Owing to the experimental discovery of magnetic skyrmions stabilized by the Dzyaloshinskii-Moriya and/or dipolar interactions in thin films, there is a recent upsurge of interest in magnetic skyrmions with antiferromagnetic spins in order to overcome the fundamental limitations inherent with skyrmions in ferromagnetic materials. Here, we report on the observation of compact ferrimagnetic skyrmions for the class of amorphous alloys consisting of 4f rare-earth and 3d transition-metal elements with perpendicular magnetic anisotropy, using a DyCo$_3$ film, that are identified by combining x-ray magnetic scattering, scanning transmission x-ray microscopy, and Hall transport technique. These skyrmions, with antiparallel aligned Dy and Co magnetic moments and a characteristic core radius of about 40~nm, are formed during the nucleation and annihilation of the magnetic maze-like domain pattern exhibiting a topological Hall effect contribution. Our findings provide a promising route for fundamental research in the field of ferrimagnetic/antiferromagnetic spintronics towards practical applications.
Orientation-resolved ultrafast spin reorientation dynamics in ferrimagnetic DyCo$_5$
Max-Born-Institut für Nichtlineare Optik und Kurzzeitspektroskopie（马克斯·玻恩非线性光学和超快光谱学研究所）；Leibniz-Institut für Kristallzüchtung（莱布尼茨晶体生长研究所）；European XFEL（欧洲X射线自由电子激光设施）；Technische Universität Berlin, Institut für Optik und Atomare Physik（柏林工业大学光学与原子物理研究所）
Magnetic skyrmions are swirling magnetic textures with novel characteristics suitable for future spintronic and topological applications. Recent studies confirmed the room-temperature stabilization of skyrmions in ultrathin ferromagnets. However, such ferromagnetic skyrmions show undesirable topological effect, the skyrmion Hall effect, which leads to their current-driven motion towards device edges, where skyrmions could easily be annihilated by topographic defects. Recent theoretical studies have predicted enhanced current-driven behaviour for antiferromagnetically exchange-coupled skyrmions…
Magnetic skyrmions are swirling magnetic textures that can be efficiently driven with spin-orbit torques with a deflected trajectory. However, pinning slows skyrmions down and alters their trajectory, which prevents a quantitative comparison to analytical models. Here, we study skyrmions driven by spin-orbit torques at room temperature in ferrimagnetic GdCo thin films, an amorphous material with low pinning. Above a sharp current depinning threshold, we observe a clearly linear velocity increase with current that extrapolates to zero and a constant deflection angle, reaching high velocities up…
Ferrimagnetic Skyrmions in a Tetragonal Mn1.9Co0.1Sb Single Crystal at Room Temperature
Anhui University（安徽大学）；Wuhan University of Technology（武汉理工大学）；High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences（中国科学院合肥物质科学研究院强磁场科学中心）
We have investigated the RE atomic distribution and its magnetic moment orientation at the region near the surface of DyCo$_{4.4 \& 4.6}$ ferrimagnetic amorphous films with perpendicular magnetic anisotropy (PMA). XMCD spectroscopy of the films at the Dy $M_{4,5}$ and Co $L_{2,3}$ edges using total electron yield (TEY) detection was performed at 2 K and 300 K temperatures, and at sample orientations ranged from 0$^{\circ}$ to 70$^{\circ}$ with respect to the magnetic easy axis. The measurements showed an apparent partial decoupling between the cobalt and dysprosium magnetic sublattices. At RT,…
Interfacial mixing of elements is a well-known phenomenon found in thin film deposition. For thin-film magnetic heterostructures, interfacial compositional inhomogeneities can have drastic effects on the resulting functionalities. As such, care must be taken to characterize the compositional and magnetic properties of thin films intended for device use. Recently, ferrimagnetic Mn$_4$N thin films have drawn considerable interest due to exhibiting perpendicular magnetic anisotropy, high domain-wall mobility, and good thermal stability. In this study, we employed X-ray photoelectron spectroscopy …
Electrical detection of topological magnetic textures such as skyrmions is currently limited to conducting materials. While magnetic insulators offer key advantages for skyrmion technologies with high speed and low loss, they have not yet been explored electrically. Here, we report a prominent topological Hall effect in Pt/Tm$_3$Fe$_5$O$_{12}$ bilayers, where the pristine Tm$_3$Fe$_5$O$_{12}$ epitaxial films down to 1.25 unit cell thickness allow for tuning of topological Hall stability over a broad range from 200 to 465 K through atomic-scale thickness control. Although Tm$_3$Fe$_5$O$_{12}$ i…
Skyrmions can be stabilized in magnetic systems with broken inversion symmetry and chiral interactions, such as Dzyaloshinskii-Moriya interactions (DMI). Further, compensation of magnetic moments in ferrimagnetic materials can significantly reduce magnetic dipolar interactions, which tend to favor large skyrmions. Tuning DMI is essential to control skyrmion properties, with symmetry breaking at interfaces offering the greatest flexibility. However, in contrast to the ferromagnet case, few studies have investigated interfacial DMI in ferrimagnets. Here we present a systematic study of DMI in fe…
Materials hosting magnetic skyrmions at room temperature could enable new computing architectures as well as compact and energetically efficient magnetic storage such as racetrack memories. In a racetrack device, information is coded by the presence/absence of magnetic skyrmions forming a chain that is moved through the device. The skyrmion Hall effect that would eventually lead to an annihilation of the skyrmions at the edges of the racetrack can be suppressed for example by anti-ferromagnetically-coupled skyrmions. However, avoiding modifications of the inter-skyrmion distances in the racetr…
Skyrmions and antiskyrmions are topologically protected spin structures with opposite topological charge. Particularly in coexisting phases, these two types of magnetic quasi-particles may show fascinating physics and potential for spintronic devices. While skyrmions are observed in a wide range of materials, until now antiskyrmions were exclusive to materials with D2d symmetry. In this work, we show first and second-order antiskyrmions stabilized by magnetic dipole-dipole interaction in Fe/Gd-based multilayers. We modify the magnetic properties of the multilayers by Ir insertion layers. Using…
The interfacial Dzyaloshinskii-Moriya interaction (DMI) in multilayers of heavy metal and ferromagnetic metals enables the stabilization of novel chiral spin structures such as skyrmions. Magnetic insulators, on the other hand can exhibit enhanced dynamics and properties such as lower magnetic damping and therefore it is of interest to combine the properties enabled by interfacial DMI with insulating systems. Here, we demonstrate the presence of interfacial DMI in heterostructures that include insulating magnetic layers. We use a bilayer of perpendicularly magnetized insulating thulium iron ga…
Recently, magnetic skyrmion has emerged as an active topic of fundamental study and applications in magnetic materials research. Magnetic skyrmions are vortex-like spin excitations with topological protection and therefore are more robust to pinning compared with magnetic domain walls. We employ atomistic simulations to create room-temperature ultra-small Neel skyrmions in amorphous ferrimagnet. The fast propagation and low-dissipation dynamics of ultra-small ferrimagnetic skyrmions make them attractive for utilization as an alternative to domain walls in spin-based memory and logic devices.
Spintronic devices based on magnetic skyrmions are a promising candidate for next-generation memory applications due to their nanometre-size, topologically-protected stability and efficient current-driven dynamics. Since the recent discovery of room-temperature magnetic skyrmions, there have been reports of current-driven skyrmion displacement on magnetic tracks and demonstrations of current pulse-driven skyrmion generation. However, the controlled annihilation of a single skyrmion at room temperature has remained elusive. Here we demonstrate the deterministic writing and deleting of single is…
Thermal Evolution of Skyrmions in Synthetic Ferrimagnets of Co/Gd Heterostructure for Topological Spintronic Applications
National Institute of Science Education and Research (NISER)（印度科学教育研究所）；Homi Bhabha National Institute (HBNI)（霍米·巴巴国立大学）；Indian Institute of Science Education and Research (IISER) Mohali（印度科学教育研究学院莫哈利分校）；Durham University（杜伦大学）
We report spin-current generation related with skyrmion dynamics resonantly excited by a microwave in a helimagnetic insulator $\mathrm{Cu_2OSeO_3}$. A Pt layer was fabricated on $\mathrm{Cu_2OSeO_3}$ and voltage in the Pt layer was measured upon magnetic resonance of $\mathrm{Cu_2OSeO_3}$ to electrically detect injected spin currents via the inverse spin Hall effect (ISHE) in Pt. We found that ISHE-induced electromotive forces appear in the skyrmion phase of $\mathrm{Cu_2OSeO_3}$ as well as in the ferrimagnetic phase, which shows that magnetic skyrmions can contribute to the spin pumping effe…
Chiral magnetic phases with an unconventional topological twist in the magnetization are of huge interest due to their potential in spintronics applications. Here, we present a general method to induce such exotic magnetic phases using interfacial phase frustration within artificially grown superlattices. To demonstrate our method, we consider a multilayer with two different chiral magnetic phases as the competing orders at the top and bottom and show, using Monte Carlo calculations, that the interfacial phase frustration is realized at the central layer. In particular, we obtain three unconve…
Charged particles exhibit the Hall effect in the presence of magnetic fields. Analogously, ferromagnetic skyrmions with non-zero topological charges and finite fictitious magnetic fields exhibit the skyrmion Hall effect, which is detrimental for applications. The skyrmion Hall effect has been theoretically predicted to vanish for antiferromagnetic skyrmions because the fictitious magnetic field, proportional to net spin density, is zero. We experimentally confirm this prediction by observing current-driven transverse elongation of pinned ferrimagnetic bubbles. Remarkably, the skyrmion Hall eff…
Emergence of a spin Hall topological Hall effect in the non-collinear phase of the ferrimagnetic insulator terbium-iron garnet
Institute of Physics, Johannes Gutenberg University Mainz（美因茨约翰内斯·古腾堡大学物理研究所）；Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons (ER-C-1), Forschungszentrum Jülich GmbH（于利希研究中心格恩斯特·鲁斯卡电子显微与光谱中心（ER-C-1））；Center for Quantum Spintronics, Department of Physics, Norwegian University of Science and Technology（挪威科技大学量子自旋电子学中心）
We present long-wavelength neutron diffraction data measured on both single crystal and polycrystalline samples of the skyrmion host material Cu$_{2}$OSeO$_{3}$. We observe magnetic satellites around the $(0\bar{1}1)$ diffraction peak not accessible to other techniques, and distinguish helical from conical spin textures in reciprocal space. We confirm successive transitions from helical to conical to field polarised ordered spin textures as the external magnetic field is increased. The formation of a skyrmion lattice with propagation vectors perpendicular to the field direction is observed in …
Solitonic magnetic excitations such as domain walls and, specifically, skyrmionics enable the possibility of compact, high density, ultrafast,all-electronic, low-energy devices, which is the basis for the emerging area of skyrmionics. The topological winding of skyrmion spins affects their overall lifetime, energetics and dynamical behavior. In this review, we discuss skyrmionics in the context of the present day solid state memory landscape, and show how their size, stability and mobility can be controlled by material engineering, as well as how they can be nucleated and detected. Ferrimagnet…
The manipulation of magnetism with a gate voltage is expected to lead the way towards the realization of energy-efficient spintronics devices and high-performance magnetic memories. Exploiting magneto-ionic effects under micro-patterned electrodes in solid-state devices adds the possibility to modify magnetic properties locally, in a non-volatile and reversible way. Tuning magnetic anisotropy, magnetization and Dzyaloshinskii-Moriya interaction allows modifying at will the dynamics of non trivial magnetic textures such as skyrmions and chiral domain walls in magnetic race tracks. In this work,…
Anisotropic mesoscale magnetic scattering across the spin-reorientation transition in TbMn6Sn6
Spallation Neutron Source Science Center（散裂中子源科学中心）；Institute of High Energy Physics, Chinese Academy of Sciences (CAS)（中国科学院高能物理研究所）；Guangdong Provincial Key Laboratory of Extreme Conditions（广东省极端条件重点实验室）
