Radon-induced backgrounds, particularly from $^{222}$Rn and its beta-emitting progeny, present a critical challenge for next-generation liquid xenon (LXe) detectors aimed at probing dark matter down to the neutrino fog. To address this, we developed a compact hermetic gaseous xenon (GXe) detector. This device physically isolates the active volume from external radon sources by using a PTFE vessel sealed between two quartz flanges with mechanically compressed ePTFE gaskets. To quantify radon sealing performance, we implemented a dual-loop GXe circulation system and conducted a 670-hour radon-injection measurement campaign. Radon ingress into the hermetic detector was monitored using electrostatic radon detectors and photomultiplier tubes (PMTs). From these two independent measurements, the steady-state ratios of the radon concentrations inside the hermetic detector to those outside were estimated to be $ (1.1 \pm 0.1) \times 10^{-2} $ and $ (1.1 \pm 0.2) \times 10^{-2} $, corresponding to radon-leakage flows of $ (2.9 \pm 0.3) \times 10^{-11} $ and $ (2.6 \pm 0.4) \times 10^{-11} $ $ \thinspace $m$^{3}$ $ \thinspace $ $\mathrm{s}^{-1}$, respectively. An extrapolation to a 60-tonne LXe TPC such as XLZD suggests that the radon leakage could amount to $ 1.2 \times 10^{-2} $ $ \thinspace $mBq, which is negligible compared to the expected natural radon emanation inside the detector, typically 3$ \thinspace $mBq. These results demonstrate that flange-based mechanical sealing provides an effective solution for realizing radon-isolated inner detectors in large-scale LXe experiments.
The continuous emanation of $^{222}$Rn from detector surfaces causes the dominant background in current liquid xenon time projection chambers (TPCs) searching for dark matter. A significant reduction is required for the next generation of detectors which are aiming to reach the neutrino floor, such as DARWIN. $^{222}$Rn-induced back\-grounds can be reduced using a hermetic TPC, in which the sensitive target volume is mechanically separated from the rest of the detector containing the majority of Rn-emanating surfaces. We present a hermetic TPC that mainly follows the well-established design of…
The idea of a hermetic quartz chamber in a dual-phase xenon time projection chamber (TPC) has the potential to improve the detector sensitivity for direct dark matter searches in the future. A major challenge facing TPC detectors in future dark matter experiments will be the reduction of the internal background such as $^{222}$Rn and the deterioration of the ionization signal due to electronegative impurities. The hermetic quartz chamber can isolate the TPC's sensitive volume from external interference and is thus expected to prevent contamination caused by the radioactive and electronegative …
An online cryogenic distillation system for the removal of krypton and radon from xenon was designed and constructed for PandaX-4T, a highly sensitive dark matter detection experiment. The krypton content in a commercial xenon product is expected to be reduced by 7 orders of magnitude with 99% xenon collection efficiency at a flow rate of 10 kg/h by design. The same system can reduce radon content in xenon by reversed operation, with an expected radon reduction factor of about 1.8 in PandaX-4T under a flow rate of 56.5 kg/h. The commissioning of this system was completed, with krypton and rado…
A high-flow radon removal system based on cryogenic distillation was developed and constructed to reduce radon-induced backgrounds in liquid xenon detectors for rare event searches such as XENONnT. A continuous purification of the XENONnT liquid xenon inventory of 8.4 tonnes at process flows up to 71 kg/h (200 slpm) is required to achieve a radon reduction by a factor two for radon sources inside the detector. To reach such high flows, the distillation column's design features liquid xenon inlet and outlets along with novel custom-made bath-type heat exchangers with high liquefaction capabilit…
An important background in detectors using liquid xenon for rare event searches arises from the decays of radon and its daughters. We report for the first time a reduction of $^{222}$Rn in the gas phase above a liquid xenon reservoir. We show a reduction factor of $\gtrsim 4$ for the $^{222}$Rn concentration in boil-off xenon gas compared to the radon enriched liquid phase. A semiconductor-based $α$-detector and miniaturized proportional counters are used to detect the radon. As the radon depletion in the boil-off gas is understood as a single-stage distillation process, this result establishe…
The radioactive daughters isotope of 222Rn are one of the highest risk contaminants in liquid xenon detectors aiming for a small signal rate. The noble gas is permanently emanated from the detector surfaces and mixed with the xenon target. Because of its long half-life 222Rn is homogeneously distributed in the target and its subsequent decays can mimic signal events. Since no shielding is possible this background source can be the dominant one in future large scale experiments. This article provides an overview of strategies used to mitigate this source of background by means of material selec…
Long-lived radon daughters are a critical background source in experiments searching for low-energy rare events. Originating from radon in ambient air, radioactive polonium, bismuth and lead isotopes plate-out on materials that are later employed in the experiment. In this paper, we examine cleaning procedures for their capability to remove radon daughters from PTFE surfaces, a material often used in liquid xenon TPCs. We found a large difference between the removal efficiency obtained for the decay chains of $^{222}$Rn and $^{220}$Rn, respectively. This indicates that the plate-out mechanism …
We have built and operated a crystalline/vapor xenon TPC, with the goal of improving searches for dark matter. The motivation for this instrument is the fact that beta decays from the radon decay chain to the ground state presently limit the state-of-the-art liquid/vapor xenon experiments. In contrast, a crystalline xenon target has the potential to tag and reject radon-chain backgrounds, due to the time and energy signature of their decays. The present article is the first demonstration of a crystalline/vapor xenon TPC with electroluminescence (gas gain) for the electron signal readout. It al…
The radioactive noble gas radon-222 ($\mathrm{^{222}Rn}$, or Rn) produced in the uranium series is a crucial background source in many underground experiments. We have estimated the adsorption property of Rn with Activated Carbon Fibers (ACFs) in air (Air), argon (Ar), and xenon (Xe) gas. In this study, we evaluated six ACFs, named A-7, A-10, A-15, A-20, A-25, and S-25, provided from UNITIKA Ltd. We measured intrinsic radioactivity of these ACF samples, and found A-20's radioactivity of the uranium series is $<5.5$~$\mathrm{mBq/kg}$ with $90\%$ confidence level. In Air and Ar gas, we found ACF…
The noble elements, argon and xenon, are frequently employed as the target and event detector for weakly interacting particles such as neutrinos and Dark Matter. For such rare processes, background radiation must be carefully minimized. Radon provides one of the most significant contaminants since it is an inevitable product of trace amounts of natural uranium. To design a purification system for reducing such contamination, the adsorption characteristics of radon in nitrogen, argon, and xenon carrier gases on various types of charcoals with different adsorbing properties and intrinsic radioac…
The LZ dark matter detector, like many other rare-event searches, will suffer from backgrounds due to the radioactive decay of radon daughters. In order to achieve its science goals, the concentration of radon within the xenon should not exceed $2μ$Bq/kg, or 20 mBq total within its 10 tonnes. The LZ collaboration is in the midst of a program to screen all significant components in contact with the xenon. The four institutions involved in this effort have begun sharing two cross-calibration sources to ensure consistent measurement results across multiple distinct devices. We present here five p…
We describe the purification of xenon from traces of the radioactive noble gas radon using a cryogenic distillation column. The distillation column is integrated into the gas purification loop of the XENON100 detector for online radon removal. This enabled us to significantly reduce the constant $^{222}$Rn background originating from radon emanation. After inserting an auxiliary $^{222}$Rn emanation source in the gas loop, we determined a radon reduction factor of R > 27 (95% C.L.) for the distillation column by monitoring the $^{222}$Rn activity concentration inside the XENON100 detector.
We discuss an in-situ evaluation of the $^{85}$Kr, $^{222}$Rn, and $^{220}$Rn background in PandaX-I, a 120-kg liquid xenon dark matter direct detection experiment. Combining with a simulation, their contributions to the low energy electron-recoil background in the dark matter search region are obtained.
The throttling refrigeration system for high cooling power recovery of the PandaX-xT cryogenic distillation system for radon removal
SJTU Paris Elite Institute of Technology, Shanghai Jiao Tong University（上海交通大学巴黎卓越工程师学院）；New Cornerstone Science Laboratory, Tsung-Dao Lee Institute, Shanghai Jiao Tong University（新Cornerstone科学实验室，汤川秀树研究所，上海交通大学）；School of Physics and Astronomy, Shanghai Jiao Tong University（上海交通大学物理与天文学院）；Shanghai Jiao Tong University Sichuan Research Institute（上海交通大学四川研究院）；Jinping Deep Underground Frontier Science and Dark Matter Key Laboratory of Sichuan Province（四川省锦屏深地下前沿科学与暗物质重点实验室）；Vacree Technologies Co., Ltd.（沃瑞科技有限公司）；School of Chemical Engineering, Zhengzhou University（郑州大学化学工程与应用学院）；School of Physics, Sun Yat-Sen University（中山大学物理学院）；Department of Physics, University of Maryland, College Park（马里兰大学帕克分校物理系）；Yalong River Hydropower Development Company, Ltd.（雅砻江流域水电开发有限公司）
A Rn-220 source is deployed on the XENON100 dark matter detector in order to address the challenges in calibration of tonne-scale liquid noble element detectors. We show that the Pb-212 beta emission can be used for low-energy electronic recoil calibration in searches for dark matter. The isotope spreads throughout the entire active region of the detector, and its activity naturally decays below background level within a week after the source is closed. We find no increase in the activity of the troublesome Rn-222 background after calibration. Alpha emitters are also distributed throughout the…
We have developed a low-energy electron recoil (ER) calibration method with $^{220}$Rn for the PandaX-II detector. $^{220}$Rn, emanated from natural thorium compounds, was fed into the detector through the xenon purification system. From 2017 to 2019, we performed three dedicated calibration campaigns with different radon sources. We studied the detector response to $α$, $β$, and $γ$ particles with focus on low energy ER events. During the runs in 2017 and 2018, the amount of radioactivity of $^{222}$Rn were on the order of 1\% of that of $^{220}$Rn and thorium particulate contamination was ne…
We investigate the prospects for real-time detection of solar neutrinos via the charged-current neutrino-nucleus scattering process in liquid xenon time projection chambers. We use a nuclear shell model, benchmarked with experimental data, to calculate the cross sections for populating specific excited states of the caesium nuclei produced by neutrino capture on $^{131}$Xe and $^{136}$Xe. The shell model is further used to compute the decay schemes of the low-lying $1^{+}$ excited states of $^{136}$Cs, for which there is sparse experimental data. We explore the possibility of tagging the chara…
In this paper, we describe the XENON100 data analyses used to assess the target-intrinsic background sources radon ($^{222}$Rn), thoron ($^{220}$Rn) and krypton ($^{85}$Kr). We detail the event selections of high-energy alpha particles and decay-specific delayed coincidences. We derive distributions of the individual radionuclides inside the detector and quantify their abundances during the main three science runs of the experiment over a period of $\sim$ 4 years, from January 2010 to January 2014. We compare our results to external measurements of radon emanation and krypton concentrations wh…
The measurement of the internal $^{222}$Rn activity in the NEXT-White detector during the so-called Run-II period with $^{136}$Xe-depleted xenon is discussed in detail, together with its implications for double beta decay searches in NEXT. The activity is measured through the alpha production rate induced in the fiducial volume by $^{222}$Rn and its alpha-emitting progeny. The specific activity is measured to be $(38.1\pm 2.2~\mathrm{(stat.)}\pm 5.9~\mathrm{(syst.)})$~mBq/m$^3$. Radon-induced electrons have also been characterized from the decay of the $^{214}$Bi daughter ions plating out on t…
Low-Energy Radon Backgrounds from Electrode Grids in Dual-Phase Xenon TPCs
SLAC National Accelerator Laboratory（斯坦福直线加速器中心）；Kavli Institute for Particle Astrophysics and Cosmology, Stanford University（卡弗里粒子天体物理与宇宙学研究所，斯坦福大学）；University College London (UCL)（伦敦大学学院）；Brown University（布朗大学）；University of Wisconsin-Madison（威斯康星大学麦迪逊分校）；University of California, Santa Barbara（加州大学圣塔芭芭拉分校）；Imperial College London（帝国理工学院）；University of Maryland（马里兰大学）
