We present a complete theoretical description of atomic storage states in the multimode framework by including spatial coherence in atomic collective operators and atomic storage states. We show that atomic storage states are Dicke states with the maximum cooperation number. In some limits, a set of multimode atomic storage states has been established in correspondence with multimode Fock states of the electromagnetic field. This gives better understanding of both the quantum and coherent information of optical field can be preserved and recovered in ultracold medium. In this treatment, we discuss in detail both the adiabatic and dynamic transfer of quantum information between the field and the ultracold medium.
We experimentally demonstrate electromagnetically induced transparency and light storage with ultracold 87Rb atoms in a Mott insulating state in a three dimensional optical lattice. We have observed light storage times of about 240 ms, to our knowledge the longest ever achieved in ultracold atomic samples. Using the differential light shift caused by a spatially inhomogeneous far detuned light field we imprint a "phase gradient" across the atomic sample, resulting in controlled angular redirection of the retrieved light pulse.
Advanced data analysis techniques have proved to be crucial for extracting information from noisy images. Here we show that principal component analysis can be successfully applied to ultracold gases to unveil their collective excitations. By analyzing the correlations in a series of images we are able to identify the collective modes which are excited, determine their population, image their eigenfunction, and measure their frequency. Our method allows to discriminate the relevant modes from other noise components and is robust with respect to the data sampling procedure. It can be extended t…
We derive a master equation describing the collective decay of two-level atoms inside a single mode cavity in the dispersive limit. By considering atomic decay in the collective thermostat, we found a decoherence-free subspace of the multiparticle entangled states of the W-like class. We present a scheme for writing and storing these states in collective thermostat.
We theoretically analyze interference patterns of parametrically driven one dimensional ultracold atomic gases. By modulating the interaction strength periodically in time, we propose to excite collective modes in a pair of independent one dimensional gases at energies corresponding to the drive frequency. The excited collective modes lead to spatial oscillations in the correlations of the interference pattern, which can be analyzed to obtain the sound velocity of the collective modes. We discuss both bosonic and fermionic systems, and how such experiments could be used to probe spin charge se…
We demonstrate optical nonlinearities due to the interaction of weak optical fields with the collective motion of a strongly dispersive ultracold gas. The combination of a recoil-induced resonance (RIR) in the high gain regime and optical waveguiding within the dispersive medium enables us to achieve a collective atomic cooperativity of $275 \pm 50$ even in the absence of a cavity. As a result, we observe optical bistability at input powers as low as 20 pW. The present scheme allows for dynamic optical control of the dispersive properties of the ultracold gas using very weak pulses of light. T…
The quantum optical response of high density ultracold atomic systems is critical to a wide range of fundamentally and technically important physical processes. These include quantum image storage, optically based quantum repeaters and ultracold molecule formation. We present here a microscopic analysis of the light scattering on such a system, and we compare it with a corresponding description based on macroscopic Maxwell theory. Results are discussed in the context of the spectral resonance structure, time-dependent response, and the light localization problem.
We study the nonlinear dynamics of an ensemble of cold trapped atoms with a hyperfine transition magnetically coupled to a resonant microwave cavity mode. Despite the minute single atom coupling one obtains strong coupling between collective hyperfine qubits and microwave photons enabling coherent transfer of an excitation between the long lived atomic qubit state and the mode. Evidence of strong coupling can be obtained from the cavity transmission spectrum even at finite thermal photon number. The system makes it possible to study further prominent collective phenomena such as superradiant d…
Quantum states with long-lived coherence are essential for quantum computation, simulation and metrology. The nuclear spin states of ultracold molecules prepared in the singlet rovibrational ground state are an excellent candidate for encoding and storing quantum information. However, it is important to understand all sources of decoherence for these qubits, and then eliminate them, in order to reach the longest possible coherence times. Here, we fully characterise the dominant mechanisms for decoherence of a storage qubit in an optically trapped ultracold gas of RbCs molecules using high-reso…
Current research on micro-mechanical resonators strives for quantum-limited detection of the motion of macroscopic objects. Prerequisite to this goal is the observation of measurement backaction consistent with quantum metrology limits. However, thermal noise presently dominates measurements and precludes ground-state preparation of the resonator. Here we establish the collective motion of an ultracold atomic gas confined tightly within a Fabry-Perot optical cavity as a system for investigating the quantum mechanics of macroscopic bodies. The cavity-mode structure selects a single collective v…
We present an analysis of transfer of quantum information between the collective spin degrees of freedom of a large ensemble of two-level systems and a single central qubit. The coupling between the central qubit and the individual ensemble members may be varied and thus provides access to more than a single storage mode. Means to store and manipulate several independent qubits are derived for the case where the variation in coupling strengths does not allow addressing of orthogonal modes of the ensemble. While our procedures and analysis may apply to a number of different physical systems, fo…
The collective modes of a quantum liquid shape and impact its properties profoundly, including its emergent phenomena such as superfluidity. Here we present how a two-dimensional Bose gas responds to a moving lattice potential. In particular we discuss how the induced heating rate depends on the interaction strength and the temperature. This study is motivated by the recent measurements of Sobirey {\it et al.} arXiv:2005.07607 (2020), for which we provide a quantitative understanding. Going beyond the existing measurements, we demonstrate that this probing method allows to identify first and s…
Coherent control of collective spontaneous emission in an extended atomic ensemble resonantly interacting with single-photon wave packets is analyzed. A scheme for coherent manipulation of collective atomic states is developed such that superradiant states of the atomic system can be converted into subradiant ones and vice versa. Possible applications of such a scheme for optical quantum state storage and single-photon wave packet shaping are discussed. It is shown that also in the absence of inhomogeneous broadening of the resonant line, single-photon wave packets with arbitrary pulse shape m…
We consider the non-equilibrium orbital dynamics of spin-polarized ultracold fermions in the first excited band of an optical lattice. A specific lattice depth and filling configuration is designed to allow the $p_x$ and $p_y$ excited orbital degrees of freedom to act as a pseudo-spin. Starting from the full Hamiltonian for p-wave interactions in a periodic potential, we derive an extended Hubbard-type model that describes the anisotropic lattice dynamics of the excited orbitals at low energy. We then show how dispersion engineering can provide a viable route to realizing collective behavior d…
In many experiments isolated atoms and ions have been inserted into high-finesse optical resonators for the study of fundamental quantum optics and quantum information. Here, we introduce another application of such a system, as the realization of cavity optomechanics where the collective motion of an atomic ensemble serves the role of a moveable optical element in an optical resonator. Compared with other optomechanical systems, such as those incorporating nanofabricated cantilevers or the large cavity mirrors of gravitational observatories, our cold-atom realization offers direct access to t…
Quantum information platforms made great progress in the control of many-body entanglement and the implementation of quantum error correction, but it remains a challenge to realize both in the same setup. Here, we propose a mixture of two ultracold atomic species as a platform for universal quantum computation with long-range entangling gates, while providing a natural candidate for quantum error-correction. In this proposed setup, one atomic species realizes localized collective spins of tunable length, which form the fundamental unit of information. The second atomic species yields phononic …
Epitaxially grown quantum dots (QDs) are promising sources of non-classical states of light such as single photons and entangled photons. However, in order for them to be used as a resource for long-distance quantum communication, distributed quantum computation, or linear optics quantum computing, these photons must be coupled efficiently to long-lived quantum memories as part of a quantum repeater network. Here, we theoretically examine the prospects for efficient storage and retrieval of a QD-generated single photon with a 1 ns lifetime in a multi-level atomic system. We calculate using an …
High-density and ultracold atomic gases have emerged as promising media for storage of individual photons for quantum memory applications. In this paper we provide an overview of our theoretical and experimental efforts in this direction, with particular attention paid to manipulation of light storage (a) through complex recurrent optical scattering processes in very high density gases (b) by an external control field in a characteristic electromagnetically induced transparency configuration.
Experiments in dense, ultracold gases of rubidium Rydberg atoms show a considerable decrease of the radiative excited state lifetimes compared to dilute gases. This accelerated decay is explained by collective and cooperative effects, leading to superradiance. A novel formalism to calculate effective decay times in a dense Rydberg gas shows that for these atoms the decay into nearby levels increases by up to three orders of magnitude. Excellent agreement between theory and experiment follows from this treatment of Rydberg decay behavior.
Einstein, Podolsky & Rosen (EPR) pointed out that correlations induced between quantum objects will persist after these objects have ceased to interact. Consequently, their joint continuous variables (CV), e.g., the difference of their positions and the sum of their momenta, may be specified, regardless of their distance, with arbitrary precision. EPR correlations give rise to two fundamental notions: {\em nonlocal ``steering''} of the quantum state of one object by measuring the other, and inseparability ({\em entanglement}) of their quantum states. EPR entanglement is a resource of quantum i…
A near perfect, storage time-extended photon echo-based quantum memory protocol has been analyzed by solving the Maxwell-Bloch equations for a backward scheme in a three-level system. The backward photon echo scheme is combined with a controlled coherence conversion process via control Rabi flopping to a third state, where the control Rabi flopping collectively shifts the phase of the ensemble coherence. The propagation direction of photon echoes is coherently determined by the phase matching condition between the data (quantum) and the control (classical) pulses. Herein we discuss the classic…
We theoretically investigate the generation of microscopic atomic NOON states, corresponding to the coherent |N,0> + |0,N> superposition with N ~ 5 particles, via collective tunneling of interacting ultracold bosonic atoms within a symmetric double-well potential in the self-trapping regime. We show that a periodic driving of the double well with suitably tuned amplitude and frequency parameters allows one to substantially boost this tunneling process without altering its collective character. The time scale to generate the NOON superposition, which corresponds to half the tunneling time and w…
We study the resonant electronic excitation dynamics for ultracold atoms trapped in a deep optical lattice prepared in a Mott insulator state. Excitons in these artificial crystals are similar to Frenkel excitons in Noble atom or molecular crystals. They appear when the atomic excited state line width is smaller than the exciton band width generated by dipole-dipole coupling. When the atoms are placed within a cavity the electronic excitations and the quantized cavity mode get coupled. In the collective strong coupling regime excitations form two branches of cavity polaritons with Rabi splitti…
Ultracold collisions of Bose-Einstein condensates can be used to generate a large number of counterpropagating pairs of entangled atoms, which collectively form a thin spherical shell in momentum space, called a scattering halo. Here we generate a scattering halo composed almost entirely of pairs in a symmetric entangled state and observe a scattering angle-dependent mixing to the anti-symmetric state due to the presence of an inhomogeneous magnetic field. We report on a proof-of-principle application of the observed parity dynamics to demonstrate magnetic gradiometry, insensitive to common-mo…
To overcome fundamental limitations of the πoptical pulse-induced population inversion and optical decay-caused short storage time in conventional photon echoes, a coherent control of collective atoms is studied for inversion-free, optical decay-halted photon echoes, where the constraint of photon storage time is now replaced by a spin population decay process. Using phase-controlled double rephasing, an inversion-free photon echo scheme is obtained, where no spontaneous or stimulated emission-driven quantum noise exists. Thus, the present method can be applied for ultralong quantum memories i…
The influence of decoherence on the fidelity of quantum memories for photonic qubits based on dark-state polaritons in atomic ensembles is discussed. It is shown that despite the large entanglement of the collective storage states corresponding to single photons or nonclassical states of light the sensitivity to decoherence does not scale with the number of atoms. This is due to the existence of equivalence classes of storage states corresponding to states with the same number of dark-state polariton excitations but arbitrary excitations in other polariton modes. Several decoherence processes …
We study the transmission spectra of ultracold rubidium atoms coupled to a high-finesse optical cavity. Under weak probing with pi-polarized light, the linear response of the system is that of a collective spin with multiple levels coupled to a single mode of the cavity. By varying the atom number, we change the collective coupling of the system. We observe the change in transmission spectra when going from a regime where the collective coupling is much smaller than the separation of the atomic levels to a regime where both are of comparable size. The observations are in good agreement with a …
We report on Kerr nonlinearity and dispersive optical bistability of a Fabry-Perot optical resonator due to the displacement of ultracold atoms trapped within. In the driven resonator, such collective motion is induced by optical forces acting upon up to $10^5$ $^{87}$Rb atoms prepared in the lowest band of a one-dimensional intracavity optical lattice. The longevity of atomic motional coherence allows for strongly nonlinear optics at extremely low cavity photon numbers, as demonstrated by the observation of both branches of optical bistability at photon numbers below unity.
We study cavity optomechanics of a mixture of ultracold atoms with tunable nonlinear collisions. We show that atomic collisions provide linear couplings between fictitious condensate oscillators, leading to possibilities of achieving a globally coupled quantum optomechanical network with an integrated atom chip. Potential applications range from simulating collective nonequilibrium dynamics in fields well past physics to probing unique properties of quantum mixtures.
Based on the developed quantum microscopic theory, the interaction of weak electromagnetic radiation with dense ultracold atomic clouds is described in detail. The differential and total cooperative scattering cross sections are calculated for monochromatic radiation as particular examples of application of the general theory. The angular, spectral, and polarization properties of scattered light are determined. The dependence of these quantities on the sample size and concentration of atoms is studied and the influence of collective effects is analyzed.
Electron and nuclear spins have good coherence times and an ensemble of spins is a promising candidate for a quantum memory. By employing holographic techniques via field gradients a single ensemble may be used to store many bits of information. Here we present a coherent memory using a pulsed magnetic field gradient, and demonstrate the storage and retrieval of up to 100 weak 10 GHz coherent excitations in collective states of an electron spin ensemble. We further show that such collective excitations in the electron spin can then be stored in nuclear spin states, which offer coherence times …
Ultracold ground-state molecules can be formed from ultracold atoms via photoassociation followed by a spontaneous emission process. Typically, the molecular products are distributed over a range of final states. Here, we propose to use an optical cavity with high cooperativity to selectively enhance the population of a pre-determined final state by controlling the spontaneous emission. During this process, a photon will be emitted into the cavity mode. Detection of this photon heralds a single reaction. We discuss the efficiency and the dynamics of cavity-assisted molecule formation in the fr…
We report the experimental demonstration of a quantum memory for collective atomic states in a far-detuned optical dipole trap. Generation of the collective atomic state is heralded by the detection of a Raman scattered photon and accompanied by storage in the ensemble of atoms. The optical dipole trap provides confinement for the atoms during the quantum storage while retaining the atomic coherence. We probe the quantum storage by cross-correlation of the photon pair arising from the Raman scattering and the retrieval of the atomic state stored in the memory. Non-classical correlations are ob…
A scheme for coherent manipulation of collective atomic states is developed such that total subradiant states, in which spontaneous emission is suppressed into all directions due to destructive interference between neighbor atoms, can be created in an extended atomic ensemble. The optimal conditions for creation of such states and suitability of them for quantum storage are discussed. It is shown that in order to achieve the maximum signal-to-noise ratio the shape of a light pulse to be stored and reconstructed using a homogeneously broadened absorbtion line of an atomic system should be a tim…
We investigate the collective aspects of Rydberg excitation in ultracold mesoscopic systems. Strong interactions between Rydberg atoms influence the excitation process and impose correlations between excited atoms. The manifestations of the collective behavior of Rydberg excitation are the many-body Rabi oscillations, spatial correlations between atoms as well as the fluctuations of the number of excited atoms. We study these phenomena in detail by numerically solving the many-body Schrëdinger equation.
Prospects for reaching persistent entanglement between two spatially separated atomic Bose-Einstein condensates are outlined. The system set-up comprises of two condensates loaded in an optical lattice, which, in return, is confined within a high-Q optical resonator. The system is driven by an external laser that illuminates the atoms such that photons can scatter into the cavity. In the superradiant phase a cavity field is established and we show that the emerging cavity mediated interactions between the two condensates is capable of entangling them despite photon losses. This macroscopic ato…
In this article we discuss and compare different ways to engineer an interface between ultracold atoms and micro- and nanomechanical oscillators. We start by analyzing a direct mechanical coupling of a single atom or ion to a mechanical oscillator and show that the very different masses of the two systems place a limit on the achievable coupling constant in this scheme. We then discuss several promising strategies for enhancing the coupling: collective enhancement by using a large number of atoms in an optical lattice in free space, coupling schemes based on high-finesse optical cavities, and …
We present a theoretical framework to describe the collective emission of light by entangled atomic states. Our theory applies to the low excitation regime, where most of the atoms are initially in the ground state, and relies on a bosonic description of the atomic excitations. In this way, the problem of light emission by an ensemble of atoms can be solved exactly, including dipole-dipole interactions and multiple light scattering. Explicit expressions for the emitted photonic states are obtained in several situations, such as those of atoms in regular lattices and atomic vapors. We determine…
Using collective atom phase control a population inversion-free photon echo scheme has been studied for quantum memory applications. For the inversion-free photon echoes a double rephasing method is combined with optical locking, where the optical locking coherently controls each atom phase excited by weak data pulses. As a result, intensity flattened, normally ordered, storage time-extended, and noise-free photon echoes are obtained.
Two-dimensional regular arrays of atoms are a promising platform for quantum networks, with collective subradiant states providing long-lived storage and collimated emission allowing for natural coherent links between arrays in free space. However, a single-layer lattice can only efficiently absorb or emit light symmetrically in the forward and backward directions. Here we show how a bilayer lattice can absorb a single photon either incident from a single direction or an arbitrary superposition of forward and backward propagating components. The excitation can be stored in a subradiant state, …
Ultracold atoms uniformly filling an optical lattice can be treated like an artificial crystal. An implementation including the atomic occupation of a single excited atomic state can be represented by a two-component Bose-Hubbard model. Its phase diagram exhibits a quantum phase transition from a superfluid to a Mott insulator phase. The dynamics of electronic excitations governed by electrostatic dipole-dipole interactions in the ordered regime can be well described by wave-like collective excitations called excitons. Here we present an extensive study of such excitons for a wide range of geo…
We investigate an attractive force caused by light induced dipole-dipole interactions in freely expanding ultracold 87Rb atoms. This collective, light-triggered effect results in a self-confining potential with interesting features: it exhibits nonlocal properties, is attractive for both red and blue-detuned light fields and induces a remarkably strong force that depends on the gradient of the atomic density. The experimental data are discussed in the framework of a theoretical model based on a local-field approach for the light scattered by the atomic cloud.
Quantum mechanics is an inherently linear theory. However, collective effects in many body quantum systems can give rise to effectively nonlinear dynamics. In the present work, we analyze whether and to what extent such nonlinear effects can be exploited to enhance the rate of quantum evolution. To this end, we compute a suitable version of the quantum speed limit for numerical and analytical examples. We find that the quantum speed limit grows with the strength of the nonlinearity, yet it does not trivially scale with the ``degree'' of nonlinearity. This is numerically demonstrated for the pa…
Confining ultracold gases in cavities creates a paradigm of quantum trapping potentials. We show that this allows to bridge models with global collective and short-range interactions as novel quantum phases possess properties of both. Some phases appear solely due to quantum light-matter correlations. Due to global, but spatially structured, interaction, the competition between quantum matter and light waves leads to multimode structures even in single-mode cavities, including delocalized dimers of matter-field coherences (bonds), beyond density orders as supersolids and density waves.
The effects of decoherence on the transfer and storage of coherent quantum states in hybrid systems are studied within the Caldeira-Leggett approach. In general, we find that a high transfer fidelity can be achieved even if the decoherence time is less than an order of magnitude larger than the transfer time, which is approximately half a Rabi period and determined by the qubit-qubit coupling strength. Finally, we apply our results to assess the feasibility of a hybrid quantum memory system, comprised of the hyperfine qubit states of an ultracold atomic Bose-Einstein condensate and the flux qu…
An ensemble of excited atoms can synchronize emission of light collectively in a process known as superradiance when its characteristic size is smaller than the wavelength of emitted photons. The underlying superradiance depends strongly on electromagnetic (photon) fields surrounding the atomic ensemble. High mode densities of microwave photons from $300\,$K blackbody radiation (BBR) significantly enhance decay rates of Rydberg states to neighbouring states, enabling superradiance that is not possible with bare vacuum induced spontaneous decay. Here we report observations of the superradiance …
Triple-NOON states are superpositions of the form $e^{i φ_1} |{N,0,0}\rangle + e^{i φ_2} |{0,N,0}\rangle + e^{i φ_3} |{0,0,N}\rangle$ involving $N$ bosonic quanta distributed over three modes. We theoretically show how such highly entangled states can be generated with interacting ultracold bosonic atoms in a symmetric three-site lattice. The basic protocol consists in preparing all atoms on one site of the lattice and then letting the system evolve during a specific time such that collective tunneling of the atoms to the other two sites takes place. The key point put forward here is that this…
We propose a mechanism to realize high-yield molecular formation from ultracold atoms. Atom pairs are continuously excited by a laser, and a collective decay into the molecular ground state is induced by a coupling to a lossy cavity mode. Using a combination of analytical and numerical techniques, we demonstrate that the molecular yield can be improved by simply increasing the number of atoms, and can overcome efficiencies of state-of-the-art association schemes. We discuss realistic experimental setups for diatomic polar and nonpolar molecules, opening up collective light matter interactions …
Resonant dipole-dipole interaction modifies the energy and decay rate of electronic excitations for finite one dimensional chains of ultracold atoms in an optical lattice. We show that collective excited states of the atomic chain can be divided into dark and bright modes, where a superradiant mode with an enhanced collective effective dipole dominates the optical scattering. Studying the generic case of two chain segments of different length and position exhibits an interaction blockade and spatially structured light emission. Ultimately, an extended system of several interfering segments mod…
Coherent scattering of light from ultracold atoms involves an exchange of energy and momentum introducing a wealth of non-linear dynamical phenomena. As a prominent example particles can spontaneously form stationary periodic configurations which simultaneously maximize the light scattering and minimize the atomic potential energy in the emerging optical lattice. Such self-ordering effects resulting in periodic lattices via bimodal symmetry breaking have been experimentally observed with cold gases and Bose-Einstein condensates (BECs) inside an optical resonator. Here we study a new regime of …
In contrast to the fully projective limit of strong quantum measurement, where the evolution is locked to a small subspace (quantum Zeno dynamics), or even frozen completely (quantum Zeno effect), the weak non-projective measurement can effectively compete with standard unitary dynamics leading to nontrivial effects. Here we consider global weak measurement addressing collective variables, thus preserving quantum superpositions due to the lack of which path information. While for certainty we focus on ultracold atoms, the idea can be generalized to other multimode quantum systems, including va…
We use a microwave field to control the quantum state of optical photons stored in a cold atomic cloud. The photons are stored in highly excited collective states (Rydberg polaritons) enabling both fast qubit rotations and control of photon-photon interactions. Through the collective read-out of these pseudo-spin rotations it is shown that the microwave field modifies the long-range interactions between polaritons. This technique provides a powerful interface between the microwave and optical domains, with applications in quantum simulations of spin liquids, quantum metrology and quantum netwo…
We report the storage and retrieval of a small microwave field from a superconducting resonator into collective excitations of a spin ensemble. The spins are nitrogen-vacancy centers in a diamond crystal. The storage time of the order of 30 ns is limited by inhomogeneous broadening of the spin ensemble.
We present a wave atom optics theory of the Collective Atomic-Recoil Laser, where the atomic center-of-mass motion is treated quantum mechanically. It extends the previous ray atom optics theory, which treated the center-of-mass atomic motion classically, to the realm of ultracold atoms. For the case of a far off resonant pump laser we derive an analytical solution which gives the linear response of the CARL system for both the quantum and classical regimes. A linear stability analysis reveals significant qualitative differences between these two regimes, which arise from the effects of diffra…
