There have been recent suggestions for searching for the electron electric dipole moment, using solid state experiments with compounds containing Gd 3+ ions. These experiments could improve the sensitivity compared to present atomic and molecular experiments by several orders of magnitude. The analysis of the problem requires a calculation of the enhancement coefficient K for the electron electric dipole moment in the Gd 3+ ion. In this work we perform this calculation. The result is K = -4.9 +- 1.6. Limitations of the accuracy of the calculation are mainly due to the lack of data on Gd 3+ excitation spectra. We formulate which quantities have to be measured and/or calculated to improve the accuracy.
The prospects for a new search for the electron electric dipole moment in solid Gadolinium iron garnet ceramics
我们解决了一些问题，固态电子电偶极矩（EDM）的实验，专注于钆铁石榴石（简称GdIG，化学式Gd $_3$ Fe $_5$ O $_{12}$）作为可能的样品材料。GdIG保持其高磁化率低至4.2 K，这增强了置于电场中的样品的EDM诱导磁化。我们估计晶格极化率产生的EDM增强因子约为20。我们还计算了各种样品的几何形状和磁导率的退磁场的效果。固有的GdIG磁化噪声的测量，和波动耗散定理是用来比较我们的数据与GdIG磁导率的虚部在4.2 K的测量，显示出良好的协议以上的频率的几个赫兹。我们还观察到退磁场如何抑制噪声引起的磁通量，证实了我们的计算。基于固体GdIG样品的EDM搜索的统计灵敏度估计与目前的实验极限处于同一水平。考虑到所涉及的完全不同的方法和系统，这种测量是有价值的。在这样的实验中最重要的系统是磁滞和磁电效应。我们的分析表明，在统计敏感性水平上控制这些是可能的。
We report results of an experimental search for the intrinsic Electric Dipole Moment (EDM) of the electron using a solid-state technique. The experiment employs a paramagnetic, insulating gadolinium gallium garnet (GGG) that has a large magnetic response at low temperatures. The presence of the eEDM would lead to a small but non-zero magnetization as the GGG sample is subject to a strong electric field. We search for the resulting Stark-induced magnetization with a sensitive magnetometer. Recent progress on the suppression of several sources of background allows the experiment to run free of s…
The multiconfiguration Dirac-Hartree-Fock (MCDHF) method was employed to calculate atomic electric dipole moments (EDM) of the superheavy element copernicium (Cn, $Z=112$). The EDM enhancement factors of Cn, here calculated for the first time, are about one order of magnitude larger than those of Hg. The exponential dependence of enhancement factors on atomic number $Z$ along group 12 of the periodic table was derived from the EDMs of the entire homolog series, $^{69}_{30}$Zn, $^{111}_{\phantom{1}48}$Cd, $^{199}_{\phantom{1}80}$Hg, $^{285}_{112}$Cn, and $^{482}_{162}$Uhb. These results show th…
Comment on "Reappraisal of the Electric Dipole Moment Enhancement Factor for Thallium"
Nataraj { \em et al}（Phys. Rev. Lett. { \bf 106}，200403（2011））提供了T1的EDM增强因子的计算，其与先前最精确的计算不一致。作者声称，由于对高阶相关性的更完整处理，他们对TI EDM的计算是最准确的。在本说明中，我们认为这一主张没有足够的证据支持。Nataraj { \em et al}也对我们的计算给出了误导性的评论。我们解释了我们的方法并回复了Nataraj { \em et al}的评论。
We provide a physical explanation for enhancement of the low-energy electron production by sensitizing nanoparticles due to irradiation by fast ions. It is demonstrated that a significant increase in the number of emitted electrons arises from the collective electron excitations in the nanoparticle. We predict a new mechanism of the yield enhancement due to the plasmon excitations and quantitatively estimate its contribution to the electron production. Revealing the nanoscale mechanism of the electron yield enhancement, we provide an efficient tool for evaluating the yield of emitted electron …
Polyatomic polar molecules are promising systems for future experiments that search for violation of time-reversal and parity symmetries due to their advantageous electronic and vibrational structure, which allows laser cooling, full polarisation of the molecule, and reduction of systematic effects [I. Kozyryev and N.R. Hutzler, Phys, Rev. Lett. {\bf 119}, 133002 (2017)]. In this work we investigate the enhancement factor of the electric dipole moment of the electron ($E_\text{eff}$) in the triatomic monohydroxide molecules BaOH and YbOH within the high-accuracy relativistic coupled cluster me…
The reaction between He$^+$ and CH$_3$F forming predominantly CH$_2^+$ and CHF$^+$ has been studied at collision energies $E_{\rm coll}$ between 0 and $k_{\rm B}\cdot 10$~K in a merged-beam apparatus. To avoid heating of the ions by stray electric fields, the reaction was observed within the orbit of a highly excited Rydberg electron. Supersonic beams of CH$_3$F and He($n$) Rydberg atoms with principal quantum number $n= 30$ and 35 were merged and their relative velocity tuned using a Rydberg-Stark decelerator and deflector, allowing an energy resolution of 150 mK. A strong enhancement of the …
The relativistic coupled-cluster (RCC) method is a powerful many-body method, particularly in the evaluation of electronic wave functions of heavy atoms and molecules, and can be used to calculate various atomic and molecular properties. One such atomic property is the enhancement factor (R) of the atomic electric dipole moment (EDM) due to an electron EDM needed in electron EDM searches. The EDM of the electron is a sensitive probe of CP-violation, and its search could provide insights into new physics beyond the Standard Model, as well as open questions in cosmology. Electron EDM searches us…
We present mean-field calculations of azimuthally averaged retarded dipole-dipole interactions in a Bose-Einstein condensate induced by a laser, at both long and short wavelengths. Our calculations demonstrate that dipole-dipole interactions become significantly stronger at shorter wavelengths, by as much as 30-fold, due to retardation effects. This enhancement, along with inclusion of the dynamic polarizability, indicate a method of inducing long-range interatomic interactions in neutral atom condensates at significantly lower intensities than previously realized.
Dipole-dipole interactions are at the origin of long-lived collective atomic states, often called subradiant, which are explored for their potential use in novel photonic devices or in quantum protocols. Here, we study subradiance beyond linear optics and experimentally demonstrate a two hundred-fold increase in the population of these modes, as the saturation parameter of the driving field is increased. We attribute this enhancement to a mechanism similar to optical pumping through the well-coupled superradiant states. The lifetimes are unaffected by the pump strength, as the system is ultima…
The energy dependence of the rates of the reactions between He$^+$ and ammonia (NY$_3$, Y= {H,D}), forming NY$_2^+$, Y and He as well as NY$^+$, Y$_2$ and He, and the corresponding product branching ratios have been measured at low collision energies between 0 and $k_{\mathrm{B}}\cdot40$ K using a recently developed merged-beam technique [Allmendinger {\it et al.}, ChemPhysChem {\bf 17}, 3596 (2016)]. To avoid heating of the ions by stray electric fields, the reactions are observed within the large orbit of a highly excited Rydberg electron. A beam of He Rydberg atoms was merged with a superso…
Hyperfine-induced electric dipole contributions may significantly increase probabilities of otherwise very weak electric octupole and magnetic quadrupole atomic clock transitions (e.g. transitions between $s$ and $f$ electron orbitals). These transitions can be used for exceptionally accurate atomic clocks, quantum information processing and search for dark matter. They are very sensitive to new physics beyond the Standard Model, such as temporal variation of the fine structure constant, the Lorentz invariance and Einstein equivalence principle violation. We formulate conditions under which th…
