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arXiv 2406.09628cond-mat.mtrl-sci
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拓扑绝缘体 Sm,Fe:Bi2Se3 单晶中的有质量 Dirac 费米子与强 Shubnikov-de Haas 振荡

Massive Dirac Fermions and Strong Shubnikov-de Haas Oscillations in Topological Insulator Sm,Fe:Bi2Se3 Single Crystals

Weiyao Zhao, Chi Xuan Trang, Qile Li, Lei Chen, Zengji Yue, Abdulhakim Bake, Cheng Tan, Lan Wang, Mitchell Nancarrow, Mark Edmonds, David Cortie, Xiaolin Wang

AI总结:

该研究在 Bi2Se3 单晶中采用 Sm 与 Fe 共掺杂,实现铁磁序、44 meV 表面带隙和高迁移率下的强 SdH 振荡,为 QAHE 与有质量 Dirac 费米子器件提供路径。

摘要:

拓扑绝缘体(TI)是一类具有独特能带结构的新兴材料,使人们能够研究固体中的量子效应,并有助于实现高性能量子器件。为了获得更好的 TI 性能,本文提出一种共掺杂策略,在 Bi2Se3 单晶中协同使用稀土 Sm 掺杂剂和过渡金属 Fe 掺杂剂,从而兼具过渡金属掺杂 TI(高铁磁有序温度且已观测到 QAHE)与稀土掺杂 TI(大磁矩和显著自旋轨道耦合)的优势。在原生单晶中观察到了铁磁有序的明确证据。角分辨光电子能谱表明,铁磁性在表面 Dirac 点处打开了一个 44 meV 的带隙。此外,3 K 下的载流子迁移率约为 7400 cm²/Vs,因此我们在纵向电阻率中观测到超强 Shubnikov-de Haas 振荡,并在低于 14 T 时于横向电阻率中观测到 Hall 台阶。我们的输运和角分辨光电子能谱结果表明,在 Bi2Se3 体系中进行稀土与过渡金属共掺杂,是实现量子反常 Hall 效应以及在电子器件中利用有质量 Dirac 费米子的一条有前景途径。

英文摘要:

Topological insulators (TIs) are emergent materials with unique band structure, which allow the study of quantum effect in solids, as well as contribute to high performance quantum devices. To achieve the better performance of TI, here we present a co-doping strategy using synergistic rare-earth Sm and transition-metal Fe dopants in Bi2Se3 single crystals, which combine the advantages of both transition metal doped TI (high ferromagnetic ordering temperature and observed QAHE), and rare-earth doped TI (large magnetic moments and significant spin orbit coupling). In the as-grown single crystals, clear evidences of ferromagnetic ordering were observed. The angle resolve photoemission spectroscopy indicate the ferromagnetism opens a 44 meV band gap at surface Dirac point. Moreover, the carrier mobility at 3 K is ~ 7400 cm2/Vs, and we thus observed an ultra-strong Shubnikov-de Haas oscillation in the longitudinal resistivity, as well as the Hall steps in transverse resistivity below 14 T. Our transport and angular resolved photoemission spectroscopy results suggest that the rare-earth and transition metal co-doping in Bi2Se3 system is a promising avenue implement the quantum anomalous Hall effect, as well as harnessing the massive Dirac fermion in electrical devices.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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