We present a wave atom optics theory of the Collective Atomic-Recoil Laser, where the atomic center-of-mass motion is treated quantum mechanically. It extends the previous ray atom optics theory, which treated the center-of-mass atomic motion classically, to the realm of ultracold atoms. For the case of a far off resonant pump laser we derive an analytical solution which gives the linear response of the CARL system for both the quantum and classical regimes. A linear stability analysis reveals significant qualitative differences between these two regimes, which arise from the effects of diffraction on the atomic center-of-mass motion.
The recoil of atoms in arrays due to the emission or absorption of photons is studied for sub-wavelength interatomic spacing. The atoms in the array interact with each other through collective dipole-dipole interactions and with the incident laser field in the low intensity limit. Shining uniform light on the array gives rise to patterns of excitation and recoil in the array. These arise due to the interference of different eigenmodes of excitation. The relation between the recoil and the decay dynamics is studied when the array is in its excitation eigenstates. The recoil experienced by a sub…
We demonstrate clear collective atomic recoil motion in a dilute, momentum-squeezed, ultra-cold degenerate fermion gas by circumventing the effects of Pauli blocking. Although gain from bosonic stimulation is necessarily absent because the quantum gas obeys Fermi-Dirac statistics, collective atomic recoil motion from the underlying wave-mixing process is clearly visible. With a single pump pulse of the proper polarization, we observe two mutually-perpendicular wave-mixing processes occurring simultaneously. Our experiments also indicate that the red-blue pump detuning asymmetry observed with B…
Self-organization effects related to light amplification in the collective atomic recoil laser system with the driven atoms confined in a harmonic trap are investigated further. In the dispersive parametric region, our study reveals that the spontaneously formed structures in the phase space contributes an important role to the light amplification of the probe field under the atomic motion being modified by the trap.
We observe the buildup of a frequency-shifted reverse light field in a unidirectionally pumped high-$Q$ optical ring cavity serving as a dipole trap for cold atoms. This effect is enhanced and a steady state is reached, if via an optical molasses an additional friction force is applied to the atoms. We observe the displacement of the atoms accelerated by momentum transfer in the backscattering process and interpret our observations in terms of the collective atomic recoil laser. Numerical simulations are in good agreement with the experimental results.
We formulate a wave atom optics theory of the Collective Atomic Recoil Laser, where the atomic center-of-mass motion is treated quantum mechanically. By comparing the predictions of this theory with those of the ray atom optics theory, which treats the center-of-mass motion classically, we show that for the case of a far off-resonant pump laser the ray optics model fails to predict the linear response of the CARL when the temperature is of the order of the recoil temperature or less. This is due to the fact that in theis temperature regime one can no longer ignore the effects of matter-wave di…
We demonstrate optical nonlinearities due to the interaction of weak optical fields with the collective motion of a strongly dispersive ultracold gas. The combination of a recoil-induced resonance (RIR) in the high gain regime and optical waveguiding within the dispersive medium enables us to achieve a collective atomic cooperativity of $275 \pm 50$ even in the absence of a cavity. As a result, we observe optical bistability at input powers as low as 20 pW. The present scheme allows for dynamic optical control of the dispersive properties of the ultracold gas using very weak pulses of light. T…
We consider the effects of the trap environment on the atomic and optical quantum statistical properties and on the atom-photon correlations in the Collective Atomic-Recoil Laser. Atomic and optical statistical properties, as well as the atom-photon correlations are dependent on the optical field intensity and phase. In particular, depending on the values of the optical field intensity and phase, the fields statistics varies from coherent to superchaotic.
We extend the Collective Atomic Recoil Lasing (CARL) model including the effects of friction and diffusion forces acting on the atoms due to the presence of optical molasses fields. The results from this model are consistent with those from a recent experiment by Kruse et al. [Phys. Rev. Lett. 91, 183601 (2003)]. In particular, we obtain a threshold condition above which collective backscattering occurs. Using a nonlinear analysis we show that the backscattered field and the bunching evolve to a steady-state, in contrast to the non-stationary behaviour of the standard CARL model. For a proper …
Free Electron Laser (FEL) and Collective Atomic Recoil Laser (CARL) are described by the same model of classical equations for properly defined scaled variables. These equations are extended to the quantum domain describing the particle's motion by a Schrödinger equation coupled to a self-consistent radiation field. The model depends on a single collective parameter $\bar ρ$ which represents the maximum number of photons emitted per particle. We demonstrate that the classical model is recovered in the limit $\bar ρ\gg 1$, in which the Wigner function associated to the Schrödinger equation obey…
Networks of globally coupled oscillators exhibit phase transitions from incoherent to coherent states. Atoms interacting with the counterpropagating modes of a unidirectionally pumped high-finesse ring cavity form such a globally coupled network. The coupling mechanism is provided by collective atomic recoil lasing (CARL), i.e. cooperative Bragg scattering of laser light at an atomic density grating, which is self-induced by the laser light. Under the rule of an additional friction force, the atomic ensemble is expected to undergo a phase transition to a state of synchronized atomic motion. We…
We study a system represented by a Bose-Einstein condensate interacting with a cavity field in presence of a strong off-resonant pumping laser. This system can be described by a three-mode Gaussian state, where two are the atomic modes corresponding to atoms populating upper and lower momentum sidebands and the third mode describes the scattered cavity field light. We show that, as a consequence of the collective atomic recoil instability, these modes possess a genuine tripartite entanglement that increases unboundedly with the evolution time and is larger than the bipartite entanglement in an…
We propose an experiment to realize radiation to atom continuous variable quantum mapping, i.e. to teleport the quantum state of a single mode radiation field onto the collective state of atoms with a given momentum out of a Bose-Einstein condensate. The atoms-radiation entanglement needed for the teleportation protocol is established through the interaction of a single mode with the condensate in presence of a strong far off-resonant pump laser, whereas the coherent atomic displacement is obtained by the same interaction with the radiation in a classical coherent field. In principle, verifica…
We describe a method for non-degenerate four-wave mixing in a cold sample of 4-level atoms. An integral part of the four-wave mixing process is a collective instability which spontaneously generates a periodic density modulation in the cold atomic sample with a period equal to half of the wavelength of the generated high-frequency optical field. Due to the generation of this density modulation, phase-matching between the pump and scattered fields is not a necessary initial condition for this wave-mixing process to occur, rather the density modulation acts to "self phase-match" the fields durin…
We address the dynamics induced by collective atomic recoil in a Bose-Einstein condensate in presence of radiation losses and atomic decoherence. In particular, we focus on the linear regime of the lasing mechanism, and analyze the effects of losses and decoherence on the generation of entanglement. The dynamics is that of three bosons, two atomic modes interacting with a single-mode radiation field, coupled with a bath of oscillators. The resulting three-mode dissipative Master equation is solved analytically in terms of the Wigner function. We examine in details the two complementary limits …
An analytical perturbation theory of short-pulse, matter-wave superradiant scatterings is presented. We show that Bragg resonant enhancement is incapacitated and both positive and negative order scatterings contribute equally. We further show that propagation gain is small and scattering events primarily occur at the end of the condensate where the generated field has maximum strength, thereby explaining the apparent ``asymmetry" in the scattered components with respect to the condensate center. In addition, the generated field travels near the speed of light in a vacuum, resulting in signific…
We experimentally investigate the formation of subradiant atomic momentum states in Bose-Einstein condensates inside a recoil resolving optical ring resonator according to the theoretical proposal of Cola, Bigerni, and Piovella. The atoms are pumped from the side with laser light that contains two frequency components. They resonantly drive cavity assisted Raman transitions between three discreet atomic momentum states. Within a few hundred microseconds, the system evolves into a stationary subradiant state. In this state, the condensate develops two density gratings suitable to diffract the t…
The recoil effects of spontaneous photon emissions during optical pumping of a trapped three-level atom are exactly calculated. Without resort to the Lamb-Dicke approximation, and considering arbitrary detuning and saturation of the pump laser, the density of recoil shifts in phase space is derived. It is shown that this density is not of Gaussian shape, and that it becomes isotropic in phase space only for a branching ratio corresponding to fluorescence scattering but unfavorable for optical pumping. The dependence of its anisotropy on the laser saturation is discussed in the resonant case, a…
We report on the storage of light via the phenomenon of recoil-induced resonance in a pure two- level system of cold cesium atoms. We use a strong coupling beam and a weak probe beam to couple different external momentum states of the cesium atom via two-photon Raman interaction which leads to the storage of the optical information of the probe beam. We have also measured the probe transmission spectrum, as well as the light storage spectrum which reveals very narrow subnatural resonance features showing absorption and gain. We have demonstrated that this memory presents the unique property of…
A mean field theory for Raman superradiance (SR) with recoil is presented, where the typical SR signatures are recovered, such as quadratic dependence of the intensity on the number of atoms and inverse proportionality of the time scale to the number of atoms. A comparison with recent experiments and theories on Rayleigh SR and collective atomic recoil lasing (CARL) are included. The role of recoil is shown to be in the decay of atomic coherence and breaking of the symmetry of the SR end-fire modes.
We directly measure the quantized collective motion of a gas of thousands of ultracold atoms, coupled to light in a high-finesse optical cavity. We detect strong asymmetries, as high as 3:1, in the intensity of light scattered into low- and high-energy motional sidebands. Owing to high cavity-atom cooperativity, the optical output of the cavity contains a spectroscopic record of the energy exchanged between light and motion, directly quantifying the heat deposited by a quantum position measurement's backaction. Such backaction selectively causes the phonon occupation of the observed collective…
A superfluid atomic gas is prepared inside an optical resonator with an ultra-narrow band width on the order of the single photon recoil energy. When a monochromatic off-resonant laser beam irradiates the atoms, above a critical intensity the cavity emits superradiant light pulses with a duration on the order of its photon storage time. The atoms are collectively scattered into coherent superpositions of discrete momentum states, which can be precisely controlled by adjusting the cavity resonance frequency. With appropriate pulse sequences the entire atomic sample can be collectively accelerat…
The collective dynamics of mobile scatterers and light in optical resonators generates complex behaviour. For strong transverse illumination a phase transition from homogeneous to crystalline particle order appears. In contrast, a gas inside a single-side pumped ring cavity exhibits an instability towards bunching and collective acceleration called collective atomic recoil lasing (CARL). We demonstrate that by driving two orthogonally polarized counter propagating modes of a ring resonator one realises both cases within one system. The corresponding phase diagram depending on the two pump inte…
We use an optically dense, anisotropic magneto-optical trap to study recoil-induced resonances (RIRs) in the transient, high-gain regime. We find that two distinct mechanisms govern the atomic dynamics: the finite, frequency-dependent atomic response time, and momentum-space population redistribution. At low input probe intensities, the residual Doppler width of the atoms, combined with the finite atomic response time, result in a linear, transient hysteretic effect that modifies the locations, widths, and magnitudes of the resulting gain spectra depending on the sign of the scan chirp. When l…
We derive a markovian master equation for the internal dynamics of an ensemble of two-level atoms including all effects related to the quantization of their motion. Our equation provides a unifying picture of the consequences of recoil and indistinguishability of atoms beyond the Lamb-Dicke regime on both their dissipative and conservative dynamics, and applies equally well to distinguishable and indistinguishable atoms. We give general expressions for the decay rates and the dipole-dipole shifts for any motional states, and we find closed-form formulas for a number of relevant states (Gaussia…
Ultracold atoms interacting with the optical modes of a high-Q optical ring cavity can synchronize their motion. The collective behavior makes the system interesting for quantum computing applications. This paper is devoted to the study of the collective coupling. We report on the first observation of a collective dynamics and on the realization of a laser, the gain mechanism of which is based on collective atomic recoil. We show that, if the atoms are subject to a friction force, starting from an unordered distribution they spontaneously form a moving density grating. Furthermore, we demonstr…
We derive the quantum-mechanical master equation (generalized optical Bloch equation) for an atom in the vicinity of a flat dielectric surface. This equation gives access to the semiclassical radiation pressure force and the atomic momentum diffusion tensor, that are expressed in terms of the vacuum field correlation function (electromagnetic field susceptibility). It is demonstrated that the atomic center-of-mass motion provides a nonlocal probe of the electromagnetic vacuum fluctuations. We show in particular that in a circularly polarized evanescent wave, the radiation pressure force experi…
We observe vacuum Rabi splitting in a lossy nearly confocal cavity indicating the strong coupling regime, despite a weak single-atom single-mode coupling. Strong collective interaction manifests itself in the typical $\sqrt{N}$-dependence of the normal mode splitting on the number of atoms $N$. The $TEM_{00}$-mode coupling parameters are $(g,κ,γ)=2π\times(0.12,0.8,2.6)$ MHz and up to $(1.33\pm 0.08)\times10^5$ cesium atoms were loaded into the mode volume.
Using collective atom phase control a population inversion-free photon echo scheme has been studied for quantum memory applications. For the inversion-free photon echoes a double rephasing method is combined with optical locking, where the optical locking coherently controls each atom phase excited by weak data pulses. As a result, intensity flattened, normally ordered, storage time-extended, and noise-free photon echoes are obtained.
We report on Kerr nonlinearity and dispersive optical bistability of a Fabry-Perot optical resonator due to the displacement of ultracold atoms trapped within. In the driven resonator, such collective motion is induced by optical forces acting upon up to $10^5$ $^{87}$Rb atoms prepared in the lowest band of a one-dimensional intracavity optical lattice. The longevity of atomic motional coherence allows for strongly nonlinear optics at extremely low cavity photon numbers, as demonstrated by the observation of both branches of optical bistability at photon numbers below unity.
We present a theory of recoil effects in two zone Ramsey spectroscopy, particularly adapted to microwave frequency standards using laser cooled atoms. We describe the atoms by a statistical distribution of Gaussian wave packets which enables us to derive and quantify effects that are related to the coherence properties of the atomic source and that have not been considered previously. We show that, depending on the experimental conditions, the expected recoil frequency shift can be partially cancelled by these effects which can be significant at microwave wavelengths whilst negligible at optic…
In this work we perform a detailed theoretical and experimental investigation of an atomic memory based on recoil-induced resonance in cold cesium atoms. We consider the interaction of a nearly degenerated pump and probe beams with an ensemble of two-level atoms. A full theoretical density matrix calculation in the extended Hilbert space of the internal and external atomic degrees of freedom allows us to obtain, from first principles, the transient and stationary responses determining the probe transmission and the forward four-wave mixing spectra. These two signals are generated together at t…
We report on the observation of collective atomic recoil lasing and superradiant Rayleigh scattering with ultracold and Bose-Einstein condensed atoms in an optical ring cavity. Both phenomena are based on instabilities evoked by the collective interaction of light with cold atomic gases. This publication clarifies the link between the two effects. The observation of superradiant behavior with thermal clouds as hot as several tens of $μ\textrm{K}$ proves that the phenomena are driven by the cooperative dynamics of the atoms, which is strongly enhanced by the presence of the ring cavity.
Collective interaction of light with an atomic gas can give rise to superradiant instabilities. We experimentally study the sudden build-up of a reverse light field in a laser-driven high-finesse ring cavity filled with ultracold thermal or condensed atoms. While superradiant Rayleigh scattering from atomic clouds is normally only observed at very low temperatures (i.e. well below $1 μ$K), the presence of the ring cavity enhances cooperativity and allows for superradiance with thermal clouds as hot as several $10 μ$K. A characterization of the superradiance at various temperatures and cooperat…
We study photoionization of cold rubidium atoms in a strong infrared laser field using a magneto-optical trap (MOT) recoil ion momentum spectrometer. Three types of cold rubidium target are provided, operating in two-dimension (2D) MOT, 2D molasses, and 3D MOT with densities in the orders of $10^7$ atoms/cm$^3$, $10^8$ atoms/cm$^3$, and $10^9$ atoms/cm$^3$, respectively. The density profile and the temperature of 3D MOT are characterized using the absorption imaging and photoionization. The momentum distributions of Rb$^+$ created by absorption of two- or three-photon illuminate a dipole-like …
We explore how to cool atomic collective excitations in an optically-driven three-level atomic ensemble, which may be described by a model of coupled two harmonic oscillators (HOs) with a time-dependent coupling. Moreover, the coupled two-HO model is further generalized to address other cooling issues, where the lower-frequency HO can be cooled whenever the cooling process dominates over the heating one during the sideband transitions. Unusually, due to the absence of the heating process, the optimal cooling of our first cooling protocol for collective excitations in an atomic ensemble could b…
We report on collective non-linear dynamics in an optical lattice formed inside a high finesse ring cavity in a so far unexplored regime, where the light shift per photon times the number of trapped atoms exceeds the cavity resonance linewidth. We observe bistability and self-induced squeezing oscillations resulting from the retro-action of the atoms upon the optical potential wells. We can well understand most of our observations within a simplified model assuming adiabaticity of the atomic motion. Non-adiabatic aspects of the atomic motion are reproduced by solving the complete system of cou…
We propose a search for low mass dark matter particles through momentum recoils caused by their scattering from trapped, nm-scale objects. Our projections show that even with a modest array of fg-mass sensors, parameter-space beyond the reach of existing experiments can be explored. The case of smaller, ag-mass sensors is also analyzed - where dark matter can coherently scatter from the entire sensor - enabling a large enhancement in the scattering cross-section relative to interactions with single nuclei. Large arrays of such sensors have the potential to explore new parameter space down to d…
The minimum requirements for entanglement detection are discussed for a spin chain in which the spins cannot be individually accessed. The methods presented detect entangled states close to a cluster state and a many-body singlet state, and seem to be viable for experimental realization in optical lattices of two-state bosonic atoms. The entanglement criteria are based on entanglement witnesses and on the uncertainty of collective observables.
We report the observation of collective-emission-induced, velocity-dependent light forces. One third of a falling sample containing 3 x 10^6 cesium atoms illuminated by a horizontal standing wave is stopped by cooperatively emitting light into a vertically oriented confocal resonator. We observe decelerations up to 1500 m/s^2 and cooling to temperatures as low as 7 uK, well below the free space Doppler limit. The measured forces substantially exceed those predicted for a single two-level atom.
Resonant dipole-dipole interaction modifies the energy and decay rate of electronic excitations for finite one dimensional chains of ultracold atoms in an optical lattice. We show that collective excited states of the atomic chain can be divided into dark and bright modes, where a superradiant mode with an enhanced collective effective dipole dominates the optical scattering. Studying the generic case of two chain segments of different length and position exhibits an interaction blockade and spatially structured light emission. Ultimately, an extended system of several interfering segments mod…
We calculate radiative lifetimes of collective electronic excitations of atoms in an infinite one dimensional lattice. The translational symmetry along the lattice restricts the photon wave vector component parallel to the lattice to the exciton wave number and thus the possible emission directions. The resulting radiation damping rate and emission pattern of the exciton strongly deviates from independent atom. For some wave numbers and polarizations the excitons superradiantly decay very fast, while other excitons show zero radiation damping rate and form propagating meta-stable excitations. …
We explore quantum many-body physics of a driven Bose-Einstein condensate in optical lattices. The laser field induces a gap in the generalized Bogoliubov spectrum proportional to the effective Rabi frequency. The lowest lying modes in a driven condensate are characterized by zero group velocity and non-zero current. Thus, the laser field induces roton modes, which carry interaction in a driven condensate. We show that collective excitations below the energy of the laser-induced gap remain undamped, while above the gap they are characterized by a significantly suppressed Landau damping rate.
The two-particle wave function of neutrino and recoil nucleus is found as a solution of an initial value problem in the far zone for a time longer than the electron capture decay lifetime of a hydrogenlike ion. The neutrino-recoil entanglement arising in such a process is a consequence of the momentum conservation and is closely related to the wave packet structure of the state. Because of neutrino mixing, the joint wave packet involves the coherent superposition of the neutrino mass eigenstate packets. This is the new physical realization of the Einstein-Podolsky-Rosen thought experiment, whi…
