We demonstrate a technique for precisely measuring hyperfine intervals in alkali atoms. The atoms form a three-level $Λ$ system in the presence of a strong control laser and a weak probe laser. The dressed states created by the control laser show significant linewidth reduction. We have developed a technique for Doppler-free spectroscopy that enables the separation between the dressed states to be measured with high accuracy even in room-temperature atoms. The states go through an avoided crossing as the detuning of the control laser is changed from positive to negative. By studying the separation as a function of detuning, the center of the level-crossing diagram is determined with high precision, which yields the hyperfine interval. Using room-temperature Rb vapor, we obtain a precision of 44 kHz. This is a significant improvement over the current precision of ~ 1 MHz.
We demonstrate an iterative scheme for coupled-cluster properties calculations without truncating the dressed properties operator. For validation, magnetic dipole hyperfine constants of alkaline Earth ions are calculated with relativistic coupled-cluster and role of electron correlation examined. Then, a detailed analysis of the higher order terms is carried out. Based on the results, we arrive at an optimal form of the dressed operator. Which we recommend for properties calculations with relativistic coupled-cluster theory.
We study the spectral signatures and coherence properties of radiofrequency dressed hyperfine Zeeman sub-levels of 87Rb. Experimentally, we engineer combinations of static and RF magnetic fields to modify the response of the atomic spin states to environmental magnetic field noise. We demonstrate analytically and experimentally the existence of 'magic' dressing conditions where decoherence due to electromagnetic field noise is strongly suppressed. Building upon this result, we propose a bi-chromatic dressing configuration that reduces the global sensitivity of the atomic ground states to low-f…
Techniques to manipulate the individual constituents of an ultracold mixture are key to investigating impurity physics. In this work, we confine a mixture of the hyperfine ground states of Rb-87 in a double-well potential. The potential is produced by dressing the atoms with multiple radiofrequencies. The amplitude and phase of each frequency component of the dressing field are individually controlled to independently manipulate each species. Furthermore, we verify that our mixture of hyperfine states is collisionally stable, with no observable inelastic loss.
We consider two clouds of ground state alkali atoms in two distinct hyperfine ground states. Each level is far off-resonantly coupled to a Rydberg state, which leads to dressed ground states with a weak admixture of the Rydberg state properties. Due to this admixture, for a proper choice of the Rydberg states, the atoms experience resonant dipole-dipole interactions that induce mechanical forces acting on all atoms within both clouds. This behavior is in contrast to the dynamics predicted for bare dipole-dipole interactions between Rydberg superatoms, where only a single atom per cloud is subj…
We explore properties of atoms whose magnetic hyperfine sub-levels are coupled by an external magnetic radio frequency (rf) field. We perform a thorough theoretical analysis of this driven system and present a number of systematic approximations which eventually give rise to dressed adiabatic radio frequency potentials. The predictions of this analytical investigation are compared to numerically exact results obtained by a wave packet propagation. We outline the versatility and flexibility of this new class of potentials and demonstrate their potential use to build atom optical elements such a…
We study the hyperfine spectrum of atoms of $^{87}$Rb dressed by a radio-frequency field, and present experimental results in three different situations: freely falling atoms, atoms trapped in an optical dipole trap and atoms in an adiabatic radio-frequency dressed shell trap. In all cases, we observe several resonant side bands spaced (in frequency) at intervals equal to the dressing frequency, corresponding to transitions enabled by the dressing field. We theoretically explain the main features of the microwave spectrum, using a semi-classical model in the low field limit and the Rotating Wa…
The recently realized spin-orbit coupled quantum gases (Y.-J Lin {\it et al}., Nature 471, 83-86 (2011); P. Wang {\it et al}., PRL 109, 095301 (2012); L. W. Cheuk {\it et al}., PRL 109, 095302 (2012)) mark a breakthrough in the cold atom community. In these experiments, two hyperfine states are selected from a hyperfine manifold to mimic a pseudospin-1/2 spin-orbit coupled system by the method of Raman dressing, which is applicable to both bosonic and fermionic gases. In this work, we show that the method used in these experiments can be generalized to create any large pseudospin spin-orbit co…
We propose a flexible and robust scheme to create closed quasi-one dimensional guides for ultra-cold atoms through the dressing of hyperfine sub-levels of the atomic ground state. The dressing field is spatially modulated by inductive effects over a micro-engineered conducting loop, freeing the trapping region from leading wires in its proximity. We show that arrays of connected ring traps can also be created by carefully designing the shape of the conducting loop. We report on characteristics of the trap and mechanisms that limit the range of parameters available for experimental implementati…
We use the dressed atom formalism to calculate the frequency shift in a hydrogen maser induced by applied radiation near the Zeeman frequency, and find excellent agreement with a previous calculation made in the bare atom basis. The maser oscillates on the Delta_F = 1, Delta_m_F = 0 hyperfine transition, while the applied field is swept through the F = 1, Delta_m_F = \pm 1 Zeeman resonance. We determine the effect of the applied field on the Zeeman levels using the dressed atom picture, and then calculate the maser frequency shift by coupling the dressed states to the microwave cavity. Qualita…
We calculate the rates of inelastic collisions for ultracold alkali-metal atoms in radiofrequency-dressed traps, using coupled-channel scattering calculations on accurate potential energy surfaces. We identify an rf-induced loss mechanism that does not exist in the absence of rf radiation. This mechanism is not suppressed by a centrifugal barrier in the outgoing channel, and can be much faster than spin relaxation, which is centrifugally suppressed. We explore the dependence of the rf-induced loss rate on singlet and triplet scattering lengths, hyperfine splittings and the strength of the rf f…
A semiclassical, four-level model of a nanosecond, chirped pulse interacting with all optically accessible hyperfine states in the ultracold Rb atom is analyzed aiming at population inversion within $5S_{1/2}$ electronic state. The nature of two-photon adiabatic passage performed by such a single pulse having a bandwidth smaller than the hyperfine splitting of $5S_{1/2}$ state is investigated in the framework of the dressed state picture. It is shown that two dressed states are involved in the adiabatic dynamics of population inversion. The excited state manifold appeared to play an important …
In Rydberg dressed ultra-cold gases, ground state atoms inherit properties of a weakly admixed Rydberg state, such as sensitivity to long-range interactions. We show that through hyperfine-state dependent interactions, a pair of atom clouds can evolve into a spin and subsequently into a spatial Schrödinger's cat state: The pair, containing 20 atoms in total, is in a coherent superposition of two configurations, with cloud locations separated by micrometers. The mesoscopic nature of the superposition state can be proven with absorption imaging, while the coherence can be revealed though recombi…
We develop the research achievement of recent work [M. Gärttner, et.al., Phys. Rev. Letts. 113, 233002 (2014)], in which an anomalous excitation enhancement is observed in a three-level Rydberg-atom ensemble with many-body coherence. In our novel theoretical analysis, this effect is ascribed to the existence of a quasi-dark state as well as its avoided crossings to nearby Rydberg-dressed states. Moreover, we show that with an appropriate control of the optical detuning to the intermediate state, the enhancement can evoke a direct facilitation to atom-light coupling that even breaks through the…
In a recent publication [Phys. Rev. A 79, 065602 (2009)] it was shown that an avoided-crossing resonance can be defined in different ways, according to level-structural or dynamical aspects, which do not coincide in general. Here a simple $3$-level system in a $Λ$ configuration is discussed, where the difference between both definitions of the resonance may be observed. We also discuss the details of a proposed experiment to observe this difference, using microwave fields coupling hyperfine magnetic sublevels in alkali atoms.
We demonstrate theoretically the existence of a linear dc Stark shift of the individual substates of an alkali atom in its ground state, dressed by a circularly polarized laser field. It arises from the electroweak nuclear anapole moment violating P but not T. It is characterized by the pseudoscalar equal to the mixed product formed with the photon angular momentum and static electric and magnetic fields. We derive the relevant left-right asymmetry with its complete signature in a field configuration selected for a precision measurement with cold atom beams. The 3,3 to 4,3 Cs hyperfine-transit…
We remind the reader that it is possible to tell if two or more eigenvalues of a matrix are equal, without calculating the eigenvalues. We then use this property to detect (avoided) crossings in the spectra of quantum Hamiltonians representable by matrices. This approach provides a pedagogical introduction to (avoided) crossings, is capable of handling realistic Hamiltonians analytically, and offers a way to visualize crossings which is sometimes superior to that provided by the spectrum. We illustrate the method using the Breit-Rabi Hamiltonian to describe the hyperfine-Zeeman structure of th…
We demonstrate that Ramsey spectroscopy can be used to observe Rydberg-dressed interactions. In contrast to many prior proposals, our scheme operates comfortably within experimentally measured lifetimes, and accesses a regime where quantum superpositions are crucial. The key idea is to build a spin-1/2 from one level that is Rydberg-dressed and another that is not. These levels may be hyperfine or long-lived electronic states. An Ising spin model governs the Ramsey dynamics, for which we derive an exact solution. Due to the structure of Rydberg interactions, the dynamics differs significantly …
High-resolution Zeeman spectroscopy of electronic-nuclear hyperfine levels of ${^5\mathrm{I}_8}\rightarrow{^5\mathrm{I}_7}$ transitions in Ho$^{3+}$:Y$_2$SiO$_5$ is reported. Crystal-field parameters determined for the two $C_1$ symmetry sites in Er$^{3+}$:Y$_2$SiO$_5$ are successfully used to model the Zeeman-hyperfine data, including the prediction of avoided crossings between hyperfine levels under the influence of an external magnetic field. The two six- and seven-coordinate substitutional sites may be distinguished by comparing the spectra with crystal-field calculations.
We evaluate the impact that nonlinear Zeeman shifts have on resonant radio-frequency (RF) dressed traps in an atom-chip configuration. The degeneracy of the resonance between Zeeman levels is lifted at large intensities of a static field, modifying the spatial dependence of the atomic adiabatic potential. In this context, we find effects that are important for the next generation of atom chips with tight trapping: in particular, that the vibrational frequency of the atom trap is sensitive to the RF frequency and, depending on the sign of the Landé factor, can produce significantly weaker, or t…
Light-induced states are commonly observed in the photoionization spectra of laser-dressed atoms. The properties of autoionizing polaritons, entangled states of light and Auger resonances, however, are largely unexplored. We employ attosecond transient-absorption spectroscopy to study the evolution of autoionizing states in argon, dressed by a tunable femtosecond laser pulse. The avoided crossings between the $3s^{-1}4p$ and several light-induced states indicates the formation of polariton multiplets. We measure a controllable stabilization of the polaritons against ionization, in excellent ag…
Floquet Interpretation of Avoided Crossings in AC Stark-Shifted Rydberg-EIT Spectra
National Institute of Standards and Technology（美国国家标准与技术研究院）；Department of Electrical, Computer, and Engineering, University of Colorado, Boulder（科罗拉多大学博尔德分校电气、计算机与工程学院）
We study collision of two atoms with formation of Feshbach resonance at combined interaction with the external magnetic field and laser radiation. In cases of one- and two-photon resonances of laser radiation with two discrete vibrational molecular levels, we show that Feshbach resonances appear at interaction of external magnetic field with dressed states formed via Autler-Townes effect. In addition, in case of one-photon resonance the lower vibrational molecular state is coupled by laser radiation with the continuum of the elastic channel and forms laser-induced Feshbach resonance via both A…
