Multiple filamentation in air of high-power ultrashort laser radiation with transverse intensity profile resembling a "corona" composed by incoherent combining of several annularly distributed independent top-hat sub-beams is theoretically studied. Through the numerical solution of time-averaged nonlinear Schrodinger equation, we study the spatio-angular dynamics of synthesized near-infrared "corona-beam" (CB) along the optical path by varying the number and power of the beamlets (corona-spikes). For the first time to our knowledge, the evident advances in the multiple filamentation region manipulating of synthesized CB are demonstrated. Particularly, by adjusting the number and aperture of the constituting sub-beams it makes possible to significantly delay the CB filamentation onset distance and increase the filamentation length in air. In addition, at the post-filamentation stage of femtosecond pulse propagation under certain conditions the synthesized corona-beams exhibit significantly lower angular divergence of its most intense part (post-filamentation light channel) compared to the beams with regular uni-modal intensity profiles (Gaussian, plateau-like) that provides enhancing of laser power delivered to the receiver over the atmospheric links.
The filamentational instability of spatially broadband femtosecond optical pulses in air is investigated by means of a kinetic wave equation for spatially incoherent photons. An explicit expression for the spatial amplification rate is derived and analyzed. It is found that the spatial spectral broadening of the pulse can lead to stabilization of the filamentation instability. Thus, optical smoothing techniques could optimize current applications of ultra-short laser pulses, such as atmospheric remote sensing.
The propagation of high-power femtosecond laser pulses in air under conditions of superposed spatial phase modulation is considered theoretically. The numerical simulations are carried out on the basis of the reduced form of nonlinear Schrodinger equation (NLSE) for time-averaged electric field envelope. Initial spatial modulations are applied to pulse wavefront profiling by a staggered (TEM33) phase plate which is simulated numerically. The dynamics of laser pulse self-focusing, filamentation, and post-filamentation self-channeling after the phase plates with variable phase jumps is studied. …
An influence of plasma channel created by a filament of focused UV or IR femtosecond laser pulse (λ=248 nm or 740 nm) on characteristics of other plasma channel formed by a femtosecond pulse at the same wavelength following the first one with varied nanosecond time delay was experimentally studied. A dependence of optical transparency of the first channel and plasma density of the second channel on the time delay was demonstrated to be quite different for such a double UV and IR femtosecond pulses.
The results of investigation of extremely compressed wave packet-light bullet (LB) penetration through an air gap under single-pulse femtosecond Mid IR filamentation in LiF are presented. It is revealed by the laser coloration method and from numerical simulations that a single-cycle LB, which was formed before an air gap up to 0.5 mm width, completely recovered after passing some distance in LiF after the gap. This distance increases nonlinearly with the gap width and LB pathway before the gap. LB in the air gap has a strongly convergent wave front with focusing radius of 20-100 μm and its di…
The axial dependence of femtosecond filamentation in air is measured under conditions of varying laser pulsewidth, energy, and focusing f-number. Filaments are characterized by the ultrafast z-dependent absorption of energy from the laser pulse and diagnosed by measuring the local single cycle acoustic wave generated. Results are compared to 2D+1 simulations of pulse propagation, whose results are highly sensitive to the instantaneous (electronic) part of the nonlinear response of $N_2$ and $O_2$. We find that recent measurements of the nonlinear refractive index ($n_2$) in [J.K. Wahlstrand et…
We experimentally investigate generation of backward 357 nm N2 laser in a gas mixture of N2/Ar using 800-nm femtosecond laser pulses, and examine the involved gain dynamics based on pump-probe measurements. Our findings show that a minimum lifetime of population inversion in the excited N2 molecules is required for generating intense backward nitrogen lasers, which is ~0.8 ns under our experimental conditions. The results shed new light on the mechanism for generating intense backward lasers from ambient air, which are highly in demand for high sensitivity remote atmospheric sensing applicatio…
We demonstrate that Freeman resonances have a strong impact on the nonlinear optical response in femtosecond filaments. These resonances decrease the transient refractive index within a narrow intensity window and strongly affect the filamentation dynamics. In particular, we demonstrate that the peak intensity of the filament can be clamped at these resonances, hinting at the existence of new regimes of filamentation with electron densities considerably lower than predicted by the standard model. This sheds a new light on the phenomenon of filamentary intensity clamping and the plasmaless fila…
In this work, sub-ppb aerosol detection is achieved by femtosecond laser filament with a single pulse energy of 4 mJ at a distance of 30 m. A concave mirror with an open aperture of 41.4 cm is employed in an off-axis optical system to focus the femtosecond laser beam and collect the fluorescence of NaCl aerosol. The simulation and experimental results show that the astigmatism can be greatly reduced when femtosecond laser beam is incident non-symmetrically on the concave mirror. Compared with the case that femtosecond laser strikes at the center of the concave mirror, the intensity of the opti…
Using femtosecond laser pulses at 800 and 400 nm, we characterize the formation of underdense channels in air generated by laser filamentation at the millijoule energy level by means of transverse interferometry. We find that using tight focusing conditions, filamentation generates a shock wave and that the resulting low-density channel lasts for more than 90 ms. Comparison of these results with hydrodynamic simulations using an Eulerian hydrodynamic code gives an good agreement and allows us to estimate the initial gas peak temperature at $\sim$ 1000 K. The influence of experimental parameter…
According to a recent experiment, the instantaneous electronic Kerr effect in air exhibits a strong intensity dependence, the nonlinear refractive index switching sign and crossing over from a self-focusing to a de-focusing nonlinearity. A subsequent theoretical work has demonstrated that this has paradigm-changing consequences for the understanding of filamentation in air, so it is important to subject the idea of higher-order nonlinearities to stringent tests. Here we use numerical modeling to propose an experiment capable of discriminating between the standard and the new intensity-dependen…
An influence of pass-through optics on femtosecond laser pulse filamentation in ambient air is analyzed for the first time both experimentally and numerically. Propagation of high-power femtosecond laser pulse through solid optical elements introduces spatiotemporal phase modulation due to the Kerr effect. This modulation may have a strong ef-fect on the pulse filamentation in air. We demonstrated that the phase modulation obtained in the thin pass-through dielectric plate reduces the distance to the filament onset and increases the plasma channel length
High-power femtosecond laser radiation propagates nonlinearly in air exhibiting pulse self-focusing and strong multiphoton medium ionization, which leads to the spatial fragmentation of laser pulse into highly-localized light channels usually called the filaments. The filaments are characterized by high optical intensity, reduced (even zero) angular spreading and can contain laser plasma or be plasmaless (postfilaments). The presence of optical turbulence on the propagation path dramatically changes pulse filamentation dynamics and in some cases causes pulse fragmentation enhancement and colla…
In this paper, an inverse variational problem is solved for the nonlocal nonlinear Schrdinger equation used in modeling filamentation in various nonlinear media. The corresponding integral relations are found which generalize the conservation laws for the non-conservative case.
The introduction of mid-IR optical parametric chirped pulse amplifiers (OPCPAs) has catalyzed interest in multi-millijoule, infrared femtosecond pulse-based filamentation. As tunneling ionization is a fundamental first stage in these high-intensity laser-matter interactions, characterizing the process is critical to understand derivative topical studies on femtosecond filamentation and self-focusing. Here, we report constructive-elastic microwave scattering-based measurements of total electron count, electron number densities, and photoionization rates generated by 3.9 micron femtosecond mid-i…
This work compares computational methods for laser pulse propagation in hollow waveguides filled with rare gases at high pressures, with applications in extreme nonlinear optics in the mid-infrared wavelength region. As the wavelength of light λ=2π/k increases with respect to the transverse size R of a leaky waveguide, the loss of light out of the waveguide upon propagation, in general, increases. The now standard numerical approach for studying such structures is based on expansion of the propagating field into approximate leaky waveguide modes. We compare this approach to a new method that r…
Ionizing 800-nm femtosecond laser pulses propagating in silica glass and in potassium dihydrogen phosphate (KDP) crystal are investigated by means of a unidirectional pulse propagation code. Filamentation in fused silica is compared with the self-channeling of light in KDP accounting for the presence of defect states and electron-hole dynamics. In KDP, laser pulses produce intense filaments with higher clamping intensities up to 200 TW/cm$^2$ and longer plasma channels with electron densities above $10^{16}$ cm$^{-3}$. Despite these differences, the propagation dynamics in silica and KDP are a…
The processes of energy gain and redistribution in a dense gas subject to an intense ultrashort laser pulse are investigated theoretically for the case of high-pressure argon. The electrons released via strong-field ionization and driven by oscillating laser field collide with neutral neighbor atoms, thus effecting the energy gain in the emerging electron gas via a short-range inverse Bremsstrahlung interaction. These collisions also cause excitation and impact ionization of the atoms thus reducing the electron-gas energy. A kinetic model of these competing processes is developed which predict…
We experimentally demonstrate energy exchange between a delay-tuned femtosecond beam and two delay-fixed ones as they spatiotemporally overlapped and experienced filamentation in air. The energy exchange process in the relative time delay is dramatically elongated up to 40 ps in the presence of plasma grating, indicating that filamentary beams coupling may be an effective method for filament control.
We investigate beam pointing dynamics in filamentation in gases driven by high repetition rate femtosecond laser pulses. Upon suddenly exposing a gas to a kilohertz train of filamenting pulses, the filament is steered from its original direction to a new stable direction whose equilibrium is determined by a balance among buoyant, viscous, and diffusive processes in the gas. Results are shown for Xe and air, but are broadly applicable to all configurations employing high repetition rate femtosecond laser propagation in gases.
Laser filamentation in transparent material has a wide range of applications, from three dimensional manufacturing to biological technologies. Various experimental results showed that femtosecond laser pulse filamentation in fused silica strongly depends on laser focusing conditions. However, the physical mechanism governing each regime has not been fully understood. For the first time, single and multiple re-focusing of the laser pulse in interaction of femtosecond laser pulse with fused silica, and consequent single and multiple damage zones (filaments) have been observed in our extensive th…
We report on experimental realization of impulsive rotational Raman scattering from neutral nitrogen molecules in a femtosecond laser filament using an intense self-induced white-light seeding "air laser" generated during the filamentation of an 800 nm Ti: Sapphire laser in nitrogen gas. The impulsive rotational Raman fingerprint signals are observed with a maximum conversion efficiency of ~0.8%. Our observation provides a promising way of remote identification and location of chemical species in atmosphere by rotational Raman scattering of molecules.
We demonstrate numerically and experimentally the generation of powerful supercontinuum vortices from femtosecond vortex beams by using multiple thin fused silica plates. The supercontinuum vortices are shown to preserve the vortex phase profile of the initial beam for spectral components ranging from 500 nm to 1200 nm. The transfer of the vortex phase profile results from the inhibition of multiple filamentation and the preservation of vortex ring with relatively uniform intensity distribution by means of the thin-plate scheme, where the supercontinuum is mainly generated from the self-phase …
The propagation of intense picosecond laser pulses in air in the presence of strong nonlinear self-action effects and air ionization is investigated experimentally and numerically. The model used for numerical analysis is based on the nonlinear propagator for the optical field coupled with the rate equations for the production of various ionic species and plasma temperature. Our results show that the phenomenon of plasma-driven intensity clamping, which is paramount in femtosecond laser filamentation, holds for picosecond pulses. Furthermore, the temporal pulse distortions are limited and the …
We demonstrate theoretically that few-cycle vortex beam with subterawatt peak power can be generated by self-compression of mid-infrared femtosecond vortex beam using the thin-plate scheme. The 3 μm femtosecond vortex beam with input duration of 90 fs is compressed to 15.1 fs with the vortex characteristics preserved. The conversion efficiency is as high as 91.5% and the peak power reaches 0.18 TW. The generation of the high-peak-power few-cycle vortex beam is owing to the proper spatiotemporal match by this novel scheme, where the spectrum is broadened enough, the negative group velocity disp…
We experimentally studied intense femtosecond pulse filamentation and propagation in water for Gaussian, Laguerre-Gaussian, and Bessel-Gaussian incident beams. These different transverse modes for incident laser pulses were created from an initial Gaussian beam by using a computer generated hologram technique. We found that the length of the filament induced by the Bessel-Gaussian incident beam was longer than that for the other transverse modes under the conditions of the same peak intensity, pulse duration, and the size of the central part of the beam. To better understand the Bessel-Gaussia…
We report the first generation of quasi-steady-state air waveguides capable of guiding high average power laser beams. The guides are produced by high-repetition rate patterned filamentation of femtosecond laser pulses. We demonstrate near-continuous guiding of a CW probe beam with significantly higher efficiency than transient guides at lower repetition rates.
Broadband laser sources based on supercontinuum generation by femtosecond laser filamentation have enabled applications from stand-off sensing and spectroscopy to the generation and self-compression of high-energy few-cycle pulses. Filamentation relies on the dynamic balance between self-focusing and plasma defocusing, mediated by the Kerr nonlinearity and multiphoton ionization respectively. The filament properties, including the supercontinuum generation, are therefore highly sensitive to the properties of both the laser source and the propagation medium. Here, we report the anomalous spectr…
Since their discovery in the mid-1990s, ultrafast laser filaments in gases have been described as products of a dynamic balance between Kerr self-focusing and defocusing by free electric charges that are generated via multi-photon ionization on the beam axis. This established paradigm has been recently challenged by a suggestion that the Kerr effect saturates and even changes sign at high intensity of light, and that this sign reversal, not free-charge defocusing, is the dominant mechanism responsible for the extended propagation of laser filaments. We report qualitative tests of the new theor…
Filamentation of ultrashort laser pulses in the atmosphere offers unique opportunities for long-range transmission of high-power laser radiation and standoff detection. With the critical power of self-focusing scaling as the laser wavelength squared, the quest for longer-wavelength drivers, which would radically increase the peak power and, hence, the laser energy in a single filament, has been ongoing over two decades, during which time the available laser sources limited filamentation experiments in the atmosphere to the near-infrared and visible ranges. Here, we demonstrate filamentation of…
The absence of ionization and observation of white continuum in the initial moment of filamentation of powerful femtosecond laser pulses, propagating in silica glasses, as well as the filamentation without plasma channels observed in the experiments in air, forced us to look for other nonlinear mechanisms of description the above mentioned effects. For this reason we present in this paper new parametric conversion mechanism for asymmetric spectrum broadening of femtosecond laser pulses towards the higher frequencies in isotropic media. This mechanism includes cascade generation with THz spectr…
A dramatic spectral modulation of third-order harmonic (TH) emission generated in a near in- frared femtosecond (fs) pulse filamentation, assisted by a two-dimensional plasma grating formed by two pump femtosecond pulses, is experimentally demonstrated when their spatiotemporal overlap is achieved. It is mainly attributed to strong cross-phase modulation induced by the fundamental wave of the probe pulse and two pump ones. The delay dynamic of TH spectra indicates the influence of two retarded nonlinear responses on the TH generation. The dependences of TH generation on the energies of probe a…
Femtosecond Engineering of PolyMethylPentene(PMP) Nonlinearity via NA, Spin/orbital angular momentum (OAM), and In-Situ SC Diagnostics
Hong Kong Polytechnic University（香港理工大学）；Chongqing University of Arts and Sciences（重庆文理学院）；University of Liverpool（利物浦大学）；John Moores University（约翰摩尔斯大学）；TPM3D Direct Manufacturing Co., Ltd.（TPM3D直接制造有限公司）
We study the possibility of efficient self-compression of femtosecond laser pulses in nonlinear media with anomalous dispersion of group velocity during the self-focusing of wave packets with a power several times greater than the critical self-focusing power. The results of qualitative analysis of the evolution of three-dimensional wave packets with the quasi-soliton field distribution are confirmed by the computer simulation. The simulation proves that the considered regime of compression of high-power laser pulses with initial durations of about ten optical cycles is stable relative to fila…
Propagation of a tightly focused high-power ultrashort laser pulse in an optical medium is usually substantially influenced by the medium optical nonlinearity that can noticeably affect the laser pulse parameters around the nonlinear focus and lead to unavoidable and often undesirable spatial distortions of the focal waist. We present the results of our experimental study and numerical simulations on a femtosecond Ti-Sapphire laser pulse propagation in air under different spatial focusing. We concentrated our study on spectral-angular and spatial pulse transformations under different focusing …
We present space and time resolved measurements of the air hydrodynamics induced by ultrafast laser pulse excitation of the air gap between two electrodes at high potential difference. We explore both plasma-based and plasma-free gap excitation. The former uses the plasma left in the wake of femtosecond filamentation, while the latter exploits air heating by multiple-pulse resonant excitation of quantum molecular wavepackets. We find that the cumulative electrode-driven air density depression channel initiated by the laser plays the dominant role in the gap evolution leading to breakdown.
Femtosecond lasers interacting with Kerr nonlinear optical materials, propagate in form of filaments due to the balance of beam diffraction by self-focusing induced by the Kerr nonlinearity. Femtosecond laser filamentation is a universal phenomenon that belongs to a general class of processes proper to ultrashort lasers processing systems, associated with the competition between nonlinearity and dispersion also known to promote optical solitons. The present work considers a model describing femtosecond laser inscriptions in a transparent medium with Kerr nonlinearity. Upon inscription, the las…
The distant projection of high peak and average power laser beams in the atmosphere is a longstanding goal with a wide range of applications. Our early proof-of-principle experiments [Phys. Rev. X 4, 011027 (2014)] presented one solution to this problem, employing the energy deposition of femtosecond filaments in air to sculpt millisecond lifetime sub-meter length air waveguides. Here, we demonstrate air waveguiding at the 50 meter scale, 60X longer, making many practical applications now possible. We employ a new method for filament energy deposition: multi-filamentation of Laguerre-Gaussian …
Supercontinuum generation by femtosecond filaments in air is investigated for different laser wavelengths ranging from ultraviolet to infrared. Particular attention is paid on the role of third-harmonic generation and temporal steepening effects, which enlarge the blue part of the spectrum. A unidirectional pulse propagation model and nonlinear evolution equations are numerically integrated and their results are compared. Apart from the choice of the central wavelength, we emphasize the importance of the saturation intensity reached by self-guided pulses, together with their temporal duration …
Motivated by the ongoing controversy on the origin of the nonlinear index saturation and subsequent intensity clamping in femtosecond filaments, we study the atomic nonlinear polarization induced by a high-intensity and ultrashort laser pulse in hydrogen by numerically solving the time dependent Schrödinger equation. Special emphasis is given to the efficient modeling of the nonlinear polarization at central laser frequency corresponding to 800 nm wavelength. Here, the recently proposed model of the Higher-Order Kerr Effect (HOKE) and two versions of the Standard model for femtosecond filament…
Supercontinuum (SC) light source has advanced ultrafast laser spectroscopy in condensed matter science, biology, physics, and chemistry. Compared to the frequently used photonic crystal fibers and bulk materials, femtosecond laser filamentation in gases is damage-immune for supercontinuum generation. A bottleneck problem is the strong jitters from filament induced self-heating at kHz repetition rate level. We demonstrate stable kHz supercontinuum generation directly in air with multiple mJ level pulse energy. This is achieved by applying an external DC electric field to the air plasma filament…
Low-threshold efficient N${_2^+}$ lasing driven by sub-cycle soliton dynamics in a hollow waveguide
State Key Laboratory of Ultra-intense Laser Science and Technology, Shanghai Institute of Optics and Fine Mechanics (SIOM), Chinese Academy of Sciences (CAS)（中国科学院上海光学精密机械研究所超强度激光科学与技术国家重点实验室）；Russell Centre for Advanced Lightwave Science, Shanghai Institute of Optics and Fine Mechanics (SIOM) and Hangzhou Institute of Optics and Fine Mechanics (HIOM)（上海光学精密机械研究所与杭州光学精密机械研究所先进光波科学中心）；Zhejiang Key Laboratory of Microstructured Specialty Optical Fiber, Hangzhou Institute of Optics and Fine Mechanics (HIOM)（杭州光学精密机械研究所微结构特种光纤浙江省重点实验室）；School of Optoelectronic Engineering, Xidian University（西安电子科技大学光电工程学院）；School of Optical-Electrical and Computer Engineering, University of Shanghai for Science and Technology（上海理工大学光电信息与计算机工程学院）；Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences（中国科学院大学杭州高等研究院）；Zhangjiang Laboratory（张江实验室）
In the world of epsilon-near-zero (ENZ) materials, the plasma is unique for its natural ENZ properties at the plasma frequency (wp). However, for the air plasma during femtosecond laser filamentation with wp in terahertz (THz) band, which is also known as a broadband THz emitter, the possible ENZ effect has long been neglected. In this work, interactions between the laser plasma in air and the radiated THz waves were investigated, and the THz resonance absorption at the ENZ point, which gave rise to the generation of surface plasmon waves, has been theoretically and experimentally demonstrated…
