Trade-off relations place fundamental limits on the operations that physical systems can perform. This Letter presents a trade-off relation that bounds the correlation function, which measures the relationship between a system's current and future states, in Markov processes. The obtained bound, referred to as the thermodynamic correlation inequality, states that the change in the correlation function has an upper bound comprising the dynamical activity, a thermodynamic measure of the activity of a Markov process. Moreover, by applying the obtained relation to the linear response function, it is demonstrated that the effect of perturbation can be bounded from above by the dynamical activity.
The third law of thermodynamics in the form of the unattainability principle states that exact ground-state cooling requires infinite resources. Here we investigate the amount of non-equilibrium resources needed for approximate cooling. We consider as resource any system out of equilibrium, allowing for resources beyond the i.i.d. assumption and including the input of work as a particular case. We establish in full generality a sufficient and a necessary condition for cooling and show that for a vast class of non-equilibrium resources these two conditions coincide, providing a single necessary…
Various quantum thermodynamic bounds are shown to stem from a single tighter and more general inequality, consequence of the operator concavity of the logarithmic function. Such an inequality, which we call the "thermodynamic reverse bound", is compactly expressed as a quantum relative entropy, from which it inherits mathematical properties and meaning. As concrete examples, we apply our bound to evaluate the thermodynamic length for open processes, the heat exchange in erasure processes, and the maximal energy outflow in general quantum evolutions.
We present a new inequality which holds in the thermodynamical processes with measurement and feedback controls with using only the Helmholtz free energy and the entanglement of formation: $W_{\mathrm{ext}}\le-ΔF-k_{B}TΔE_{F}$. The quantity $-ΔE_{F}$, which is positive, expresses the amount of entanglement transfer from the system $S$ to the probe $P$ through the interaction $\hat{U}_{SP}$ during the measurement. It is easier to achieve the upper bound in the new inequality than in the Sagawa-Ueda inequality [Phys. Rev. Lett. 100 080403 (2008)]. The new inequality has clear physical meaning: i…
The main thread that links classical thermodynamics and the thermodynamics of small quantum systems is the celebrated Clausius inequality form of the second law. However, its application to small quantum systems suffers from two cardinal problems: (i) The Clausius inequality does not hold when the system and environment are initially correlated - a commonly encountered scenario in microscopic setups. (ii) In some other cases, the Clausius inequality does not provide any useful information (e.g. in dephasing scenarios). We address these deficiencies by developing the notion of global passivity …
In Phys. Rev. Lett. 128, 200501 (2022) the authors consider the thermodynamic cost of quantum metrology. One of the main results is $\mathcal{S} \geq \log(2) \| h_λ\|^{-2} F_Q [ψ_λ]$, which purports to relate the Shannon entropy $\mathcal{S}$ of an optimal measurement (i.e., in the basis of the symmetric logarithmic derivative) to the quantum Fisher information $F_Q$ of the pure state $|ψ_λ\rangle$. However, we show that in the setting considered by the authors we have $\mathcal{S} = \log(2)$ and $\| h_λ\|^{2} = \max_{ψ_λ} F_Q[ψ_λ]$, so that their inequality reduces to the trivial inequality $…
Thermodynamic uncertainty principles make up one of the few rare anchors in the largely uncharted waters of nonequilibrium systems, the fluctuation theorems being the more familiar. In this work we aim to trace the uncertainties of thermodynamic quantities in nonequilibrium systems to their quantum origins, namely, to the quantum uncertainty principles. Our results enable us to make this categorical statement: For Gaussian systems, thermodynamic functions are functionals of the Robertson-Schrodinger uncertainty function, which is always non-negative for quantum systems, but not necessarily so …
We report two results complementing the second law of thermodynamics for Markovian open quantum systems coupled to multiple reservoirs with different temperatures and chemical potentials. First, we derive a nonequilibrium free energy inequality providing an upper bound for a maximum power output, which for systems with inhomogeneous temperature is not equivalent to the Clausius inequality. Secondly, we derive local Clausius and free energy inequalities for subsystems of a composite system. These inequalities differ from the total system one by the presence of an information-related contributio…
Accurate thermodynamic simulations of correlated fermions using path integral Monte Carlo (PIMC) methods are of paramount importance for many applications such as the description of ultracold atoms, electrons in quantum dots, and warm-dense matter. The main obstacle is the fermion sign problem (FSP), which leads to an exponential increase in computation time both with increasing the system-size and with decreasing temperature. Very recently, Hirshberg et al. [J. Chem. Phys. 152, 171102 (2020)] have proposed to alleviate the FSP based on the Bogoliubov inequality. In the present work, we extend…
We show that complete positivity is not only sufficient but also necessary for the validity of the quantum data-processing inequality. As a consequence, the reduced dynamics of a quantum system are completely positive, even in the presence of initial correlations with its surrounding environment, if and only if such correlations do not allow any anomalous backward flow of information from the environment to the system. Our approach provides an intuitive information-theoretic framework to unify and extend a number of previous results.
We prove that for a single-component many-body system at zero temperature the inequality $E_{\rm int} \leq\, P\,V$ holds, where $E_{\rm int}$ is the interaction energy, $P$ is pressure and $V$ is volume. This inequality is proven under rather general assumptions with the use of Anderson-type bound relating ground state energies of systems with different numbers of particles. We also consider adding impurity particles to the system and derive inequalities on the chemical potential of the impurity and binding energy of the bound state of two impurities.
An inequality is deduced from Einstein's locality and a supplementary assumption. This inequality defines an experiment which can actually be performed with present technology to test local realism. Quantum mechanics violate this inequality a factor of 1.5. In contrast, quantum mechanics violates previous inequalities (for example, Clauser-Horne-Shimony-Holt inequality of 1969, Freedman-Clauser inequality of 1972, Clauser-Horne inequality of 1974) by a factor of $\sqrt 2$. Thus the magnitude of violation of the inequality derived in this paper is approximately $20.7%$ larger than the magnitude…
We generalize the correlation functions of the Clauser-Horne-Shimony-Holt (CHSH) inequality to arbitrarily high-dimensional systems. Based on this generalization, we construct the general CHSH inequality for bipartite quantum systems of arbitrarily high dimensionality, which takes the same simple form as CHSH inequality for two-dimension. This inequality is optimal in the same sense as the CHSH inequality for two dimensional systems, namely, the maximal amount by which the inequality is violated consists with the maximal resistance to noise. We also discuss the physical meaning and general def…
We propose a new form of the Second Law inequality that defines a tight bound for extractable work from the non-equilibrium quantum state. In classical thermodynamics, the optimal work is given by the difference of free energy, what according to the result of Skrzypczyk \emph{et al.} can be generalized for individual quantum systems. The saturation of this bound, however, requires an infinite bath and an ideal energy storage that is able to extract work from coherences. The new inequality, defined in terms of the ergotropy (rather than free energy), incorporates both of those important microsc…
We generalize the correlation functions of the Clauser-Horne-Shimony-Holt (CHSH) inequality to multipartite d-dimensional systems. All the Bell inequalities based on this generalization take the same simple form as the CHSH inequality. For small systems, numerical results show that the new inequalities are tight and we believe this is also valid for higher dimensional systems. Moreover, the new inequalities are relevant to the previous ones and for bipartite system, our inequality is equivalent to the Collins-Gisin-Linden-Masser-Popescu (CGLMP) inequality.
Proofs of Bell's theorem and the data analysis used to show its violation have commonly assumed a spatially stationary underlying process. However, it has been shown recently that the appropriate Bell's inequality holds identically for cross correlations of three or four lists of + or - 1's, independently of statistical assumptions. When data consistent with its derivation are analyzed without imposition of the stationarity assumption, the resulting correlations satisfy the Bell inequality.
In this paper we prove that the inequality introduced by Collins, Gisin, Linden, Massar and Popescu is tight, or in other words, it is a facet of the convex polytope generated by all local-realistic joint probabilities of d outcomes. This means that this inequality is optimal. We also show that, for correlation functions generalized to deal with three-outcome measurements, the satisfyability of this inequality is a necessary and sufficient condition for the existence of a local-realistic model accounting for them.
Violation of a Bell inequality guarantees the existence of quantum correlations in a quantum state. A pure bipartite quantum state, having nonvanishing quantum correlation, always violates a Bell inequality. Such correspondence is absent for multipartite pure quantum states. For a shared multipartite quantum state, we establish a connection between the monogamy of Bell inequality violation and genuine multi-site entanglement as well as monogamy-based multiparty quantum correlation measures. We find that generalized Greenberger-Horne-Zeilinger states and another single-parameter family states w…
It is not generally known, that the inequality that Bell derived using three random variables must be identically satisfied by any three corresponding data sets of plus and minus 1s that are writable on paper.This surprising fact is not immediately obvious from Bell's inequality derivation based on causal random variables, but follows immediately if the same mathematical operations are applied to finite data sets.For laboratory data, the inequality is identically satisfied as a fact of pure algebra, and its satisfaction is independent of whether the processes generating the data are local, non…
Violation of modified Wigner inequality by means binary bipartite quantum system allows the discrimination between the quantum world and the classical local-realistic one, and also ensures the security of Ekert-like quantum key distribution protocol. In this paper we study both theoretically and experimentally the bounds of quantum correlation associated to the modified Wigner's inequality finding the optimal experimental configuration for its maximal violation. We also extend this analysis to the implementation of Ekert's protocol.
Quantum mechanics exhibits a very peculiar form of contextuality. Identifying and connecting the simplest scenarios in which more general theories can or cannot be more contextual than quantum mechanics is a fundamental step in the quest for the principle that singles out quantum contextuality. The former scenario corresponds to the Klyachko-Can-Binicioglu-Shumovsky (KCBS) inequality. Here we show that there is a simple tight inequality, twin to the KCBS, for which quantum contextuality cannot be outperformed. In a sense, this twin inequality is the simplest tool for recognizing fully contextu…
The correct laws of thermodynamics, either classical or quantum without probabilities of statistical quantum mechanics are valid for all systems, large or small, including systems of one spin or one particle only. So no violations can occur in nanoscale electric circuits.
The relativistic version of the Greenberger-Horne-Zeilinger experiment with massive particles is proposed. We point out that, in the moving frame, GHZ correlations of spins in original directions transfer to different directions due to the Wigner rotation. Its effect on the degree of violation of Bell-type inequality is also discussed.
We design a heat engine with multi-heat-reservoir, ancillary system and quantum memory. We then derive an inequality related with the second law of thermodynamics, and give a new limitation about the work gain from the engine by analyzing the entropy change and quantum mutual information change during the process. In addition and remarkably, by combination of two independent engines and with the help of the entropic uncertainty relation with quantum memory, we find that the total maximum work gained from those two heat engines should be larger than a quantity related with quantum entanglement …
We numerically demonstrate that "mode-entangled states" based on the transverse modes of classical optical fields in multimode waveguides violate Bell's inequality. Numerically simulating the correlation measurement scheme of Bell's inequality, we obtain the normalized correlation functions of the intensity fluctuations for the two entangled classical fields. By using the correlation functions, the maximum violations of Bell's inequality are obtained. This implies that the two classical fields in the mode-entangled states, although spatially separated, present a nonlocal correlation.
In this paper I demonstrate that the quantum correlations of polarization (or spin) observables used in Bell's argument against local realism have to be interpreted as {\it conditional} quantum correlations. By taking into account additional sources of randomness in Bell's type experiments, i.e., supplementary to source randomness, I calculate (in the standard quantum formalism) the complete quantum correlations. The main message of the quantum theory of measurement (due to von Neumann) is that complete correlations can be essentially smaller than the conditional ones. Additional sources of ra…
We find a single parameter family of genuinely entangled three qubit pure states, called the maximally Bell inequality violating states (MBV), which exhibit maximum Bell inequality violation by the reduced bipartite system for a fixed amount of genuine tripartite entanglement quantified by the so called tangle measure. This in turn implies that there holds a complementary relation between the Bell inequality violation by the reduced bipartite systems and the tangle present in the three qubit states, not necessarily pure. The MBV states also exhibit maximum Bell inequality violation by the redu…
We formulate the Einstein-Podolsky-Rosen (EPR) gedankenexperiment within the framework of relativistic quantum theory to analyze a situation in which measurements are performed by moving observers. We point out that under certain conditions the perfect anti-correlation of an EPR pair of spins in the same direction is deteriorated in the moving observers' frame due to the Wigner rotation, and show that the degree of the violation of Bell's inequality prima facie decreases with increasing the velocity of the observers if the directions of the measurement are fixed. However, this does not imply a…
The characterization of quantum information quantifiers has attracted a considerable attention of the scientific community, since they are a useful tool to verify the presence of quantum correlations in a quantum system. In this context, in the present work we show a theoretical study of some quantifiers, such as entanglement witness, entanglement of formation, Bell's inequality violation and geometric quantum discord as a function of the diffractive properties of neutron scattering. We provide one path toward identifying the presence of quantum correlations and quantum nonlocality in a molecu…
In multiparty quantum systems, the monogamy inequality proposes an upper bound on the distribution of bipartite quantum correlation between a single party and each of the remaining parties in the system, in terms of the amount of quantum correlation shared by that party with the rest of the system taken as a whole. However, it is well-known that not all quantum correlation measures universally satisfy the monogamy inequality. In this work, we aim at determining the non-trivial value by which the monogamy inequality can be violated by a quantum correlation measure. Using an information-theoreti…
In constructing his theorem, Bell assumed that correlation functions among non-commuting variables are the same as those among commuting variables. However, in quantum mechanics, multiple data values exist simultaneously for commuting operations while for non-commuting operations data are conditional on prior outcomes, or may be predicted as alternative outcomes of the non-commuting operations. Given these qualitative differences, there is no reason why correlation functions among non-commuting variables should be the same as those among commuting variables, as assumed by Bell. When data for c…
We present a generalized quantum scattering circuit which can be used to perform non-invasive quantum measurements, and implement it on NMR qubits. Such a measurement is a key requirement for testing temporal non-contextual inequalities. We use this circuit to experimentally demonstrate the violation of the Peres-Mermin inequality (which is the temporal analog of a Klyachko-Can- Binicioglu-Shumovsky (KCBS) inequality), on a three-qubit NMR quantum information processor. Further, we experimentally demonstrate the violation of a transformed Bell-type inequality (the spatial equivalent of the tem…
We analyze the correlation structure of bipartite arbitrary-dimensional Bell inequalities via novel conditions of correlations in terms of differences of joint probabilities called correlators. The conditions of correlations are shown to be necessary for the multi-level Bell state. In particular, we find that the bipartite arbitrary-dimensional Bell-type inequalities introduced by Collins-Gisin-Linden-Massar-Popescu [Phys. Rev. Lett. 88, 040404 (2002)] and Son-Lee-Kim [Phys. Rev. Lett. 96, 060406 (2006)] are composed of correlators, and we reveal that the maximal violations by the Bell state j…
Correlations for the Bell gedankenexperiment are constructed using probabilities given by quantum mechanics, and nonlocal information. They satisfy Bell's inequality and exhibit spatial non stationarity in angle. Correlations for three successive local spin measurements on one particle are computed as well. These correlations also exhibit non stationarity, and satisfy the Bell inequality. In both cases, the mistaken assumption that the underlying process is wide-sense-stationary in angle results in violation of Bell's inequality. These results directly challenge the wide-spread belief that vio…
According to the second law, the efficiency of cyclic heat engines is limited by the Carnot bound that is attained by engines that operate between two thermal baths under the reversibility condition whereby the total entropy does not increase. Quantum engines operating between a thermal and a squeezed-thermal bath have been shown to surpass this bound. Yet, their maximum efficiency cannot be determined by the reversibility condition, which may yield an unachievable efficiency bound above unity. Here we identify the fraction of the exchanged energy between a quantum system and a bath that neces…
We propose a new inequality that we call the conditional ageing inequality (CAIN). The CAIN is a slight generalization to non-equilibrium situations of the Second Law of thermodynamics. The goal of this paper is to study the consequences of the CAIN. We use the CAIN to discuss Maxwell demon processes (i.e., thermodynamic processes with feedback.) In particular, we apply the CAIN to four cases of the Szilard engine: for a classical or a quantum system with either one or two correlated particles. Besides proposing this new inequality that we call the CAIN, another novel feature of this paper is …
We proved when random-variable fluctuations obey the central limit theorem the equality of the uncertainty relation corresponds to the thermodynamic equilibrium state. The inequality corresponds to the thermodynamic non-equilibrium state. The uncertainty relation is a quantum-mechanics expression of the second law of thermodynamics originated in wave-particle duality. Formulas of mean square-deviations changes adjusted by random fluctuations under the minimal uncertainty relation are obtained. Finally, an assumption is made which is waiting for examination. We except phase transitions in our d…
We derive a new inequality that is necessary and sufficient to show EPR-steering in a scenario employing only correlations between two arbitrary dichotomic measurements on each party. Thus the inequality is a complete steering analogy of the CHSH inequality, a generalisation of the result of Cavalcanti et al, JOSA B, 32(4), A74 (2015). We show that violation of the inequality only requires measuring over equivalence classes of mutually unbiased measurements on the trusted party and in fact assuming a general two qubit system arbitrary pairs of distinct projective measurements at the trusted pa…
It is one of the most remarkable features of quantum physics that measurements on spatially separated systems cannot always be described by a locally causal theory. In such a theory, the outcomes of local measurements are determined in advance solely by some unknown (or hidden) variables and the choice of local measurements. Correlations that are allowed within the framework of a locally causal theory are termed classical. Typically, the fact that quantum mechanics does not always result in classical correlations is revealed by the violation of Bell inequalities, which are constraints that hav…
Cirel'son inequality states that the absolute value of the combination of quantum correlations appearing in the Clauser-Horne-Shimony-Holt (CHSH) inequality is bound by $2 \sqrt 2$. It is shown that the correlations of two qubits belonging to a three-qubit system can violate the CHSH inequality beyond $2 \sqrt 2$. Such a violation is not in conflict with Cirel'son's inequality because it is based on postselected systems. The maximum allowed violation of the CHSH inequality, 4, can be achieved using a Greenberger-Horne-Zeilinger state.
It is possible for two parties, Alice and Bob, to establish a secure communication link by sharing an ensemble of entangled particles, and then using these particles to generate a secret key. One way to establish that the particles are indeed entangled is to verify that they violate a Bell inequality. However, it might be the case that Bob is not trustworthy and wishes Alice to believe that their communications are secure, when in fact they are not. He can do this by managing to have prior knowledge of Alice's measurement device settings and then modifying his own settings based upon this info…
The EPR correlation matrix admit a Hilbert model if it can be extended to a positive full correlation matrix. A simple proof of the corresponding Tsirelson bound is given and the relations to PR boxes and indefinite inner product spaces are briefly discussed.
Explicit local hidden variables models are exhibited that assume a correlation between detection events produced in the same detector at different times. It is shown that some models give predictions closer to the Bell limit than models without time correlation.
In this paper, we use Bell inequality and nonlocality to study the bipartite correlation in an exactly soluble two-dimensional mixed spin system. Bell inequality turns out to be a valuable detector for phase transitions in this model. It can detect not only the quantum phase transition, but also the thermal phase transitions, of the system. The property of bipartite correlation in the system is also analyzed. In the quantum anti-ferromagnetic phase, the Bell inequality is violated thus nonlocality is present. It is interesting that the nonlocality is enhanced by thermal fluctuation, and simila…
We provide a characterization of energy in the form of exchanged heat and work between two interacting constituents of a closed, bipartite, correlated quantum system. By defining a binding energy we derive a consistent quantum formulation of the first law of thermodynamics, in which the role of correlations becomes evident, and this formulation reduces to the standard classical picture in relevant systems. We next discuss the emergence of the second law of thermodynamics under certain---but fairly general---conditions such as the Markovian assumption. We illustrate the role of correlations and…
We study the polarization dependent second order correlation of a pair of photons emitted in a four level radiative cascade driven by an external field. It is found that the quantum correlations of the emitted photons, degraded by the energy splitting of the intermediate levels in the radiative cascade can be efficiently revived by a far detuned external field. The physics of this revival is linked to an induced stark shift and the formation of dressed states in the system by the non-resonant external field. Further, we investigated the competition between the effect of the coherent external f…
We consider optical beams with topological singularities which possess Schmidt decomposition and show that such classical beams share many features of two mode entanglement in quantum optics. We demonstrate the coherence properties of such beams through the violations of Bell inequality for continuous variables using the Wigner function. This violation is a consequence of correlations between the $(x, p_x)$ and $(y, p_y)$ spaces which mathematically play the same role as nonlocality in quantum mechanics. The Bell violation for the LG beams is shown to increase with higher orbital angular momen…
For an even qudit dimension $d\geq 2,$ we introduce a class of two-qudit states exhibiting perfect correlations/anticorrelations and prove via the generalized Gell-Mann representation that, for each two-qudit state from this class, the maximal violation of the original Bell inequality is bounded from above by the value $3/2$ - the upper bound attained on some two-qubit states. We show that the two-qudit Greenberger-Horne-Zeilinger (GHZ) state with an arbitrary even $d\geq 2$ exhibits perfect correlations/anticorrelations and belongs to the introduced two-qudit state class. These new results ar…
Franson-type nonlocal correlation is a testing tool for Bell inequality violation using noninterfering interferometers, where coincidence measurements involve an interference fringe of g^((1)) correlation between noninterfering photon pairs. Like the Bell inequality, Franson correlation is also limited to a microscopic regime of entangled photon pairs. Here, randomness-based macroscopic Franson-type nonlocal correlation is presented using polarization-basis coherent superposition of laser light, where probabilistic randomness between bipartite orthonormal bases plays an important role for both…
Quantum Correlations are studied extensively in quantum information domain. Entanglement Measures and Quantum Discord are good examples of these actively studied correlations. Detection of violation in Bell inequalities is also a widely active area in quantum information theory world. In this work, we revisit the problem of analyzing the behavior of quantum correlations and violation of Bell inequalities in noisy channels. We extend the problem defined in [1] by observing the changes in negativity measure, quantum discord and a modified version of Horodecki measure for violation of Bell inequa…
Quantum thermodynamics and quantum information are two frameworks for employing quantum mechanical systems for practical tasks, exploiting genuine quantum features to obtain advantages with respect to classical implementations. While appearing disconnected at first, the main resources of these frameworks, work and correlations, have a complicated yet interesting relationship that we examine here. We review the role of correlations in quantum thermodynamics, with a particular focus on the conversion of work into correlations. We provide new insights into the fundamental work cost of correlation…
Bell inequality violation is one of the most widely known manifestations of entanglement in quantum mechanics; indicating that experiments on physically separated quantum mechanical systems cannot be given a local realistic description. However, despite the importance of Bell inequalities, it is not known in general how to determine whether a given entangled state will violate a Bell inequality. This is because one can choose to make many different measurements on a quantum system to test any given Bell inequality and the optimization over measurements is a high-dimensional variational problem…
In the paper the EPR-Bohm scenario will be reproduced in an algebraic quantum field theoretical setting with locally finite degrees of freedom. It will be shown that for a set of spatially separated correlating events (projections) maximally violating the Clauser-Horne inequality there can be given a common causal explanation if commutativity is abandoned between the common cause and the correlating events. Moreover, the noncommuting common cause will be local and supported in the common past of the correlating events.
Adopting the frame of mesoscopic physics, we describe a Bell type experiment involving time-delayed two-particle correlation measurements. The indistinguishability of quantum particles results in a specific interference between different trajectories. We show how the non-locality in the time-delayed correlations due to the indistinguishability of the quantum particles manifests itself in the violation of a Bell inequality, where the degree of violation is related to the accuracy of the measurement. We demonstrate how the interrelation between the orbital- and the spin exchange symmetry can by …
In contrast to Bell's inequalities which test the correlations between multiple spatially separated systems, the Leggett-Garg inequalities test the temporal correlations between measurements of a single system. We experimentally demonstrate the violation of the Leggett-Garg inequality in a classical optical system using only the polarization degree-of-freedom of a laser beam. Our results show maximal violations of the Leggett-Garg inequality.
