The radioactive noble gas radon-222 ($\mathrm{^{222}Rn}$, or Rn) produced in the uranium series is a crucial background source in many underground experiments. We have estimated the adsorption property of Rn with Activated Carbon Fibers (ACFs) in air (Air), argon (Ar), and xenon (Xe) gas. In this study, we evaluated six ACFs, named A-7, A-10, A-15, A-20, A-25, and S-25, provided from UNITIKA Ltd. We measured intrinsic radioactivity of these ACF samples, and found A-20's radioactivity of the uranium series is $<5.5$~$\mathrm{mBq/kg}$ with $90\%$ confidence level. In Air and Ar gas, we found ACF A-15 has the adsorption efficiency of $1/10000$ reduction at maximum before saturation of Rn adsorption, and more than $97\%$ adsorption efficiency after the saturation. In Xe gas, we found ACF A-20 has the best Rn adsorption ability among tested ACFs. We also found S-25, A-25, and A-15 have similar Rn adsorption performance.
A high-flow radon removal system based on cryogenic distillation was developed and constructed to reduce radon-induced backgrounds in liquid xenon detectors for rare event searches such as XENONnT. A continuous purification of the XENONnT liquid xenon inventory of 8.4 tonnes at process flows up to 71 kg/h (200 slpm) is required to achieve a radon reduction by a factor two for radon sources inside the detector. To reach such high flows, the distillation column's design features liquid xenon inlet and outlets along with novel custom-made bath-type heat exchangers with high liquefaction capabilit…
An important background in detectors using liquid xenon for rare event searches arises from the decays of radon and its daughters. We report for the first time a reduction of $^{222}$Rn in the gas phase above a liquid xenon reservoir. We show a reduction factor of $\gtrsim 4$ for the $^{222}$Rn concentration in boil-off xenon gas compared to the radon enriched liquid phase. A semiconductor-based $α$-detector and miniaturized proportional counters are used to detect the radon. As the radon depletion in the boil-off gas is understood as a single-stage distillation process, this result establishe…
The radioactive daughters isotope of 222Rn are one of the highest risk contaminants in liquid xenon detectors aiming for a small signal rate. The noble gas is permanently emanated from the detector surfaces and mixed with the xenon target. Because of its long half-life 222Rn is homogeneously distributed in the target and its subsequent decays can mimic signal events. Since no shielding is possible this background source can be the dominant one in future large scale experiments. This article provides an overview of strategies used to mitigate this source of background by means of material selec…
The noble elements, argon and xenon, are frequently employed as the target and event detector for weakly interacting particles such as neutrinos and Dark Matter. For such rare processes, background radiation must be carefully minimized. Radon provides one of the most significant contaminants since it is an inevitable product of trace amounts of natural uranium. To design a purification system for reducing such contamination, the adsorption characteristics of radon in nitrogen, argon, and xenon carrier gases on various types of charcoals with different adsorbing properties and intrinsic radioac…
Long-lived radon daughters are a critical background source in experiments searching for low-energy rare events. Originating from radon in ambient air, radioactive polonium, bismuth and lead isotopes plate-out on materials that are later employed in the experiment. In this paper, we examine cleaning procedures for their capability to remove radon daughters from PTFE surfaces, a material often used in liquid xenon TPCs. We found a large difference between the removal efficiency obtained for the decay chains of $^{222}$Rn and $^{220}$Rn, respectively. This indicates that the plate-out mechanism …
An online cryogenic distillation system for the removal of krypton and radon from xenon was designed and constructed for PandaX-4T, a highly sensitive dark matter detection experiment. The krypton content in a commercial xenon product is expected to be reduced by 7 orders of magnitude with 99% xenon collection efficiency at a flow rate of 10 kg/h by design. The same system can reduce radon content in xenon by reversed operation, with an expected radon reduction factor of about 1.8 in PandaX-4T under a flow rate of 56.5 kg/h. The commissioning of this system was completed, with krypton and rado…
Radon and radon daughters pose significant backgrounds to rare-event searching experiments. Activated carbon, which has very strong adsorption capacity for radon, can be used for radon removal and radon enrichment. The internal $^{226}$Ra concentration ultimately limits its radon enrichment ability. In order to measure the intrinsic background and study the radon adsorption capability of Saratech activated carbon at various temperatures, a radon-emanation measurement system with a high-sensitivity radon detector and an adsorption-performance research-system have been developed. In this paper, …
In order to reduce backgrounds from radon-daughter plate-out onto detector surfaces, an ultra-low-radon cleanroom is being commissioned at the South Dakota School of Mines and Technology. An improved vacuum-swing-adsorption radon mitigation system and cleanroom build upon a previous design implemented at Syracuse University that achieved radon levels of $\sim$0.2$\,$Bq$\,$m$^{-3}$. This improved system will employ a better pump and larger carbon beds feeding a redesigned cleanroom with an internal HVAC unit and aged water for humidification. With the rebuilt (original) radon mitigation system,…
The LZ dark matter detector, like many other rare-event searches, will suffer from backgrounds due to the radioactive decay of radon daughters. In order to achieve its science goals, the concentration of radon within the xenon should not exceed $2μ$Bq/kg, or 20 mBq total within its 10 tonnes. The LZ collaboration is in the midst of a program to screen all significant components in contact with the xenon. The four institutions involved in this effort have begun sharing two cross-calibration sources to ensure consistent measurement results across multiple distinct devices. We present here five p…
Long-lived alpha and beta emitters in the $^{222}$Rn decay chain on (and near) detector surfaces may be the limiting background in many experiments attempting to detect dark matter or neutrinoless double-beta decay, and in screening detectors. In order to reduce backgrounds from radon-daughter plate-out onto the wires of the BetaCage during its assembly, an ultra-low-radon cleanroom is being commissioned at Syracuse University using a vacuum-swing-adsorption radon-mitigation system. The radon filter shows ~20$\times$ reduction at its output, from 7.47$\pm$0.56 to 0.37$\pm$0.12 Bq/m$^3$, and th…
A high performance gas displacement pump based on four individual cylinders was developed. The magnetically-coupled pistons and the hermetically-sealed housings as well as the special cleanliness in terms of out-gassing and radio-purity make the four cylinder pump interesting for the usage in low background experiments dealing with noble gases as target. An optimized inner flow path as well as reduced dead volume with respect to the prototype single cylinder pump of the XENON1T experiment combined with advanced polymer piston gaskets and a piston coupling force of (3177 $\pm$ 162) N ensures a …
We describe the purification of xenon from traces of the radioactive noble gas radon using a cryogenic distillation column. The distillation column is integrated into the gas purification loop of the XENON100 detector for online radon removal. This enabled us to significantly reduce the constant $^{222}$Rn background originating from radon emanation. After inserting an auxiliary $^{222}$Rn emanation source in the gas loop, we determined a radon reduction factor of R > 27 (95% C.L.) for the distillation column by monitoring the $^{222}$Rn activity concentration inside the XENON100 detector.
We have built and operated a crystalline/vapor xenon TPC, with the goal of improving searches for dark matter. The motivation for this instrument is the fact that beta decays from the radon decay chain to the ground state presently limit the state-of-the-art liquid/vapor xenon experiments. In contrast, a crystalline xenon target has the potential to tag and reject radon-chain backgrounds, due to the time and energy signature of their decays. The present article is the first demonstration of a crystalline/vapor xenon TPC with electroluminescence (gas gain) for the electron signal readout. It al…
The continuous emanation of radon due to trace amounts of uranium and thorium in detector materials introduces radon to the active detection volume of low-background rare event search detectors. $^{222}$Rn produces a particularly problematic background in the physics region of interest by the ``naked'' beta decay of its $^{214}$Pb daughter nucleus. While charcoal-based adsorption traps are expected to be effective for radon reduction in auxiliary circulation loops that service the warm components of current {ton-scale} detectors at slow flow rates $(0.5-2\;SLPM)$, radon reduction in the entire…
We discuss an in-situ evaluation of the $^{85}$Kr, $^{222}$Rn, and $^{220}$Rn background in PandaX-I, a 120-kg liquid xenon dark matter direct detection experiment. Combining with a simulation, their contributions to the low energy electron-recoil background in the dark matter search region are obtained.
Two cryogenic bath-type heat exchangers for ultra-pure noble gas applications were developed with particular emphasis on noble gas liquefaction in cryogenic distillation systems. The main objective was to construct heat exchangers for xenon from materials that do not emanate radon and that fulfill ultra-high vacuum standards. Therefore, only high-quality copper and stainless steel materials were used. Especially, large-area oxygen-free copper fins with high conductivity in a new design ensure efficient heat transfer. One bath-type Xe-Xe heat exchanger was designed with a diameter of 50 cm to a…
NEXT-DEMO is a 1:4.5 scale prototype of the NEXT100 detector, a high-pressure xenon gas TPC that will search for the neutrinoless double beta decay of $^{136}$Xe. X-ray energy depositions produced by the de-excitation of Xenon atoms after the interaction of gamma rays from radioactive sources have been used to characterize the response of the detector obtaining the spatial calibration needed for close-to-optimal energy resolution. Our result, 5.5% FWHM at 30 keV, extrapolates to 0.6% FWHM at the Q value of $^{136}$Xe. Additionally, alpha decays from radon have been used to measure several dete…
We have developed a low-energy electron recoil (ER) calibration method with $^{220}$Rn for the PandaX-II detector. $^{220}$Rn, emanated from natural thorium compounds, was fed into the detector through the xenon purification system. From 2017 to 2019, we performed three dedicated calibration campaigns with different radon sources. We studied the detector response to $α$, $β$, and $γ$ particles with focus on low energy ER events. During the runs in 2017 and 2018, the amount of radioactivity of $^{222}$Rn were on the order of 1\% of that of $^{220}$Rn and thorium particulate contamination was ne…
The throttling refrigeration system for high cooling power recovery of the PandaX-xT cryogenic distillation system for radon removal
SJTU Paris Elite Institute of Technology, Shanghai Jiao Tong University（上海交通大学巴黎卓越工程师学院）；New Cornerstone Science Laboratory, Tsung-Dao Lee Institute, Shanghai Jiao Tong University（新Cornerstone科学实验室，汤川秀树研究所，上海交通大学）；School of Physics and Astronomy, Shanghai Jiao Tong University（上海交通大学物理与天文学院）；Shanghai Jiao Tong University Sichuan Research Institute（上海交通大学四川研究院）；Jinping Deep Underground Frontier Science and Dark Matter Key Laboratory of Sichuan Province（四川省锦屏深地下前沿科学与暗物质重点实验室）；Vacree Technologies Co., Ltd.（沃瑞科技有限公司）；School of Chemical Engineering, Zhengzhou University（郑州大学化学工程与应用学院）；School of Physics, Sun Yat-Sen University（中山大学物理学院）；Department of Physics, University of Maryland, College Park（马里兰大学帕克分校物理系）；Yalong River Hydropower Development Company, Ltd.（雅砻江流域水电开发有限公司）
The Neutrino Experiment with a Xenon TPC (NEXT), intended to investigate the neutrinoless double beta decay using a high-pressure xenon gas TPC filled with Xe enriched in 136Xe at the Canfranc Underground Laboratory in Spain, requires ultra-low background conditions demanding an exhaustive control of material radiopurity and environmental radon levels. An extensive material screening process is underway for several years based mainly on gamma-ray spectroscopy using ultra-low background germanium detectors in Canfranc but also on mass spectrometry techniques like GDMS and ICPMS. Components from…
We report on results obtained with the NEXT-DEMO prototype of the NEXT-100 high-pressure xenon gas time projection chamber (TPC), exposed to an alpha decay calibration source. Compared to our previous measurements with alpha particles, an upgraded detector and improved analysis techniques have been used. We measure event-by-event correlated fluctuations between ionization and scintillation due to electron-ion recombination in the gas, with correlation coeffcients between -0.80 and -0.56 depending on the drift field conditions. By combining the two signals, we obtain a 2.8 % FWHM energy resolut…
Low-Energy Radon Backgrounds from Electrode Grids in Dual-Phase Xenon TPCs
SLAC National Accelerator Laboratory（斯坦福直线加速器中心）；Kavli Institute for Particle Astrophysics and Cosmology, Stanford University（卡弗里粒子天体物理与宇宙学研究所，斯坦福大学）；University College London (UCL)（伦敦大学学院）；Brown University（布朗大学）；University of Wisconsin-Madison（威斯康星大学麦迪逊分校）；University of California, Santa Barbara（加州大学圣塔芭芭拉分校）；Imperial College London（帝国理工学院）；University of Maryland（马里兰大学）
