The generation of a laser filament through clouds produces a shockwave which displaces the small water droplets from the air to create a quasi-transparent channel through which, information can be transmitted. We present a robust method that utilizes the channel for free-space optical communication using structured light beams coupled with a femtosecond filament. Vortex beams based on their spatial profiles and non-diffractive characteristics are perfectly suited to propagate around the filament. We have also developed a 4-bit communication channel using these structured light beam. We introduce a method dubbed segmented space division multiplexing. Our system demonstrates resilience to noise and is unaffected by the filament. This method can improve the scalability, robustness, and capacity of the free optical channel.
A giant blue shift of an isolated visible band of supercontinuum was discovered and studied in the single filament regime of Mid-IR femtosecond laser pulse at powers slightly exceeding critical power for self-focusing in fluorides.
We investigate beam pointing dynamics in filamentation in gases driven by high repetition rate femtosecond laser pulses. Upon suddenly exposing a gas to a kilohertz train of filamenting pulses, the filament is steered from its original direction to a new stable direction whose equilibrium is determined by a balance among buoyant, viscous, and diffusive processes in the gas. Results are shown for Xe and air, but are broadly applicable to all configurations employing high repetition rate femtosecond laser propagation in gases.
Femtosecond laser filament generates strong terahertz (THz) pulse in air. In this paper, THz pulse waveform generated by femtosecond laser filament has been experimentally investigated as a function of the length of the filament. Superluminal propagation of THz pulse has been uncovered, indicating that the filament creates a THz waveguide in air. Numerical simulation has confirmed that the waveguide is formed because of the radially non-uniform refractive index distribution inside the filament. The underlying physical mechanisms and the control techniques of this type THz pulse generation meth…
An influence of pass-through optics on femtosecond laser pulse filamentation in ambient air is analyzed for the first time both experimentally and numerically. Propagation of high-power femtosecond laser pulse through solid optical elements introduces spatiotemporal phase modulation due to the Kerr effect. This modulation may have a strong ef-fect on the pulse filamentation in air. We demonstrated that the phase modulation obtained in the thin pass-through dielectric plate reduces the distance to the filament onset and increases the plasma channel length
Polarization dependence on clamping intensity inside femtosecond filament was experimentally measured in air. By tuning the laser pulse ellipse from linear polarization to circular polarization, the measured clamping intensity inside laser filament is gradually increased up to 1.7 times. The experimental results are in good agreement with the simulation results by solving the extended nonlinear Schrodinger equation (NLSE). The polarization sensitive clamping intensity inside filaments offers an important factor towards fully understanding the polarization related phenomenon observed so far.
The filamentational instability of spatially broadband femtosecond optical pulses in air is investigated by means of a kinetic wave equation for spatially incoherent photons. An explicit expression for the spatial amplification rate is derived and analyzed. It is found that the spatial spectral broadening of the pulse can lead to stabilization of the filamentation instability. Thus, optical smoothing techniques could optimize current applications of ultra-short laser pulses, such as atmospheric remote sensing.
An influence of plasma channel created by a filament of focused UV or IR femtosecond laser pulse (λ=248 nm or 740 nm) on characteristics of other plasma channel formed by a femtosecond pulse at the same wavelength following the first one with varied nanosecond time delay was experimentally studied. A dependence of optical transparency of the first channel and plasma density of the second channel on the time delay was demonstrated to be quite different for such a double UV and IR femtosecond pulses.
A general form of the kinetic equation for filament number density considering the effects of their generation and decay is stated. It is consists of the phenomenological parameters, which have been determined from the direct numerical simulation of propagation of a high-power femtosecond laser pulse (HPFLP) based on the stationary nonlinear Schrödinger equation (NSE) for a series of the threshold particular cases.
We demonstrate that Freeman resonances have a strong impact on the nonlinear optical response in femtosecond filaments. These resonances decrease the transient refractive index within a narrow intensity window and strongly affect the filamentation dynamics. In particular, we demonstrate that the peak intensity of the filament can be clamped at these resonances, hinting at the existence of new regimes of filamentation with electron densities considerably lower than predicted by the standard model. This sheds a new light on the phenomenon of filamentary intensity clamping and the plasmaless fila…
We report on experimental realization of impulsive rotational Raman scattering from neutral nitrogen molecules in a femtosecond laser filament using an intense self-induced white-light seeding "air laser" generated during the filamentation of an 800 nm Ti: Sapphire laser in nitrogen gas. The impulsive rotational Raman fingerprint signals are observed with a maximum conversion efficiency of ~0.8%. Our observation provides a promising way of remote identification and location of chemical species in atmosphere by rotational Raman scattering of molecules.
We report on strong backward stimulated emission at 337 nm in Nitrogen gas pumped by circularly polarized femtosecond laser pulses at 800 nm. A distinct dependence of the backward UV spectrum on pump laser polarization and intensity is observed, pointing to the occurrence of backward amplified spontaneous emission inside filaments. We attribute the population inversion to inelastic collision between the free electrons produced by the pump laser and neutral N2 molecules. The addition of Oxygen molecules is detrimental for the gain, reducing it to near threshold at atmospheric concentration.
Terahertz (THz) imaging provides cutting edge technique in biology, medical sciences and non-destructive evaluation. However, due to the long wavelength of the THz wave, the obtained resolution of THz imaging is normally a few hundred microns and is much lower than that of the traditional optical imaging. We introduce a sub-wavelength resolution THz imaging technique which uses the THz radiation generated by a femtosecond laser filament in air as the probe. This method is based on the fact that the femtosecond laser filament forms a waveguide for the THz wave in air. The diameter of the THz be…
We experimentally studied intense femtosecond pulse filamentation and propagation in water for Gaussian, Laguerre-Gaussian, and Bessel-Gaussian incident beams. These different transverse modes for incident laser pulses were created from an initial Gaussian beam by using a computer generated hologram technique. We found that the length of the filament induced by the Bessel-Gaussian incident beam was longer than that for the other transverse modes under the conditions of the same peak intensity, pulse duration, and the size of the central part of the beam. To better understand the Bessel-Gaussia…
We present direct measurements of the gas acoustic dynamics following interaction of spatial single- and multi-mode 50 fs, 800 nm pulses in air at 10 Hz and 1 kHz repetition rates. Results are in excellent agreement with hydrodynamic simulations. Under no conditions for single filaments do we find on-axis enhancement of gas density; this occurs only with multi-filaments. We also investigate the propagation of probe beams in the gas density profile induced by a single extended filament. We find that light trapping in the expanding annular acoustic wave can create the impression of on-axis guidi…
We report, for what we believe to be the first time, on the generation of remote self-seeding laser amplification by using only one 800 nm Ti:Sapphire femtosecond laser pulse. The laser pulse (~ 40 fs) is first used to generate a filament either in pure nitrogen or in ambient air in which population inversion between ground and excited states of nitrogen molecular ions is realized. Self-induced white light inside the filament is then serving as the seed to be amplified. The self-induced narrow-band laser at 428 nm has a pulse duration of ~2.6 ps with perfect linear polarization property. This …
In this work, sub-ppb aerosol detection is achieved by femtosecond laser filament with a single pulse energy of 4 mJ at a distance of 30 m. A concave mirror with an open aperture of 41.4 cm is employed in an off-axis optical system to focus the femtosecond laser beam and collect the fluorescence of NaCl aerosol. The simulation and experimental results show that the astigmatism can be greatly reduced when femtosecond laser beam is incident non-symmetrically on the concave mirror. Compared with the case that femtosecond laser strikes at the center of the concave mirror, the intensity of the opti…
Multiple filamentation in air of high-power ultrashort laser radiation with transverse intensity profile resembling a "corona" composed by incoherent combining of several annularly distributed independent top-hat sub-beams is theoretically studied. Through the numerical solution of time-averaged nonlinear Schrodinger equation, we study the spatio-angular dynamics of synthesized near-infrared "corona-beam" (CB) along the optical path by varying the number and power of the beamlets (corona-spikes). For the first time to our knowledge, the evident advances in the multiple filamentation region man…
The results of investigation of extremely compressed wave packet-light bullet (LB) penetration through an air gap under single-pulse femtosecond Mid IR filamentation in LiF are presented. It is revealed by the laser coloration method and from numerical simulations that a single-cycle LB, which was formed before an air gap up to 0.5 mm width, completely recovered after passing some distance in LiF after the gap. This distance increases nonlinearly with the gap width and LB pathway before the gap. LB in the air gap has a strongly convergent wave front with focusing radius of 20-100 μm and its di…
High-power femtosecond laser radiation propagates nonlinearly in air exhibiting pulse self-focusing and strong multiphoton medium ionization, which leads to the spatial fragmentation of laser pulse into highly-localized light channels usually called the filaments. The filaments are characterized by high optical intensity, reduced (even zero) angular spreading and can contain laser plasma or be plasmaless (postfilaments). The presence of optical turbulence on the propagation path dramatically changes pulse filamentation dynamics and in some cases causes pulse fragmentation enhancement and colla…
Stable propagation of large, multifilament arrays over long distances in air paves new ways for microwave-radiation manipulation. Although, the dynamics of a single or a few filaments was discussed in some of the previous studies, we show that the stability of large plasma filament arrays is significantly more complicated and is constrained by several trade-offs. Here, we analyze the stability properties of rectangular arrays as a function of four parameters: relative phase of the generating beams, number of filaments, separation between them, and initial power. We find that arrays with altern…
We experimentally demonstrate energy exchange between a delay-tuned femtosecond beam and two delay-fixed ones as they spatiotemporally overlapped and experienced filamentation in air. The energy exchange process in the relative time delay is dramatically elongated up to 40 ps in the presence of plasma grating, indicating that filamentary beams coupling may be an effective method for filament control.
Using femtosecond laser pulses at 800 and 400 nm, we characterize the formation of underdense channels in air generated by laser filamentation at the millijoule energy level by means of transverse interferometry. We find that using tight focusing conditions, filamentation generates a shock wave and that the resulting low-density channel lasts for more than 90 ms. Comparison of these results with hydrodynamic simulations using an Eulerian hydrodynamic code gives an good agreement and allows us to estimate the initial gas peak temperature at $\sim$ 1000 K. The influence of experimental parameter…
Recently, S. Mitryukovskiy et al. presented experimental evidence showing that backward stimulated radiation at 337 nm can be obtained from plasma filaments in nitrogen gas pumped by circularly polarized 800 nm femtosecond pulses (Opt. Express, 22, 12750 (2014)). Here, we report that this backward stimulated radiation is enhanced by a factor of ~ 16 in the presence of a seed pulse. This enhanced stimulated radiation can be either linearly or circularly polarized, dictated by the seeding pulse, which is distinct from the non-polarized nature of the ASE without seeding pulse. We also measured th…
We experimentally investigate generation of backward 357 nm N2 laser in a gas mixture of N2/Ar using 800-nm femtosecond laser pulses, and examine the involved gain dynamics based on pump-probe measurements. Our findings show that a minimum lifetime of population inversion in the excited N2 molecules is required for generating intense backward nitrogen lasers, which is ~0.8 ns under our experimental conditions. The results shed new light on the mechanism for generating intense backward lasers from ambient air, which are highly in demand for high sensitivity remote atmospheric sensing applicatio…
A wavelength-degenerate pump-probe spectroscopy is used to study the ultrafast dynamics of strong-field ionization in femtosecond-laser subwavelength-structured fused silica. The comparative spectra demonstrate that femtosecond-laser subwavelength structuring always give rise to great enhancement for strong-field ionization as well as third-order nonlinear optical effects, which is the direct evidence of great local field enhancement in subwavelength apertures of fs-laser highly-excited surface. In short, the study shows the prominent subwavelength spatial effect of strong-field ionization in …
The absence of ionization and observation of white continuum in the initial moment of filamentation of powerful femtosecond laser pulses, propagating in silica glasses, as well as the filamentation without plasma channels observed in the experiments in air, forced us to look for other nonlinear mechanisms of description the above mentioned effects. For this reason we present in this paper new parametric conversion mechanism for asymmetric spectrum broadening of femtosecond laser pulses towards the higher frequencies in isotropic media. This mechanism includes cascade generation with THz spectr…
Numerous techniques have been demonstrated for effective generation of orbital angular momentum-carrying radiation, but intracavity generation of continuously tunable pulses in the femtosecond regime remains challenging. Even if such a creation was realized, the generated pulses, like all pulses in reality, are complex and transitory objects that can only be comprehensively characterized via multidimensional spaces. An integrated lasing system that generates pulses while simultaneously quantifies them can achieve adaptive pulse tailoring. Here, we report a femtosecond pulse scope that unifies …
A high contrast imaging technique based on an optical vortex coronagraph (OVC) is used to measure the spatial phase profile induced by an air plasma generated by a femtosecond laser pulse. The sensitivity of the OVC method significantly surpassed both in-line holographic and direct imaging methods based on air plasma fluorescence. The estimated phase sensitivity of 0.046 waves provides opportunities for OVC applications in areas such as bioimaging, material characterization, as well as plasma diagnostics.
We demonstrate numerically and experimentally the generation of powerful supercontinuum vortices from femtosecond vortex beams by using multiple thin fused silica plates. The supercontinuum vortices are shown to preserve the vortex phase profile of the initial beam for spectral components ranging from 500 nm to 1200 nm. The transfer of the vortex phase profile results from the inhibition of multiple filamentation and the preservation of vortex ring with relatively uniform intensity distribution by means of the thin-plate scheme, where the supercontinuum is mainly generated from the self-phase …
We demonstrate theoretically that few-cycle vortex beam with subterawatt peak power can be generated by self-compression of mid-infrared femtosecond vortex beam using the thin-plate scheme. The 3 μm femtosecond vortex beam with input duration of 90 fs is compressed to 15.1 fs with the vortex characteristics preserved. The conversion efficiency is as high as 91.5% and the peak power reaches 0.18 TW. The generation of the high-peak-power few-cycle vortex beam is owing to the proper spatiotemporal match by this novel scheme, where the spectrum is broadened enough, the negative group velocity disp…
We demonstrate that femtosecond filaments can set up an extended and robust thermal waveguide structure in air with a lifetime of several milliseconds, making possible the very long range guiding and distant projection of high energy laser pulses and high average power beams. As a proof of principle, we demonstrate guiding of 110 mJ, 7 ns, 532 nm pulses with 90% throughput over ~15 Rayleigh lengths in a 70 cm long air waveguide generated by the long timescale thermal relaxation of an array of femtosecond filaments. The guided pulse was limited only by our available laser energy. In general, th…
We investigate two types of nonlinear interaction between collinear femtosecond laser pulses with power slightly above the critical for self-focusing $P_{cr}$. In the first case we study energy exchange between filaments. The model describes this process through degenerate four-photon parametric mixing (FPPM) scheme and requests initial phase difference between the waves. When there are no initial phase difference between the pulses, the FPPM process does not work. In this case it is obtained the second type of interaction as merging between two, three or four filaments in a single filament wi…
Since their discovery in the mid-1990s, ultrafast laser filaments in gases have been described as products of a dynamic balance between Kerr self-focusing and defocusing by free electric charges that are generated via multi-photon ionization on the beam axis. This established paradigm has been recently challenged by a suggestion that the Kerr effect saturates and even changes sign at high intensity of light, and that this sign reversal, not free-charge defocusing, is the dominant mechanism responsible for the extended propagation of laser filaments. We report qualitative tests of the new theor…
We experimentally demonstrate ultrafast dynamic of generation of a strong 337-nm nitrogen laser by injecting an external seed pulse into a femtosecond laser filament pumped by a circularly polarized laser pulse. In the pump-probe scheme, it is revealed that the population inversion between the excited and ground states of N2 for the free-space 337-nm laser is firstly built up on the timescale of several picoseconds, followed by a relatively slow decay on the timescale of tens of picoseconds, depending on the nitrogen gas pressure. By measuring the intensities of 337-nm signal from nitrogen gas…
Experimental and numerical studies of a temporal evolution of a light bullet formed in isotropic LiF by Mid IR femtosecond pulse (2500 to 3250 nm) of power, slightly exceeding the critical power for self-focusing, are presented. For the first time regular oscillations of the light bullet intensity during its propagation in a filament were registered by investigation of induced color centers in LiF. It was revealed that color centers in a single laser pulse filament have a strictly periodic structure with a length of separate sections about 30 mcm, which increases with a laser pulse wavelength …
Femtosecond lasers interacting with Kerr nonlinear optical materials, propagate in form of filaments due to the balance of beam diffraction by self-focusing induced by the Kerr nonlinearity. Femtosecond laser filamentation is a universal phenomenon that belongs to a general class of processes proper to ultrashort lasers processing systems, associated with the competition between nonlinearity and dispersion also known to promote optical solitons. The present work considers a model describing femtosecond laser inscriptions in a transparent medium with Kerr nonlinearity. Upon inscription, the las…
We propose to use femtosecond direct laser writing technique to realize dielectric optical elements from photo-resist materials for the generation of structured light from purely geometrical phase transformations. This is illustrated by the fabrication and characterization of spin-to-orbital optical angular momentum couplers generating optical vortices of topological charge from 1 to 20. In addition, the technique is scalable and allows obtaining microscopic to macroscopic flat optics. These results thus demonstrate that direct 3D photopolymerization technology qualifies for the realization of…
We present an analytical approach to the theory of nonlinear propagation of femtosecond optical pulses with broad-band spectrum in gases. The vector character of the nonlinear third-order polarization is investigated in details, taking into account the carrier to envelope phase. The corresponding system of vector amplitude equations is written by using left-hand and right-hand circular components of the electrical field. We found that this system nonlinear equations admits $3D+1$ vector soliton solution with Lorentz shape. The solution presents relatively stable propagation and rotation with G…
We report a novel scheme to generate laser-induced, ultrafast, intense (Tesla scale), spatially isolated, magnetic fields. Three-dimensional particle-in-cell simulations show that a femtosecond azimuthally-polarized infrared vector beam, aimed to a conducting circular aperture, produces an intense axially polarized tip-shaped femtosecond magnetic field, extending over micrometer distances and being isolated from the electric field. Our results are backed-up by an analytic model, demonstrating the underlying physics and guiding for optimal parameters. In particular, we find the conditions under…
Supercontinuum (SC) light source has advanced ultrafast laser spectroscopy in condensed matter science, biology, physics, and chemistry. Compared to the frequently used photonic crystal fibers and bulk materials, femtosecond laser filamentation in gases is damage-immune for supercontinuum generation. A bottleneck problem is the strong jitters from filament induced self-heating at kHz repetition rate level. We demonstrate stable kHz supercontinuum generation directly in air with multiple mJ level pulse energy. This is achieved by applying an external DC electric field to the air plasma filament…
Polarization plays crucial role in light-matter interactions; hence its overall manipulation is an essential key to unlock the versatility of light manufacturing, especially in femtosecond laser direct writing. Existing polarization-shaping techniques, however, only focus on the manipulation in transverse plane of a light beam, namely a two-dimensional control. In this paper, we propose a novel passive strategy that exploits a class of femtosecond laser written space varying birefringent elements, to shape the polarization state along the optical path. As a demonstration, we generate a three-d…
The use of structured ultrashort pulses with coupled spatiotemporal properties is emerging as a key tool for ultrafast manipulation. Ultrafast vector beams are opening exciting opportunities in different fields such as microscopy, time-resolved imaging, nonlinear optics, particle acceleration or attosecond science. Here, we implement a technique for the full characterization of structured time-dependent polarization light waveforms with spatiotemporal resolution, using a compact twofold spectral interferometer, based on in-line bulk interferometry and fibre-optic coupler assisted interferometr…
We present an analytical approach to the theory of nonlinear propagation in gases of femtosecond optical pulses with broad-band spectrum . The vector character of the nonlinear third-order polarization of the electrical field in air is investigated in details. A new polarization state is presented by using left-hand and right-hand circular components of the electrical field . The corresponding system of vector amplitude equations is derived in the rotating basis. We found that this system of nonlinear equations has $3D+1$ vector soliton solutions with Lorentz shape. The solution presents a rel…
Nonlinear propagation of intense femtosecond laser pulses in bulk transparent media leads to a specific propagation regime, termed femtosecond filamentation, which in turn produces dramatic spectral broadening, or superbroadening, termed supercontinuum generation. Femtosecond supercontinuum generation in transparent solids represents a compact, efficient and alignment-insensitive technique for generation of coherent broadband radiation at various parts of the optical spectrum, which finds numerous applications in diverse fields of modern ultrafast science. During recent years, this research fi…
The distant projection of high peak and average power laser beams in the atmosphere is a longstanding goal with a wide range of applications. Our early proof-of-principle experiments [Phys. Rev. X 4, 011027 (2014)] presented one solution to this problem, employing the energy deposition of femtosecond filaments in air to sculpt millisecond lifetime sub-meter length air waveguides. Here, we demonstrate air waveguiding at the 50 meter scale, 60X longer, making many practical applications now possible. We employ a new method for filament energy deposition: multi-filamentation of Laguerre-Gaussian …
Femtosecond Engineering of PolyMethylPentene(PMP) Nonlinearity via NA, Spin/orbital angular momentum (OAM), and In-Situ SC Diagnostics
Hong Kong Polytechnic University（香港理工大学）；Chongqing University of Arts and Sciences（重庆文理学院）；University of Liverpool（利物浦大学）；John Moores University（约翰摩尔斯大学）；TPM3D Direct Manufacturing Co., Ltd.（TPM3D直接制造有限公司）
