The dynamics of correlated systems is relevant in many fields ranging from cosmology to plasma physics. However, they are challenging to predict and understand even for classical systems due to the typically large numbers of particles involved. Here, we study the evolution of an ultracold, correlated many-body system with repulsive interactions and initial correlations set by the Rydberg blockade using the analytical framework of Kinetic Field Theory (KFT). The KFT formalism is based on the path-integral formulation for classical mechanics and was first developed and successfully used in cosmology to describe structure formation in Dark Matter. The theoretical framework offers a high flexibility regarding the initial configuration and interactions between particles and, in addition, is computationally cheap. More importantly, the analytic approach allows us to gain better insight into the processes which dominate the dynamics. In this work we show that KFT can be applied in a much more general context and study the evolution of a correlated ion plasma. We find good agreement between the analytical KFT results for the evolution of the correlation function and results obtained from numerical simulations. We use the correlation functions obtained with KFT to compute the temperature increase in the ionic system due to disorder-induced heating. For certain choices of parameters we observe that the effect can be reversed, leading to correlation cooling. Due to its numerical efficiency as compared to numerical simulations, a detailed study using KFT can help to constrain parameter spaces where disorder-induced heating is minimal in order to reach the regime of strong coupling.
We propose an experimentally realizable scheme to produce triatomic ultralong-range Rydberg molecules (TURM), formed in ultracold KRb traps. A near resonant coupling of the non-zero quantum defect Rydberg levels with the KRb molecule in N=0 and N=2 rotational levels, is engineered which exploits the unique Rydberg electron-molecule anisotropic dipole interaction. This near resonant coupling enhances the TURM binding and produces favorable Franck-Condon factors. Schemes for both postassium and rubidium excitations are demonstrated.
We have studied the associative ionization of a Rydberg atom and a ground state atom in an ultracold Rydberg gas. The measured scattering cross section is three orders of magnitude larger than the geometrical size of the produced molecule. This giant enhancement of the reaction kinetics is due to an efficient directed mass transport which is mediated by the Rydberg electron. We also find that the total inelastic scattering cross section is given by the geometrical size of the Rydberg electron's wavefunction.
We investigate the spectral properties of a finite laser-driven lattice of ultracold Rydberg atoms exploiting the dipole blockade effect in the frozen Rydberg gas regime. Uniform one-dimensional lattices as well as lattices with variable spacings are considered. In the case of a weak laser coupling, we find a multitude of many-body Rydberg states with well-defined excitation properties which are adiabatically accessible starting from the ground state. A comprehensive analysis of the degeneracies of the spectrum as well as of the single and pair excitations numbers of the eigenstates is perform…
We characterize the two-photon excitation of an ultracold gas of Rubidium atoms to Rydberg states analysing the induced atomic losses from an optical dipole trap. Extending the duration of the Rydberg excitation to several ms, the ground state atoms are continuously coupled to the formed positively charged plasma. In this regime we measure the $n$-dependence of the blockade effect and we characterise the interaction of the excited states and the ground state with the plasma. We also investigate the influence of the quasi-electrostatic trapping potential on the system, confirming the validity o…
We study ultracold Rydberg-dressed Bose gases subject to artificial gauge fields in the fractional quantum Hall (FQH) regime. The characteristics of the Rydberg interaction gives rise to interesting many-body ground states different from standard FQH physics in the lowest Landau level (LLL). The non-local but rapidly decreasing interaction potential favors crystalline ground states for very dilute systems. While a simple Wigner crystal becomes energetically favorable compared to the Laughlin liquid for filling fractions $ν<1/12$, a correlated crystal of composite particles emerges already for …
Engineering quantum phases with spontaneously broken symmetries is a major goal of research in different fields. Trapped ultracold Rydberg-excited atoms in optical lattices are a promising platform for realizing quantum phases with broken lattice translational symmetry since they are interacting over distances larger than the lattice constant. Although numerous theoretical works on trapped Rydberg-excited gases have predicted such phases, in particular density wave or supersolid phases, their experimental observation proves to be difficult due to challenges such as scattering processes and the…
Several recent experiments have established by measuring the Mandel Q parameter that the number of Rydberg excitations in ultracold gases exhibits sub-Poissonian statistics. This effect is attributed to the Rydberg blockade that occurs due to the strong interatomic interactions between highly-excited atoms. Because of this blockade effect, the system can end up in a state in which all particles are either excited or blocked: a jamming limit. We analyze appropriately constructed random-graph models that capture the blockade effect, and derive formulae for the mean and variance of the number of …
We describe a quantum information architecture consisting of a hybrid array of optically-trapped molecules and atoms. This design leverages the large transition dipole moments of Rydberg atoms to mediate fast, high-fidelity gates between qubits encoded in coherent molecular degrees of freedom. Error channels of detuning, decay, pulse area noise, and leakage to other molecular states are discussed. The molecule-Rydberg interaction can also be used to enable nondestructive molecule detection and rotational state readout. We consider a specific near-term implementation of this scheme using NaCs m…
We present a combined experimental and theoretical study of the effects of Rydberg interactions on Autler-Townes spectra of ultracold gases of atomic strontium. Realizing two-photon Rydberg excitation via a long-lived triplet state allows us to probe the thus far unexplored regime where Rydberg state decay presents the dominant decoherence mechanism. The effects of Rydberg interactions are observed in shifts, asymmetries, and broadening of the measured atom-loss spectra. The experiment is analyzed within a one-body density matrix approach, accounting for interaction-induced level shifts and de…
We show that the excitation of long-range Rydberg molecules in a three-dimensional optical lattice can be used as a position- and time-sensitive probe of the site occupancy in the system. To this end, we detect the ions which are continuously generated by the decay of the formed Rydberg molecules. While a superfluid gas shows molecule formation for all parameters, a Mott insulator with $n=1$ filling reveals a strong suppression of the number of formed molecules. In the limit of weak probing, the technique can be used to probe the superfluid to Mott-insulator transition in real-time. Our method…
The non-equilibrium dynamics of a gas of cold atoms in which Rydberg states are off-resonantly excited is studied in the presence of noise. The interplay between interaction and off-resonant excitation leads to an initial dynamics where aggregates of excited Rydberg atoms slowly nucleate and grow, eventually reaching long-lived meta-stable arrangements which then relax further on much longer timescales. This growth dynamics is governed by an effective Master equation which permits a transparent and largely analytical understanding of the underlying physics. By means of extensive numerical simu…
Dense Rydberg gases are out-of-equilibrium systems where strong density-density interactions give rise to effective kinetic constraints. They cause dynamic arrest associated with highly-constrained many-body configurations, leading to slow relaxation and glassy behavior. Multi-component Rydberg gases feature additional long-range interactions such as excitation-exchange. These are analogous to particle swaps used to artificially accelerate relaxation in simulations of atomistic models of classical glass formers. In Rydberg gases, however, swaps are real physical processes, which provide dynami…
We study the out-of-equilibrium dynamics of dissipative gases of atoms excited to two or more high-lying Rydberg states. This situation bears interesting similarities to classical binary (in general $p$-ary) mixtures of particles. The effective forces between the components are determined by the inter-level and intra-level interactions of Rydberg atoms. These systems permit to explore new parameter regimes which are physically inaccessible in a classical setting, for example one in which the mixtures exhibit non-additive interactions. In this situation the out-of-equilibrium evolution is chara…
The theory of quantum scarring -- a remarkable violation of quantum unique ergodicity -- rests on two complementary pillars: the existence of unstable classical periodic orbits and the so-called quasimodes, i.e., the non-ergodic states that strongly overlap with a small number of the system's eigenstates. Recently, interest in quantum scars has been revived in a many-body setting of Rydberg atom chains. While previous theoretical works have identified periodic orbits for such systems using time-dependent variational principle (TDVP), the link between periodic orbits and quasimodes has been mis…
Out-of-equilibrium, strong correlation in a many-body system triggers emergent properties that can act in important ways to constrain the natural dissipation of energy and matter. Networks of atoms, intricately engineered to arrange positions and tune interaction energies, exhibit striking dynamics. But, strong correlation itself can also act to restrict available phase space. Relaxation confined by strong correlation gives rise to scale invariance and density distributions characteristic of self-organized criticality. For some time, we have observed signs of self-organization in the avalanche…
In this paper, we study Bose-Einstein condensation of Rydberg-dressed atoms considering finite range interactions. We use Hartree-Fock-Bogoliubov approximation based on Mean-Field approach. Moreover, within this approximation modified by the finite-range character of the two-body interaction we shall obtain analytical expressions for thermodynamic quantities of Rydberg-dressed Bose gas. The imaginary part of the quasiparticle spectrum of a BEC signals the instability of the roton mode with respect to the formation of supersolid state. Our theory predicts a second-order quantum phase transition…
We discuss techniques to generate long-range interactions in a gas of groundstate alkali atoms, by weakly admixing excited Rydberg states with laser light. This provides a tool to engineer strongly correlated phases with reduced decoherence from inelastic collisions and spontaneous emission. As an illustration, we discuss the quantum phases of dressed atoms with dipole-dipole interactions confined in a harmonic potential, as relevant to experiments. We show that residual spontaneous emission from the Rydberg state acts as a heating mechanism, leading to a quantum-classical crossover.
Many-body correlations govern a variety of important quantum phenomena such as the emergence of superconductivity and magnetism. Understanding quantum many-body systems is thus one of the central goals of modern sciences. Here we demonstrate an experimental approach towards this goal by utilizing an ultracold Rydberg gas generated with a broadband picosecond laser pulse. We follow the ultrafast evolution of its electronic coherence by time-domain Ramsey interferometry with attosecond precision. The observed electronic coherence shows an ultrafast oscillation with a period of 1 femtosecond, who…
The emergent phases of strongly correlated spin-1/2 Fermi gases of Rydberg dressed atoms in a one dimensional optical lattice are theoretically investigated. At weak coupling a bosonization description is used to demonstrate the ability to drive alternating quantum phase transitions between distinct Luttinger liquids. At strong coupling the ground state develops non-trivial phase separation exhibiting Luttinger liquid ''puddles'' separated by magnetic domain walls due to the interplay of the incommensurate filling and the Rydberg core length scale. These phases can be detected in ultracold gas…
We investigate the possibility of realizing supersolid quantum phases in bosonic Rydberg-excited quantum lattice gases in the presence of non-unitary processes, by simulating the dynamical evolution starting from initial preparation in non-dissipative equilibrium states. Within Gutzwiller theory, we first analyze the many-body ground-state of a bosonic Rydberg-excited quantum gas in a two dimensional optical lattice for variable atomic hopping rates and Rabi detunings. Furthermore, we perform time evolution of different supersolid phases using the Lindblad-master equation. With the inclusion o…
We study the long-range interaction of a single ion with a highly excited ultracold Rydberg atom and report on the direct observation of ion-induced Rydberg excitation blockade mediated over tens of micrometer distances. Our hybrid ion-atom system is directly produced from an ultracold atomic ensemble via near-threshold photo-ionization of a single Rydberg excitation, employing a two-photon scheme which is specifically suited for generating a very low-energy ion. The ion's motion is precisely controlled by small electric fields, which allows us to analyze the blockade mechanism for a range of …
We study the non-equilibrium steady state arising from the interplay between coherent and dissipative dynamics in strongly interacting Rydberg gases using a recently introduced variational method [H. Weimer, Phys. Rev. Lett. 114, 040402 (2015)]. We give a detailed discussion of the properties of this novel approach, and we provide a comparison with methods related to the Bogoliubov-Born-Green-Kirkwood-Yvon hierarchy. We find that the variational approach offers some intrinsic advantages, and we also show that it is able to explain the experimental results obtained in an ultracold Rydberg gas o…
We theoretically investigate the response of a two component Fermi gas to vector potentials which couple separately to the two spin components. Such vector potentials may be implemented in ultracold atomic gases using optically dressed states. Our study indicates that light-induced gauge potentials may be used to probe the properies of the interacting ultracold Fermi gas, providing. amongst other things, ways to measure the superfluid density and the strength of pairing.
We report the experimental observation of strong two-color optical nonlinearity in an ultracold gas of $^{85}\mathrm{Rb}$-$^{87}\mathrm{Rb}$ atom mixture. By simultaneously coupling two probe transitions of $^{85}$Rb and $^{87}$Rb atoms to Rydberg states in electromagnetically induced transparency (EIT) configurations, we observe significant suppression of the transparency resonance for one probe field when the second probe field is detuned at $\sim1~\mathrm{GHz}$ and hitting the EIT resonance of the other isotope. Such a cross-absorption modulation to the beam propagation dynamics can be desc…
We show how density dependent gauge potentials can be induced in dilute gases of ultracold atoms using light-matter interactions. We study the effect of the resulting interacting gauge theory and show how it gives rise to novel topological states in the ultracold gas. We find in particular that the onset of persistent currents in a ring geometry is governed by a critical number of particles. The density-dependent gauge potential is also found to support chiral solitons in a quasi-one-dimensional ultracold Bose gas.
We present photo-excitation of ultra-long-range Rydberg molecules as a probe of spatial correlations in quantum gases. Rydberg molecules can be created with well-defined internuclear spacing, set by the radius of the outer lobe of the Rydberg electron wavefunction $R_n$. By varying the principal quantum number $n$ of the target Rydberg state, the molecular excitation rate can be used to map the pair-correlation function of the trapped gas $g^{(2)}(R_n)$. We demonstrate this with ultracold Sr gases and probe pair-separation length scales ranging from $R_n = 1400 - 3200$ $a_0$, which are on the …
We study a two-dimensional lattice gas of atoms that are photo-excited to high-lying Rydberg states in which they interact via the van-der-Waals interaction. We explore the regime of dominant nearest neighbor interaction where this system is intimately connected to a quantum version of Baxter's hard squares model. We show that the strongly correlated ground state of the Rydberg gas can be analytically described by a projected entangled pair state that constitutes the ground state of the quantum hard squares model. This correspondence allows us to identify a first order phase boundary where the…
One of the major challenges in realizing a strongly interacting lattice gas using Rydberg states is the occurrence of avalanche loss processes. As these are directly proportional to the total Rydberg fraction, the commonly suggested solution is using far off-resonantly excited Rydberg states. We instead propose the realization of a correlated bosonic lattice gas at near-resonant excitation, where the total Rydberg fraction in the bulk is low due to the strong, interaction-driven effective detuning. Using real-space dynamical mean-field theory we show that its reduced effect at the boundary of …
We have investigated formation of structures of Rydberg atoms excited from a disordered gas of ultracold atoms, using rate equations for two-photon Rydberg excitation in a single atom without eliminating the intermediate state. We have explored the validity range of these rate equations and defined a simple measure to determine, whether our model is applicable for a given set of laser parameters. We have applied these rate equations in Monte Carlo simulations of ultracold gases, for different laser beam profiles, and compared these simulations to experimental observations and find a general ag…
We propose a novel scheme to efficiently tune the scattering length of two colliding ground-state atoms by off-resonantly coupling the scattering-state to an excited Rydberg-molecular state using laser light. For the s-wave scattering of two colliding ${^{87}}\mathrm{Rb}$ atoms, we demonstrate that the effective optical length and pole strength of this Rydberg optical Feshbach resonance can be tuned over several orders of magnitude, while incoherent processes and losses are minimised. Given the ubiquity of Rydberg molecular states, this technique should be generally applicable to homo-nuclear …
We clarify some technical issues in the present generalized effective-potential Landau theory (GEPLT) that makes the GEPLT more consistent and complete. Utilizing this clarified GEPLT, we analytically study the quantum phase transitions of ultracold Bose gases in bipartite superlattices at zero termparture. The corresponding quantum phase boundaries are analytically calculated up to the third-order hopping, which are in excellent agreement with the quantum Monte Carlo (QMC) simulations.
We present an analytical theory for the nonlinear optical response of a strongly interacting Rydberg gas under conditions of electromagnetically induced transparency. Simple formulae for the third order optical susceptibility are derived and shown to be in excellent agreement with recent experiments. The obtained expressions reveal strong nonlinearities, which in addition are of highly nonlocal character. This property together with enormous strength of the Rydberg-induced nonlinearities is shown to yield a unique laboratory platform for nonlinear wave phenomena, such as collapse-arrested modu…
The object of study of this thesis are dipolar systems in the quantum degenerate regime. In general, dealing with many-body systems and evaluating their properties requires to deal with the Schrödinger equation. In the present study we employ different Monte Carlo methods, that are stochastic techniques that allow to find numerical solutions to it.
In this chapter, we describe scattering resonance phenomena in general, and focus on the mechanism of Feshbach resonances, for which a multi-channel treatment is required. We derive the dependence of the scattering phase shift on magnetic field and collision energy. From this, the scattering length and effective range coefficient can be extracted, expressions which are particularly useful for ultracold gases.
We show that simple laser configurations can give rise to "optical flux lattices", in which optically dressed atoms experience a periodic effective magnetic flux with high mean density. These potentials lead to narrow energy bands with non-zero Chern number. Optical flux lattices will greatly facilitate the achievement of the quantum Hall regime for ultracold atomic gases.
Ultracold atomic gases have developed into prime systems for experimental studies of Efimov three-body physics and related few-body phenomena, which occur in the universal regime of resonant interactions. In the last few years, many important breakthroughs have been achieved, confirming basic predictions of universal few-body theory and deepening our understanding of such systems. We review the basic ideas along with the fast experimental developments of the field, focussing on ultracold cesium gases as a well-investigated model system. Triatomic Efimov resonances, atom-dimer Efimov resonances…
In this work we investigate the unique properties of ultracold Bose gases in one and two dimensions. In two dimensions, we present simulations of the Berezinskii-Kosterlitz-Thouless (BKT) phase transition using the projected Gross-Pitaevskii equation formalism. We confirm the presence of the BKT phase by observing algebraic decay in the first-order correlation function, unbinding of vortex pairs, and behaviour of the superfluid fraction. In one dimension we use a transverse Gaussian ansatz and the Lagrangian approach to derive an effective equation of motion for the one dimensional Bose gas at…
We numerically investigate the quantum crystallographic phases of a Rydberg-dressed Bose gas loaded on a square lattice by using the mean-field Gross--Pitaevskii model. For a relatively weak lattice confinement, the phases of ground state undergo amorphism, polycrystal, and polymorphism following the increase of the blockade radius, and if the confinement is stronger, a single crystal with a specific filling factor will be formed. In order to distinctively characterize these phases, the structure function is also studied. In such an anisotropic system, we report that the first diagonal element…
Penning ionization releases electrons in a state-selected Rydberg gas of nitric oxide entrained in a supersonic molecular beam. Subsequent processes of electron impact avalanche, bifurcation, and quench form a strongly coupled, spatially correlated ultracold plasma of NO$^+$ ions and electrons that exhibits characteristics of self-organized criticality. This plasma contains a residue of nitric oxide Rydberg molecules. A conventional fluid dynamics of ion-electron-Rydberg quasi-equilibrium predicts rapid decay to neutral atoms. Instead, the NO plasma endures for a millisecond or more, suggestin…
This article provides a brief review of how various spectroscopies have been used to investitage many-body quantum phenomena in the context of ultracold Fermi gases. In particular, work done with RF spectroscopy, Bragg spectroscopy and lattice modulation spectroscopy is considered. The theoretical basis of these spectroscopies, namely linear response theory in the many-body quantum physics context is briefly presented. Experiments related to the BCS-BEC crossover, imbalanced Fermi gases, polarons, possible pseudogap and Fermi liquid behaviour and measuring the contact are discussed. Remaining …
We systematically investigate the topological properties of spin polarized Rydberg-dressed fermionic atoms loaded in a bilayer optical lattice. Through tuning the Rydberg coupling strength and the inter-layer tunneling amplitude, we identify different types of topological superfluid states generated from the inter-layer pairing and relative gauge phase modulation of the couples 2D $p$-wave superfluids. These phases includes gapped/gapless with/without time reversal symmetry. One of the most interesting states is a gapless paired topological superfluid with both the time-reversal symmetry and p…
Atoms excited into high-lying Rydberg states and under strong dipole-dipole interactions exhibit phenomena associated with highly correlated and complex systems. We perform first principles numerical simulations on the dynamics of such systems. The emergence of a roton minimum in the excitation spectrum, as expected in strongly correlated gases and accurately described by Feynman's theory of liquid helium, is shown to significantly inhibit particle transport, with a strong suppression of the diffusion coefficient, due to the emerging spatial order. We also demonstrate how the ability to tempor…
Recent experiments with strongly interacting, driven Rydberg ensembles have introduced a promising setup for the study of self-organized criticality (SOC) in cold atom systems. Based on this setup, we theoretically propose a control mechanism for the paradigmatic avalanche dynamics of SOC in terms of a time-dependent drive amplitude. This gives access to a variety of avalanche dominated, self-organization scenarios, prominently including self-organized criticality, as well as sub- and supercritical dynamics. We analyze the dependence of the dynamics on external scales and spatial dimensionalit…
We present optimal control protocols to prepare different many-body quantum states of Rydberg atoms in optical lattices. Specifically, we show how to prepare highly ordered many-body ground states, GHZ states as well as some superposition of symmetric excitation number Fock states, that inherit the translational symmetry from the Hamiltonian, within sufficiently short excitation times minimizing detrimental decoherence effects. For the GHZ states, we propose a two-step detection protocol to experimentally verify the optimal preparation of the target state based only on standard measurement tec…
Two-dimensional (2D) spectroscopy uses multiple electromagnetic pulses to infer the properties of a complex system. A paradigmatic class of target systems are molecular aggregates, for which one can obtain information on the eigenstates, various types of static and dynamic disorder and on relaxation processes. However, two-dimensional spectra can be difficult to interpret without precise knowledge of how the signal components relate to microscopic Hamiltonian parameters and system-bath interactions. Here we show that two-dimensional spectroscopy can be mapped in the microwave domain to highly …
The recent advances in single atom detection and manipulation in experiments with ultracold quantum gases are reviewed. The discussion starts with the basic principles of trapping, cooling and detecting single ions and atoms. The realization of single atom detection in ultracold quantum gases is presented in detail and the employed methods, which are based on light scattering, electron scattering, field ionization and direct neutral particle detection are discussed. The microscopic coherent manipulation of single atoms in a quantum gas is also covered. Various examples are given in order to hi…
The statistics of strongly interacting, ultracold Rydberg gases are governed by the interplay of two factors: geometrical restrictions induced by blockade effects, and quantum mechanical effects. To shed light on their relative roles in the statistics of Rydberg gases, we compare three models in this paper: a quantum mechanical model describing the excitation dynamics within a Rydberg gas, a Random Sequential Adsorption (RSA) process on a Random Geometric Graph (RGG), and a RSA process on a Decomposed Random Intersection Graph (DRIG). The latter model is new, and refers to choosing a particula…
Electron lattice potentials for ultracold atoms using circular Rydberg orbitals
Max-Planck Institut für Physik komplexer Systeme（马克斯·普朗克复杂系统物理研究所）；Joint Quantum Centre (JQC) Durham-Newcastle, Department of Chemistry, Durham University（杜伦大学化学系）；Physikalisches Institut and Center for Integrated Quantum Science and Technology, Universität Stuttgart（斯图加特大学第五物理研究所及综合量子科学技术中心）；Department of Physics and Astronomy, Purdue University（普渡大学物理与天文学系）
We suggest pump-probe spectroscopy to study pair correlations that determine the many-body dynamics in weakly interacting, dilute ultracold gases. A suitably chosen, short laser pulse depletes the pair density locally, creating a 'hole' in the electronic ground state. The dynamics of this non-stationary pair density is monitored by a time-delayed probe pulse. The resulting transient signal allows to spectrally decompose the 'hole' and to map out the pair correlation functions.
We theoretically analyze interference patterns of parametrically driven one dimensional ultracold atomic gases. By modulating the interaction strength periodically in time, we propose to excite collective modes in a pair of independent one dimensional gases at energies corresponding to the drive frequency. The excited collective modes lead to spatial oscillations in the correlations of the interference pattern, which can be analyzed to obtain the sound velocity of the collective modes. We discuss both bosonic and fermionic systems, and how such experiments could be used to probe spin charge se…
