In this article, we review the history, current status, physical mechanisms, experimental methods, and applications of nonlinear magneto-optical effects in atomic vapors. We begin by describing the pioneering work of Macaluso and Corbino over a century ago on linear magneto-optical effects (in which the properties of the medium do not depend on the light power) in the vicinity of atomic resonances, and contrast these effects with various nonlinear magneto-optical phenomena that have been studied both theoretically and experimentally since the late 1960s. In recent years, the field of nonlinear magneto-optics has experienced a revival of interest that has led to a number of developments, including the observation of ultra-narrow (1-Hz) magneto-optical resonances, applications in sensitive magnetometry, nonlinear magneto-optical tomography, and the possibility of a search for parity- and time-reversal-invariance violation in atoms.
The operation of a high sensitive atomic magnetometer using resonant elliptically polarized light is demonstrated. The experimental geometry allows autonomous frequency stabilization of the laser, thereby offers compact operation of the overall device. The magnetometry is based on measurement of the zero magnetic field resonance in degenerate two level system using polarimetric detection and has a preliminary sensitivity of <10 pT/Hz1/2 @ 1 Hz.
We report a new technique for generating magnetic resonance with synchronous modulation of two-photon resonant light fields. Magnetic resonances in fluorescence from a sodium cell are measured to demonstrate suitability of this technique for remote magnetometry. A strong magnetic resonance with its dip corresponding to the Larmor frequency is produced in the presence of a transverse magnetic field. An additional resonance at 3\{Omega_L} is observed, which can be used to determine the magnetic field orientation. We have developed a theoretical model based on the density matrix equations to veri…
Results of a fairly straightforward experiment on resonant magneto-optical rotation by rubidium-87 atoms revealed strong time-dependence of the polarization plane of light emerging from atomic vapors following a sudden irradiation with a laser beam. The rotation of the plane appears as a not direct consequence of the influence of the magnetic field on atoms. Reported measurements conducted using a vapor cell without any buffer gas or an anti-relaxation wall coating show that transmitted light has initially the same (linear) polarization as the incident one. Rotation of the polarization plane c…
An additional channel opens for photoionization of atom $A$ by an electromagnetic field if it traverses a gas of atoms $B$ resonantly coupled to this field. We show that this channel, in which $A$ is ionized via resonant photoexcitation of $B$ with subsequent energy transfer to $A$ through two-center electron correlations and which is very efficient when $A$ and $B$ constitute a bound system, can strongly dominate the ionization of $A$ also in collisions where the average distance between $A$ and $B$ exceeds the typical size of a bound system by orders of magnitude.
Electron scattering and dielectronic recombination with an ion in the presence of a neighboring atom is studied. The incident electron is assumed to be captured by the ion, leading to resonant excitation of the atom which afterwards may stabilize either by electron re-emission or radiative decay. We show that the participation of the atom can strongly affect, both quantitatively and qualitatively, the corresponding processes of electron scattering and recombination. Various ion-atom systems and electronic transitions are considered. In particular we show that electron scattering under backward…
We propose and demonstrate a radio-frequency atomic magnetometer with sub-Doppler laser cooled rubidium-87. With a simple and compact design, our system demonstrates a sensitivity of $330~pT/\sqrt{Hz}$ in an unshielded environment, thus matching or surpassing previously reported cold atoms designs. By merging the multiple uses and robustness of radio-frequency atomic magnetometers with the detailed control of laser cooling, our cold atom radio-frequency magnetometer has the potential to move applications of atomic magnetometry to high spatial resolution. Direct impact in metrology for applied …
We develop an approach to generate finite-range atomic interactions via optical Rydberg-state excitation and study the underlying excitation dynamics in theory and experiment. In contrast to previous work, the proposed scheme is based on resonant optical driving and the establishment of a dark state under conditions of electromagnetically induced transparency (EIT). Analyzing the driven dissipative dynamics of the atomic gas, we show that the interplay between coherent light coupling, radiative decay and strong Rydberg-Rydberg atom interactions leads to the emergence of sizeable effective inte…
Radio communication through attenuating media necessitates the use of very-low frequency (VLF) and ultra-low frequency (ULF) carrier bands, which are frequently used in underwater and under-ground communication applications. Quantum sensing techniques can be used to circumvent hard constraints on the size, weight and noise floor of classical signal transducers. In this low-frequency range, an optically pumped atomic sample can be used to detect carrier wave modulation resonant with ground-state Zeeman splitting of alkali atoms. Using a compact, self-calibrating system we demonstrate a resonant…
We have demonstrated the resonant control of the elastic scattering cross sections in the vicinity of Feshbach resonances between $^{23}$Na$^{40}$K molecules and $^{40}$K atoms by studying the thermalization between them. The elastic scattering cross sections vary by more than two orders of magnitude close to the resonance, and can be well described by an asymmetric Fano profile. The parameters that characterize the magnetically tunable s-wave scattering length are determined from the elastic scattering cross sections. The observation of resonantly controlled elastic scattering cross sections …
Magnetic resonance in an ensemble of laser-cooled trapped Rb atoms is excited using a micro- cantilever with a magnetic tip. The cantilever is mounted on a multi-layer chip designed to capture, cool, and magnetically transport cold atoms. The coupling is observed by measuring the loss from a magnetic trap as the oscillating cantilever induces Zeeman state transitions in the atoms. Interfacing cold atoms with mechanical devices could enable probing and manipulating atomic spins with nanometer spatial resolution and single-spin sensitivity, leading to new capabilities in quantum computation, qua…
We perform a comprehensive investigation of Förster resonant energy transfer in a room-temperature thermal mixture of ammonia molecules and rubidium Rydberg atoms. Fully state-resolved measurement of the Rydberg-atom populations is achieved by combining millimeter-wave state transfer with state-selective field ionization. This allows aspects of the energy transfer process such as state dependence, ammonia pressure dependence, and dependence on the energy resonance condition to be investigated in detail. Our results pave the way for future quantum experiments combining polar molecules and Rydbe…
It is shown that the influence of the undulator field on the motion of a relativistic electron leads to a significant increase of the bremsstrahlung cross section on an atom near the end of the spectrum of undulator radiation. Observation of this effect is quite a realistic task.
We study theoretically the scattering of light by an ensemble of $N$ resonant atoms in a sub-wavelength volume. We consider the low intensity regime so that each atom responds linearly to the field. While $N$ non-interacting atoms would scatter $N^2$ more than a single atom, we find that $N$ interacting atoms scatter less than a single atom near resonance. In addition, the scattered power presents strong fluctuations, either from one realization to another or when varying the excitation frequency. We analyze this counter-intuitive behavior in terms of collective modes resulting from the light-…
We consider the resonant Casimir-Polder interaction of an excited alkali-type atom which has a single (electric dipole) transition with a Chern insulator. The Chern insulator has a nonzero, time reversal symmetry breaking Hall conductance, leading to an additional contribution to the resonant Casimir-Polder interaction which depends on the coupling between the Hall conductance and the circular polarization state of the atomic transition. We find that the resonant Casimir-Polder shift can be significantly enhanced for de-excitation frequencies near values associated with the van Hove singularit…
We experimentally study resonant light scattering by a one-dimensional randomly filled chain of cold two-level atoms. By a local measurement of the light scattered along the chain, we observe constructive interferences in light-induced dipole-dipole interactions between the atoms. They lead to a shift of the collective resonance despite the average interatomic distance being larger than the wavelength of the light. This result demonstrates that strong collective effects can be enhanced by structuring the geometrical arrangement of the ensemble. We also explore the high intensity regime where a…
When an atom is placed into an oscillating electric field with frequency far from atomic resonances, the atomic electrons partly shield this field at the nucleus. It is conjectured that when the frequency of electric field reaches an atomic resonance, the electric field at the nucleus may be significantly enhanced. In this paper, we systematically study the mechanisms of this enhancement and show that it may reach five orders in magnitude in particular cases. As an application, we consider laser-assisted neutron capture in 139-Lanthanum nucleus and screening and resonance enhancement of nuclea…
