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arXiv 2507.21997cond-mat.mes-hallcond-mat.mtrl-sci
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邻近屏蔽极大提升石墨烯的电子质量

Proximity screening greatly enhances electronic quality of graphene

Daniil Domaretskiy, Zefei Wu, Van Huy Nguyen, Ned Hayward, Ian Babich, Xiao Li, Ekaterina Nguyen, Julien Barrier, Kornelia Indykiewicz, Wendong Wang, Roman V. G… 展开作者

Daniil Domaretskiy, Zefei Wu, Van Huy Nguyen, Ned Hayward, Ian Babich, Xiao Li, Ekaterina Nguyen, Julien Barrier, Kornelia Indykiewicz, Wendong Wang, Roman V. Gorbachev, Na Xin, Kenji Watanabe, Takashi Taniguchi, Lee Hague, Vladimir I. Fal'ko, Irina V. Grigorieva, Leonid A. Ponomarenko, Alexey I. Berdyugin, Andre K. Geim

AI总结:

本文通过采用间距1 nm的紧邻石墨栅极实现邻近屏蔽,将石墨烯电荷不均匀性降低两个数量级,量子迁移率达10⁷ cm²/Vs(超半导体异质结构一个量级),并观测到低场量子输运现象,为二维系统电子质量提升及新物理探索提供可靠途径。

摘要:

二维系统的电子质量在探索量子输运现象时至关重要。在半导体异质结构中,数十年的优化已产生创纪录质量的二维电子气,其输运迁移率和量子迁移率分别接近10⁸和10⁶ cm²/Vs。尽管石墨烯器件的质量也在提升,但仍相对较低。本文报道了通过采用紧邻石墨烯(间距1 nm)的石墨栅极,实现石墨烯电子质量的突破性提升。由此产生的屏蔽将电荷不均匀性降低两个数量级,降至约10⁷ cm⁻²,并将电势波动限制在1 meV以下。量子迁移率达到10⁷ cm²/Vs,比最高质量半导体异质结构的量子迁移率高一个数量级,输运迁移率则与后者的纪录相当。这种质量使石墨烯在低至1 mT的磁场中出现舒勃尼科夫-德哈斯振荡,在5 mT以下出现量子霍尔平台。尽管邻近屏蔽可预见地抑制电子-电子相互作用,但分数量子霍尔态仍可观测到,其能隙仅比未屏蔽器件降低3-5倍,表明空间尺度短于10 nm的多体现象仍保持稳健。我们的结果为提升石墨烯和其他二维系统的电子质量提供了可靠途径,这将有助于探索此前被无序掩盖的新物理现象。

英文摘要:

The electronic quality of two-dimensional systems is crucial when exploring quantum transport phenomena. In semiconductor heterostructures, decades of optimization have yielded record-quality two-dimensional gases with transport and quantum mobilities reaching close to 10$^8$ and 10$^6$ cm$^2$/Vs, respectively. Although the quality of graphene devices has also been improving, it remains comparatively lower. Here we report a transformative improvement in the electronic quality of graphene by employing graphite gates placed in its immediate proximity, at 1 nm separation. The resulting screening reduces charge inhomogeneity by two orders of magnitude, bringing it down to a few 10$^7$ cm$^-2$ and limiting potential fluctuations to less than 1 meV. Quantum mobilities reach 10$^7$ cm$^2$/Vs, surpassing those in the highest-quality semiconductor heterostructures by an order of magnitude, and the transport mobilities match their record. This quality enables Shubnikov-de Haas oscillations in fields as low as 1 mT and quantum Hall plateaus below 5 mT. Although proximity screening predictably suppresses electron-electron interactions, fractional quantum Hall states remain observable with their energy gaps reduced only by a factor of 3-5 compared to unscreened devices, demonstrating that many-body phenomena at spatial scales shorter than 10 nm remain robust. Our results offer a reliable route to improving electronic quality in graphene and other two-dimensional systems, which should facilitate the exploration of new physics previously obscured by disorder.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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