Complete controllability is a fundamental issue in the field of control of quantum systems, not least because of its implications for dynamical realizability of the kinematical bounds on the optimization of observables. In this paper we investigate the question of complete controllability for finite-level quantum systems subject to a single control field, for which the interaction is of dipole form. Sufficient criteria for complete controllability of a wide range of finite-level quantum systems are established and the question of limits of complete controllability is addressed. Finally, the results are applied to give a classification of complete controllability for four-level systems.
We consider a control scheme where a quantum system S is put in contact with an auxiliary quantum system A and the control can affect A only, while S is the system of interest. The system S is then controlled indirectly through the interaction with A. Complete controllability of S +A means that every unitary state transformation for the system S +A can be achieved with this scheme. Indirect controllability means that every unitary transformation on the system S can be achieved. We prove in this paper, under appropriate conditions and definitions, that these two notions are equivalent in finite…
Complete controllability of finite dimensional quantum systems with energy level degeneracy is investigated using two different approaches. One approach is to apply a weak constant field to eliminate the degeneracy and then control it using techniques developed for non-degenerate quantum systems. Conditions for the elimination of degeneracy are found and the issue of influence of relaxation time of constant external field to the target state are addressed through the fidelity. Another approach is to control the degenerate system by a single control field directly. It is found that the system w…
Sufficient conditions for complete controllability of $N$-level quantum systems subject to a single control pulse that addresses multiple allowed transitions concurrently are established. The results are applied in particular to Morse and harmonic-oscillator systems, as well as some systems with degenerate energy levels. Morse and harmonic oscillators serve as models for molecular bonds, and the standard control approach of using a sequence of frequency-selective pulses to address a single transition at a time is either not applicable or only of limited utility for such systems.
We prove complete controllability for rotational states of an asymmetric top molecule belonging to degenerate values of the orientational quantum number M. Based on this insight, we construct a pulse sequence that energetically separates population initially distributed over degenerate M-states, as a precursor for orientational purification. Introducing the concept of enantio-selective controllability, we determine the conditions for complete enantiomer-specific population transfer in chiral molecules and construct pulse sequences realizing this transfer for population initially distributed ov…
We discuss the use of incoherent light as a resource to control the atomic dynamics and review the proposed in Phys. Rev. A 84, 042106 (2011) method for a controlled transfer between any pure and mixed states of quantum systems using a combination of incoherent and coherent light. Formally, the method provides a constructive proof for an approximate open-loop Markovian state-transfer controllability of quantum system in the space of all density matrices---the strongest possible degree of quantum state control.
Quantum phenomena of interest in connection with applications to computation and communication almost always involve generating specific transfers between eigenstates, and their linear superpositions. For some quantum systems, such as spin systems, the quantum evolution equation (the Schrödinger equation) is finite-dimensional and old results on controllability of systems defined on on Lie groups and quotient spaces provide most of what is needed insofar as controllability of non-dissipative systems is concerned. However, in an infinite-dimensional setting, controlling the evolution of quantum…
Controllability properties for discrete-time, Markovian quantum dynamics are investigated. We find that, while in general the controlled system is not finite-time controllable, feedback control allows for arbitrary asymptotic state-to-state transitions. Under further assumption on the form of the measurement, we show that finite-time controllability can be achieved in a time that scales linearly with the dimension of the system, and we provide an iterative procedure to design the unitary control actions.
Various notions from geometric control theory are used to characterize the behavior of the Markovian master equation for N-level quantum mechanical systems driven by unitary control and to describe the structure of the sets of reachable states. It is shown that the system can be accessible but neither small-time controllable nor controllable in finite time. In particular, if the generators of quantum dynamical semigroups are unital, then the reachable sets admit easy characterizations as they monotonically grow in time. The two level case is treated in detail.
Complete controllability of degenerate quantum system using quantum accessor modeled as a qubit chain with nearest neighborhood coupling is investigated. Sufficient conditions on the length of accessor and the way of coupling between controlled system and accessor are obtained. General approach to arbitrary finite system is presented and two and three level degenerate systems are investigated in detail.
A closed quantum system is defined as completely controllable if an arbitrary unitary transformation can be executed using the available controls. In practice, control fields are a source of unavoidable noise. Can one design control fields such that the effect of noise is negligible on the time-scale of the transformation? Complete controllability in practice requires that the effect of noise can be suppressed for an arbitrary transformation. The present study considers a paradigm of control, where the Lie-algebraic structure of the control Hamiltonian is fixed, while the size of the system in…
Manipulation of infinite dimensional quantum systems is important to controlling complex quantum dynamics with many practical physical and chemical backgrounds. In this paper, a general investigation is casted to the controllability problem of quantum systems evolving on infinite dimensional manifolds. Recognizing that such problems are related with infinite dimensional controllability algebras, we introduce an algebraic mathematical framework to describe quantum control systems possessing such controllability algebras. Then we present the concept of smooth controllability on infinite dimensio…
This paper provides a framework for the control of quantum mechanical systems with scattering states, i.e., systems with continuous spectra. We present the concept and prove a criterion of the approximate strong smooth controllability. Our results make non-trivial extensions from quantum systems with finite dimensional control Lie algebras to those with infinite dimensions. It also opens up many interesting problems for future studies.
The reachable set for a finite dimensional quantum system is shown to be the orbit of the group corresponding to the internal and control Hamiltonians, even if this group is not compact.
In coherent quantum feedback control schemes, a target quantum system S is put in contact with an auxiliary system A and the coherent control can directly affect only A. The system S is controlled 'indirectly' through the interaction with A. The system S is said to be indirectly controllable if every unitary transformation can be performed on the state of S with this scheme. The indirect controllability of S will depend on the `dynamical Lie algebra' L characterizing the dynamics of the total system S+A and on the initial state of the auxiliary system A. In this paper we describe this characte…
A quantum mechanical system S is indirectly controlled when the control affects an ancillary system A and the evolution of S is modified through the interaction with A only. A study of indirect controllability gives a description of the set of states that can be obtained for S with this scheme. In this paper, we study the indirect controllability of quantum systems in the finite dimensional case. After discussing the relevant definitions, we give a general necessary condition for controllability in Lie algebraic terms. We present a detailed treatment of the case where both systems, S and A, ar…
A new notion of controllability, eigenstate controllability, is defined for finite-dimensional bilinear quantum mechanical systems which are neither strongly completely controllably nor completely controllable. And a quantum control algorithm based on Grover iteration is designed to perform a quantum control task of steering a system, which is eigenstate controllable but may not be (strongly) completely controllable, from an arbitrary state to a target state.
We consider the optimal control problem of transferring population between states of a quantum system where the coupling proceeds only via intermediate states that are subject to decay. We pose the question whether it is generally possible to carry out this transfer. For a single intermediate decaying state, we recover the Stimulated Raman Adiabatic Passage (STIRAP) process which we identify as the global optimum in the limit of infinite control time. We also present analytic solutions for the case of transfer that has to proceed via two consecutive intermediate decaying states. We show that i…
Qualitative differences in the robust controllability of model two-qubit systems
Macquarie University（麦考瑞大学）；ARC Centre of Excellence for Engineered Quantum Systems, Macquarie University（麦考瑞大学工程量子系统卓越研究中心）；Friedrich-Alexander Universität of Erlangen-Nuremberg（埃尔朗根-纽伦堡弗里德里希·亚历山大大学）
Indirect controllability of an arbitrary finite dimensional quantum system (N-dimensional qudit) through a quantum accessor is investigated. Here, The qudit is coupled to a quantum accessor which is modeled as a fully controllable spin chain with nearest neighbor (anisotropic) XY-coupling. The complete controllability of such indirect control system is investigated in detail. The general approach is applied to the indirect controllability of two and three dimensional quantum systems. For two and three dimensional systems, a simpler indirect control scheme is also presented.
We prove approximate controllability of the bilinear Schrödinger equation in the case in which the uncontrolled Hamiltonian has discrete non-resonant spectrum. The results that are obtained apply both to bounded or unbounded domains and to the case in which the control potential is bounded or unbounded. The method relies on finite-dimensional techniques applied to the Galerkin approximations and permits, in addition, to get some controllability properties for the density matrix. Two examples are presented: the harmonic oscillator and the 3D well of potential, both controlled by suitable potent…
In quantum control theory, the fundamental issue of controllability covers the questions whether and under which conditions a system can be steered from one pure state into another by suitably tuned time evolution operators. Even though Lie theoretic methods to analyze these aspects are well-established for finite dimensional systems, they fail to apply to those with an infinite number of levels. The Jaynes-Cummings-Hubbard model - describing two-level systems in coupled cavities - is such an infinite dimensional system. In this contribution we study its controllability. In the two cavity case…
This paper presents a constructive proof of complete kinematic state controllability of finite-dimensional open quantum systems whose dynamics are represented by Kraus maps. For any pair of states (pure or mixed) on the Hilbert space of the system, we explicitly show how to construct a Kraus map that transforms one state into another. Moreover, we prove by construction the existence of a Kraus map that transforms all initial states into a predefined target state (such a process may be used, for example, in quantum information dilution). Thus, in sharp contrast to unitary control, Kraus-map dyn…
