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arXiv 2605.30173cond-mat.mes-hall
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量子点中的相干与耗散自旋扭矩:量子自旋动力学的统一框架

Coherent and Dissipative Spin Torques in Quantum Dots: A Unified Framework for Quantum Spin Dynamics

ETH Zurich(苏黎世联邦理工学院)

Dominic Ruckert, Stepan Kovarik, Richard Schlitz, Mirco Grellmann, Aishwarya Vishwakarma, Pietro Gambardella, Sebastian Stepanow

AI总结:

本文提出一个统一理论框架,通过Lindblad主方程描述分子量子点中自旋转移、自旋扭矩和自旋共振,涵盖相干交换相互作用和耗散自旋扭矩效应,并扩展到耦合自旋系统,揭示自旋相干性和纠缠对局域自旋扭矩的响应。

摘要:

通过自旋极化隧穿对单自旋的操控为原子尺度的量子控制开辟了新途径。我们提出了一个理论框架,描述弱耦合到磁性电极的分子量子点中的自旋转移、自旋扭矩和自旋共振。通过从微观隧穿过程推导Lindblad主方程,我们在统一方法中捕获了相干交换相互作用和耗散自旋扭矩效应。我们分析了通过局域轨道的电荷输运如何影响自旋动力学,并表明随时间调制隧穿率可以诱导电子自旋共振。该框架进一步扩展到耦合自旋系统,揭示了自旋相干性和纠缠如何响应局域自旋扭矩,并强调了输运驱动的退相干源。我们的结果提供了一个通用模型来解释自旋分辨隧穿实验,并将经典自旋扭矩概念扩展到量子领域。

英文摘要:

The manipulation of single spins through spin-polarized tunneling opens new routes for quantum control at the atomic scale. We present a theoretical framework describing spin-transfer, spin torques and spin resonance in molecular quantum dots weakly coupled to magnetic electrodes. By deriving a Lindblad master equation from microscopic tunneling processes, we capture both coherent exchange interactions and dissipative spin torque effects within a unified approach. We analyze how charge transport through localized orbitals influences spin dynamics and show that modulating the tunneling rates in time can induce electron spin resonance. This framework is further extended to coupled spin systems, revealing how spin coherence and entanglement respond to local spin torques and highlighting sources of transport-driven decoherence. Our results provide a general model to interpret spin-resolved tunneling experiments and extend classical spin torque concepts into the quantum regime.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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