The pure electric field level-crossing of m_F Zeeman sublevels of hyperfine F levels at two-step laser excitation was described theoretically and studied experimentally for the nD_3/2 states in Cs with n = 7,9, and 10, by applying a diode laser in the first 6S_1/2 to 6P_3/2 step and a diode or dye laser for the second 6P_3/2 to nD_3/2 step. Level-crossing resonance signals were observed in the nD_3/2 to 6P_1/2 fluorescence. A theoretical model was developed to describe quantitatively the resonance signals by correlation analysis of the optical Bloch equations in the case when an atom simultaneously interacts with two laser fields in the presence of an external dc electric field. The simulations described well the experimental signals. The tensor polarizabilities (in Bohr radii cubed) were determined to be 7.45(20) x 10^4 for the 7D_3/2 state and 1.183(35) x 10^6 for the 9D_3/2 state; a well established tensor polarizability value for 10D_3/2 was used to calibrate the electric field. The tensor polarizability value for the 7D_3/2 state differed by ca. 15% from the existing experimentally measured value.
We present an experimental and theoretical investigation of the polarizabilities and hyperfine constants of D_J states in 133Cs for J=3/2 and J=5/2. New experimental values for the hyperfine constant A are obtained from level-crossing signals of the (7,9,10)D_5/2 states of 133Cs and precise calculations of the tensor polarizabilities alpha_2. The results of relativistic many-body calculations for scalar and tensor polarizabilities of the (5-10)D_3/2 and (5-10)D_5/2 states are presented and compared with measured values from the literature. Calculated values of the hyperfine constants A for the…
We demonstrate a technique for precisely measuring hyperfine intervals in alkali atoms. The atoms form a three-level $Λ$ system in the presence of a strong control laser and a weak probe laser. The dressed states created by the control laser show significant linewidth reduction. We have developed a technique for Doppler-free spectroscopy that enables the separation between the dressed states to be measured with high accuracy even in room-temperature atoms. The states go through an avoided crossing as the detuning of the control laser is changed from positive to negative. By studying the separa…
Using a newly developed laser-microwave-laser resonance method, we observed a pair of microwave transitions between hyperfine levels of the $(n,L)=(37,35)$ state of antiprotonic helium. This experiment confirms the quadruplet hyperfine structure due to the interaction of the antiproton orbital angular momentum, the electron spin and the antiproton spin as predicted by Bakalov and Korobov. The measured frequencies of $ν_{\text HF}^+ =12.89596 \pm 0.00034$ GHz and $ν_{\text HF}^- =12.92467 \pm 0.00029$ GHz agree with recent theoretical calculations on a level of $ 6 \times10^{-5}$.
A two-step, two-color laser spectroscopy technique has been used to measure the hyperfine splittings of the $8p$ excited states in $^{203}$Tl and $^{205}$Tl, as well as the $7s - 8p$ transition isotope shifts. For the case of the $8p_{3/2}$ state, our results show a hyperfine anomaly consistent with our recent measurements of other hyperfine splittings, and in disagreement with older results for this state. Our measurement of the $8p_{1/2}$ isotope shift is also in disagreement with earlier work. In this series of experiments, a UV laser was locked to the first-step transition and directed thr…
Isotope shifts and hyperfine structure of tungsten were studied in the near UV range. We have used laser induced fluorescence spectroscopy on a pulsed supersonic beam to probe the 5D0 -> 5F1 transition at 384.9 nm, 7S3 -> 7P4 transition at 400.9 nm, and 7S3 -> 7P3 transition at 407.4 nm. Three new magnetic hyperfine constants are reported for 7P3,7P4, and 5F1 states. The isotope shifts of the 384.9 nm transition are presented for the first time, and the isotope shifts of 400.9 nm and 407.4 nm transition are measured with an order of magnitude higher precision compared to the previous measureme…
We report on the measurement of the isotope shifts of the $3d^74s \,\, a \, {}^5\!F_5 - 3d^74p \,\, z \, {}^5\!G^o_6$ Fe~I line at 358~nm between all four stable isotopes ${}^{54}$Fe, ${}^{56}$Fe, ${}^{57}$Fe and ${}^{58}$Fe, as well as the hyperfine structure of that line for ${}^{57}$Fe, the only stable isotope having a nonzero nuclear spin. This line is of primary importance for laser cooling applications. In addition, an experimental value of the field and specific mass shift coefficients of the transition is reported as well as the hyperfine structure magnetic dipole coupling constant $A$…
We present measurements of the hyperfine splitting in the Yb-173 $6s6p~^1P_1^{\rm o} (F^{\prime}=3/2,7/2)$ states that disagree significantly with those measured previously by Das and Natarajan [Phys. Rev. A 76, 062505 (2007)]. We point out inconsistencies in their measurements and suggest that their error is due to optical pumping and improper determination of the atomic line center. Our measurements are made using an optical frequency comb. We use an optical pumping scheme to improve the signal-to-background ratio for the $F^{\prime}=3/2$ component.
The simple structure of the BH molecule makes it an excellent candidate for direct laser cooling. We measure the branching ratios for the decay of the ${\rm A}^{1}Π(v'=0)$ state to vibrational levels of the ground state, ${\rm X}^{1}Σ^{+}$, and find that they are exceedingly favourable for laser cooling. We verify that the branching ratio for the spin-forbidden transition to the intermediate ${\rm a}^{3}Π$ state is inconsequentially small. We measure the frequency of the lowest rotational transition of the X state, and the hyperfine structure in the relevant levels of both the X and A states, …
Detailed analysis of spectral line broadening and variations in relative intensities of hyperfine spectral components due to optical pumping is presented. Hyperfine levels of sodium $3p_{1/2}$ and $3p_{3/2}$ levels are selectively excited in a supersonic beam at various laser intensities under the conditions when optical pumping time is shorter than transit time of atoms through the laser beam. The excitation spectra exhibit significant line broadening at laser intensities well below the saturation intensity, and redistribution of intensities of hyperfine spectral components is observed, which…
The CREMA collaboration is pursuing a measurement of the ground-state hyperfine splitting (HFS) in muonic hydrogen ($μ$p) with 1 ppm accuracy by means of pulsed laser spectroscopy to determine the two-photon-exchange contribution with $2\times10^{-4}$ relative accuracy. In the proposed experiment, the $μ$p atom undergoes a laser excitation from the singlet hyperfine state to the triplet hyperfine state, {then} is quenched back to the singlet state by an inelastic collision with a H$_2$ molecule. The resulting increase of kinetic energy after the collisional deexcitation is used as a signature …
A two-step, two-color laser spectroscopy technique has been used to measure the hyperfine splitting of the 7p$_{1/2}$ excited state in $^{203}$Tl and $^{205}$Tl, as well as the isotope shift within the 7s$_{1/2}$ - 7p$_{1/2}$ transition. Our measured values for the hyperfine splittings, 2153.2(7) MHz (in $^{203}$Tl) and 2173.3(8) MHz (in $^{205}$Tl), each differ by 20 MHz from previously published values which quoted comparable precision. The transition isotope shift of $^{203}$Tl relative to $^{205}$Tl was measured to be 534.4(9) MHz. In our experiment, one laser was locked to the thallium gr…
Laser Excitation of Muonic 1S Hydrogen Hyperfine Transition: Effects of Multi-pass Cell Interference
NOVA School of Science and Technology, NOVA University Lisbon（新大学科学技术学院，新里斯本大学）；PSI Center for Neutron and Muon Sciences（瑞士保罗谢勒研究所中子与μ子科学中心）；LIBPhys-UC, Department of Physics, University of Coimbra（科英布拉大学物理系LIBPhys-UC）；Institute for Particle Physics and Astrophysics, ETH Zurich（苏黎世联邦理工学院粒子物理与天体物理研究所）
In a frequency-modulation spectroscopy experiment, using the radiation from a single frequency diode laser, the spectra of molecular iodine hyperfine structure near 640 nm were recorded on the transition $B^3Π_{0_u^{+}}-X^1Σ^+_{g}$. The frequency reference given by the value of the modulation frequency (12.5 MHz in given experiment) allows determination of the frequency differences between hyperfine components with accuracy better than 0.1 MHz using the fitting procedure in experiment with only one laser.
We demonstrate a technique for directly measuring the fine-structure interval in alkali atoms using two frequency-stabilized diode lasers. Each laser has a linewidth of order 1 MHz and precise tunability: one laser is tuned to a hyperfine transition in the D_1 line, and the other laser to a hyperfine transition in the D_2 line. The outputs of the lasers are fed into a scanning Michelson interferometer that measures the ratio of their wavelengths accurately. To illustrate the technique, we measure the fine-structure interval in Rb, and obtain a value of 237.6000(3)(5) cm^-1 for the hyperfine-fr…
An overview is presented of laser spectroscopy experiments with cold, trapped, highly-charged ions, which will be performed at the HITRAP facility at GSI in Darmstadt (Germany). These high-resolution measurements of ground state hyperfine splittings will be three orders of magnitude more precise than previous measurements. Moreover, from a comparison of measurements of the hyperfine splittings in hydrogen- and lithium-like ions of the same isotope, QED effects at high electromagnetic fields can be determined within a few percent. Several candidate ions suited for these laser spectroscopy studi…
We consider a simplified model of the optical multi-pass cavity that is being currently developed by the FAMU collaboration for the measurement of the hyperfine splitting in the ground state of muonic hydrogen and of the Zemach radius of the proton. The model is focused on the time distribution of the events of laser-stimulated hyperfine transitions in the muonuc atom and may be helpful in the preliminary design of the FAMU experimental set-up and, more generally, in the optimization of multi-pass optical cavities for experiments with pulsed lasers.
The absolute frequencies of the hyperfine components of the R(26) 62-0 transition in molecular iodine at 501.7 nm are measured for the first time with an optical clockwork based on a femtosecond laser frequency comb generator. The set-up is composed of an Ar+ laser locked to a hyperfine component of the R(26) 62-0 transition detected in a continuously pumped low-pressure cell (0.33 Pa). The detected resonances show a linewidth of 45 kHz (half-width at half-maximum). The uncertainty of the frequency measurement is estimated to be 250 Hz.
We report measurements of absolute transition frequencies and hyperfine coupling constants for the 8S_{1/2}, 9S_{1/2}, 7D_{3/2}, and 7D_{5/2} states in ^{133}Cs vapor. The stepwise excitation through either the 6P_{1/2} or 6P_{3/2} intermediate state is performed directly with broadband laser light from a stabilized femtosecond laser optical-frequency comb. The laser beam is split, counter-propagated and focused into a room-temperature Cs vapor cell. The repetition rate of the frequency comb is scanned and we detect the fluorescence on the 7P_{1/2,3/2} -> 6S_{1/2} branches of the decay of the …
We demonstrate the first application of a liquid-metal ion source for collinear laser spectroscopy in proof-of-principle measurements on naturally abundant In$^+$. The superior beam quality, i.e., the actively stabilized current and energy of a beam with very low transverse emittance, allowed us to perform precision spectroscopy on the $5s^2\;^1\mathrm{S}_0 \rightarrow 5s5p\;^3\mathrm{P}_1$ intercombination transition in $^{115}$In$^+$, which is to our knowledge the slowest transition measured with collinear fluorescence laser spectroscopy so far. By applying collinear and anticollinear spectr…
We studied magneto-optical resonances caused by excited-state level crossings in a nonzero magnetic field. Experimental measurements were performed on the transitions of the $D_2$ line of rubidium. These measured signals were described by a theoretical model that takes into account all neighboring hyperfine transitions, the mixing of magnetic sublevels in an external magnetic field, the coherence properties of the exciting laser radiation, and the Doppler effect. Good agreement between the experimental measurements and the theoretical model could be achieved over a wide range of laser power de…
Hyperfine and Zeeman Optical Pumping and Transverse Laser Cooling of a Thermal Atomic Beam of Dysprosium Using a Single 421 nm Laser
Johannes Gutenberg-Universität Mainz（约翰内斯·古腾堡美因茨大学）；Helmholtz-Institut Mainz, GSI Helmholtzzentrum für Schwerionenforschung（亥姆霍兹美因茨研究所，GSI重离子研究中心）；Department of Physics, Indian Institute of Technology Tirupati（蒂鲁帕蒂印度理工学院物理系）；Korea National University of Education（韩国国立教育大学）；Department of Physics, University of California, Berkeley（加州大学伯克利分校物理系）
Hyperfine-structures of highly charged ions (HCIs) are favourable spectroscopic targets for exploring fundamental physics as well as nuclear properties. Recent proposals of HCI atomic clocks highlight their importance, especially for many-electron HCIs, and they have been theoretically investigated by refining atomic-structure calculations. Nonetheless, no established spectroscopic method is currently available to verify these theoretical calculations. Here, we demonstrate hyperfine-structure-resolved laser spectroscopy of HCIs in an electron beam ion trap plasma, employing the magnetic-dipole…
We use the technique of coherent population trapping (CPT) to access the ground hyperfine interval (clock transition) in $^{133}$Cs. The probe and control beams required for CPT are obtained from a single compact diode laser system. The phase coherence between the beams, whose frequency difference is the clock frequency, is obtained by frequency modulating the laser with an electro-optic modulator (EOM). The EOM is fiber coupled and hence does not require alignment, and the atoms are contained in a vapor cell. Both of these should prove advantageous for potential use as atomic clocks in satell…
We report on the improved measurement of the hyperfine structure of $4f^{12}(^3 H_6)5d_{5/2}6s^2$ $(J=9/2)$ excited state in Tm-169 which is involved in the second-stage laser cooling of Tm. To measure the absolute value of the hyperfine splitting interval we used Doppler-free frequency modulation saturated absorption spectroscopy of Tm atoms in a vapor cell. The sign of the hyperfine constant was determined independently by spectroscopy of laser cooled Tm atoms. The hyperfine constant of the level equals $A_J=-422.112(32)$ MHz that corresponds to the energy difference between two hyperfine su…
We use the phenomenon of electromagnetically-induced transparency in a three-level atomic system for hyperfine spectroscopy of upper states that are not directly coupled to the ground state. The three levels form a ladder system: the probe laser couples the ground state to the lower excited state, while the control laser couples the two upper states. As the frequency of the control laser is scanned, the probe absorption shows transparency peaks whenever the control laser is resonant with a hyperfine level of the upper state. As an illustration of the technique, we measure hyperfine structure i…
A measurement of the hyperfine coefficients and isotope shifts for the Dy I 421.291 nm transition [$4f^{10}6s^2 (J=8)\to4f^{10}6s6p (J=9)$] using atomic beam laser-induced fluorescence spectroscopy is presented. A King Plot analysis is performed to determine a specific mass shift of $δν_{sms}^{164-162}=11(7)$ Hz for the 421-nm transition, confirming the pure $4f^{10}6s6p$ configuration of the excited state. This transition is currently being explored for laser cooling of an atomic beam of dysprosium used in a search for a temporal variation of the fine-structure constant.
Absolute frequency measurement of molecular iodine hyperfine transitions at 554 nm and its application to stabilize a 369 nm laser for Yb+ ions cooling
Hyperfine spectroscopy and laser cooling of the fermionic isotopes $^{47}$Ti and $^{49}$Ti
University of California, Berkeley（加州大学伯克利分校）；Challenge Institute for Quantum Computation（挑战量子计算研究所）；Joint Quantum Institute, National Institutes for Standards and Technology（国家标准与技术研究院联合量子研究所）；Department of Physics, University of Chicago（芝加哥大学物理系）；Department of Physics and Astronomy, University of Delaware（特拉华大学物理与天文学系）
We report absolute frequency measurements of the molecular iodine P(46) 5-4 $a_{1}$, $a_{10}$, and $a_{15}$ hyperfine transitions at 647 nm with a fiber-based frequency comb. The light source is based on a Littrow-type external-cavity diode laser. A frequency stability of 5 $\times$ 10$^{-12}$ at a 200 s integration time is achieved when the light source is stabilized to the P(46) 5-4 $a_{15}$ line. The pressure shift is determined to be -8.3(7) kHz/Pa. Our determination of the line centers reached a precision of 21 kHz. The light source can serve as a reference laser for lithium atom spectros…
Relativistic self-consistent-field calculations of the radial hyperfine integrals have been performed in the 4d-shell element ions. The comparison with available experimental results gives an estimate of configuration interaction effects in the hyperfine interaction in these ions. The results can also be used to derive nuclear moments from laserspectroscopic measurements of radioactive isotopes. PACS Numbers: 31.15.Ne, 31.30.Gs, 32.10.Fn
We demonstrate a technique to lock simultaneously two laser frequencies to each step of a two-photon transition in the presence of a magnetic field sufficiently large to gain access to the hyperfine Paschen-Back regime. A ladder configuration with the 5S$_{1/2}$, 5P$_{3/2}$ and 5D$_{5/2}$ terms in a thermal vapour of $^{87}$Rb atoms is used. The two lasers remain locked for more than 24 hours. For the sum of the laser frequencies, which represents the stability of the two-photon lock, we measure a frequency instability of less than the Rb D$_2$ natural linewidth of 6 MHz for nearly all measure…
We have measured and analyzed the hyperfine structure of two lines, one at 583nm and one at 401nm, of the only stable fermionic isotope of atomic erbium as well as determined its isotope shift relative to the four most-abundant bosonic isotopes. Our work focuses on the J->J+1 laser cooling transitions from the [Xe] 4f12 6s2 (3H6) ground state to two levels of the excited [Xe] 4f12 6s6p configuration, which are of major interest for experiments on quantum degenerate dipolar Fermi gases. From a fit to the observed spectra of the strong optical transition at 401nm we find that the magnetic dipole…
We demonstrate a new technique for measuring the absolute frequencies of atomic transitions. The technique uses a ring-cavity resonator whose length is calibrated using a reference laser locked to the D_2 line in {87}Rb. The frequency of this line is known to be 384 230 484.468(10) MHz. Using a second laser locked to the D_1 line of Rb, we measure the frequencies of various hyperfine transitions in the D_1 and D_2 lines with a precision of 30 kHz. We obtain the following values: 120.687(17) MHz and 406.520(25) MHz for the 5P_{1/2} hyperfine constant A in {85}Rb and {87}Rb; 377 107 385.623(50) …
We report the initial results from a systematic study of the hyperfine (HF) structure of antiprotonic helium (n,l) = (37,~35) carried out at the Antiproton Decelerator (AD) at CERN. We performed a laser-microwave-laser resonance spectroscopy using a continuous wave (cw) pulse-amplified laser system and microwave cavity to measure the HF transition frequencies. Improvements in the spectral linewidth and stability of our laser system have increased the precision of these measurements by a factor of five and reduced the line width by a factor of three compared to our previous results. A compariso…
Molecular hydrogen ions are of metrological relevance due to the possibility of precise theoretical evaluation of their spectrum and of external-field-induced shifts. In homonuclear molecular ions the electric dipole $E1$ transitions are strongly suppressed, and of primary laser spectroscopy interest is the electric quadrupole ($E2$) transition spectrum. In continuation of previous work on the H$_2^+$ ion, we report here the results of the calculations of the hyperfine structure of the laser-induced electric quadrupole transitions between a large set of ro-vibrational states of D$_2^+$; the in…
We remind the reader that it is possible to tell if two or more eigenvalues of a matrix are equal, without calculating the eigenvalues. We then use this property to detect (avoided) crossings in the spectra of quantum Hamiltonians representable by matrices. This approach provides a pedagogical introduction to (avoided) crossings, is capable of handling realistic Hamiltonians analytically, and offers a way to visualize crossings which is sometimes superior to that provided by the spectrum. We illustrate the method using the Breit-Rabi Hamiltonian to describe the hyperfine-Zeeman structure of th…
We perform high resolution spectroscopy on $^{176}$Lu$^+$ including the $^1S_0\leftrightarrow{^3}D_1$ and $^1S_0\leftrightarrow{^3}D_2$ clock transitions. Hyperfine structures and optical frequencies relative to the $^1S_0$ ground state of four low lying excited states are given to a few tens of kHz resolution. This covers the most relevant transitions involved in clock operation with this isotope. Additionally, measurements of the $^3D_2$ hyperfine structure may provide access to higher order nuclear moments, specifically the magnetic octupole and electric hexadecapole moments.
We present our experimental investigation of an optical Raman transition between the magnetic clock states of $^{87}$Rb in an atom chip magnetic trap. The transfer of atomic population is induced by a pair of diode lasers which couple the two clock states off-resonantly to an intermediate state manifold. This transition is subject to destructive interference of two excitation paths, which leads to a reduction of the effective two-photon Rabi-frequency. Furthermore, we find that the transition frequency is highly sensitive to the intensity ratio of the diode lasers. Our results are well describ…
Experimental signals of non-linear magneto-optical resonances at D1 excitation of natural rubidium in a vapor cell have been obtained and described with experimental accuracy by a detailed theoretical model based on the optical Bloch equations. The D1 transition of rubidium is a challenging system to analyze theoretically because it contains transitions that are only partially resolved under Doppler broadening. The theoretical model took into account all nearby transitions, the coherence properties of the exciting laser radiation, and the mixing of magnetic sublevels in an external magnetic fi…
We report on telecom laser frequency stabilization to narrow iodine hyperfine line in the green range of the optical domain, after a frequency tripling process using two nonlinear PPLN crystals. We have generated up to 300 mW optical power in the green (P3w), from 800 mW of infrared power (Pw). This result corresponds to an optical conversion efficiency eta= P3w/Pw ~ 36 %. To our knowledge, this is the best value ever demonstrated for a CW frequency tripling process. We have used a narrow linewidth iodine hyperfine line (component a1 of the 127I2 R 35 (44-0) line) to stabilize the IR laser yie…
We describe an atom trapping mechanism based upon differential optical pumping between metastable hyperfine states by partially-displaced laser beams in the absence of a magnetic field. With realistic laser powers, trap spring constants should match or exceed those typical of magneto-optical traps, and highly flexible tailored trap shapes should be achievable. In a proof-of-principle experiment, we have combined a 1D implementation with magneto-optical trapping in the orthogonal directions, capturing ~10000 85Rb atoms. This is an author-created, un-copyedited version of an article published in…
Advances in laser spectroscopy of superheavy ($Z>100$) elements enabled determination of the nuclear moments of the heaviest nuclei, which requires high-precision atomic calculations of the relevant hyperfine structure (HFS) constants. Here, we calculated the HFS constants and energy levels for a number of nobelium (Z=102) states using the hybrid approach, combining linearized coupled-cluster and configuration interaction methods. We also carried out an extensive study of the No energies using 16-electron configuration interaction method to determine the position of the (5f^{13}7s^2 6d) and (5…
Electro-optic frequency combs with tooth spacings as low as 100 Hz were employed to probe electromagnetically induced transparency (EIT) and hyperfine pumping in rubidium and potassium vapor cells. From the potassium EIT transition we were able to determine the ground state hyperfine splitting with a fit uncertainty of 8 Hz. Importantly, because of the mutual coherence between the control and probe beams, which originate from a single laser, features with linewidths several orders-of-magnitude narrower than the laser linewidth could be observed in a multiplexed fashion. This approach removes t…
A simple and efficient scheme based on one-dimensional nanometric thin cell filled with Rb and strong permanent ring magnets allowed direct observation of hyperfine Paschen-Back regime on D1 line in 0.5 - 0.7 T magnetic field. Experimental results are perfectly consistent with the theory. In particular, with sigma+ laser excitation, the slopes of B-field dependence of frequency shift for all the 10 individual transitions of 85,87Rb are the same and equal to 18.6 MHz/mT. Possible applications for magnetometry with submicron spatial resolution and tunable atomic frequency references are discusse…
We investigated experimentally and theoretically angular momentum alignment-to-orientation conversion created by the joint interaction of laser radiation and an external magnetic field with atomic rubidium at room temperature. In particular we were interested in alignment-to-orientation conversion in atomic ground state. Experimentally the laser frequency was fixed to the hyperfine transitions of $D_1$ line of rubidium. We used a theoretical model for signal simulations that takes into account all neighboring hyperfine levels, the mixing of magnetic sublevels in an external magnetic field, the…
Simple and efficient "λ-method" and "λ/2-method" (λis the resonant wavelength of laser radiation) based on nanometric-thickness cell filled with rubidium are implemented to study the splitting of hyperfine transitions of 85Rb and 87Rb D_1 line in an external magnetic field in the range of B = 0.5 - 0.7 T. It is experimentally demonstrated from 20 (12) Zeeman transitions allowed at low B-field in 85Rb (87Rb) spectra in the case of σ+ polarized laser radiation, only 6 (4) remain at B > 0.5 T, caused by decoupling of the total electronic momentum J and the nuclear spin momentum I (hyperfine Pasch…
We describe the operation of two GaN-based diode lasers for the laser spectroscopy of gallium at 403 nm and 417 nm. Their use in an external cavity configuration enabled the investigation of absorption spectroscopy in a gallium hollow cathode. We have analyzed the Doppler broadened profiles accounting for hyperfine and isotope structure and extracting both the temperature and densities of the neutral atomic sample produced in the glow discharge. We have also built a setup to produce a thermal atomic beam of gallium. Using the GaN-based diode lasers we have studied the laser induced fluorescenc…
We demonstrate subpicosecond-time-scale population transfer between the pair of hyperfine ground states of atomic rubidium using a single laser-pulse. Our scheme utilizes the geometric and dynamic phases induced during Rabi oscillation through the fine-structure excited state in order to construct an $X$ rotation gate for the hyperfine-state qubit system. Experiment performed with a femtosecond laser and cold rubidium atoms, in a magneto-optical trap, shows over 98\% maximal population transfer between the clock states.
Selective reflection of a laser radiation from an interface formed by a dielectric window and a potassium atomic vapour confined in a nano-cell with $350~$nm gap thickness is implemented for the first time to study the atomic transitions of K D$_2$ line in external magnetic fields. In moderate $B$-fields, there are 44 individual Zeeman transitions which reduce to two groups (one formed by $σ^+$ the other one by $σ^-$ circularly-polarised light), each containing eight atomic transitions, as the magnetic field increases. Each of these groups contains one so-called "guiding" transition whose part…
We report high-precision measurements on the thallium fluoride $\tilde{J} = 1$ hyperfine manifold of the $B^3Π_1$ ($ν= 0$) state. This state is of special interest because it is central to an optical cycling scheme that is envisioned to play an important role in enhancing the sensitivity of the CeNTREX nuclear Schiff-moment experiment presently under construction. The measurements are made by monitoring the fluorescence induced by narrow-band laser excitation of a cryogenic molecular beam. We use a multipass arrangement of the laser beam to enhance fluorescence. When viewed with a camera, we c…
