A systematic perturbation scheme is developed for approximate solutions to the time-dependent Schroedinger equation with a space-adiabatic Hamiltonian. For a particular isolated energy band, the basic approach is to separate kinematics from dynamics. The kinematics is defined through a subspace of the full Hilbert space for which transitions to other band subspaces are suppressed to all orders and the dynamics operates in that subspace in terms of an effective intraband Hamiltonian. As novel applications we discuss the Born-Oppenheimer theory to second order and derive the nonperturbative definition of the g-factor of the electron within nonrelativistic quantum electrodynamics.
We introduce high-order dynamical decoupling strategies for open system adiabatic quantum computation. Our numerical results demonstrate that a judicious choice of high-order dynamical decoupling method, in conjunction with an encoding which allows computation to proceed alongside decoupling, can dramatically enhance the fidelity of adiabatic quantum computation in spite of decoherence.
The use of the nuclear spins surrounding electron spin qubits as quantum registers and long-lived memories opens the way to new applications in quantum information and biological sensing. Hence, there is a need for generic and robust forms of control of the nuclear registers. Although adiabatic gates are widely used in quantum information, they can become too slow to outpace decoherence. Here, we introduce a technique whereby adiabatic gates arise from the dynamical decoupling protocols that simultaneously extend coherence. We illustrate this pulse-based adiabatic control for nuclear spins aro…
In the quantum-computation scenario, geometric phase-gates are becoming increasingly attractive for their intrinsic fault tolerance to disturbance. With an adiabatic cyclic evolution, Berry phase appears to realize a geometric transformation. Performing the quantum gates as many as possible within the timescale of coherence, however, remains an inconvenient bottleneck due to the systematic errors. Here we propose an accelerated adiabatic quantum gate based on the Berry phase, the transitionless driving, and the dynamical decoupling. It reconciles a high fidelity with a high speed in the presen…
The high fidelity generation of strongly entangled states of many particles, such as cat states, is a particularly demanding challenge. One approach is to drive the system, within a certain final time, as adiabatically as possible, in order to avoid the generation of unwanted excitations. However, excitations can be generated also by the presence of dissipative effects such as dephasing. Here we compare the effectiveness of Local Adiabatic and the FAst QUasi ADiabatic protocols in achieving a high fidelity for a target superposition state both with and without dephasing. In particular we consi…
Quantum dynamical decoupling is a procedure to cancel the effective coupling between two systems by applying sequences of fast actuations, under which the coupling Hamiltonian averages out to leading order(s). One of its prominent uses is to drive a target system in such a way as to decouple it from a less protected one. The present manuscript investigates the dual strategy: acting on a noisy "environment" subsystem such as to decouple it from a target system. The potential advantages are that actions on the environment commute with system operations, and that imprecisions in the decoupling ac…
The Uhrig dynamical decoupling sequence achieves high-order decoupling of a single system qubit from its dephasing bath through the use of bang-bang Pauli pulses at appropriately timed intervals. High-order decoupling of single and multiple qubit systems from baths causing both dephasing and relaxation can also be achieved through the nested application of Uhrig sequences, again using single-qubit Pauli pulses. For the 3-qubit decoherence free subsystem (DFS) and related subsystem encodings, Pauli pulses are not naturally available operations; instead, exchange interactions provide all require…
We introduce universally robust sequences for dynamical decoupling, which simultaneously compensate pulse imperfections and the detrimental effect of a dephasing environment to an arbitrary order, work with any pulse shape, and improve performance for any initial condition. Moreover, the number of pulses in a sequence grows only linearly with the order of error compensation. Our sequences outperform the state-of-the-art robust sequences for dynamical decoupling. Beyond the theoretical proposal, we also present convincing experimental data for dynamical decoupling of atomic coherences in a soli…
We develop a hierarchical functional derivative method to investigate the reduced dynamics of a quantum dissipative system within the framework of a stochastic decoupling description. Keeping only the lowest order truncation of the hierarchical functional derivatives, one can recover the second order Nakajima-Zwanzig quantum master equation. Taking into account the higher-order corrections, our method can be implemented as a highly efficient numerical scheme for a general quantum dissipative system beyond the usual Markovian, rotating-wave, and weak-coupling approximations.
Dynamical decoupling (DD) sequences were invented to eliminate the direct coupling between qubit and its environment. We further investigate the possibility of decoupling the indirect qubit-qubit interaction induced by a common environment, and sucessfully find simplified solutions that preserve the bipartite quantum states to arbitrary order. Through analyzing the exact dynamics of the controlled two-qubit density matrix, we have proven that applying independent Uhrig Dynamical Decoupling (UDD) on each qubit will effectively eliminate both the qubit- environment and indirect qubit-qubit coupl…
We show that the physical mechanism of population transfer in a 3-level system with a closed loop of coherent couplings (loop-STIRAP) is not equivalent to an adiabatic rotation of the dark-state of the Hamiltonian but coresponds to a rotation of a higher-order trapping state in a generalized adiabatic basis. The concept of generalized adiabatic basis sets is used as a constructive tool to design pulse sequences for stimulated Raman adiabatic passage (STIRAP) which give maximum population transfer also under conditions when the usual condition of adiabaticty is only poorly fulfilled. Under cert…
We study the performance of dynamical decoupling in suppressing decoherence caused by soft-cutoff Gaussian noise, using short-time expansion of the noise correlations and numerical optimization. For the noise with soft cutoff at high frequencies, there exists no dynamical decoupling scheme to eliminate the decoherence to arbitrary orders of the short time, regardless of the timing or pulse shaping of the control under the population conserving condition. We formulate the equations for optimizing pulse sequences that minimizes decoherence up to the highest possible order of the short time for t…
In this paper we present an invariant perturbation theory to adiabatic process according to the concepts of adiabatic orbits, adiabatic evolution orbit and U(1)-invariant adiabatic orbit. The probabilities of keeping the adiabatic orbit in the first-order and the second-order approximation are calculated, respectively. We also give a convenient sufficient condition.
Quantum adiabatic evolution is a dynamical evolution of a quantum system under slow external driving. According to the quantum adiabatic theorem, no transitions occur between non-degenerate instantaneous eigen-energy levels in such a dynamical evolution. However, this is true only when the driving rate is infinitesimally small. For a small nonzero driving rate, there are generally small transition probabilities between the energy levels. We develop a classical mechanics framework to address the small deviations from the quantum adiabatic theorem order by order. A hierarchy of Hamiltonians are …
In the continuum limit (large number of qubits), adiabatic quantum algorithms display a remarkable similarity to sweeps through quantum phase transitions. We find that transitions of second or higher order are advantageous in comparison to those of first order. With this insight, we propose a novel adiabatic quantum algorithm for the solution of 3-satisfiability (3-SAT) problems (exact cover), which is significantly faster than previous proposals according to numerical simulations (up to 20 qubits). These findings suggest that adiabatic quantum algorithms can solve NP-complete problems such as…
We present a novel continuous dynamical decoupling scheme for the construction of a robust qubit in a three-level system. By means of a clock transition adjustment, we first show how robustness to environmental noise is achieved, while eliminating drive-noise, to first-order. We demonstrate this scheme with the spin sub-levels of the NV-centre's electronic ground state. By applying drive fields with moderate Rabi frequencies, the drive noise is eliminated and an improvement of 2 orders of magnitude in the coherence time is obtained compared to the pure dephasing time. We then show how the cloc…
When a composite Lindblad system consists of weakly coupled sub-systems with fast and slow timescales, the description of slow dynamics can be simplified by discarding fast degrees of freedom. This model reduction technique is called adiabatic elimination. While second-order perturbative expansion with respect to the timescale separation has revealed that the evolution of a reduced state is completely positive, this paper presents an example exhibiting complete positivity violation in the fourth-order expansion. Despite the non-uniqueness of slow dynamics parametrization, we prove that complet…
Dynamical decoupling can be used to preserve arbitrary quantum states despite undesired interactions with the environment, using control Hamiltonians affecting the system only. We present a system-independent analysis of dynamical decoupling based on leading order decoupling error estimates, valid for bounded-strength environments. Using as a key tool a renormalization transformation of the effective system-bath coupling Hamiltonian, we delineate the reliability domain of dynamical decoupling used for quantum state preservation, in a general setting for a single qubit. We specifically analyze …
Adiabatic elimination is a perturbative model reduction technique based on timescale separation and often used to simplify the description of composite quantum systems. We here analyze a quantum experiment where the perturbative expansion can be carried out to arbitrary order, such that: (i) we can formulate in the end an exact reduced model in quantum form; (ii) as the series provides accuracy for ever larger parameter values, we can discard any condition on the timescale separation, thereby analyzing the intermediate regime where the actual experiment is performing best; (iii) we can clarify…
We demonstrate the use of dynamic decoupling techniques to extend the coherence time of a single memory qubit by nearly two orders of magnitude. By extending the Hahn spin-echo technique to correct for unknown, arbitrary polynomial variations in the qubit precession frequency, we show analytically that the required sequence of pi-pulses is identical to the Uhrig dynamic decoupling (UDD) sequence. We compare UDD and CPMG sequences applied to a single Ca-43 trapped-ion qubit and find that they afford comparable protection in our ambient noise environment.
The task of decoupling, i.e., removing unwanted interactions in a system Hamiltonian and/or couplings with an environment (decoherence), plays an important role in controlling quantum systems. There are many efficient decoupling schemes based on combinatorial concepts like orthogonal arrays, difference schemes and Hadamard matrices. So far these (combinatorial) decoupling schemes have relied on the ability to effect sequences of instantaneous, arbitrarily strong control Hamiltonians (bang-bang controls). To overcome the shortcomings of bang-bang control Viola and Knill proposed a method called…
Based on a theorem we establish on dynamical decoupling of time-dependent systems, we present a scheme of nested Uhrig dynamical decoupling (NUDD) to protect multi-qubit systems in generic quantum baths to arbitrary decoupling orders, using only single-qubit operations. The number of control pulses in NUDD increases polynomially with the decoupling order. For general multi-level systems, this scheme can preserve a set of unitary Hermitian system operators which mutually either commute or anti-commute, and hence all operators in the Lie algebra generated from this set of operators, generating a…
Topological orders are exotic phases of matter existing in strongly correlated quantum systems, which are beyond the usual symmetry description and cannot be distinguished by local order parameters. Here we report an experimental quantum simulation of the Wen-plaquette spin model with different topological orders in a nuclear magnetic resonance system, and observe the adiabatic transition between two $Z_2$ topological orders through a spin-polarized phase by measuring the nonlocal closed-string (Wilson loop) operator. Moreover, we also measure the entanglement properties of the topological ord…
We examine both quantum and classical versions of the problem of spin evolution in a slowly varying magnetic field. Main attention is given to the first- and second-order adiabatic corrections in the case of in-plane variations of the magnetic field. While the first-order correction relates to the adiabatic Berry phase and Coriolis-type lateral deflection of the spin, the second-order correction is shown to be responsible for the next-order geometric phase and in-plain deflection. A comparison between different approaches, including the exact (non-adiabatic) geometric phase, is presented.
Topological order characterizes those phases of matter that defy a description in terms of symmetry and cannot be distinguished in terms local order parameters. This type of order plays a key role in the theory of the fractional quantum Hall effect, as well as in topological quantum information processing. Here we show that a system of n spins forming a lattice on a Riemann surface can undergo a second order quantum phase transition between a spin-polarized phase and a string-net condensed phase. This is an example of a phase transition between magnetic and topological order. We furthermore sh…
Nested Uhrig dynamical decoupling (NUDD) is a highly efficient quantum error suppression scheme that builds on optimized single axis UDD sequences. We prove the universality of NUDD and analyze its suppression of different error types in the setting of generalized control pulses. We present an explicit lower bound for the decoupling order of each error type, which we relate to the sequence orders of the nested UDD layers. We find that the error suppression capabilities of NUDD are strongly dependent on the parities and relative magnitudes of all nested UDD sequence orders. This allows us to pr…
Topological orders are a class of exotic states of matter characterized by patterns of long-range entanglement. Certain topologically ordered systems are proposed as potential realization of fault-tolerant quantum computation. Topological orders can arise in two-dimensional spin-lattice models. In this paper, we engineer a time-dependent Hamiltonian to prepare a topologically ordered state through adiabatic evolution. The other sectors in the degenerate ground-state space of the model are obtained by applying nontrivial operations corresponding to closed string operators. Each sector is highly…
We simulate the quantum adiabatic algorithm (QAA) for the exact cover problem for sizes up to N=256 using quantum Monte Carlo simulations incorporating parallel tempering. At large N we find that some instances have a discontinuous (first order) quantum phase transition during the evolution of the QAA. This fraction increases with increasing N and may tend to 1 for N -> infinity.
We construct efficient deterministic dynamical decoupling schemes protecting continuous variable degrees of freedom. Our schemes target decoherence induced by quadratic system-bath interactions with analytic time-dependence. We show how to suppress such interactions to $N$-th order using only $N$ pulses. Furthermore, we show to homogenize a $2^m$-mode bosonic system using only $(N+1)^{2m+1}$ pulses, yielding - up to $N$-th order - an effective evolution described by non-interacting harmonic oscillators with identical frequencies. The decoupled and homogenized system provides natural decoherenc…
We investigate the connection between local minima in the problem Hamiltonian and first order quantum phase transitions during an adiabatic quantum computation. We demonstrate how some properties of the local minima can lead to an extremely small gap that is exponentially sensitive to the Hamiltonian parameters. Using perturbation expansion, we derive an analytical formula that can not only predict the behavior of the gap, but also provide insight on how to controllably vary the gap size by changing the parameters. We show agreement with numerical calculations for a weighted maximum independen…
The scattering properties of any complex scattering potential, v:R -> C, can be obtained from the dynamics of a particular non-unitary two-level quantum system S_v. The application of the adiabatic approximation to S_v yields a semiclassical treatment of the scattering problem. We examine the adiabatic series expansion for the evolution operator of S_v and use it to obtain corrections of arbitrary order to the semiclassical formula for the transfer matrix of v. This results in a high-energy approximation scheme that unlike the semiclassical approximation can be applied for potentials with larg…
We study the growth dynamics of ordered structures of strongly interacting polar molecules in optical lattices. Using dipole blockade of microwave excitations, we map the system onto an interacting spin-1/2 model possessing ground states with crystalline order, and describe a way to prepare these states by non-adiabatically driving the transitions between molecular rotational levels. The proposed technique bypasses the need to cross a phase transition and allows for the creation of ordered domains of considerably larger size compared to approaches relying on adiabatic preparation.
The loss of quantum information due to interaction with external degrees of freedom, which is known as decoherence, remains one of the main obstacles for large-scale implementations of quantum computing. Accordingly, different measures are being explored for reducing its effect. One of them is dynamical decoupling (DD) which offers a practical solution because it only requires the application of control pulses to the system qubits. Starting from basic DD sequences, more sophisticated schemes were developed that eliminate higher-order terms of the system-environment interaction and are also mor…
The rovibrational intervals of the $^4$He$_2^+$ molecular ion in its $X\ ^2Σ_\text{u}^+$ ground electronic state are computed by including the non-adiabatic, relativistic, and leading-order quantum-electrodynamics corrections. Good agreement of theory and experiment is observed for the rotational excitation series of the vibrational ground state and the fundamental vibration. The lowest-energy rotational interval is computed to be $70.937\ 69(10)$ cm$^{-1}$ in agreement with the most recently reported experimental value, $70.937\ 589(23)(60)_\text{sys}$ cm$^{-1}$ [L. Semeria, P. Jansen, G.-M. …
