We propose a scheme to generate superpositions of coherent states for the vibrational motion of a laser cooled trapped-ion. It is based on the interaction with a standing wave making use of the counter-rotating terms, i.e. not applying the rotating wave approximation. We also show that the same scheme can be exploited for quantum state measurement, i.e. with the same scheme non-classical states may be reconstructed
We show how to generate quasi-rectangle-states of the vibrational motion of an ion, this is, states that have the same probability in a given position interval. We produce those states by repeated ion-laser interactions followed by conditional measurements that generate a superposition of squeezed states. The squeeze parameter of the initial state may be tuned in order to obtain such highly localized rectangle states.
We propose an ideal scheme for preparing vibrational $\mathrm{SU(1,1)} \otimes \mathrm{SU(1,1)}$ states in a two-dimensional ion trap using red and blue second sideband resolved driving of two orthogonal vibrational modes. Symmetric and asymmetric driving provide two regimes to realize quantum state engineering of the vibrational modes. In one regime, we show that time evolution synthesizes so-called $\mathrm{SU}(1,1)$ Perelomov coherent states, that is separable squeezed states and their superposition too. The other regime allows engineering of lossless 50/50 $\mathrm{SU}(2)$ beam splitter st…
Molecular matter-wave interferometry enables novel strategies for manipulating the internal mechanical motion of complex molecules. Here, we show how chiral molecules can be prepared in a quantum superposition of two enantiomers by far-field matter-wave diffraction and how the resulting tunnelling dynamics can be observed. We determine the impact of ro-vibrational phase averaging and propose a setup for sensing enantiomer-dependent forces, parity-violating weak interactions, and environment-induced superselection of handedness, as suggested to resolve Hund's paradox. Using ab-initio tunnelling…
The manipulation of massive ro-vibronic superpositions using time-frequency-resolved coherent anti-Stokes Raman scattering (TFRCARS): from quantum control to quantum computing
Properties and applications of a plasmonic cross-shaped nano-antenna is presented and compared to those of array of holes. A simple analytical model based on the superposition of waves are proposed and compared to the numerical results. A direct consequence of unequal path for two orthogonal surface waves leads to a coherent quantum interferometer with interesting properties. Mechanism behind the rotating surface charge densities and consequently, the formation of rotating resultant dipole moments is identified and the concept of Dipole-SPP-LSP-Stokes coupling is introduced. All of which leads…
A chirped-pulse quantum control scheme applicable to Coherent Anti-Stokes Raman Scattering spectroscopy, named as C-CARS, is presented aimed at maximizing the vibrational coherence in molecules. It implies chirping of three incoming pulses in the four-wave mixing process of CARS, the pump, the Stokes and the probe, to fulfil the conditions of adiabatic passage. The scheme is derived in the framework of rotating wave approximation and adiabatic elimination of excited state manifold simplifying the four-level model system into a ``super-effective'' two level system. The robustness, spectral sele…
We demonstrate the preparation and coherent control of the angular momentum state of a two-ion crystal. The ions are prepared with an average angular momentum of $7780\hbar$ freely rotating at 100~kHz in a circularly symmetric potential, allowing us to address rotational sidebands. By coherently exciting these motional sidebands, we create superpositions of states separated by up to four angular momentum quanta. Ramsey experiments show the expected dephasing of the superposition which is dependent on the number of quanta separating the states. These results demonstrate coherent control of a co…
