We propose a mechanism to realize high-yield molecular formation from ultracold atoms. Atom pairs are continuously excited by a laser, and a collective decay into the molecular ground state is induced by a coupling to a lossy cavity mode. Using a combination of analytical and numerical techniques, we demonstrate that the molecular yield can be improved by simply increasing the number of atoms, and can overcome efficiencies of state-of-the-art association schemes. We discuss realistic experimental setups for diatomic polar and nonpolar molecules, opening up collective light matter interactions as a tool for quantum state engineering, enhanced molecule formation, collective dynamics, and cavity mediated chemistry.
While the recently realized dissipative time crystal in a laser-pumped atom-cavity system in the experiment of Keßler et al. [Phys. Rev. Lett. 127, 043602 (2021)] is qualitatively consistent with a theoretical description in an idealized limit, here, we investigate the stability of this dissipative time crystal in the presence of an inhomogeneous potential provided by a harmonic trap, and competing short- and infinite-range interactions. We note that these features are ubiquitous in any realization of atom-cavity systems. By mapping out the dynamical phase diagram and studying how it is modifi…
Supersolids are characterized by the counter-intuitive coexistence of superfluid and crystalline order. Here we study a supersolid phase emerging in the steady state of a driven-dissipative system. We consider a transversely pumped Bose-Einstein condensate trapped along the axis of a ring cavity and coherently coupled to a pair of degenerate counter-propagating cavity modes. Above a threshold pump strength the interference of photons scattered into the two cavity modes results in an emergent superradiant lattice, which spontaneously breaks the continuous translational symmetry towards a period…
In dissipative quantum systems, strong symmetries can lead to the existence of conservation laws and multiple steady states. In this work we investigate a strong symmetry for bosonic atoms coupled to an optical cavity, an experimentally relevant system, generalizing the adiabatic elimination techniques and using numerically exact matrix product state methods. We show that for ideal bosons coupled to the cavity multiple steady states exist and in each symmetry sector a dissipative phase transition occurs at a different critical point. This implies that phases of very different nature can coexis…
We present a theoretical study on the robustness of multi-photon states in a frustrated lattice of coupled nonlinear optical cavities, which are described by a driven-dissipative Bose-Hubbard model. In particular, we focus here on a Lieb lattice with two elementary cells and periodic boundary conditions. Due to the geometric frustration of the lattice, the non-equilibrium steady state can exhibit dark sites with low photon density and strong correlations, ascribable to the population of multi-photon modes. We explore the sensitivity of such strong correlations on the random inhomogeneity of th…
We study the collective emission of a beam of atomic dipoles into an optical cavity. Our focus lies on the effect of a finite detuning between the atomic transition frequency and the cavity resonance frequency. By developing a theoretical description of the coupled atom-cavity dynamics we analyze the stationary atomic configurations including a superradiant phase where the atoms undergo continuous monochromatic collective emission. In addition, we derive an analytical formula for the cavity pulling coefficient which characterizes the displacement of the emission frequency towards the cavity fr…
Pumps are transport mechanisms in which direct currents result from a cyclic evolution of the potential. As Thouless has shown, the pumping process can have topological origins, when considering the motion of quantum particles in spatially and temporally periodic potentials. However, the periodic evolution that drives these pumps has always been assumed to be imparted from outside, as was the case in the experimental systems studied so far. Here we report on an emergent mechanism for pumping in a quantum gas coupled to an optical resonator, where we observe a particle current without applying …
We numerically obtain the full time-evolution of a parametrically-driven dissipative Bose-Einstein condensate in an optical cavity and investigate the implications of driving for the phase diagram. Beyond the normal and superradiant phases, a third nonequilibrium phase emerges as a manybody parametric resonance. This dynamical normal phase switches between two symmetry-broken superradiant configurations. The switching implies a breakdown of the system's mapping to the Dicke model. Unlike the other phases, the dynamical normal phase shows features of nonintegrability and thermalization.
We propose the dynamical stabilization of a nonequilibrium order in a driven dissipative system comprised an atomic Bose-Einstein condensate inside a high finesse optical cavity, pumped with an optical standing wave operating in the regime of anomalous dispersion. When the amplitude of the pump field is modulated close to twice the characteristic limit-cycle frequency of the unmodulated system, a stable subharmonic response is found. The dynamical phase diagram shows that this subharmonic response occurs in a region expanded with respect to that where stable limit-cycle dynamics occurs for the…
We study the XY model with infinite-range interactions (Lipkin-Meshkov-Glick model) in the presence of dissipation from spontaneous decay. We show that independent and collective decay lead to qualitatively different phase transitions of the steady state, even though the phase boundary is the same. Independent decay leads to a second-order phase transition to a ferromagnet, while collective decay leads to a first-order transition to a time-dependent oscillatory phase. Then we show that the addition of a drive leads to infinite spin squeezing for collective decay in the thermodynamic limit. Our…
We observe vacuum Rabi splitting in a lossy nearly confocal cavity indicating the strong coupling regime, despite a weak single-atom single-mode coupling. Strong collective interaction manifests itself in the typical $\sqrt{N}$-dependence of the normal mode splitting on the number of atoms $N$. The $TEM_{00}$-mode coupling parameters are $(g,κ,γ)=2π\times(0.12,0.8,2.6)$ MHz and up to $(1.33\pm 0.08)\times10^5$ cesium atoms were loaded into the mode volume.
We describe an efficient numerical method for simulating the dynamics and steady states of collective spin systems in the presence of dephasing and decay. The method is based on the Schwinger boson representation of spin operators and uses an extension of the truncated Wigner approximation to map the exact open system dynamics onto stochastic differential equations for the corresponding phase space distribution. This approach is most effective in the limit of very large spin quantum numbers, where exact numerical simulations and other approximation methods are no longer applicable. We benchmar…
We investigate the near-critical dynamics of atomic density fluctuations in the non-equilibrium self-organization transition of an optically driven quantum gas coupled to a single mode of a cavity. In this system cavity-mediated long-range interactions between atoms, tunable by the drive strength, lead to softening of an excitation mode recently observed in experiments. This phenomenon has previously been studied within a two-mode approximation for the collective motional degrees of freedom of the atomic condensate which results in an effective open-system Dicke model. Here, including the full…
Fluctuation-Induced Bistability in the Dissipative Dynamics of Generic Cavity-Matter Quantum Systems
Univ. Grenoble Alpes, CEA, Grenoble INP, IRIG, Pheliqs（格勒诺布尔阿尔卑斯大学）；Physikalisches Institut, University of Bonn（波恩大学物理研究所）；Max Planck Institute for the Physics of Complex Systems（马克斯·普朗克复杂系统物理研究所）
By exploiting the nonlinear nature of the Jaynes Cumming's interaction, one can get photon population trapping in cavity-QED arrays. However, the unavoidable dissipative effects in a realistic system would destroy the self-trapped state by continuous photon leakage. To circumvent this issue, we show that a careful engineering of drive, dissipation and Hamiltonian results in achieving indefinitely sustained self-trapping. We show that the intricate interplay between drive, dissipation, and light-matter interaction results in requiring an optimal window of drive strengths in order to achieve suc…
We predict a new mechanism to induce collective excitations and a nonequilibrium phase transition of fermionic superfluids via a sudden switch-on of two-body loss, for which we extend the BCS theory to fully incorporate a change in particle number. We find that a sudden switch-on of dissipation induces an amplitude oscillation of the superfluid order parameter accompanied by a chirped phase rotation as a consequence of particle loss. We demonstrate that when dissipation is introduced to one of the two superfluids coupled via a Josephson junction, it gives rise to a nonequilibrium dynamical pha…
We theoretically study the driven-dissipative Harper-Hofstadter model on a 2D square lattice in the presence of a weak harmonic trap. Without pumping and loss, the eigenstates of this system can be understood, in certain limits, as momentum-space toroidal Landau levels, where the Berry curvature, a geometrical property of an energy band, acts like a momentum-space magnetic field. We show that key features of these eigenstates can be observed in the steady-state of the driven-dissipative system under a monochromatic coherent drive, and present a realistic proposal for an optical experiment usin…
We investigate the dynamics of fermionic atoms in a high-finesse optical resonator after a sudden switch on of the coupling between the atoms and the cavity. The atoms are additionally confined by optical lattices to a ladder geometry. The tunneling mechanism on a rung of a ladder is induced by a cavity assisted Raman process. At long times after the quantum quench the arising steady state can carry a chiral current. In this work we employ exact diagonalization techniques on small system sizes to study the dissipative attractor dynamics after the quench towards the steady state and deviations …
We present a technique, based on atoms coupled to an optical cavity, for non-destructive detection of trapped ions. We demonstrate the vacuum-Rabi splitting (VRS), arising due to the collective strong coupling of ultracold Rb atoms to a cavity, to change in presence of trapped Rb+ ions. The Rb+ ions are optically dark and the Rb atoms are prepared in a dark magneto-optical trap (MOT). The VRS is measured on an optically open transition of the initially dark Rb atoms. The measurement itself is fast, non-destructive and has sufficient fidelity to permit the measurement of atomic-state selective …
We use the Bethe Ansatz technique to study dissipative systems experiencing loss. The method allows us to exactly calculate the Liouvillian spectrum. This opens the possibility of analytically calculating the dynamics of a wide range of experimentally relevant models including cold atoms subjected to one and two body losses, coupled cavity arrays with bosons escaping the cavity, and cavity quantum electrodynamics. As an example of our approach we study the relaxation properties in a boundary driven XXZ spin chain. We exactly calculate the Liouvillian gap and find different relaxation rates wit…
We study collective scattering with Bose-Einstein condensates interacting with a high-finesse ring cavity. The condensate scatters the light of a transverse pump beam superradiantly into modes which, in contrast to previous experiments, are not determined by the geometrical shape of the condensate, but specified by a resonant cavity mode. Moreover, since the recoil-shifted frequency of the scattered light depends on the initial momentum of the scattered fraction of the condensate, we show that it is possible to employ the good resolution of the cavity as a filter selecting particular quantized…
