We report the generation of a macroscopic singlet state in a cold atomic sample via quantum non-demolition (QND) measurement induced spin squeezing. We observe 3 dB of spin squeezing and detect entanglement of up to $5.5\times10^5 $ atoms with $5σ$ statistical significance using a generalized spin squeezing inequality. The degree of squeezing implies at least 50% of the atoms have formed singlets, while the response to a magnetic field gradient indicates entanglement bonds at all length scales, a characteristic of quantum spin liquids.
It is shown that 100% squeezed output can be produced in the resonance fluorescence from a coherently driven two-level atom interacting with a squeezed vacuum. This is only possible for $N=1/8$ squeezed input, and is associated with a pure atomic state, i.e., a completely polarized state. The quadrature for which optimal squeezing occurs depends on the squeezing phase $Φ,$ the Rabi frequency $Ω,$ and the atomic detuning $Δ$. Pure states are described for arbitrary $Φ,$ not just $Φ=0$ or $π$ as in previous work. For small values of $N,$ there may be a greater degree of squeezing in the output f…
In this paper the interaction between a two-level atom and a single-mode field in the $k$-photon Jaynes-Cummings model (JCM) in the presence of Stark shift and Kerr medium is studied. All terms in the respected Hamiltonian, such as the single-mode field, its interaction with the atom, the contribution of the Stark shift and the Kerr medium effects are considered to be $f$-deformed. In particular, the effect of the initial state of radiation field on the dynamical evolution of some physical properties such as atomic inversion and entropy squeezing are investigated by considering different initi…
We squeeze unconditionally the collective spin of a dilute ensemble of laser-cooled rubidium-87 atoms using their interaction with a driven optical resonator. The shape and size of the resulting spin uncertainty region are well described by a simple analytical model [M.H.S., I.D.L., V.V., arXiv:0911.3936] through two orders of magnitude in the effective interaction strength, without free parameters. We deterministically generate states with up to 5.6(6) dB of metrologically relevant spin squeezing on the canonical rubidium-87 hyperfine clock transition.
A scheme is proposed to prepare squeezed states and Schrödinger cat-like states of the collective spin degrees of freedom associated with a pair of ground states in an atomic ensemble. The scheme uses an effective Jaynes-Cummings interaction which can be provided by excitation of the atoms to Rydberg states and an effective J_x interaction implemented by a resonant Raman coupling between the atomic ground states. Both dynamical evolution with a constant Hamiltonian and with adiabatic variation of the two interaction terms are studied. We show that by the application of further resonant laser f…
The manuscript investigates the entropy squeezing of a qubit (two-level atom) interacting with the cavity field in the Schrödinger cat states. The effects of the Schrödinger cat states of the field on the squeezing are examined. Our results suggest that entropy squeezing is not sensitive to the superposition features of two coherent states of the Schrödinger cat states. Furthermore, it is found that entropy squeezing occurs as the qubit initially close to its maximally coherent state, and the qubit initially in the maximally coherent state can generate optimal squeezing. This also demonstrates…
The strong light-matter coupling attainable in optical cavities enables the generation of highly squeezed states of atomic ensembles. It was shown in [Phys. Rev. A 66, 022314 (2002)] how an effective one-axis twisting Hamiltonian can be realized in a cavity setup. Here, we extend this work and show how an effective two-axis twisting Hamiltonian can be realized in a similar cavity setup. We compare the two schemes in order to characterize their advantages. In the absence of decoherence, the two-axis Hamiltonian leads to more squeezing than the one-axis Hamiltonian. If limited by decoherence fro…
The coherent population trapping (CPT) effect is used for making compact atomic clocks. There are two types of CPT clocks: the one in which the Raman beams are applied continuously and the one in which two CPT pulses separated by a dark period are applied (Ramsey scheme). It is obvious that the technique of spin squeezing can only be applied to the Ramsey CPT clock to enhance the sensitivity. However, it is not apparent how to adapt to the CPT clock the protocols for the microwave clock using one-axis-twist squeezing (OATS), since the Ramsey CPT clock is not trivially equivalent to the Ramsey …
We analyze the creation of spin squeezed atomic ensembles by simultaneous dispersive interactions with several optical frequencies. A judicious choice of optical parameters enables optimization of an interferometric detection scheme that suppresses inhomogeneous light shifts and keeps the interferometer operating in a balanced mode that minimizes technical noise. We show that when the atoms interact with two-frequency light tuned to cycling transitions the degree of spin squeezing $ξ^2$ scales as $ξ^2\sim 1/d$ where $d$ is the resonant optical depth of the ensemble. In real alkali atoms there …
We study the process of squeezing of an ensemble of cold atoms in a pulsed optical lattice. The problem is treated both classically and quantum-mechanically under various thermal conditions. We show that a dramatic compression of the atomic density near the minima of the optical potential can be achieved with a proper pulsing of the lattice. Several strategies leading to the enhanced atomic squeezing are suggested, compared and optimized.
We present a scheme to generate steady-state atomic spin squeezing in a cavity QED system using cavity-mediated Raman transitions to engineer effective atom-photon interactions, which include both linear and nonlinear (dispersive) atom-cavity couplings, on a potentially equal footing. We focus on a regime where the dispersive coupling is very large and find that the steady state of the system can in fact be a strongly spin-squeezed Dicke state, $|N/2,0\rangle$, of the atomic ensemble. These states offer Heisenberg-limited metrological properties and feature genuine multipartite entanglement am…
The unconditionally squeezing of the collective spin of an atomic ensemble in a laser driven optical cavity (I. D. Leroux, M. H. Schleier-Smith, and V. Vuletic, Phys. Rev. Lett 104, 073602 (2010)) is studied and analyzed theoretically. Surprisingly, we find that the largely detuned driving laser can improve the scaling of cavity squeezing from $S^{-2/5}$ to $S^{-2/3}$, where S is the total atomic spin. Moreover, we also demonstrate that the experimental imperfection of photon scattering into free space can be efficiently suppressed by detuning.
We propose and analyze a scheme for generating entangled atomic beams out of a Bose-Einstein condensate using spin-exchanging collisions. In particular, we show how to create both atomic squeezed states and entangled states of pairs of atoms.
We investigate the quantum non-demolition (QND) measurement of an atomic population based on a heterodyne detection and show that the induced back-action allows to prepare both spin-squeezed and Dicke states. We use a wavevector formalism to describe the stochastic process of the measurement and the associated atomic evolution. Analytical formulas of the atomic distribution momenta are derived in the weak coupling regime both for short and long time behavior, and they are in good agreement with those obtained by a Monte-Carlo simulation. The experimental implementation of the proposed heterody…
We observed squeezed vacuum light at 795 nm in 87Rb vapor via resonant polarization self-rotation, and report noise sidebands suppression of ~1 dB below shot noise level spanning from acoustic (30 kHz) to MHz frequencies. This is the first demonstration of sub-MHz quadrature vacuum squeezing in atomic systems. The spectral range of observed squeezing matches well typical bandwidths of electromagnetically induced transparency (EIT) resonances, making this simple technique for generation of optical fields with non-classical statistics at atomic transitions wavelengths attractive for EIT-based qu…
In spin-1 collective atomic systems, the spin and nematic-tensor operators constitute the su(3) Lie algebra whose su(2) subalgebras are shown to give two distinct classes of squeezing which are unitarily equivalent to spin squeezing and spin-nematic squeezing. We explicitly construct a unitary operator that generates an arbitrary squeezed spin-nematic state from an arbitrary Fock state. In particular, we demonstrate that squeezed spin states can be generated from a polar state and that squeezed spin-nematic sates can be generated from a fully spin-polarized state.
We analyze a model for spin squeezing based on the so-called counter-twisting Hamiltonian, including the effects of dissipation and finite system size. We discuss the conditions under which the Heisenberg limit, i.e. phase sensitivity $\propto 1/N$, can be achieved. A specific implementation of this model based on atom-atom interactions via quantized photon exchange is presented in detail. The resulting excitation corresponds to the creation of spin-flipped atomic pairs and can be used for fast generation of entangled atomic ensembles, spin squeezing and apllications in quantum information pro…
Unitary control of qudits can improve the collective spin squeezing of an atomic ensemble. Preparing the atoms in a state with large quantum fluctuations in magnetization strengthens the entangling Faraday interaction. The resulting increase in interatomic entanglement can be converted into metrologically useful spin squeezing. Further control can squeeze the internal atomic spin without compromising entanglement, providing an overall multiplicative factor in the collective squeezing. We model the effects of optical pumping and study the tradeoffs between enhanced entanglement and decoherence.…
Atomic squeezing is studied for the case of large systems of radiating atoms, when collective effects are well developed. All temporal stages are analyzed, starting with the quantum stage of spontaneous emission, passing through the coherent stage of superradiant emission, and going to the relaxation stage ending with stationary solutions. A method of governing the temporal behaviour of the squeezing factor is suggested. The influence of a squeezed effective vacuum on the characteristics of collective emission is also investigated.
Resonant interaction of a collection of two-level atoms with a single-mode coherent cavity field is considered in the framework of the Dicke model. We focus on the role of collective atomic effects in the phenomenon of collapses and revivals of the Rabi oscillations. It is shown that the behavior of the system strongly depends on the initial atomic state. In the case of the initial half-excited Dicke state we account for a number of interesting phenomena. The correlations between the atoms result in a suppression of the revival amplitude, and the revival time is halved, compared to the uncorre…
We propose a simple scheme to measure squeezing and phase properties of a harmonic oscillator. We treat in particular the case of a the field, but the scheme may be easily realized in ion traps. It is based on integral transforms of measured atomic properties as atoms exit a cavity. We show that by measuring atomic polarizations it is possible, after a given integration, to measure several properties of the field.
In this article we discuss a scheme of teleportation of atomic states making use of three-level lambda atoms. The experimental realization proposed makes use of cavity QED involving the interaction of Rydberg atoms with a micromaser cavity prepared in a coherent state. We start presenting a scheme to prepare atomic EPR states involving two-level atoms via the interaction of these atoms with a cavity. In our scheme the cavity and some atoms play the role of auxiliary systems used to achieve the teleportation.
Ultracold atoms in an ultrahigh-finesse optical cavity are a powerful platform to produce spin squeezing since photon of cavity mode can induce nonlinear spin-spin interaction and thus generate a one-axis twisting Hamiltonian $H_{\text{OAT}}=qJ_{x}^{2}$, whose corresponding maximal squeezing factor scales as $N^{-2/3}$, where $N$ is the atomic number. On the contrary, for the other two-axis twisting Hamiltonian $H_{\text{TAT}}=q(J_{x}^{2}-J_{y}^{2})$, the maximal squeezing factor scales as $N^{-1}$, approaching the Heisenberg limit. In this paper, inspired by recent experiments of cavity-assis…
We investigate theoretically and experimentally a nondestructive interferometric measurement of the state population of an ensemble of laser cooled and trapped atoms. This study is a step towards generation of (pseudo-) spin squeezing of cold atoms targeted at the improvement of the Caesium clock performance beyond the limit set by the quantum projection noise of atoms. We calculate the phase shift and the quantum noise of a near resonant optical probe pulse propagating through a cloud of cold 133Cs atoms. We analyze the figure of merit for a quantum non-demolition (QND) measurement of the col…
Spin squeezing of collective atomic spins can be achieved conditionally via probing with light and subsequent homodyne detection, as is done in a Quantum Nondemolition measurement. Recently it has been shown that squeezing can also be created unconditionally by a properly designed dissipative dynamics. We compare the two approaches in a Gaussian description, and optimize over all Gaussian light-matter interactions. We find that in the optimal unconditional scheme based on dissipation the level of squeezing scales as $d^{-1/2}$. In contrast, the optimal conditional scheme based on measurement o…
Spin squeezing is a form of entanglement that can improve the stability of quantum sensors operating with multiple particles, by inducing inter-particle correlations that redistribute the quantum projection noise. Previous analyses of potential metrological gain when using spin squeezing were performed on theoretically ideal states, without incorporating experimental imperfections or inherent limitations which result in non-unitary quantum state evolution. Here, we show that potential gains in clock stability are substantially reduced when the spin squeezing is non-unitary, and derive analytic…
