We present a technique, based on atoms coupled to an optical cavity, for non-destructive detection of trapped ions. We demonstrate the vacuum-Rabi splitting (VRS), arising due to the collective strong coupling of ultracold Rb atoms to a cavity, to change in presence of trapped Rb+ ions. The Rb+ ions are optically dark and the Rb atoms are prepared in a dark magneto-optical trap (MOT). The VRS is measured on an optically open transition of the initially dark Rb atoms. The measurement itself is fast, non-destructive and has sufficient fidelity to permit the measurement of atomic-state selective ion-atom collision rate. This demonstration illustrates a method based on atom-cavity coupling to measure two particle interactions generically and non-destructively.
We demonstrate a new method of cavity-enhanced non-destructive detection of atoms for a strontium optical lattice clock. The detection scheme is shown to be linear in atom number up to at least 10,000 atoms, to reject technical noise sources, to achieve signal to noise ratio close to the photon shot noise limit, to provide spatially uniform atom-cavity coupling, and to minimize inhomogeneous ac Stark shifts. These features enable detection of atoms with minimal perturbation to the atomic state, a critical step towards realizing an ultra-high-stability, quantum-enhanced optical lattice clock.
Rydberg atoms are at the core of an increasing number of experiments, which frequently rely on destructive detection methods, such as field ionization. Here, we present an experimental realization of single-shot non-destructive detection of ensembles of helium Rydberg atoms. We use the dispersive frequency shift of a superconducting microwave cavity interacting with the ensemble. By probing the transmission of the cavity and measuring the change in its phase, we determine the number of Rydberg atoms or the populations of Rydberg quantum states when the ensemble is prepared in a superposition. …
Bloch oscillations are a hallmark of coherent wave dynamics in periodic potentials. They occur as the response of quantum mechanical particles in a lattice if a weak force is applied. In optical lattices with their perfect periodic structure they can be readily observed and employed as a quantum mechanical force sensor, for example, for precise measurements of the gravitational acceleration. However, the destructive character of the measurement process in previous experimental implementations poses serious limitations for the precision of such measurements. In this article we show that the use…
Non-destructive cavity readout of molecules for precision measurements
University of Florida（佛罗里达大学）；Johns Hopkins University（约翰斯·霍普金斯大学）；University of Chicago（芝加哥大学）；Massachusetts Institute of Technology（麻省理工学院）；Argonne National Laboratory（阿贡国家实验室）
Laser spectroscopy of cold and trapped molecular ions is a powerful tool for fundamental physics, including the determination of fundamental constants, the laboratory test for their possible variation, and the search for a possible electric dipole moment of the electron. Optical clocks based on molecular ions sensitive to some of these effects are expected to achieve uncertainties approaching the $10^{-18}$ level. While the complexity of molecular structure facilitates these applications, the absence of cycling transitions poses a challenge for direct laser cooling, quantum state control, and …
We present and implement a non-destructive detection scheme for the transition probability readout of an optical lattice clock. The scheme relies on a differential heterodyne measurement of the dispersive properties of lattice-trapped atoms enhanced by a high finesse cavity. By design, this scheme offers a 1st order rejection of the technical noise sources, an enhanced signal-to-noise ratio, and an homogeneous atom-cavity coupling. We theoretically show that this scheme is optimal with respect to the photon shot noise limit. We experimentally realize this detection scheme in an operational str…
We theoretically study non-destructive detection of ultracold molecules, using a Fabry-Perot cavity. Specifically, we consider vacuum Rabi splitting where we demonstrate the use of collective strong coupling for detection of molecules with many participating energy levels. We also consider electromagnetically induced transparency and transient response of light for the molecules interacting with a Fabry-Perot cavity mode, as a mean for non-destructive detection. We identify the parameters that are required for the detection of molecules in the cavity electromagnetically induced transparency co…
Various techniques are used to detect the presence of charged particles stored in electromagnetic traps, their energy, their mass, or their internal states. Detection methods can rely on the variation of the number of trapped particles (destructive methods) or the use of the ion's interaction with electromagnetic radiation as a non-destructive tool to probe the trapped particles. This review gives an introduction into various methods, discussing the basic mode of operation completed by the description of recent realizations.
We investigate how superpositions of motional coherent states naturally arise in the dynamics of a two-level trapped ion coupled to the quantized field inside a cavity. We extend our considerations including a more realistic set up where the cavity is not ideal and photons may leak through its mirrors. We found that a detection of a photon outside the cavity would leave the ion in a pure state. The statistics of the ionic state still keeps some interference effects that might be observed in the weak coupling regime.
We propose a hardware architecture and protocol for connecting many local quantum processors contained within an optical cavity. The scheme is compatible with trapped ions or Rydberg arrays, and realizes teleported gates between any two qubits by distributing entanglement via single-photon transfers through a cavity. Heralding enables high-fidelity entanglement even for a cavity of moderate quality. For processors composed of trapped ions in a linear chain, a single cavity with realistic parameters successfully transfers photons every few $μ$s, enabling the any-to-any entanglement of 20 ion ch…
We report on the fast production and weakly destructive detection of a Fermi gas with tunable interactions in a high finesse cavity. The cavity is used both with far off-resonant light to create a deep optical dipole trap, and with near-resonant light to reach the strong light-matter coupling regime. The cavity-based dipole trap allows for an efficient capture of laser-cooled atoms, and the use of a lattice-cancellation scheme makes it possible to perform efficient intra-cavity evaporative cooling. After transfer in a crossed optical dipole trap, we produce deeply degenerate unitary Fermi gase…
We demonstrate that it is possible, with sub-micron precision, to locate the absolute center of a Fabry-Pérot resonator oriented along the rf-field-free axis of a linear Paul trap through the application of two simultaneously resonating optical fields. In particular, we apply a probe field, which is near-resonant with an electronic transition of trapped ions, simultaneously with an off-resonant strong field acting as a periodic AC Stark-shifting potential. Through the resulting spatially modulated fluorescence signal we can find the cavity center of an 11.7 mm-long symmetric Fabry- Pérot cavit…
We prepare a maximally entangled state of two ions and couple both ions to the mode of an optical cavity. The phase of the entangled state determines the collective interaction of the ions with the cavity mode, that is, whether the emission of a single photon into the cavity is suppressed or enhanced. By adjusting this phase, we tune the ion--cavity system from sub- to superradiance. We then encode a single qubit in the two-ion superradiant state and show that this encoding enhances the transfer of quantum information onto a photon.
We present a novel hybrid system where an optical cavity is integrated with a microfabricated planar-electrode ion trap. The trap electrodes produce a tunable periodic potential allowing the trapping of up to 50 separate ion chains spaced by 160 $μ$m along the cavity axis. Each chain can contain up to 20 individually addressable Yb\textsuperscript{+} ions coupled to the cavity mode. We demonstrate deterministic distribution of ions between the sites of the electrostatic periodic potential and control of the ion-cavity coupling. The measured strength of this coupling should allow access to the …
We propose a scheme for implementation of logical gates in a trapped ion inside a high-Q cavity. The ion is simultaneously interacting with a (classical) laser field as well as with the (quantized) cavity field. We demonstrate that simply by tuning the ionic internal levels with the frequencies of the fields, it is possible to construct a controlled-NOT gate in a three step procedure, having the ion's internal as well as motional levels as qubits. The cavity field is used as an auxiliary qubit and basically remains in the vacuum state.
We investigate the dynamics of a cold trapped ion coupled to the quantized field inside a high-finesse cavity, considering exact resonance between the ionic internal levels and the field (carrier transition). We derive an intensity-dependent hamiltonian in which terms proportional to the square of the Lamb-Dicke parameter ($η$) are retained. We show that different nonclassical effects arise in the dynamics of the ionic population inversion, depending on the initial states of the vibrational motion/field and on the values of $η$.
We propose to build a bad cavity laser using forbidden transitions in large ensembles of cold ions that form a Coulomb crystal in a linear Paul trap. This laser might realize an active optical frequency standard able to serve as a local oscillator in next-generation optical clock schemes. In passive optical clocks, large ensembles of ions appear less promising, as they suffer from inhomogeneous broadening due to quadrupole interactions and micromotion-relates shifts. In bad cavity lasers however, the radiating dipoles can synchronize and generate stable and narrow-linewidth radiation. Furtherm…
We report on our progress in the construction of a continuous matter-wave interferometer for inertial sensing via the non-destructive observation of Bloch oscillations. At the present stage of the experiment, around $10^5$strontium-88 atoms are cooled down to below 1$μ$μK. Pumped by lasers red-tuned with respect to the 7.6 kHz broad intercombination transition of strontium, the two counterpropagating modes of the ring cavity form a one-dimensional optical lattice in which the atoms, accelerated by gravity, will perform Bloch oscillations. The atomic motion can be monitored in real-time via its…
Three orders of magnitude cavity-linewidth narrowing in a rare-earth-ion-doped crystal cavity, induced by strong intra-cavity dispersion caused by off-resonant interaction with dopant ions is demonstrated. The strong dispersion is created by semi-permanent but rapidly reprogrammable changes of the rare earth absorption profiles using optical pumping techniques. Several cavity modes are shown within the spectral transmission window. Potential applications are discussed.
We demonstrate light-induced localization of Coulomb-interacting particles in multi-dimensional structures. Subwavelength localization of ions within small multi-dimensional Coulomb crystals by an intracavity optical standing wave field is evidenced by measuring the difference in scattering inside symmetrically red- and blue-detuned optical lattices and is observed even for ions undergoing substantial radial micromotion. These results are promising steps towards the structural control of ion Coulomb crystals by optical fields as well as for complex many-body simulations with ion crystals or fo…
We propose an approach for studying quantum information and performing high resolution spectroscopy of rotational states of trapped molecular ions using an on-chip superconducting microwave resonator. Molecular ions have several advantages over neutral molecules. Ions can be loaded into deep (1 eV) RF traps and are trapped independent of the electric dipole moment of their rotational transition. Their charge protects them from motional dephasing and prevents collisional loss, allowing 1 s coherence times when used as a quantum memory, with detection of single molecules possible in <10 ms. An a…
We present a simple, robust, narrow-linewidth, frequency-doubled semiconductor laser source suitable for laser cooling and repumping of $^9$Be$^+$ ions. A distributed Bragg reflector (DBR) laser diode operating at 626 nm is self-injection-locked to a frequency doubling cavity via phase-stabilised optical feedback when the laser is resonant with the cavity mode. The short-term laser instability is reduced from the MHz-level to approximately 20 kHz by the injection process, thus eliminating the need for a high-bandwidth feedback loop to suppress the otherwise troublesome high-frequency laser noi…
We analyze the dynamics of a chain of singly-charged ions confined in a linear Paul trap and which couple with the mode of a high-finesse optical resonator. In these settings the ions interact via the Coulomb repulsion and are subject to the mechanical forces due to scattering of cavity photons. We show that the interplay of these interactions can give rise to bistable equilibrium configurations, into which the chain can be cooled by cavity-enhanced photon scattering. We characterize the resulting equilibrium structures by determining the stationary state in the semiclassical limit for both ca…
In this work we realize a narrow spectroscopic feature using a technique that we refer to as magnetically-induced optical transparency. A cold ensemble of $^{88}$Sr atoms interacts with a single mode of a high-finesse optical cavity via the 7.5kHz linewidth, spin forbidden $^1$S$_0$ to $^3$P$_1$ transition. By applying a magnetic field that shifts two excited state Zeeman levels, we open a transmission window through the cavity where the collective vacuum Rabi splitting due to a single level would create destructive interference for probe transmission. The spectroscopic feature approaches the …
Programmable cavity QED with a fiber-integrated atomic array
Institute of Science and Technology Austria (ISTA)（奥地利科学技术研究院）；Vienna Center for Quantum Science and Technology, Atominstitut, TU Wien（维也纳量子科学与技术中心，原子物理研究所，维也纳工业大学）
Quantum-logic techniques for state preparation, manipulation, and non-destructive interrogation are increasingly being adopted for experiments on single molecular ions confined in traps. The ability to control molecular ions on the quantum level via a co-trapped atomic ion offers intriguing possibilities for new experiments in the realms of precision spectroscopy, quantum information processing, cold chemistry, and quantum technologies with molecules. The present article gives an overview of the basic experimental methods, recent developments and prospects in this field.
Precision optical spectroscopy of exotic ions reveals accurate information about nuclear properties such as charge radii and magnetic and quadrupole moments. Thorium ions exhibit unique nuclear properties with high relevance for testing symmetries of nature. We report loading and trapping of single $^{232}$Th$^+$ ions in a linear Paul trap, embedded into and sympathetically cooled by small crystals of trapped $^{40}$Ca$^+$ ions. Trapped Th ions are identified in a non-destructive manner from the voids in the laser-induced Ca fluorescence pattern emitted by the crystal, and alternatively, by me…
Ensembles of solid-state optical emitters enable broadband quantum storage and transduction of photonic qubits, with applications in high-rate optical quantum networks for secure communications, global time-keeping, and interconnecting future quantum computers. To realize coherent quantum information transfer using ensembles, spin rephasing techniques are currently used to mitigate fast decoherence resulting from inhomogeneous broadening. Here we use a dense ensemble of neodymium rare-earth ions strongly coupled to a nanophotonic resonator to demonstrate that decoherence of a single photon exc…
We evaluate the feasibility of the implementation of two quantum repeater protocols with an existing experimental platform based on a $^{40}$Ca$^+$-ion in a segmented micro trap, and a third one that requires small changes to the platform. A fiber cavity serves as an ion-light interface. Its small mode volume allows for a large coupling strength of $g_c = 2 π20$ MHz despite comparatively large losses $κ= 2 π36.6$ MHz. With a fiber diameter of 125 mu m, the cavity is integrated into the microstructured ion trap, which in turn is used to transport single ions in and out of the interaction zone i…
We present the realization of a combined trapped-ion and optical cavity system, in which a single Yb^+ ion is confined by a micron-scale ion trap inside a 230 mum-long optical fiber cavity. We characterize the spatial ion-cavity coupling and measure the ion-cavity coupling strength using a cavity-stimulated Lambda-transition. Owing to the small mode volume of the fiber resonator, the coherent coupling strength between the ion and a single photon exceeds the natural decay rate of the dipole moment. This system can be integrated into ion-photon quantum networks and is a step towards cavity quant…
We demonstrate a spatial-imaging thermometry technique for ions in a one-dimensional Coulomb crystal by relating their imaged spatial extent along the linear radiofrequency ion trap axis to normal modes of vibration of coupled oscillators in a harmonic potential. We also use the thermal spatial spread of bright ions in the case of a two-species mixed chain to measure the center-of-mass (COM) resonance frequency of the entire chain and infer the molecular composition of the co-trapped dark ions. These non-destructive techniques create new possibilities for better understanding of sympathetic co…
The hyperfine structure of the ground state of erbium doped yttrium orthosilicate is analyzed with the use of electron paramagnetic resonance experiments in a tunable microwave resonator. This work was prompted by the disagreement between the measurements made in zero magnetic field [Phys. Rev. B, 94, 075117, (2016)] and a previously published spin Hamiltonian, which is derived from standard EPR measurements at 9.5 GHz [Phys. Rev. B, 74, 214409, (2006)]. The ability to vary magnetic field strength, resonator frequency, and the orientation of our sample enabled us to monitor how the frequencies…
Incorporating optical cavities in ion traps is becoming increasingly important in the development of photonic quantum networks. However, the presence of the cavity can hamper efficient laser cooling of ions because of geometric constraints that the cavity imposes and an unfavourable Purcell effect that can modify the cooling dynamics substantially. On the other hand the coupling of the ion to the cavity can also be exploited to provide a mechanism to efficiently cool the ion. In this paper we demonstrate experimentally how cavity cooling can be implemented to improve the localisation of the io…
We propose and demonstrate real-time sub-wavelength cavity QED measurements of the spatial distribution of atoms in an optical lattice. Atoms initially confined in one "trap" standing wave of an optical cavity mode are probed with a second "probe" standing wave. With frequencies offset by one free spectral range, the nodes of the trap fall on the anti-nodes of the probe in the ${\approx}$10$^4$ lattice sites around the center of the cavity. This lattice site independent atom-cavity coupling enables high sensitivity detection of atom dynamics even with atoms spread over many lattice sites. To d…
We demonstrate a new method of light phase shift measurement using a high-finesse optical ring cavity which exhibits reduced phase noise due to cavity length fluctuations. Two laser beams with a frequency difference of one cavity free spectral range are simultaneously resonant with the cavity, demonstrating noise correlations in the error signals due to the common-mode cavity length fluctuations. The differential error signal shows a 30 dB reduction in cavity noise down to the noise floor in a frequency range up to half the cavity linewidth ($δν/2 \simeq 30$ kHz). Various noise sources are ana…
