Spontaneous and stimulated emission of an electron in the ion channel is studied. The emission processes are studied in the regime of high harmonic generation when the parameter of plasma wiggler strength is large. Like for conventional free electron laser, a synchrotron-like broadband spectrum is generated in this regime. The asymptotic expression for the radiation spectrum of the spontaneous emission is derived. The radiation spectrum emitted from axisymmetric monoenergetic electron beam is analyzed. The gain of ion-channel synchrotron-radiation laser is calculated. Use of laser-produced ion channel for efficient X-ray generation is discussed.
Do the wavepacket-size of free-electron wavefunction and its history have physical effect in its interaction with light? Here we answer this problem by analyzing a QED model, considering both spontaneous and stimulated emission of quantized radiation field. For coherent radiation (Glauber state), we confirm that stimulated emission/absorption of photons has a dependence on wavepacket size that decays when it exceeds the interacting radiation wavelength, consistently and complementarily with Schrodinger equation analysis of wavepacket acceleration in classical electromagnetic field. Furthermore…
The inclusion of atomic inversion in Raman scattering can significantly alter field dynamics in plasmonic settings. Our calculations show that large local fields and femtosecond pulses combine to yield: (i) population inversion within hot spots; (ii) gain saturation; and (iii) conversion efficiencies characterized by a switch-like transition to the stimulated regime that spans twelve orders of magnitude. While in Raman scattering atomic inversion is usually neglected, we demonstrate that in some circumstances full accounting of the dynamics of the Bloch vector is required.
We demonstrate spatially-resolved measurements of spontaneous and stimulated electron-photon interactions in nanoscale optical near fields using electron energy-loss spectroscopy (EELS), cathodoluminescence spectroscopy (CL), and photon-induced near-field electron microscopy (PINEM). Specifically, we study resonant surface plasmon modes that are tightly confined to the tip apexes of an Au nanostar, enabling a direct correlation of EELS, CL, and PINEM on the same physical structure at the nanometer length scale. Complemented by numerical electromagnetic boundary-element method calculations, we …
We estimate the Stokes wave starting power for stimulated thermal Rayleigh scattering (STRS) produced by thermal fluctuations in the fiber core that transiently alter the refractive index profile in the core. A transverse temperature gradient creates a transverse refractive index gradient via the thermo optic effect, and if the fluctuation frequency lies in the STRS gain band, it can couple light from mode LP$_{01}$ to LP$_{11}$ to seed STRS. This spontaneous Rayleigh seed may be stronger than the quantum background and may affect the mode instability thresholds of fiber amplifiers. This new s…
We introduce a quantization scheme that can be applied to surface waves propagating along a plane interface. An important result is the derivation of the energy of the surface wave for dispersive non-lossy media without invoking any specific model for the dielectric constant. Working in Coulomb's gauge, we use a modal representation of the fields. Each mode can be associated with a quantum harmonic oscillator. We have applied the formalism to derive quantum-mechanically the spontaneous emission rate of surface plasmon by a two-level system. The result is in very good agreement with Green's ten…
We report on four-wave mixing in coupled photonic crystal nano-cavities on a silicon-on-insulator platform. Three photonic wire cavities are side-coupled to obtain three modes equally separated in energy. The structure is designed to be self-filtering, and we show that the pump is rejected by almost two orders of magnitudes. We study both the stimulated and the spontaneous four-wave mixing processes: owing to the small modal volume, we find that signal and idler photons are generated with a hundred-fold increase in efficiency as compared to silicon micro-ring resonators.
We study forward stimulated Raman emission from weakly fluorescent dye 4'-diethylamino-N-methyl-4-stilbazolium tosylate (DEST) in 1,2,dichloroethane solution excited by a 28 ps, 532 nm Nd: YAG laser. Neat 1, 2, dichloroethane emits the first Stokes line at 631 nm with a spectral width of 1.6 nm corresponding to a Raman shift of 2956 per cm. We observe reduction of spectral width with the addition of DEST in 1, 2, dichloroethane solution. The single pass conversion efficiency for forward Raman emission is as high as 20 percent in a 1 cm path length sample. The pulse duration of forward stimulat…
We demonstrate stimulated Raman gain using a broadband LED Stokes source to measure vibrational spectra of aqueous glucose solutions. This versatile and cost-effective method increases Raman signal for a variety of applications. We measured both stimulated Raman and spontaneous Raman spectra of glucose solutions with concentrations up to 10 mM with a photon counter and lock-in amplifier. We built partial least squares regression models based on both stimulated Raman and spontaneous Raman spectral data measured with each instrument for predicting concentrations of the glucose solutions. The sti…
Here we present a semiclassical analysis of spontaneous and stimulated radiative emission from unmodulated and optically-modulated electron quantum wavepackets. We show that the radiative emission/absorption and corresponding deceleration/acceleration of the wavepackets depend on the controllable 'history-dependent' wavepacket size. The characteristics of the radiative interaction when a wavepacket of size (duration) is short relative to the radiation wavelength, are close to the predictions of the classical point-particle modeling. On the other hand, in the long-sized wavepacket limit, the in…
Nanoscale semiconductor lasers have been developed recently using either metal, metallo-dielectric or photonic crystal nanocavities. While the technology of nanolasers is steadily being deployed, their expected performance for on-chip optical interconnects is still largely unknown due to a limited understanding of some of their key features. Specifically, as the cavity size is reduced with respect to the emission wavelength, the stimulated and the spontaneous emission rates are modified, which is known as the Purcell effect in the context of cavity quantum electrodynamics. This effect is expec…
Building a refrigerator based on the conversion of heat into optical energy is an ongoing engineering challenge. Under well-defined conditions, spontaneous anti-Stokes fluorescence of a dopant material in a host matrix is capable of lowering the host temperature. The fluorescence is conveying away a part of the thermal energy stored in the vibrational oscillations of the host lattice. In particular, applying this principle to the cooling of (solid-state) lasers opens up many potential device applications, especially in the domain of high-power lasers. In this paper, an alternative optical cool…
Within the framework of a Hilbert space theory, we develop a maximum-``power'' variational principle (MPVP) applicable to classical spontaneous electromagnetic radiation from relativistic electron beams or other prescribed classical current sources. A simple proof is summarized for the case of three-dimensional fields propagating in vacuum, and specialization to the important case of paraxial optics is also discussed. The techniques have been developed to model undulator radiation from relativistic electron beams, but are more broadly applicable to synchrotron or other radiation problems, and …
A theoretical model for describing the emission spectra of microsphere cavities is presented, and its prediction of detailed lineshapes of emission spectra associated with whispering gallery modes (WGMs) of various orders in ZnO microspheres (MSs) are verified experimentally by photoluminescence (PL) spectroscopy. The interplay of Purcell effect, quality factor, and leaky modes in spontaneous and stimulated emission spectra related to WGMs of all orders is revealed. The key success of the theory is based on the expansion of the full Green function of the MS in terms of all possible resonance m…
Warm rubidium vapours are known to be a versatile medium for a variety of experiments in atomic physics and quantum optics. Here we present experimental results on producing the frequency converted light for quantum applications based on spontaneous and stimulated processes in rubidium vapours. In particular, we study the efficiency of spontaneously initiated stimulated Raman scattering in the Λ-level configuration and conditions of generating the coherent blue light assisted by multi-photon transitions in the diamond-level configuration. Our results will be helpful in search for new types of …
The random lasing (RL) emission of dyed vesicular polymeric films in diffusive regime of light propagation was investigated under helium temperature. It represents itself the coupling effect of stimulated emission and stimulated Raman scattering (SRS). Due to the effect a set of Raman lines reveal in RL spectrum. Distinguishing feature of the effect is the stimulated emission promotes the Raman lines revealing. Intensity of Raman lines have quadratic trend on pump intensity. Furthermore SRS in this condition has the more structured spectrum than spontaneous Raman one. It makes enable detection…
We report on strong backward stimulated emission at 337 nm in Nitrogen gas pumped by circularly polarized femtosecond laser pulses at 800 nm. A distinct dependence of the backward UV spectrum on pump laser polarization and intensity is observed, pointing to the occurrence of backward amplified spontaneous emission inside filaments. We attribute the population inversion to inelastic collision between the free electrons produced by the pump laser and neutral N2 molecules. The addition of Oxygen molecules is detrimental for the gain, reducing it to near threshold at atmospheric concentration.
The first continuous-wave two-photon absorption laser-induced stimulated emission (CTALISE) is demonstrated. The 7^1S-6^1P transition in mercury at 1014nm wavelength is used and selective lasing of different isotopes is observed.
It is known that photon pairs generated from pulse-pumped spontaneous parametric processes can be described by independent temporal modes and form a multi-temporal mode entangled state. However, the exact form of the temporal modes is not known even though the joint spectral intensity of photon pairs can be measured by the method of stimulated emission tomography. In this paper, we describe a feedback-iteration method which, combined with the stimulated emission method, can give rise to the exact forms of the independent temporal modes for the temporally entangled photon pairs.
Light emitters in a single-mode nanolaser interact with the same cavity field, that gives rise to polarization correlations which transform the cavity mode. Usually these correlations are ignored, however, collective phenomena can lead to the distinct sub- and superradiance, whose fully quantum description is challenging. Here, we develop a simple yet rigorous picture of radiative transitions in single-mode nanolasers that accounts for polarization correlations. We show that the collective behavior of emitters modifies the photonic density of states leading to gain-dependent Purcell enhancemen…
Quarter-wave OLEDS are microcavity devices that can operate in the low finesse limit and achieve high efficiency (> 300 lm/W) by using interference to reduce the onset current for the transition to stimulated emission. In this work we study the transition to stimulated emission and compare the kinetics and electrical properties of conventional and quarter-wave devices. We show that suppression of spontaneous emission into the vertical mode can result in a sharp transition to stimulated emission at (γ/eV)I ~ N_se/τ_sp where N_se/τ_sp is determined by optical parameters, and we find a previously…
In his celebrated 1916-17 papers in which he proposed the A and B coefficients for the spontaneous and stimulated emission of energy quanta from excited atoms, Einstein conjectured that stimulated emission involves the release of individual quanta (later dubbed "photons") along the direction of an incident photon with the same energy, momentum, phase, and polarization state as that of the incident photon. According to classical electrodynamics, of course, an oscillating dipole must radiate an azimuthally symmetric electromagnetic field around its axis of oscillation. Nevertheless, Einstein sug…
In this tutorial, the physical origins and mathematical analyses of laser linewidths are reviewed. The semi-classical model is based on an equation for the light-mode amplitude that includes random source terms, one term for each process that affects the amplitude (stimulated and spontaneous emission, stimulated absorption, and facet and material loss). Although the source terms are classical, their assigned strengths are consistent with the laws of quantum optics. Analysis of this equation shows that the laser linewidth is proportional to the sum of the (positive) source strengths for all gai…
In recent and future synchrotron radiation facilities, relativistic electron bunches with increasingly high charge density are needed for producing brilliant light at various wavelengths, from X-rays to terahertz. In such conditions, interaction of electrons bunches with their own emitted electromagnetic fields leads to instabilities and spontaneous formation of complex spatial structures. Understanding these instabilities is therefore key in most electron accelerators. However, investigations suffer from the lack of non-destructive recording tools for electron bunch shapes. In storage rings, …
Stimulated Raman scattering (SRS) represents a powerful tool for accessing the vibrational properties of molecular compounds or solid state systems. From a spectroscopic perspective, SRS is able to capture Raman spectra free from incoherent background processes and typically ensures a signal enhancement of several orders of magnitude with respect to its spontaneous counterpart. Since its discovery in 1962, SRS has been applied to develop technological applications, such as Raman-based lasers, frequency shifters for pulsed sources and Raman amplifiers. For the full exploitation of their potenti…
In the spin noise spectroscopy, the magnetic susceptibility spectrum is known to be provided by the spin-system untouched by any external perturbation, or, better to say, disturbed only by its thermal bath. We propose a new version of the spin noise spectroscopy, with the detected magnetization (Faraday-rotation) noise being stimulated by an external fluctuating magnetic field with a quasi-white spectrum. Experimental study of the stimulated spin noise performed on a $\text{BaF}_2 : \text{U}^{3+}$ crystal in a longitudinal magnetic field has revealed specific features of this approach and allo…
Nanoscale lasers sustain few optical modes so that the fraction of spontaneous emission $β$ funnelled into the useful (lasing) mode is high (of the order of few 10$^{-1}$) and the threshold, which traditionally corresponds to an abrupt kink in the light in- light out curve, becomes ill-defined. We propose an alternative definition of the threshold, based on the dynamical response of the laser, which is valid even for $β=1$ lasers. The laser dynamics is analyzed through a reconstruction of its phase-space trajectory for pulsed excitation. Crossing the threshold brings about a change in the shap…
Optical supercontinuum radiation, a special kind of white light, has found numerous applications in scientific research and technology. This bright, broadband radiation can be generated from nearly monochromatic light through the cooperative action of multiple nonlinear effects. Unfortunately, supercontinuum radiation is plagued by large spectral and temporal fluctuations owing to the spontaneous initiation of the generation process. While these fluctuations give rise to fascinating behavior in the form of optical rogue waves [1], they impede many critical applications of supercontinuum. Here,…
The coherent interaction of electromagnetic fields with solid-state two-level systems can yield deterministic quantum light sources for photonic quantum technologies. To date, the performance of semiconductor single-photon sources based on three-level systems is limited mainly due to a lack of high photon indistinguishability. Here, we tailor the cavity-enhanced spontaneous emission from a ladder-type three-level system in a single epitaxial quantum dot (QD) through stimulated emission. After populating the biexciton (XX) of the QD through two-photon resonant excitation (TPE), we use another l…
We fabricate a fiber coupled ultrahigh-Q resonator from a μdroplet per se; and experimentally measure stimulated Raman emission showing itself at a 160μW threshold. We observe Raman-laser lines that agree with their related calculated molecular-vibrations, as well as with a control-group experiment that uses a Raman-spectrometer. Yet, unlike spectrometers where emission is spontaneous and less directional, our droplet emitter is stimulated, single-mode-fiber coupled, resonantly enhanced with Q of 250 million, confined to a 23 um3 mode volume and has 7 orders of magnitude higher power.
Semiconductor nanocrystals can be synthesized using inexpensive, scalable, solution-based techniques, and their utility as tunable light emitters has been demonstrated in various applications, including biolabeling and light-emitting devices. By contrast, the use of colloidal nanocrystals for optical amplification and lasing has been limited by the high input power densities that have been required. In this work, we show that colloidal nanoplatelets (NPLs) produce amplified spontaneous emission (ASE) with pump-fluence thresholds as low 6 uJ/cm2 and gain as high as 600 cm-1, both a 4-fold impro…
A hallmark of spin-lasers, injected with spin-polarized carriers, is their threshold behavior with the onset of stimulated emission. Unlike the single threshold in conventional lasers with unpolarized carriers, two thresholds are expected in spin lasers. With the progress in scaled-down lasers and the use of novel two-dimensional materials it is unclear if the common description of spin lasers assuming a negligible spontaneous emission and linear optical gain remains relevant or even how to identify the lasing thresholds. Our rate-equation description addresses these questions by considering a…
We simulate the transition from amplified spontaneous emission (ASE) to lasing in random systems with varying degrees of mode overlap. This is accomplished by solving the stochastic Maxwell-Bloch equations with the finite-difference time-domain method. Below lasing threshold, the continuous emission spectra are narrowed by frequency-dependent amplification. Our simulations reproduce the stochastic emission spikes in the spectra. Well-defined peaks, corresponding to the system resonances, emerge at higher pumping and are narrowed by stimulated emission before lasing takes place. Noise tends to …
Tailoring of electromagnetic spontaneous emission predicted by E. M. Purcell more than 50 years ago has undoubtedly proven to be one of the most important effects in the rich areas of quantum optics and nanophotonics. Although during the past decades the research in this field has been focused on electric dipole emission, the recent progress in nanofabrication and study of magnetic quantum emitters, such as rare-earth ions, has stimulated the investigation of the magnetic side of spontaneous emission. Here, we review the state-of-the-art advances in the field of spontaneous emission enhancemen…
