The object of study of this thesis are dipolar systems in the quantum degenerate regime. In general, dealing with many-body systems and evaluating their properties requires to deal with the Schrödinger equation. In the present study we employ different Monte Carlo methods, that are stochastic techniques that allow to find numerical solutions to it.
A gas of ultracold molecules interacting via the long-range dipolar potential offers a highly controlled environment in which to study strongly correlated phases. However, at particle coalescence the divergent $1/r^3$ dipolar potential and associated pathological wavefunction hinder computational analysis. For a dipolar gas constrained to two dimensions we overcome these numerical difficulties by proposing a pseudopotential that is explicitly smooth at particle coalescence, resulting in a 2000-times speedup in diffusion Monte Carlo calculations. The pseudopotential delivers the scattering phas…
We study the relaxation and damping dynamics of an ultracold, but not quantum degenerate, gas consisting of dipolar particles. These simulations are performed using a direct simulation Monte Carlo method and employing the highly anisotropic differential cross section of dipoles in the Wigner threshold regime. We find that both cross-dimensional relaxation and damping of breathing modes occur at rates that are strongly dependent on the orientation of the dipole moments relative to the trap axis. The relaxation simulations are in excellent agreement with recent experimental results in erbium. Th…
We study the role of the Dipolar-Induced Resonance (DIR) in a quasi-one-dimensional system of ultracold bosons. We first describe the effect of the DIR on two particles in a harmonic trap. Then, we consider a deep optical lattice loaded with ultracold dipolar bosons. In order to describe this system, we introduce a novel atom-dimer extended Bose-Hubbard model, which is the minimal model correctly accounting for the DIR. We analyze the impact of the DIR on the phase diagram at T=0 by exact diagonalization of a small-sized system. We show that the DIR strongly affects this phase diagram. In part…
We develop a non-perturbative theoretical framework to treat collisions with generic anisotropic interactions in quasi-one-dimensional geometries. Our method avoids the limitations of pseudopotential theory allowing to include accurately long-range anisotropic interactions. Analyzing ultracold dipolar collisions in a harmonic waveguide we predict dipolar confinement-induced resonances (DCIRs) which are attributed to different angular momentum states. The analytically derived resonance condition reveals in detail the interplay of the confinement with the anisotropic nature of the dipole-dipole …
We introduce a density functional formalism to study the ground-state properties of strongly-correlated dipolar and ionic ultracold bosonic and fermionic gases, based on the self-consistent combination of the weak and the strong coupling limits. Contrary to conventional density functional approaches, our formalism does not require a previous calculation of the interacting homogeneous gas, and it is thus very suitable to treat systems with tunable long-range interactions. Due to its asymptotic exactness in the regime of strong correlation, the formalism works for systems in which standard mean-…
We study the collapse of ultracold fermionic gases into inhomogeneous states due to strong dipolar interaction in both 2D and 3D. Depending on the dimensionality, we find that two different types of inhomogeneous states are stabilized once the dipole moment reaches a critical value $d>d_c$: the {\it stripe phase} and {\it phase separation} between high and low densities. In 2D, we prove that the stripe phase is always favored for $d\gtrsim d_c$, regardless of the microscopic details of the system. In 3D, the one-loop perturbative calculation suggests that the same type of instability leads to …
We propose an effective Ising spin chain constructed with dipolar quantum gases confined in a one-dimensional optical superlattice. Mapping the motional degrees of freedom of a single particle in the lattice onto a pseudo-spin results in effective transverse and longitudinal magnetic fields. This effective Ising spin chain exhibits a quantum phase transition from a paramagnetic to a single-kink phase as the dipolar interaction increases. Particularly in the single-kink phase,a magnetic kink arises in the effective spin chain and behaves as a quasi-particle in a pinning potential exerted by the…
Ultracold ground state dipolar 40K-87Rb molecules have recently been produced in a loose harmonic trap by employing a magnetic field sweep across a Feshbach resonance followed by stimulated Raman adiabatic passage [K.-K. Ni et al., Science 322, 231 (2008)]. The overall experimental efficiency for molecule formation was around 20%. We show that the efficiency can be increased to nearly 100% if one first loads the atomic gases into an optical lattice of the appropriate depth and tunes the interspecies attraction to have exactly one atom of each species at an occupied lattice site. Our proposed s…
We study the scissors modes of dipolar boson and fermion gases trapped in a spherically symmetric potential. We use the harmonic oscillator states to solve the time-dependent Gross-Pitaevskii equation for bosons and the time-dependent Hartree-Fock equation for fermions. It is pointed out that the scissors modes of bosons and fermions can be of quite different nature.
We studied the miscibility of two dipolar quantum gases in the limit of zero temperature. The system under study is composed by a mixture of two Bose gases with dominant dipolar interaction in a two-dimensional harmonic confinement. The dipolar moments are considered all to be perpendicular to the plane, turning the dipolar potential in a purely repulsive and isotropic model. Our analysis is carried out by using the diffusion Monte Carlo method which allows for an exact solution to the many-body problem within some statistical noise. Our results show that the miscibility between the two specie…
The self-consistent field approach for the electric dipolar ultracold spin-1/2 fermions is discussed. Contribution of the exchange part of the electric dipole interaction is found. Hence we obtain a model of dipolar fermions beyond the self-consistent field approximation. It is shown that the exchange interaction of electric dipolar fermions depends on the spin-polarisation of the system. For instance the electric dipole exchange interaction equals to zero for spin-unpolarised systems, namely all low laying quantum states occupied by two-particles with opposite spins. In opposite limit of the …
This article reviews the recent theoretical and experimental advances in the study of ultracold gases made of bosonic particles interacting via the long-range, anisotropic dipole-dipole interaction, in addition to the short-range and isotropic contact interaction usually at work in ultracold gases. The specific properties emerging from the dipolar interaction are emphasized, from the mean-field regime valid for dilute Bose-Einstein condensates, to the strongly correlated regimes reached for dipolar bosons in optical lattices.
Using the time-dependent density matrix renormalization group method, we calculate transport properties of an interacting Fermi gas in an optical lattice with a confining trap after a sudden displacement of the trap center. In the regime of attractive interactions, the dipolar motion after the displacement can be classified into underdamped oscillations and overdamped relaxations, depending on the interaction strength. These numerical calculations are consistent with experimental results. In the regime of repulsive interactions, we predict a revival of the oscillations of the center of mass wh…
We consider a mixture of two-component Fermi and (one-component) dipolar Bose gases in which both dipolar interaction and s-wave scattering between fermions of opposite spins are tunable. We show that in the long wavelength limit, the anisotropy in the Fermi-Fermi interaction induced by phonons of the dipolar condensate can strongly enhance the scattering in the triplet channel. We investigate in detail the conditions for achieving optimal critical temperature at which the triplet superfluid begins to compete with the singlet superfluid.
We theoretically investigate the response of a two component Fermi gas to vector potentials which couple separately to the two spin components. Such vector potentials may be implemented in ultracold atomic gases using optically dressed states. Our study indicates that light-induced gauge potentials may be used to probe the properies of the interacting ultracold Fermi gas, providing. amongst other things, ways to measure the superfluid density and the strength of pairing.
We consider two separated pancake-shaped trapped gases interacting with a dipolar (either magnetic or electric) force. We study how the center of mass motion propagates from one cloud to the other as a consequence of the long-range nature of the interaction. The corresponding dynamics is fixed by the frequency difference between the in-phase and the out-of-phase center of mass modes of the two clouds, whose dependence on the dipolar interaction strength and the cloud separation is explicitly investigated. We discuss Fermi gases in the degenerate as well as in the classical limit and comment on…
We investigate the occurence of Wigner-localization phenomena in bosonic dipolar ultracold few-body systems with Rashba-like spin-orbit coupling. We show that the latter strongly enhances the effects of the dipole-dipole interactions, allowing to reach the Wigner-localized regime for strengths of the dipole moment much smaller than those necessary in the spin-orbit-free case.
We show how density dependent gauge potentials can be induced in dilute gases of ultracold atoms using light-matter interactions. We study the effect of the resulting interacting gauge theory and show how it gives rise to novel topological states in the ultracold gas. We find in particular that the onset of persistent currents in a ring geometry is governed by a critical number of particles. The density-dependent gauge potential is also found to support chiral solitons in a quasi-one-dimensional ultracold Bose gas.
We study the propagation of sound in a homogeneous dipolar gas at zero temperature, known as zero sound. We find that undamped sound propagation is possible only in a range of solid angles around the direction of polarization of the dipoles. Above a critical dipole moment, we find an unstable mode, by which the gas collapses locally perpendicular to the dipoles' direction.
We investigate the phase diagrams of two-dimensional lattice dipole systems with variable geometry. For bipartite square and triangular lattices with tunable vertical sublattice separation, we find rich phase diagrams featuring a sequence of easy-plane magnetically ordered phases separated by incommensurate spin-wave states.
In a combined experimental and theoretical effort, we demonstrate a novel type of dipolar system made of ultracold bosonic dipolar molecules with large magnetic dipole moments. Our dipolar molecules are formed in weakly bound Feshbach molecular states from a sample of strongly magnetic bosonic erbium atoms. We show that the ultracold magnetic molecules can carry very large dipole moments and we demonstrate how to create and characterize them, and how to change their orientation. Finally, we confirm that the relaxation rates of molecules in a quasi-two dimensional geometry can be reduced by usi…
Analytic expressions for the differential cross sections of ultracold atoms and molecules that scatter primarily due to dipolar interactions are derived within the first Born approximation, and are shown to agree with the partial wave expansion. These cross sections are applied to the problem of cross-dimensional rethermalization. Strikingly, the rate of rethermalization can vary by as much as a factor of two, depending on the orientation of polarization of the dipoles. Thus the anisotropic dipole-dipole interaction can have a profound effect even on the behavior of a nondegenerate ultracold g…
We clarify some technical issues in the present generalized effective-potential Landau theory (GEPLT) that makes the GEPLT more consistent and complete. Utilizing this clarified GEPLT, we analytically study the quantum phase transitions of ultracold Bose gases in bipartite superlattices at zero termparture. The corresponding quantum phase boundaries are analytically calculated up to the third-order hopping, which are in excellent agreement with the quantum Monte Carlo (QMC) simulations.
We consider dilute gases of dipolar bosons or fermions in the high-temperature limit in a spherically symmetric harmonic trapping potential. We examine the system using a virial expansion up to second order in the fugacity. Using the Born approximation and assuming purely dipolar interactions, we find that the second-order virial coefficient for both bosons and fermions depends quadratically on the dipole length and is negative at high temperature, indicating that to lowest order in the dipole-dipole interactions the dipolar single-component quantum gases are repulsive. If the $s$-wave scatter…
An impurity atom immersed in an ultracold atomic Fermi gas can form a quasiparticle, so-called Fermi polaron, due to impurity-fermion interaction. We consider a three-dimensional homogeneous dipolar Fermi gas as a medium, where the interatomic dipole-dipole interaction (DDI) makes the Fermi surface deformed into a spheroidal shape, and, using a Chevy-type variational method, investigate the ground-state properties of the Fermi polaron: the effective mass, the momentum distribution of a particle-hole (p-h) excitation, the drag parameter, and the medium density modification around the impurity. …
We develop a practical Hartree-Fock theory for trapped Bose and Fermi gases that interact with dipole-dipole interactions. This theory is applicable at zero and finite temperature. Our approach is based on the introduction of local momentum distortion fields that characterize the exchange effects in terms of a local effective potential. We validate our theory against existing theories, finding excellent agreement with full Hartree-Fock calculations.
Trapped degenerate dipolar Bose and Fermi gases of cylindrical symmetry with the polarization vector along the symmetry axis are only stable for the strength of dipolar interaction below a critical value. In the case of bosons, the stability of such a dipolar Bose-Einstein condensate (BEC) is investigated for different strengths of contact and dipolar interactions using variational approximation and numerical solution of a mean-field model. In the disk shape, with the polarization vector perpendicular to the plane of the disk, the atoms experience an overall dipolar repulsion and this fact sho…
We investigate the ground state properties and tunneling dynamics of ultracold dipolar bosons in a one dimensional triple well trap from a few-body ab-initio perspective. Our focus is primarily on the distinctive features of dipolar bosons compared to the contact interacting bosons. Formation of intra-well localization is observed for very strong dipolar interaction. General population rearangement as well as fragmentation and localization effects have been found, depending strongly on the particle number. The energy spectrum for two particles exhibits avoided crossings that lead to several di…
In this chapter, we describe scattering resonance phenomena in general, and focus on the mechanism of Feshbach resonances, for which a multi-channel treatment is required. We derive the dependence of the scattering phase shift on magnetic field and collision energy. From this, the scattering length and effective range coefficient can be extracted, expressions which are particularly useful for ultracold gases.
Ultracold atomic gases have developed into prime systems for experimental studies of Efimov three-body physics and related few-body phenomena, which occur in the universal regime of resonant interactions. In the last few years, many important breakthroughs have been achieved, confirming basic predictions of universal few-body theory and deepening our understanding of such systems. We review the basic ideas along with the fast experimental developments of the field, focussing on ultracold cesium gases as a well-investigated model system. Triatomic Efimov resonances, atom-dimer Efimov resonances…
In this work we investigate the unique properties of ultracold Bose gases in one and two dimensions. In two dimensions, we present simulations of the Berezinskii-Kosterlitz-Thouless (BKT) phase transition using the projected Gross-Pitaevskii equation formalism. We confirm the presence of the BKT phase by observing algebraic decay in the first-order correlation function, unbinding of vortex pairs, and behaviour of the superfluid fraction. In one dimension we use a transverse Gaussian ansatz and the Lagrangian approach to derive an effective equation of motion for the one dimensional Bose gas at…
We study a system of dipolar molecules confined in a two-dimensional trap and subject to an optical square lattice. The repulsive long-range dipolar interaction $D/r^3$ favors an equilateral triangular arrangement of the molecules, which competes against the square symmetry of the underlying optical lattice with lattice constant $b$ and amplitude $V$. We find the minimal-energy states at the commensurate density $n = 1/b^2$ and establish the complete square-to-triangular transformation pathway of the lattice with decreasing $V$ involving period-doubled, solitonic, and distorted-triangular conf…
The dipolar collision between ultracold polar molecules is an important topic both by its own right from the fundamental point of view and for the successful exploration of many-body physics with strong and long-range dipolar interactions. Here, we report the investigation of collisions between ultracold ground-state sodium-rubidium molecules in electric fields with induced electric dipole moments as large as 0.7$\;$D. We observe a step-wise enhancement of losses due to the coupling between different partial waves induced by the increasingly stronger anisotropic dipolar interactions. Varying t…
This article provides a brief review of how various spectroscopies have been used to investitage many-body quantum phenomena in the context of ultracold Fermi gases. In particular, work done with RF spectroscopy, Bragg spectroscopy and lattice modulation spectroscopy is considered. The theoretical basis of these spectroscopies, namely linear response theory in the many-body quantum physics context is briefly presented. Experiments related to the BCS-BEC crossover, imbalanced Fermi gases, polarons, possible pseudogap and Fermi liquid behaviour and measuring the contact are discussed. Remaining …
We study the dissociation of Feshbach molecules in ultracold Fermi gases with spin-orbit (SO) coupling. Since SO coupling can induce quantum transition between the Feshbach molecules and the fully polarized Fermi gas, the Feshbach molecules can be dissociated by the SO coupling. We experimentally realized this new type of dissociation in ultracold gases of 40K atoms with SO coupling created by Raman beams, and observed that the dissociation rate is highly non-monotonic on both the positive and negative Raman-detuning sides. Our results show that the dissociation of Feshbach molecules can be co…
Motivated by the search for quantum liquid crystal phases in a gas of ultracold atoms and molecules, we study the density wave and nematic instabilities of dipolar fermions on the two-dimensional square lattice (in the $x-y$ plane) with dipoles pointing to the $z$ direction. We determine the phase diagram using two complimentary methods, the Hatree-Fock mean field theory and the linear response analysis of compressibility. Both give consistent results. In addition to the staggered ($π$, $π$) density wave, over a finite range of densities and hopping parameters, the ground state of the system f…
We review recent developments in the use of magnetic lattices as a complementary tool to optical lattices for trapping periodic arrays of ultracold atoms and degenerate quantum gases. Recent advances include the realisation of Bose-Einstein condensation in multiple sites of a magnetic lattice of one-dimensional microtraps, the trapping of ultracold atoms in square and triangular magnetic lattices, and the fabrication of magnetic lattice structures with sub-micron period suitable for quantum tunnelling experiments. Finally, we describe a proposal to utilise long-range interacting Rydberg atoms …
We study the virial relations for ultracold trapped two component Fermi gases in the case of short finite range interactions. Numerical verifications for such relations are reported through the BCS-BEC crossover. As an intermediate step, it is necessary to evaluate the partial derivatives of the many body energy with respect to the inverse of the scattering length and with respect to the interaction range. They are found to have extreme values at the unitary limit. The virial results are used to check the quality of the variational wave function involved in the calculations.
Stabilized by quantum fluctuations, dipolar Bose-Einstein condensates can form self-bound liquidlike droplets in the mean-field unstable regime. However in the Bogoliubov theory, some phonon energies are imaginary in the long-wavelength limit, implying dynamical instability of this system. A similar instability appears in the Bogoliubov theory of a binary quantum droplet, and is removed due to higher-order quantum fluctuations as shown recently [1]. In this work, we study the phonon energy of a dipolar quantum droplet in the Beliaev formalism, and find that quantum fluctuations can enhance the…
The properties of ultracold quantum gases of bosons with dipole-dipole interaction is investigated at finite temperature in the frame of the representative ensembles theory. Self-consistent coupled equations of motion are derived for the condensate and the non-condensate components. Corrections due to the dipolar interaction to the condensate depletion, the anomalous density and thermodynamic quantities such as the ground state energy, the equation of state, the compressibility and the presure are calculated in the homogeneous case at both zero and finite temperatures. Effects of interaction a…
We propose an experimental scheme for studying the Fermi-Pasta-Ulam (FPU) phenomenon in a quantum mechanical regime using ultracold atoms. Specifically, we suggest and analyze a setup of one-dimensional Bose gases confined into an optical lattice. The strength of quantum fluctuations is controlled by tuning the number of atoms per lattice sites (filling factor). By simulating the real-time dynamics of the Bose-Hubbard model by means of the exact numerical method of time-evolving block decimation, we investigate the effects of quantum fluctuations on the FPU recurrence and show that strong quan…
Investigating Friedel oscillations in ultracold gases would complement the studies performed on solid state samples with scanning-tunneling microscopes. In atomic quantum gases interactions and external potentials can be tuned freely and the inherently slower dynamics allow to access non-equilibrium dynamics following a potential or interaction quench. Here, we examine how Friedel oscillations can be observed in current ultracold gas experiments under realistic conditions. To this aim we numerically calculate the amplitude of the Friedel oscillations which a potential barrier provokes in a 1D …
We show that the Bose-Hubbard Model exhibits an increase in density with temperature at fixed pressure in the regular fluid regime and in the superfluid phase. The anomaly at the Bose-Einstein condensate is the first density anomaly observed in a quantum state. We propose that the mechanism underlying both the normal phase and the superfluid phase anomalies is related to zero point entropies and ground state phase transitions. A connection with the typical experimental scales and setups is also addressed. This key finding opens a new pathway for theoretical and experimental studies of water-li…
We demonstrate a novel class of trapping potentials, time-averaged adiabatic potentials (TAAP) which allows the generation of a large variety of traps and waveguides for ultracold atoms. Multiple traps can be coupled through controllable tunneling barriers or merged altogether. We present analytical expressions for pancake-, cigar-, and ring- shaped traps. The ring-geometry is of particular interest for guided matter-wave interferometry as it provides a perfectly smooth waveguide of controllable diameter, and thus a tunable sensitivity of the interferometer.
We describe how optical dressing can be used to generate bandstructures for ultracold atoms with non-trivial Z_2 topological order. Time reversal symmetry is preserved by simple conditions on the optical fields. We first show how to construct optical lattices that give rise to Z_2 topological insulators in two dimensions. We then describe a general method for the construction of three-dimensional Z_2 topological insulators. A central feature of our approach is a new way to understand Z_2 topological insulators starting from the nearly-free electron limit.
In this letter we consider dipolar quantum gases in a quasi-one-dimensional tube with dipole moment perpendicular to the tube direction. We deduce the effective one-dimensional interaction potential and show that this potential is not purely repulsive, but rather has an attractive part due to high-order scattering processes through transverse excited states. The attractive part can induce bound state and cause scattering resonances. This represents the dipole induced resonance in low-dimension. We work out an unconventional behavior of low-energy phase shift for this effective potential and sh…
We study a quasi two dimensional dipolar gas at finite, but ultralow temperatures using the classical field approximation. The method, already used for a contact interacting gas, is extended here to samples with a weakly interacting long-range inter-atomic potential. We present statistical properties of the system for the current experiment with Chromium [Phys. Rev. A 84 053601 (2011)] and compare them with statistics for atoms with larger magnetic dipole moments. Significant enhancement of the third order correlation function, relevant for the particle losses, is found.
The symmetry properties of the Cooper pairing problem for multi-component ultra-cold dipolar molecular systems are investigated. The dipolar anisotropy provides a natural and robust mechanism for both triplet and singlet Cooper pairing to first order in the interaction strength. With a purely dipolar interaction, the triplet $p_z$-like polar pairing is the most dominant. A short-range attractive interaction can enhance the singlet pairing to be nearly degenerate with the triplet pairing. We point out that these two pairing channels can mix by developing a relative phase of $\pm\fracπ{2}$, thus…
We report on the creation of bosonic NaCs molecules in their absolute rovibrational ground state via stimulated Raman adiabatic passage. We create ultracold gases with up to 22,000 dipolar NaCs molecules at a temperature of 300(50) nK and a peak density of $1.0(4) \times 10^{12}$ cm$^{-3}$. We demonstrate comprehensive quantum state control by preparing the molecules in a specific electronic, vibrational, rotational, and hyperfine state. Employing the tunability and strength of the permanent electric dipole moment of NaCs, we induce dipole moments of up to 2.6 D. Dipolar systems of NaCs molecu…
We report the investigation on dipolar collisions in rotational state mixtures of ultracold bosonic $^{23}$Na$^{87}$Rb molecules. The large resonant dipole-dipole interaction between molecules in rotational states of opposite parities brings about significant modifications to their collisions, even when an electric field is not present. In this work, this effect is revealed by measuring the dramatically enhanced two-body loss rate constants in the mixtures. In addition, the dipolar interaction strength can be tuned by preparing the NaRb mixture in different rotational levels with microwave spe…
We produce ultracold dense trapped samples of 87Rb133Cs molecules in their rovibrational ground state, with full nuclear hyperfine state control, by stimulated Raman adiabatic passage (STIRAP) with efficiencies of 90%. We observe the onset of hyperfine-changing collisions when the magnetic field is ramped so that the molecules are no longer in the hyperfine ground state. A strong quadratic shift of the transition frequencies as a function of applied electric field shows the strongly dipolar character of the RbCs ground-state molecule. Our results open up the prospect of realizing stable bosoni…
This tutorial is a theoretical work, in which we study the physics of ultra-cold dipolar bosonic gases in optical lattices. Such gases consist of bosonic atoms or molecules that interact via dipolar forces, and that are cooled below the quantum degeneracy temperature, typically in the nK range. When such a degenerate quantum gas is loaded into an optical lattice produced by standing waves of laser light, new kinds of physical phenomena occur. These systems realize then extended Hubbard-type models, and can be brought to a strongly correlated regime. The physical properties of such gases, domin…