TbMn6Sn6 is a metallic ferrimagnet that displays signatures of band topology arising from a combination of uniaxial ferromagnetism and spin-orbit coupling within its Mn kagome layers. Whereas the low energy magnetic excitations can be described as collective spin waves using a local moment Heisenberg model, sharply defined optical and flat-band collective magnon modes are not observed. In their place, we find overdamped chiral and flat-band spin correlations that are localized to hexagonal plaquettes within the kagome layer.
The magnetization and specific heat measurements have been performed on single-crystalline Gd_3_Ru_4_Al_12_ with a distorted Kagome lattice structure. This spin system is regarded as an antiferromagnetic triangular lattice of XY like Heisenberg model at low temperatures. The magnetic phase diagrams indicate the existence of frustration and Z_2_ degeneracy. The magnetization and specific heat imply the successive phase transitions with partial disorder and a T-shaped spin structure in the ground state.
In this work, topological properties of a ferromagnetic Heisenberg model on a breathing kagome lattice are investigated extensively in the presence of Dzyaloshinskii-Moriya interaction. While the kagome ferromagnet hosts only a single first order topological phase, the breathing kagome system exhibits multiple first and second order topological phases along with their coexistence. Magnon dispersion relation is obtained by using linear spin wave theory. Flat band and Dirac cones are obtained in the absence of Dzyaloshinskii-Moriya interaction. A topological phase diagram is presented where seve…
Materials with zero energy band gap display intriguing properties including high sensitivity of the electronic band structure to external stimulus such as pressure or magnetic field. An interesting candidate for zero energy band gap are Weyl nodes at the Fermi level EF. A prerequisite for the existence of Weyl nodes is to either have inversion or time reversal symmetry broken. Weyl nodes in systems with broken time reversal symmetry are ideal to realize the tunability of the electronic band structure by magnetic field. Theoretically, it has been shown that in ferromagnetic Weyl materials, the …
Due to an uprise in the variety of candidate compounds, kagome metals have recently gained significant attention. Among other features, kagome metals host Dirac cones as a key band structure feature away from half filling, and potentially yield an exceptionally large fine structure, beyond values found in other 2D Dirac materials such as graphene. We investigate the possibility of chiral symmetry breaking in kagome metals. Based on a heuristic lattice model, we determine the critical coupling strength and the ordering pattern by means of a Schwinger-Dyson mean-field analysis. As the leading in…
We propose in this work an effective field theory description of the chiral spin liquid state in Heisenberg spin system on kagomé lattice.To this end, we derive the low-energy effective theory of kagomé (isotropic) Heisenberg antiferromagnet around its ordered ground states found numerically and show that quantum fluctuations induced by further neighbor spin exchanges are equally strong as those from first neighbor.We use a chiral order parameter theory to argue for the occurrence of finite temperature chiral symmetry breaking transition into chiral ordered state in kagomé antiferromagnet with…
The breaking of chiral and time-reversal symmetries provides a pathway to exotic quantum phenomena and topological phases. In particular, the breaking of chiral (mirror) symmetry in quantum materials has been shown to have important technological applications. Recent work has extensively explored the resulting emergence of chiral charge orders and chiral spin liquids on the kagomé lattice. Such chiral spin liquids are closely tied to bosonic fractional quantum Hall states and host anyonic quasiparticles; however, their connection to nearby magnetically ordered states has remained a mystery. He…
Novel magnetic phases are expected to occur in highly frustrated spin systems. Here we study the structurally perfect kagomé antiferromagnet CdCu$_3$(OH)$_6$(NO$_3$)$_2\cdot$H$_2$O by magnetization, magnetic torque, and heat capacity measurements using single crystals.An antiferromagnetic order accompanied by a small spontaneous magnetization that surprisingly is confined in the kagomé plane sets in at $T_\mathrm{N}\approx$4 K, well below the nearest-neighbor exchange interaction $J / k_B$ = 45 K.This suggests that a unique $\bf q = 0$ type 120$^\circ$ spin structure with "negative" (downward)…
Two Dimensional Kagome Correlations and Field Induced Order in the Ferromagnetic XY Pyrochlore Yb2Ti2O7
中子散射测量表明，铁磁XY烧绿石Yb 2 Ti 2 O 7在低温下表现出很强的准二维（2D）自旋关联，在适当的磁场作用下，这种关联让位于长程序（LRO）.由于< 111 >这些2D自旋相关性沿方向的散射棒意味着立方烧绿石系统的磁分解成解耦的可果美平面。沿[1-10]方向施加约0.5 T的磁场，诱导向3D LRO状态的转变，其特征在于长寿命的色散自旋波。我们的测量绘制出一个复杂的低温场相图，这种异国情调的烧绿石磁铁。
Using a perturbative renormalization group approach, we show that the extended ($J_1$-$J_2$-$J_d$) Heisenberg model on the kagome lattice with a staggered chiral interaction ($J_χ$) can exhibit a gapless chiral quantum spin liquid phase. Within a coupled-chains construction, this phase can be understood as a chiral sliding Luttinger liquid with algebraic decay of spin correlations along the chain directions. We calculate the low-energy properties of this gapless chiral spin liquid using the effective field theory and show that they are compatible with the predictions from parton mean-field the…
In this Letter, we identify a noncoplanar chiral spin texture on the distorted kagomé-lattice antiferromagnets induced by the presence of a magnetic field applied perpendicular to the distorted kagomé plane. The noncoplanar chiral spin texture has a nonzero scalar spin chirality similar to a chiral quantum spin liquid with broken time-reversal symmetry. In the noncoplanar regime we observe nontrivial topological magnetic excitations and thermal Hall response through the emergent field-induced scalar spin chirality in contrast to collinear ferromagnets in which the Dzyaloshinskii-Moriya (DM) sp…
We introduce $\mathrm{Nd_{3}Sb_{3}Mg_{2}O_{14}}$ with ideal kagome lattices of neodymium ions in ABC stacking. Thermodynamic measurements show a Curie-Weiss temperature of $Θ_{CW}=-0.12~$K, a Nd$^{3+}$ spin-1/2 Kramers doublet ground state, and a second order phase transition at $T_N=0.56(2)~$K. Neutron scattering reveals non-coplanar scalar chiral ${\bf k} =0$ magnetic order with a correlation length exceeding 400 Å= 55 $a$ and an ordered moment of $1.79(5)~μ_B$. This order includes a canted ferromagnetic component perpendicular to the kagome planes favored by Dzyaloshinskii-Moriya interactio…
The study of electronic and magnetic properties of kagome lattice has been an active research area searching for topological phases of matters. In particular, the kagome system with transition metal stannides and etc exhibit interesting anomalous Hall effects driven by ferromagnetic or non-collinear magnetic ordering. In this paper, motivated by these pioneer works, we study strongly correlated spin-orbit coupled electrons in kagome lattice at 1/3 filling. Using both Hartree-Fock approach and effective model analysis, we report quantum phase transitions accompanied with distinct charge and mag…
The neutron diffraction and nuclear magnetic resonance (NMR) measurements have been used to microscopically analyze the magnetic structure in the $S = 1/2$ kagome antiferromagnet CdCu$_{3}$(OH)$_{6}$(NO$_{3}$)$_{2}\cdot $H$_{2}$O. Below the magnetic ordering temperature $T_N\simeq 4$ K, magnetic Bragg reflections at (110) and (100) were found in the neutron diffraction pattern, which suggests a $q=0$ magnetic structure. Furthermore, the vector spin chirality for the $q=0$ structure was successfully identified from the internal field direction obtained by the $^{14}$N-NMR measurement. Our findi…
Superconductors with kagome lattices have been identified for over 40 years, with a superconducting transition temperature TC up to 7K. Recently, certain kagome superconductors have been found to exhibit an exotic charge order, which intertwines with superconductivity and persists to a temperature being one order of magnitude higher than TC. In this work, we use scanning tunneling microscopy (STM) to study the charge order in kagome superconductor RbV3Sb5. We observe both a 2x2 chiral charge order and nematic surface superlattices (predominantly 1x4). We find that the 2x2 charge order exhibits…
The theoretical description of non-Fermi liquids is among the most challenging questions in strongly correlated quantum matter. While there are many experimental candidates for such phases, few examples can be studied using controlled theoretical approaches. Here we introduce a novel conceptual perspective to analytically describe the non-Fermi liquid physics of gapless spin liquids arising in a family of two- and three-dimensional Kagome models. We first discuss a symmetry-protection mechanism that is responsible for the stability of the gapless phase. We then re-cast the two-dimensional Kago…
The kagome lattice is a two-dimensional network of corner-sharing triangles known as a platform for exotic quantum magnetic states. Theoretical work has predicted that the kagome lattice may also host Dirac electronic states that could lead to topological and Chern insulating phases, but these have evaded experimental detection to date. Here we study the d-electron kagome metal Fe$_3$Sn$_2$ designed to support bulk massive Dirac fermions in the presence of ferromagnetic order. We observe a temperature independent intrinsic anomalous Hall conductivity persisting above room temperature suggestiv…
We calculate dynamical spin structure factors for gapped chiral spin liquid states in the spin-1/2 Heisenberg antiferromagnet on the kagome lattice using Schwinger-boson mean-field theory. In contrast to static (equal-time) structure factors, the dynamical structure factor shows clear signatures of time-reversal symmetry breaking for chiral spin liquid states. In particular, momentum inversion $\bm{k} \to -\bm{k}$ symmetry as well as the six-fold rotation symmetry around the $Γ$-point are lost. We highlight other interesting features, such as a relatively flat onset of the two-spinon continuum…
Chiral three-spin interactions can suppress long-range magnetic order and stabilize quantum spin liquid states in frustrated lattices. We study a spin-1/2 model on the kagome lattice involving a staggered three-spin interaction $J_χ$ in addition to Heisenberg exchange couplings $J_1$ on nearest-neighbor bonds and $J_d$ across the diagonals of the hexagons. We explore the phase diagram using a combination of a classical approach, parton mean-field theory, and variational Monte Carlo methods. We obtain a variety of noncoplanar magnetic orders, including a phase that interpolates between cuboc-1 …
We present a study of the low temperature phases of the antiferromagnetic extended classical Heisenberg model in the kagome lattice, up to third nearest neighbors. First, we focus on the degenerate lines in the boundaries of the well-known staggered chiral phases. These boundaries have either semi-extensive or extensive degeneracy, and we discuss the partial selection of states by thermal fluctuations. Then, we study the model under an external magnetic field on these lines and in the staggered chiral phases. We pay particular attention to the highly frustrated point, where the three exchange …
We study $S=1$ spin liquid states on the kagome lattice constructed by Gutzwiller-projected $p_x+ip_y$ superconductors. We show that the obtained spin liquids are either non-Abelian or Abelian topological phases, depending on the topology of the fermionic mean-field state. By calculating the modular matrices $S$ and $T$, we confirm that projected topological superconductors are non-Abelian chiral spin liquid (NACSL). The chiral central charge and the spin Hall conductance we obtained agree very well with the $SO(3)_1$ (or, equivalently, $SU(2)_2$) field theory predictions. We propose a local H…
The infinite projected entangled simplex state (iPESS), a type of tensor network (TN) state, has been used successfully for simulating and characterizing {\it non-chiral} spin liquids on the kagome lattice. Here, we demonstrate that iPESS also provides a faithful representation of a {\it chiral} spin liquid (CSL) on the same lattice, namely the ground state of the spin-$1/2$ kagome Heisenberg antiferromagnet with a scalar chirality. By classifying local tensors according to SU$(2)$ and point group symmetries, we construct a chiral ansatz breaking reflection $P$ and time reversal $T$ symmetries…
The higher-order topological insulator (HOTI) protected by spacial symmetry has been studied in-depth on models with square lattice. Our work, based on an alternative model on the breathing Kagome lattice, revealed that the different types of corners in the lattice could actually be conditionally gapless, or always gapped. Using the Wilson loop formalism, we argue that these corner states occur when the eigenvalues of the Wannier Hamiltonian cross through a certain reference point during the conceptual "pumping" procedure. The results demonstrate the corner of the Kagome lattice based HOTI is …
We develop a theory for the thermal Hall coefficient in a spin-$\frac{1}{2}$ system on a strip of Kagome lattice, where a chiral spin-interaction term is present. To this end, we model the Kagome strip as a three-leg $XXZ$ spin-ladder, and use Bosonization to derive a low-energy theory for the spinons in this system. Introducing further a Dzyaloshinskii-Moriya interaction ($D$) and a tunable magnetic field ($B$), we identify three distinct $B$-dependent quantum phases: a valence-bond crystal (VBC), a "metallic" spin liquid (MSL) and a chiral spin liquid (CSL). In the presence of a temperature …
The antiferromagnetism in $α$-Cu$_3$Mg(OH)$_6$Br$_2$ was studied by magnetic-susceptibility, specific-heat and neutron-diffraction measurements. The crystal structure consists of Cu$^{2+}$ kagome layers with Mg$^{2+}$ ions occupying the centers of the hexagons, separated by Br$^{1-}$ ions. The magnetic system orders antiferromagnetically at 5.4 K with the magnetic moments aligned ferromagnetically within the kagome planes. The ordered moment is 0.94 $μ_B$, suggesting little quantum and geometrical fluctuations. By comparing the magnetic and specific-heat properties with those of the haydeeite,…
We consider a spin-$\frac{1}{2}$ kagome-like chain with competing ferro- and antiferromagnetic anisotropic exchange interactions. The ground state phase diagram of this model consists of the ferromagnetic and ferrimagnetic phases. We study the ground state and the low-temperature properties on the phase boundary between these phases. The ground state on this phase boundary is macroscopically degenerate and consists of localized magnon states. We calculate the ground state degeneracy and corresponding residual entropy. The spontaneous magnetization has a jump on the phase boundary confirming th…
The two-dimensional kagome lattice hosts Dirac fermions at its Brillouin zone corners K and K', analogous to the honeycomb lattice. In the density functional theory electronic structure of ferromagnetic kagome metal Fe$_3$Sn$_2$, without spin-orbit coupling we identify two energetically split helical nodal lines winding along $z$ in the vicinity of K and K' resulting from the trigonal stacking of the kagome layers. We find that hopping across A-A stacking introduces a layer splitting in energy while that across A-B stacking controls the momentum space amplitude of the helical nodal lines. The …
Spin Liquid Landscapes in the Kagome Lattice: A Variational Monte Carlo Study of the Chiral Heisenberg Model and Experimental Signatures
Korea Advanced Institute of Science and Technology（韩国科学技术院）；University of Notre Dame（圣母大学）；HUN-REN Wigner Research Centre for Physics（匈牙利研究与创新网络维格纳物理研究中心）
The anomalous Hall effect is investigated for ferromagnetic Fe3Sn2 single crystal with geometrically frustrated kagome bilayer of Fe. The scaling behavior between anomalous Hall resistivity rho_{xy}^{A} and longitudinal resistivity rho_{xx} is quadratic and further analysis implies that the AHE in Fe3Sn2 single crystal should be dominated by the intrinsic Karplus-Luttinger mechanism rather than extrinsic skew-scattering or side-jump mechanisms. Moreover, there is a sudden jump of anomalous Hall conductivity sigma_{xy}^{A} appearing at about 100 K where the spin-reorientation transition from th…
While the existence of a chiral spin liquid (CSL) on a class of spin-1/2 kagome antiferromagnets is by now well-established numerically, a controlled theoretical path from the lattice model leading to a low energy topological field theory is still lacking. This we provide via an explicit construction, starting from reformulating a microscopic model for a CSL as a lattice gauge theory, and deriving the low-energy form of its continuum limit. A crucial ingredient is the realisation that the bosonic spinons of the gauge theory exhibit a $U(1)$ symmetry-protected topological (SPT) phase, which upo…
We present a study of the thermal Hall effect in the extended Heisenberg model with $XXZ$ anisotropy in the kagome lattice. This model has the particularity that, in the classical case, and for a broad region in parameter space, an external magnetic field induces a chiral symmetry breaking: the ground state is a doubly degenerate $q=0$ order with either positive or negative net chirality. Here, we focus on the effect of this chiral phase transition in the thermal Hall conductivity using Linear-Spin-Waves theory. We explore the topology and calculate the Chern numbers of the magnonic bands, obt…
In frustrated magnets the Dzyaloshinsky-Moriya interaction arising from spin-orbit coupling can induce a magnetic long-range order. Here, we report a theoretical prediction of thermal Hall effect in frustrated kagomé magnets such as KCr$_3$(OH)$_6$(SO4)$_2$ and KFe$_3$(OH)$_{6}$(SO$_{4}$)$_2$. The thermal Hall effects in these materials are induced by scalar spin chirality as opposed to DMI in previous studies. The scalar spin chirality originates from magnetic-field-induced chiral spin configuration due to non-coplanar spin textures, but in general it can be spontaneously developed as a macro…
