We study the influence of off-resonant two photon transitions on high precision measurements with atom interferometers based on stimulated Raman transitions. These resonances induce a two photon light shift on the resonant Raman condition. The impact of this effect is investigated in two highly sensitive experiments: a gravimeter and a gyroscope-accelerometer. We show that it can lead to significant systematic phase shifts, which have to be taken into account in order to achieve best performances in term of accuracy and stability.
We investigate the effect of coherent population trapping (CPT) in an atom inter-ferometer gravimeter based on the use of stimulated Raman transitions. We find that CPT leads to significant phase shifts, of order of a few mrad, which may compromise the accuracy of inertial measurements. We show that this effect is rejected by the k-reversal technique, which consists in averaging inertial measurements performed with two opposite orientations of the Raman wavevector k, provided that internal states at the input of the interferometer are kept identical for both configurations.
IIn this paper we demonstrate a new scheme for Raman transitions which realize a symmetric momentum-space splitting of $4 \hbar k$, deflecting the atomic wave-packets into the same internal state. Combining the advantages of Raman and Bragg diffraction, we achieve a three pulse state labelled interferometer, intrinsically insensitive to the main systematics and applicable to all kind of atomic sources. This splitting scheme can be extended to $4N \hbar k$ momentum transfer by a multipulse sequence and is implemented on a $8 \hbar k$ interferometer. We demonstrate the area enhancement by measur…
We investigated the Raman pulse duration effect in a gravity gradiometer with two atom interferometers. Since the two atom clouds in the gradiometer experience different gravitational fields, it is hard to compensate the Doppler shifts of the two clouds simultaneously by chirping the frequency of a common Raman laser, which leads to an appreciable phase shift. When applied to an experiment measuring the Newtonian gravitational constant G, the effect contributes to a systematic offset as large as -49ppm in Nature 510, 518 (2014). Thus an underestimated value of G measured by atom interferometer…
Atom interferometers in optical cavities benefit from strong laser intensities and high-quality wavefronts. The laser frequency pairs that are needed for driving Raman transitions (often generated by phase modulating a monochromatic beam) form multiple standing waves in the cavity, resulting in a periodic spatial variation of the properties of the atom-light interaction along the cavity axis. Here, we model this spatial dependence and calculate two-photon Rabi frequencies and ac Stark shifts. We compare the model to measurements performed with varying cavity and pulse parameters such as cavity…
We present an observation of competition effect among multiple quantum paths in a Raman-type Mach-Zehnder atom interferometer. By measuring the contrast of interference fringes, the competition effect among multiple interference paths is experimentally investigated. Due to the phase competition, the contrast periodically oscillates when modulating either the phase or the interrogation time between Raman pulses. The multiple quantum paths form because of the imperfect population transfer efficiency in stimulated Raman transitions, and are verified by modulating the duration of Raman pulses. The…
We have developed a modified Michelson interferometer type Raman laser system to manipulate cold 87 Rb atoms to interfere. A frequency modulated continuous wave technique was introduced to determine the optical path difference, thus compensating it to zero to minimize the effects of common mode noise. The linewidth (full width at half maximum) of the beat signal at 6.834 GHz was measured to 1Hz limited by the resolution bandwidth of the spectral analyzer. The measured rms phase variance of the phase noise at 166 MHz was 0.015 rad2, mainly restricted by our poor performance radio frequency micr…
The use of Raman laser generated by modulation for light-pulse atom interferometer allows to have a laser system more compact and robust. However, the additional laser frequencies generated can perturb the atom interferometer. In this article, we present a precise calculation of the phase shift induced by the additional laser frequencies. The model is validated by comparison with experimental measurements on an atom gravimeter. The uncertainty of the phase shift determination limits the accuracy of our compact gravimeter at 8.10^-8 m/s^2. We show that it is possible to reduce considerably this…
We report an improved test of the weak equivalence principle by using a simultaneous $^{85}$Rb-$^{87}$Rb dual-species atom interferometer. We propose and implement a four-wave double-diffraction Raman transition scheme for the interferometer, and demonstrate its ability in suppressing common-mode phase noise of Raman lasers after their frequencies and intensity ratios are optimized. The statistical uncertainty of the experimental data for Eötvös parameter $η$ is $0.8\times10^{-8}$ at 3200 s. With various systematic errors corrected the final value is $η=(2.8\pm3.0)\times10^{-8}$. The major unc…
It is shown that using beam splitters with non-equal wave vectors results in a new recoil diagram which is qualitatively different from the well-known diagram associated with the Mach-Zehnder atom interferometer. We predict a new asymmetric Mach-Zehnder atom interferometer (AMZAI) and study it when one uses a Raman beam splitter. The main feature is that the phase of AMZAI contains a quantum part proportional to the recoil frequency. A response sensitive only to the quantum phase was found. A new technique to measure the recoil frequency and fine structure constant is proposed and studied outs…
We propose and demonstrate a method for calibrating atomic trajectories in a large-area dual-atom-interferometer gyroscope. The atom trajectories are monitored by modulating and delaying the Raman transition, and they are precisely calibrated by controlling the laser orientation and the bias magnetic field. To improve the immunity to the gravity effect and the common phase noise, the symmetry and the overlapping of two large-area atomic interference loops are optimized by calibrating the atomic trajectories and by aligning the Raman-laser orientations. The dual-atom-interferometer gyroscope is…
Using the technique of point source atom interferometry, we characterize the sensitivity of a multi-axis gyroscope based on free-space Raman interrogation of a single source of cold atoms in a glass vacuum cell. The instrument simultaneously measures the acceleration in the direction of the Raman laser beams and the component of the rotation vector in the plane perpendicular to that direction. We characterize the sensitivities for the magnitude and direction of the rotation vector measurement, which are 0.033 $^{\circ}/\mathrm{s}$ and 0.27 $^{\circ}$ with one second averaging time, respectivel…
We evaluate the sensitivity of a dual cloud atom interferometer to the measurement of vertical gravity gradient. We study the influence of most relevant experimental parameters on noise and long-term drifts. Results are also applied to the case of doubly differential measurements of the gravitational signal from local source masses. We achieve a short term sensitivity of 3*10^(-9) g/Hz^(-1/2) to differential gravity acceleration, limited by the quantum projection noise of the instrument. Active control of the most critical parameters allows to reach a resolution of 5*10^(-11) g after 8000 s on…
We present an atom interferometry technique in which the beamsplitter is split into two separate operations. A microwave pulse first creates a spin-state superposition, before optical adiabatic passage spatially separates the arms of that superposition. Despite using a thermal atom sample in a small ($600 \, μ$m) interferometry beam, this procedure delivers an efficiency of $99\%$ per $\hbar k$ of momentum separation. Utilizing this efficiency, we first demonstrate interferometry with up to $16\hbar k$ momentum splitting and free-fall limited interrogation times. We then realize a single-sourc…
We realize a Mach-Zehnder-type dual-atom-interferometer gyroscope with an interrogation arm of 40 cm length and the interference area up to 1.2 cm$^2$. The precise angular alignment of the large-scale separated Raman lasers is demonstrated by seeking the phase intersection of Ramsey-Bord$\acute{e}$ interferometers after the gravity effect is compensated and by decoupling the velocity dependent crosstalk phase shifts, and applied to build the Mach-Zehnder atom interferometer. Then a compact inertial rotation sensor is realized based on dual large-area Mach-Zehnder atom interferometers by precis…
We describe a collective state atomic interferometer (COSAIN) with the signal fringe as a function of phase-difference or rotation narrowed by $\sqrt{N}$ compared to a conventional interferometer - $N$ being the number of atoms - without entanglement. This effect arises from the interferences among collective states, and is a manifestation of interference at a Compton frequency of ten nonillion Hz, or a de Broglie wavelength of ten attometer, for $N=10^6$ and $v = 300 m/s$. The population of the collective state of interest is detected by a null measurement scheme, in which an event correspond…
In atom interferometers based on two photon transitions, the delay induced by the difference of the laser beams paths makes the interferometer sensitive to the fluctuations of the frequency of the lasers. We first study, in the general case, how the laser frequency noise affects the performance of the interferometer measurement. Our calculations are compared with the measurements performed on our cold atom gravimeter based on stimulated Raman transitions. We finally extend this study to the case of cold atom gradiometers.
A point source atom interferometer (PSI) is a device where atoms are split and recombined by applying a temporal sequence of Raman pulses during the expansion of a cloud of cold atoms behaving approximately as a point source. Unlike a conventional light pulse atom interferometer, the PSI can produce a signal that corresponds to multi-axis rotation only, independent of acceleration. In addition, it can be used to measure acceleration along one direction, independent of rotation. Here, we describe a modified PSI that can be used to measure multi-axis rotation and multi-axis acceleration. Specifi…
In the presence of Earth gravity and gravity-gradient forces, centrifugal and Coriolis forces caused by the Earth rotation, the phase of the time-domain atom interferometers is calculated with accuracy up to the terms proportional to the fourth degree of the time separation between pulses. We considered double-loop atom interferometers and found appropriate condition to eliminate their sensitivity to acceleration to get atomic gyroscope, or to eliminate the sensitivity to rotation to increase accuracy of the atomic gravimeter. Consequent use of these interferometers allows one to measure all c…
Precisely evaluating the systematic error induced by the quadratic Zeeman effect is important for developing atom interferometer gravimeters aiming at an accuracy in the regime ( ). This paper reports on the experimental investigation of Raman spectroscopy-based magnetic field measurements and the evaluation of the systematic error in the Gravimetric Atom Interferometer (GAIN) due to quadratic Zeeman effect. We discuss Raman duration and frequency step size dependent magnetic field measurement uncertainty, present vector light shift (VLS) and tensor light shift (TLS) induced magnetic field mea…
We model the formation of stable heteronuclear molecules via pulsed Raman photoassociation of a two-component Bose-Einstein condensate near a strong Feshbach resonance, for both counterintuitive and intuitive pulse sequencing. Compared to lasers alone, weak Raman photoassociation is enhanced by as much as a factor of ten (five) for a counterintuitive (intuitive) pulse sequence, whereas strong Raman photoassociation is barely enhanced at all--regardless of pulse sequence. Stronger intra-atom, molecule, or atom-molecule collisions lead to an expected decrease in conversion efficiency, but strong…
We present the realization of a compact micro-wave frequency synthesizer for an atom interferometer based on stimulated Raman transitions, applied to transportable inertial sensing. Our set-up is intended to address the hyperfine transitions of Rubidium 87 atoms at 6.8 GHz. The prototype is evaluated both in the time and the frequency domain by comparison with state-of-the-art frequency references developed at LNE-SYRTE. In free-running mode, it features a residual phase noise level of -65 dBrad$^2.Hz^{-1} at 10-Hz offset frequency and a white phase noise level in the order of -120 dBrad^2.Hz^…
We present the derivation of the frequency dependent scalar, vector, and tensor dynamical polarizabilities for the two hyperfine levels of the 87Rb atom 5s ground state. Based on the characterization of the dynamical polarizabilities, we analyze and measure the differential vector and tensor light shift between the 5s ground state sub-levels with near-resonant, stimulated Raman transitions. These results clarify that the tensor polarizabilities for the ground states of alkali atoms are absent when the light field is far-detuned from the atomic resonance and the total electronic angular momentu…
We report the observation of a novel nonlinear effect in the hard x-ray range. Upon illuminating Fe and Cu metal foils with intense x-ray pulses tuned near their respective K edges, photons at nearly twice the incoming photon energy are emitted. The signal rises quadratically with the incoming intensity, consistent with two-photon excitation. The spectrum of emitted high-energy photons comprises multiple Raman lines that disperse with the incident photon energy. Upon reaching the double K-shell ionization threshold, the signal strength undergoes a marked rise. Above this threshold, the lines c…
We present mirror and beamsplitter pulse designs that improve the fidelity of atom interferometry and increase its tolerance of systematic inhomogeneities. These designs are demonstrated experimentally with a cold thermal sample of $^{85}$Rb atoms. We first show a stimulated Raman inversion pulse design that achieves a ground hyperfine state transfer efficiency of 99.8(3)%, compared with a conventional $π$ pulse efficiency of 75(3)%. This inversion pulse is robust to variations in laser intensity and detuning, maintaining a transfer efficiency of 90% at detunings for which the $π$ pulse fideli…
Resonant Raman excitation by ultrafast vacuum ultraviolet laser pulses is a powerful means to study electron dynamics in molecules, but experiments must contend with linear background ionization: frequencies high enough to reach resonant core-valence transitions will usually ionize all occupied orbitals as well, and the ionization cross sections are usually dominant. Here we show that attosecond pulses can induce a process, transient impulsive stimulated Raman scattering, which can overwhelm valence ionization. Calculations are performed for atomic sodium, but the principal is valid for many m…
Motional ground state cooling and internal state preparation are important elements for quantum logic spectroscopy (QLS), a class of quantum information processing. Since QLS does not require the high gate fidelities usually associated with quantum computation and quantum simulation, it is possible to make simplifying choices in ion species and quantum protocols at the expense of some fidelity. Here, we report sideband cooling and motional state detection protocols for $^{138}$Ba$^+$ of sufficient fidelity for QLS without an extremely narrowband laser or the use of a species with hyperfine str…
