Anomalous 4$f$ fine structure in TmSe$_{1-x}$Te$_x$ across the metal-insulator transition
C. -H. Min, S. Müller, W. J. Choi, L. Dudy, V. Zabolotny, M. Heber, J. D. Denlinger, C. -J. Kang, M. Kalläne, N. Wind, M. Scholz, T. L. Lee, C. Schlueter, A. Gl… 展开作者
C. -H. Min, S. Müller, W. J. Choi, L. Dudy, V. Zabolotny, M. Heber, J. D. Denlinger, C. -J. Kang, M. Kalläne, N. Wind, M. Scholz, T. L. Lee, C. Schlueter, A. Gloskovskii, E. D. L. Rienks, V. Hinkov, H. Bentmann, Y. S. Kwon, F. Reinert, K. Rossnagel
备注：
5 pages, 4 figures for the main text, 6 pages and 5 figures for the supplementary
Hybridization between localized 4$f$ and itinerant 5$d$6$s$ states in heavy fermion compounds is a well-studied phenomenon and commonly captured by the paradigmatic Anderson model. However, the investigation of additional electronic interactions, beyond the standard Anderson model, has been limited, despite their predicted important role in the exotic quasiparticle formation in mixed-valence systems. We investigate the 4$f$ states in TmSe$_{1-x}$Te$_x$ throughout a semimetal-insulator phase transition, which drastically varies the interactions related to the 4$f$ states. Using synchrotron-based hard x-ray and extreme ultraviolet photoemission spectroscopy, we resolve subtle peak splitting in the 4$f$ peaks near the Fermi level in the mixed-valent semimetal phase. The separation is enhanced by several tens of meV by increasing the lattice parameter by a few percent. Our results elucidate the evolving nature of the 4$f$ state across the phase transition, and provide direct experimental evidence for electronic interactions beyond the standard Anderson model in mixed-valence systems.
The intermediate valent systems TmSe and SmB6 have been investigated up to 16 and 18 GPa by ac microcalorimetry with a pressure (p) tuning realized in situ at low temperature. For TmSe, the transition from an antiferromagnetic insulator for p<3 GPa to an antiferromagnetic metal at higher pressure has been confirmed. A drastic change in the p variation of the Neel temperature (Tn) is observed at 3 GPa. In the metallic phase (p>3 GPa), Tn is found to increase linearly with p. A similar linear p increase of Tn is observed for the quasitrivalent compound TmS which is at ambiant pressure equivalent…
Motivated by recent experiments, which give strong evidence for an excitonic insulating phase in $\rm TmSe_{0.45}Te_{0.55}$, we developed a scheme to quantitatively construct, for generic two-band models, the phase diagram of an excitonic insulator. As a first application of our approach, we calculated the phase diagram for an effective mass two-band model with long-range Coulomb interaction. The shielded potential approximation is used to derive a generalized gap equation controlling for positive (negative) energy gaps the transition from a semi-conducting (semi-metallic) phase to an insulati…
We calculate the critical temperature below which an excitonic insulator exists at the pressure-induced semiconductor-semimetal transition. Our approach is based on an effective-mass model for valence and conduction band electrons interacting via a statically screened Coulomb potential. Assuming pressure to control the energy gap, we derive, in the spirit of a BEC-BCS crossover scenario, a set of equations which determines, as a function of the energy gap (pressure), the chemical potentials for the two bands, the screening wave number, and the critical temperature. We (i) show that in leading …
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We present a comparative study of Nernst effect and resistivity in underdoped samples of Bi$_2$Sr$_2$CuO$_{6+δ}$ and La$_{2-x}$Sr$_{x}$CuO$_4$. The Nernst effect presents a peak in a region of the H-T diagram where resistivity shows a non-metallic temperature dependence. Our results illustrate that the mechanism of dissipation in the mixed state of underdoped cuprates is poorly understood. Large quantum superconducting fluctuations and vanishing vortex viscosity are among suggested explanations for an enhanced Nernst signal close to the superconductor-insulator boundary.
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Two-dimensional periodically driven systems can host an unconventional topological phase unattainable for equilibrium systems, termed the Anomalous Floquet-Anderson insulator (AFAI). The AFAI features a quasi-energy spectrum with chiral edge modes and a fully localized bulk, leading to non-adiabatic but quantized charge pumping. Here, we show how such a Floquet phase can be realized in a driven, disordered Quantum Anomalous Hall insulator, which is assumed to have two critical energies where the localization length diverges, carrying states with opposite Chern numbers. Driving the system at a …
The discovery of quadrupole topology opens a new horizon in the study of topological phenomena. However, the existing experimental realizations of quadrupole topological insulators in symmorphic lattices with $π$-fluxes often break the protective mirror symmetry. Here, we present a theory for anomalous quadrupole topological insulators in nonsymmorphic crystals without flux, using 2D sonic crystals with $p4gm$ and $p2gg$ symmetry groups as concrete examples. We reveal that the anomalous quadrupole topology is protected by two orthogonal glide symmetries in square or rectangular lattices. The d…
The anomalous Hall effect (AHE) is a quantum coherent transport phenomenon that conventionally vanishes at elevated temperatures because of thermal dephasing. Therefore, it is puzzling that the AHE can survive in heavy metal (HM)/antiferromagnetic (AFM) insulator (AFMI) heterostructures at high temperatures yet disappears at low temperatures. In this paper, we report that an unconventional high-temperature AHE in HM/AFMI is observed only around the Néel temperature of AFM, with large anomalous Hall resistivity up to 40 n$Ω$ cm. This mechanism is attributed to the emergence of a noncollinear AF…
We show theoretically that an undoped carbon nanotube might be an excitonic insulator---the long-sought phase of matter proposed by Keldysh, Kohn and others fifty years ago. We predict that the condensation of triplet excitons, driven by intervalley exchange interaction, spontaneously occurs at equilibrium if the tube radius is sufficiently small. The signatures of exciton condensation are its sizeable contributions to both the energy gap and the magnetic moment per electron. The increase of the gap might have already been measured, albeit with a different explanation [Deshpande et al., Scienc…
We consider the problem of the superconductor-insulator transition in the presence of disorder, assuming that the fermionic degrees of freedom can be ignored so that the problem reduces to one of Cooper pair localization. Weak disorder drives the critical behavior away from the pure critical point, initially towards a diffusive fixed point. We consider the effects of Coulomb interactions and quantum interference at this diffusive fixed point. Coulomb interactions enhance the conductivity, in contrast to the situation for fermions, essentially because the exchange interaction is opposite in sig…
We demonstrate the existence of a two-dimensional anomalous Floquet insulator (AFI) phase: an interacting (periodically-driven) non-equilibrium topological phase of matter with no counterpart in equilibrium. The AFI is characterized by a many-body localized bulk, exhibiting nontrivial micromotion within a driving period, and delocalized (thermalizing) chiral states at its boundaries. For a geometry without edges, we argue analytically that the bulk may be many-body localized in the presence of interactions, deriving conditions where stability is expected. We investigate the interplay between t…
In this paper, we study $(2+1)$-dimensional quantum anomalous Hall states, i.e. band insulators with quantized Hall conductance, using the exact holographic mapping. The exact holographic mapping is an approach to holographic duality which maps the quantum anomalous Hall state to a different state living in $(3+1)$-dimensional hyperbolic space. By studying topological response properties and the entanglement spectrum, we demonstrate that the holographic dual theory of a quantum anomalous Hall state is a $(3+1)$-dimensional topological insulator. The dual description enables a new characterizat…
The resistivity and the thermopower for Bi2Sr2Ca{1-x}RxCu2O8 single crystals are measured and analyzed with a special interest in the parent antiferromagnet insulators. Above room temperature, the parent insulators show an electric conduction confined in the CuO2 plane and a decreasing thermopower with temperature, which are very similar to those for high-$T_c$ cuprates. These data strongly suggest that essential anomalies of high-Tc cuprates inheres in the parent insulators.
The quantum anomalous Hall effect (QAHE) hosts the dissipationless chiral edge states associated with the nonzero Chern number, providing potentially significant applications in future spintronics. The QAHE usually occurs in a two-dimensional (2D) system with time-reversal symmetry breaking. In this work, we propose that the QAHE can exist in three-dimensional (3D) ferromagnetic insulators. By imposing inversion symmetry, we develop the topological constraints dictating the appearance of 3D QAHE based on the parity analysis at the time-reversal invariant points in reciprocal space. Moreover, u…
In the quantum anomalous Hall effect, chiral edge modes are expected to conduct spin polarized current without dissipation and thus hold great promise for future electronics and spintronics with low energy consumption. However, spin polarization of chiral edge modes has never been established in experiments. In this work, we theoretically study spin polarization of chiral edge modes in the quantum anomalous Hall effect, based on both the effective model and more realistic tight-binding model constructed from the first principles calculations. We find that spin polarization can be manipulated b…
Electronic states with non-trivial topology host a number of novel phenomena with potential for revolutionizing information technology. The quantum anomalous Hall effect provides spin-polarized dissipation-free transport of electrons, while the quantum spin Hall effect in combination with superconductivity has been proposed as the basis for realizing decoherence-free quantum computing. We introduce a new strategy for realizing these effects, namely by hole and electron doping kagome lattice Mott insulators through, for instance, chemical substitution. As an example, we apply this new approach …
We reveal the crucial effect of strong spin-charge coupling on high-harmonic generation (HHG) in Mott insulators. In a system with antiferromagnetic correlations, the HHG signal is drastically enhanced with decreasing temperature, even though the gap increases and the production of charge carriers is suppressed. This anomalous behavior, which has also been observed in recent HHG experiments on Ca$_2$RuO$_4$, originates from a cooperative effect between the spin-charge coupling and the thermal ensemble, and the strongly temperature-dependent coherence between charge carriers. We argue that the …
The search for topologically non-trivial states of matter has become an important goal for condensed matter physics. Here, we give a theoretical introduction to the quantum anomalous Hall (QAH) effect based on magnetic topological insulators in two-dimension (2D) and three-dimension (3D). In 2D topological insulators, magnetic order breaks the symmetry between the counter-propagating helical edge states, and as a result, the quantum spin Hall effect can evolve into the QAH effect. In 3D, magnetic order opens up a gap for the topological surface states, and chiral edge state has been predicted …
We search for dynamical magnetoelectric phenomena in three-dimensional correlated systems with spin-orbit coupling. We focus on the antiferromagnetic insulator phases where the dynamical axion field is realized by the fluctuation of the antiferromagnetic order parameter. It is shown that the dynamical chiral magnetic effect, an alternating current generation by magnetic fields, emerges due to the time dependences of the order parameter such as antiferromagnetic resonance. It is also shown that the anomalous Hall effect arises due to the spatial variations of the order parameter such as antifer…
The interplay of strong disorder and superconductivity is a topic of long-term interest in condensed matter physics. Here we explore the nonlinear THz response of superconducting NbN films close to the 3D metal-insulator transition. For the least disordered samples, the magnitude of the nonlinear $χ^{(3)}$ response follows the temperature dependence of the superfluid density as expected. In contrast, for high disorder samples near the metal-insulator transition the $χ^{(3)}$ nonlinearity persists to temperatures as high as even 4 times the $T_c$ of the cleanest sample. We discuss the possible …
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It is by now well established that periodically driven quantum many-body systems can realize topological nonequilibrium phases without any equilibrium counterpart. Here we show that, even in the absence of time translation symmetry, nonequilibrium topological phases of matter can exist in aperiodically driven systems for tunably parametrically long prethermal lifetimes. As a prerequisite, we first demonstrate the existence of longlived prethermal Anderson localization in two dimensions under random multipolar driving. We then show that the localization may be topologically nontrivial with a qu…
After the recognition of the possibility to implement Majorana fermions using the building blocks of solid-state matters, the detection of this peculiar particle has been an intense focus of research. Here we experimentally demonstrate a collection of Majorana fermions living in a one-dimensional transport channel at the boundary of a superconducting quantum anomalous Hall insulator thin film. A series of topological phase changes are controlled by the reversal of the magnetization, where a half-integer quantized conductance plateau (0.5e2/h) is observed as a clear signature of the Majorana ph…
The boundary of a topological insulator (TI) hosts an anomaly restricting its possible phases: e.g. 3D strong and weak TIs maintain surface conductivity at any disorder if symmetry is preserved on-average, at least when electron interactions on the surface are weak. However the interplay of strong interactions and disorder with the boundary anomaly has not yet been theoretically addressed. Here we study this combination for the edge of a 2D TI and the surface of a 3D weak TI, showing how it can lead to an "Anomalous Many Body Localized" (AMBL) phase that preserves the anomaly. We discuss how t…
