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arXiv 2501.12937cond-mat.mtrl-sci
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低温磁阻异常现象的费米面起源

Fermi surface origin of the low-temperature magnetoresistance anomaly

Yejun Feng, Yishu Wang, T. F. Rosenbaum, P. B. Littlewood, Hua Chen

AI总结:

本文证明Cr、Mo、W等大费米面良金属中也存在低温磁阻异常,并揭示尖锐费米面弧上的量子输运而非完整回旋轨道是其起源。

摘要:

低温下的磁阻(MR)异常现象已在多种体系中被观察到,从低维硫族化合物到自旋密度波和电荷密度波(SDW/CDW)金属,以及最近的拓扑半金属。在某些体系中,抛物线型磁阻可以升至其低温零场值的数十万倍。虽然这种显著效应的起源仍未解决,但这些体系通常是低载流子密度的补偿金属,其物理机制预期是准经典的。本文我们证明这种温度相关的磁阻异常也存在于具有大费米面的高电导率良金属中,即Cr、Mo和W,在线性和二次场依赖区域均存在,其非饱和分别归因于开放轨道和电子-空穴补偿。我们提供证据表明,跨越尖锐费米面弧的量子输运——但不一定是完整的回旋轨道——主导了这一低温磁阻异常。在Cr中,叠加的晶格和SDW能带结构诱导出极其尖锐的曲率。可以观察到三种现象的温度依赖性的叠加:即恒定高场下的磁阻、低场极限下的线性磁阻,以及最轻轨道的Shubnikov-de Haas(SdH)振荡。在Mo中,低温磁阻异常的温度依赖性超出了其SdH振荡的温度范围,但在Kohler标度重新出现的温度处消失。在低温和高场极限下,载流子绕量子轨道运动所产生的大磁阻是整数量子霍尔效应中载流子局域化零电导态的三维类比,尤其是在无序的不利影响方面。

英文摘要:

A magnetoresistance (MR) anomaly at low temperatures has been observed in a variety of systems, ranging from low-dimensional chalcogenides to spin and charge density wave (SDW/CDW) metals and, most recently, topological semimetals. In some systems parabolic magnetoresistance can rise to hundreds of thousands of times its low-temperature, zero-field value. While the origin of such a dramatic effect remains unresolved, these systems are often low-carrier-density compensated metals, and the physics is expected to be quasi-classical. Here we demonstrate that this MR anomaly in temperature also exists in high conductivity good metals with large Fermi surfaces, namely Cr, Mo, and W, for both linear and quadratic field-dependent regimes with their non-saturation attributed to open orbit and electron-hole compensation, respectively. We provide evidence that quantum transport across sharp Fermi surface arcs, but not necessarily the full cyclotron orbit, governs this low-temperature MR anomaly. In Cr, extremely sharp curvatures are induced by superposed lattice and SDW band structures. One observes an overlay of the temperature dependence of three phenomena: namely, MR at a constant high field, linear MR in the low-field limit, and Shubnikov-de Haas (SdH) oscillations of the lightest orbit. In Mo, the temperature dependence of low-T MR anomaly extends beyond those of its SdH oscillations but disappears at temperatures where Kohler's scaling reemerges. In the low-temperature and high-field limit, large magnetoresistance from carriers circling quantum orbits is the three-dimensional analogy to the zero-conductance state of carrier localization in the integer quantum Hall effect, especially with regard to the adverse effect of disorder.

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