The electric dipole moment (EDM) of paramagnetic atoms is sensitive to the intrinsic EDM contribution from that of its constituent electrons and a scalar--pseudo-scalar (S-PS) electron-nucleus interactions. The electron EDM and the S-PS EDM contribution to atomic EDM scales as Z^3. Thus, the heavy paramagnetic atomic systems will exhibit large enhancement factors. However, the nature of the coupling is so small that it becomes an interest of high precision atomic experiments. In this work, we have computed the EDM enhancement factors of the ground states of Rb and Cs due to both the electron EDM and the S-PS EDM using the relativistic coupled-cluster (RCC) theory. The importance of obtaining the precise enhancement factors and the experimental results in deducing a reliable limit on the electron EDM is emphasized.
We present an innovative fiber laser system for both cesium and rubidium manipulation. The architecture is based on frequency conversion of two lasers at 1560 nm and 1878 nm. By taking advantage of existing fiber components at these wavelengths, we demonstrate an all fiber laser system delivering 350 mW at 780 nm for rubidium and 210 mW at 852 nm for cesium. This result highlights the promising nature of such laser system especially for Cs manipulation for which no fiber laser system has been reported. It offers new perspectives for the development of atomic instruments dedicated to onboard ap…
Resonances in the magnetic decoupling curves for the spin relaxation of dense alkali-metal vapors prove that much of the relaxation is due to the spin-axis interaction in triplet dimers. Initial estimates of the spin-axis coupling coefficients for the dimers are 290 MHz for Rb; 2500 MHz for Cs.
We develop a theoretical treatment of polarization spectroscopy and use it to make predictions about the general form of polarization spectra in the alkali atoms. Using our model, we generate theoretical spectra for the D2 transitions in 87Rb, 85Rb, and 133Cs. Experiments demonstrate that the model accurately reproduces spectra of transitions from the upper hyperfine level of the ground state only. Among these, the closed transition F -> F' = F + 1 dominates, with a steep gradient through line center ideally suited for use as a reference in laser locking.
I searched for the ground state 6.8 and 9.2 GHz hyperfine transitions of rubidium and cesium toward M- and L-dwarfs that show Rb and Cs optical resonance lines. The optical lines can pump the hyperfine transitions, potentially forming masers. These spin-flip transitions of Rb and Cs are the principal transitions used in atomic clocks (the $^{133}$Cs hyperfine transition defines the second). If they are detected in stellar atmospheres, these transitions would provide exceptionally precise clocks that can be used as accelerometers, as exoplanet detectors, as probes of the predictions of general …
We experimentally investigated Rabi resonance-based continuously frequency-tunable microwave (MW) magnetic field detection using a single hybrid vapor cell filled with cesium and rubidium atoms. The multispecies atomic systems, with their tunable abilities in transition frequencies, enabled this atomic sensing head to cover a broader detectable MW field scope compared to the use of a single metal atom. Here, we demonstrated the simultaneous observation of atomic Rabi resonance signals with 85Rb, 87Rb, and 133Cs in the same vapor cell. Using an experimentally feasible static magnetic field (DC …
Scattering of ortho positronium (Ps) by cesium and rubidium atoms has been investigated employing a three-Ps-state coupled-channel model with Ps(1s,2s,2p) states using a time-reversal-symmetric regularized electron-exchange model potential. We find a narrow S-wave singlet resonance at 5.057 eV of width 0.003 eV in the Ps-Rb system and at 5.067 eV of width 0.003 eV in the Ps-Cs system. Singlet P-wave resonances in both systems are found at 5.3 eV of width 0.4 eV. Singlet D-wave structures are found at 5.4 eV in both systems. The pronounced P- and D-wave resonances in these systems lead to easil…
Currently the theoretical uncertainty limits the interpretation of the atomic parity non-conservation (PNC) measurements. We calculate the PNC $5s$ - $6s$ electric dipole transition amplitude in rubidium and demonstrate that rubidium is a good candidate to search for new physics beyond the standard model since accuracy of the atomic calculations in rubidium can be higher than in cesium. PNC in cesium is currently the best low-energy test of the standard model, therefore, similar measurements for rubidium present a good option for further progress in the field. We also calculate nuclear spin-de…
We have experimentally realized a hybrid trap for ultracold paramagnetic rubidium and diamagnetic ytterbium atoms by combining a bichromatic optical dipole trap for ytterbium with a Ioffe-Pritchard-type magnetic trap for rubidium. In this hybrid trap, sympathetic cooling of five different ytterbium isotopes through elastic collisions with rubidium was achieved. A strong dependence of the interspecies collisional cross section on the mass of the ytterbium isotope was observed.
We consider microwave hyperfine transitions in the ground state of cesium and rubidium atoms which are presently used as the primary and the secondary frequency standards. The atoms are confined in an optical lattice generated by a circularly polarized laser field. We demonstrate that applying an external magnetic field with appropriately chosen direction may cancel dynamic Stark frequency shift making the frequency of the clock transition insensitive to the strengths of both the laser and the magnetic fields. This can be attained for practically any laser frequency which is sufficiently dista…
We investigate the phenomenon of optical bistability in a driven ensemble of Rydberg atoms. By performing two experiments with thermal vapors of rubidium and cesium, we are able to shed light onto the underlying interaction mechanisms causing such a non-linear behavior. Due to the different properties of these two atomic species, we conclude that the large polarizability of Rydberg states in combination with electric fields of spontaneously ionized Rydberg atoms is the relevant interaction mechanism. In the case of rubidium, we directly measure the electric field in a bistable situation via tw…
Three body resonant interactions between Rydberg atoms are considered in order to perform few-body quantum gates. So far, the resonances found in cesium or rubidium atoms relied on an adjacent two-body resonance which ceases to exist for principal quantum numbers above $n \simeq 40$. We have proposed recently a new class of 3-body interaction resonances in alkali-metal Rydberg atoms [P. Cheinet \textit{et al.}, Quant. Elect. \textbf{50}, 213 (2020)], which circumvienes this limit. We investigate here the relative strength between this new class of 3-body interaction resonance and quasi-forbidd…
The enhancement factors of the electric dipole moment (EDM) of the ground states of two paramagnetic atoms; rubidium (Rb) and caesium (Cs) which are sensitive to the electron EDM are computed using the relativistic coupled-cluster theory and our results are compared with the available calculations and measurements. The possibility of improving the limit for the electron EDM using the results of our present work is pointed out.
Atomic vapor of four different paramagnetic species: gold, silver, lithium, and rubidium, is produced and studied inside several buffer gases: helium, nitrogen, neon, and argon. The paramagnetic atoms are injected into the buffer gas using laser ablation. Wires with diameters 25 $μ$m, 50 $μ$m, and 100 $μ$m are used as ablation targets for gold and silver, bulk targets are used for lithium and rubidium. The buffer gas cools and confines the ablated atoms, slowing down their transport to the cell walls. Buffer gas temperatures between 20 K and 295 K, and densities between $10^{16}$ cm$^{-3}$ and…
We measure the transverse relaxation of the spin state of an ensemble of ground-state rubidium atoms trapped in solid parahydrogen at cryogenic temperatures. We find the spin dephasing time of the ensemble (T$_2^*$) is limited by inhomogeneous broadening. We determine that this broadening is dominated by electrostatic interactions with the host matrix, and can be reduced by preparing nonclassical spin superposition states. Driving these superposition states gives significantly narrower electron paramagnetic resonance lines and the longest reported electron spin $T_2^*$ in any solid-phase syste…
We present studies of strong coupling in single-photon photoassociation of cesium dimers using an optical dipole trap. A thermodynamic model of the trap depletion dynamics is employed to extract absolute rate coefficents. From the dependence of the rate coefficient on the photoassociation laser intensity, we observe saturation of the photoassociation scattering probability at the unitarity limit in quantitative agreement with the theoretical model by Bohn and Julienne [Phys. Rev. A, 60, 414 (1999)]. Also the corresponding power broadening of the resonance width is measured. We could not observ…
The influence of negative-energy states (NES) on forbidden magnetic-dipole $ns_{1/2}-(n+1)s_{1/2}$ transitions in alkali-metal atoms is investigated. We find that the NES contributions are significant in almost all cases and for rubidium reduce the transition rate by a factor of 8. We tabulate magnetic-dipole (M_1) transition amplitudes for the alkalis. Our M_1 value for cesium, where accurate measurements are available, differs from experiment by 16%. We briefly discuss the feasibility of an experimental test of NES effects.
Electric dipole moments constitute a competitive method to search for new physics, being particularly sensitive to new CP-violating phases. Given the experimental and theoretical progress in this field and more generally in particle physics, the necessity for more reliable bounds than the ones usually employed emerges. We therefore propose an improved extraction of the electric dipole moment of the electron and the relevant coefficient of the electron-nucleon coupling, taking into account theoretical uncertainties and possible cancellations, to be used in model-dependent analyses. Specifically…
We demonstrate how Rydberg atoms and the phenomena of electromagnetically induced transparency can be used to aid in the recording of a musical instrument in real time as it is played. Also, by using two different atomic species (cesium and rubidium) in the same vapor cell, we demonstrate the ability to record two guitars simultaneously, where each atomic species detects and allows for the recording of each guitar separately. The approach shows how audio data (the musical composition) can be detected with a quantum system, illustrating how we can control ensembles of atoms to such an extent th…
We present calculations of the photoionization (PI) cross sections of rubidium and cesium Rydberg atoms for light with wavelengths ranging from the infrared to the ultraviolet, using model potentials from [M. Marinescu, H. R. Sadeghpour, and A. Dalgarno, Phys. Rev. A 49, 982 (1994)]. The origins of pronounced PI minima are identified by investigating the free-electron wavefunctions. These include broad PI minima in the $nS$ to $εP$ PI channels of both Rb and Cs, with free-electron energy $ε$, which are identified as Cooper minima. Much narrower PI minima in the $nD$ to $εF$ channels are due to…
A physics package for a compact cold atomic clock is hereby presented. The uniqueness of this package is its small dimensions that enable, for the first time, implementation of a primary cold atomic clock in a standard package of 3U height (=133mm). These dimensions are made possible by using an in-vacuum Microwave (MW) Loop Gap Resonator (LGR) whose length and diameter can be reduced from those of a typical resonator. Following our presentation of the design, we analyze the homogeneity of the MW field amplitude and phase. We find that the expected clock instability due to non-uniformity of th…
We measure the sensitivity of a broadband atomic magnetometer using quantum non-demolition spin measurements. A cold, dipole-trapped sample of rubidium atoms provides a long-lived spin system in a non-magnetic environment, and is probed non-destructively by paramagnetic Faraday rotation. The calibration procedure employs a known reference state, the maximum-entropy or 'thermal' spin state and quantitative imaging-based atom counting to identify electronic, quantum, and technical noise in both the probe and spin system. The measurement achieves sensitivity 2.8 dB better than the projection nois…
We demonstrate simultaneous electromagnetically-induced transparency (EIT) with cesium (Cs) and rubidium (Rb) Rydberg atoms in the same vapor cell with coincident (overlapping) optical fields. Each atomic system can detect radio frequency (RF) electric (E) field strengths through modification of the EIT signal (Autler-Townes (AT) splitting), which leads to a direct SI traceable RF E-field measurement. We show that these two systems can detect the same the RF E-field strength simultaneously, which provides a direct in situ comparison of Rb and Cs RF measurements in Rydberg atoms. In effect, thi…
Quantum processing architectures that include multiple qubit modalities offer compelling strategies for high-fidelity operations and readout, quantum error correction, and a path for scaling to large system sizes. Such hybrid architectures have been realized for leading platforms, including superconducting circuits and trapped ions. Recently, a new approach for constructing large, coherent quantum processors has emerged based on arrays of individually trapped neutral atoms. However, these demonstrations have been limited to arrays of a single atomic element where the identical nature of the at…
We employ collisions of individual atomic cesium (Cs) impurities with an ultracold rubidium (Rb) gas to probe atomic interaction with hyperfine- and Zeeman-state sensitivity. Controlling the Rb bath's internal state yields access to novel phenomena observed in inter-atomic spin-exchange. These can be tailored at ultra-low energies, owing to the excellent experimental control over all relevant energy scales. First, detecting spin-exchange dynamics in the Cs hyperfine state manifold, we resolve a series of previously unreported Feshbach resonances at magnetic fields below 300 mG, separated by en…
