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arXiv 2304.13698cond-mat.mtrl-sci
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亚铁磁DyCo₃薄膜中Néel型斯格明子与畴壁的直接观测

Direct observation of Néel-type skyrmions and domain walls in a ferrimagnetic DyCo$_3$ thin film

Chen Luo, Kai Chen, Victor Ukleev, Sebastian Wintz, Markus Weigand, Radu-Marius Abrudan, Karel Prokeš, Florin Radu

AI总结:

本研究以典型亚铁磁材料DyCo₃为对象,借助STXM和XMLD技术观测到其孤立斯格明子的畴壁为Néel型,证实了体系中本征DMI的存在,为亚铁磁材料手性自旋织构调控研究提供了关键依据。

摘要:

孤立磁斯格明子是稳定的、受拓扑保护的自旋织构,因其在信息技术领域的潜在应用,成为当前研究的前沿热点。稀土-过渡金属(RE-TM)亚铁磁材料是一类独特的斯格明子宿主材料。迄今为止,这类材料中斯格明子基本特性的本质与调控机制尚未被完全阐明。我们发现,对于具有强垂直各向异性的典型亚铁磁材料DyCo₃,其亚铁磁斯格明子的尺寸可通过外磁场进行调控。此外,我们利用扫描透射X射线显微镜(STXM)的高空间分辨率,并借助稀土共振边处天然存在的强X射线磁线性二向色性(XMLD)衬度,解析了亚铁磁斯格明子的磁畴壁本质。我们证明,通过该方法可以轻松区分每个独立斯格明子的畴壁属于Bloch型还是Néel型。对于所有孤立的亚铁磁斯格明子,我们观测到其畴壁均为Néel型。这一关键信息得到了微磁模拟结果的佐证,也让我们得以确定促成该亚铁磁体系中斯格明子稳定存在的Dzyaloshinskii-Moriya相互作用(DMI)的本质。证实RE-TM材料中存在本征DMI,也将有助于更深入地理解亚铁磁材料中手性自旋织构的调控。

英文摘要:

Isolated magnetic skyrmions are stable, topologically protected spin textures that are at the forefront of research interests today due to their potential applications in information technology. A distinct class of skyrmion hosts are rare earth - transition metal (RE-TM) ferrimagnetic materials. To date, the nature and the control of basic traits of skyrmions in these materials are not fully understood. We show that for an archetypal ferrimagnetic material DyCo$_3$ that exhibits a strong perpendicular anisotropy, the ferrimagnetic skyrmion size can be tuned by an external magnetic field. Moreover, by taking advantage of the high spatial resolution of scanning transmission X-ray microscopy (STXM) and utilizing a large x-ray magnetic linear dichroism (XMLD) contrast that occurs naturally at the RE resonant edges, we resolve the nature of the magnetic domain walls of ferrimagnetic skyrmions. We demonstrate that through this method one can easily discriminate between Bloch and Néel type domain walls for each individual skyrmion. For all isolated ferrimagnetic skyrmions, we observe that the domain walls are of Néel-type. This key information is corroborated with results of micromagnetic simulations and allows us to conclude on the nature of the Dzyaloshinskii-Moriya interaction (DMI) which concurs to the stabilisation of skyrmions in this ferrimagnetic system. Establishing that an intrinsic DMI occurs in RE-TM materials will also be beneficial towards a deeper understanding of chiral spin texture control in ferrimagnetic materials.

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