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arXiv 2501.05028cond-mat.str-elcond-mat.mes-hallcond-mat.mtrl-sci
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量子材料中耦合集体激发的时域研究

Time-domain study of coupled collective excitations in quantum materials

Chenhang Xu, Alfred Zong

AI总结:

本文综述量子材料中声子、磁振子、激子及极化激元等集体模式耦合的超快时域实验,阐明激光激发、探测机制及其对非平衡动力学的调控意义。

摘要:

量子材料因其引人注目的电子、磁、热和力学性质而在未来应用方面具有巨大前景,这些性质通常源于微观自由度之间复杂的相互作用。对此类相互作用的重要认识来自对电子、自旋、轨道和晶格的集体激发的研究;它们的协同运动在决定这些体系的新颖行为方面发挥着关键作用,并为我们提供了一个关键调控手段,可通过外部扰动按需改变材料性质。在这方面,超快光-物质相互作用在控制集体激发的耦合方面展现出巨大潜力,而且众多时间分辨技术向阿秒区间的快速发展显著增进了我们对耦合机制的理解,并指导我们操控量子材料的动力学性质。本综述旨在重点介绍在时域中可视化集体激发的近期实验,聚焦不同集体模式之间的耦合机制,例如声子-声子、声子-磁振子、声子-激子、磁振子-磁振子、磁振子-激子以及各种极化激元。我们介绍这些集体模式如何被超短激光脉冲激发,并由不同的超快技术探测,同时解释集体激发之间的耦合如何支配随之产生的非平衡动力学。我们还对未来研究提出若干展望,这些研究可能带来量子材料在平衡态与非平衡态下涌现性质的发现。

英文摘要:

Quantum materials hold immense promises for future applications due to their intriguing electronic, magnetic, thermal, and mechanical properties that often arise from a complex interplay between microscopic degrees of freedom. Important insights of such interactions come from studying the collective excitations of electrons, spins, orbitals, and lattice, whose cooperative motions play a crucial role in determining the novel behavior of these systems and offer us a key tuning knob to modify material properties on-demand through external perturbations. In this regard, ultrafast light-matter interaction has shown great potential in controlling the couplings of collective excitations, and rapid progress in a plethora of time-resolved techniques down to the attosecond regime has significantly advanced our understanding of the coupling mechanisms and guided us in manipulating the dynamical properties of quantum materials. This review aims to highlight recent experiments on visualizing collective excitations in the time domain, focusing on the coupling mechanisms between different collective modes such as phonon-phonon, phonon-magnon, phonon-exciton, magnon-magnon, magnon-exciton, and various polaritons. We introduce how these collective modes are excited by an ultrashort laser pulse and probed by different ultrafast techniques, and we explain how the coupling between collective excitations governs the ensuing nonequilibrium dynamics. We also provide some perspectives on future studies that can lead to discoveries of the emergent properties of quantum materials both in and out of equilibrium.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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