We demonstrate numerically and experimentally the generation of powerful supercontinuum vortices from femtosecond vortex beams by using multiple thin fused silica plates. The supercontinuum vortices are shown to preserve the vortex phase profile of the initial beam for spectral components ranging from 500 nm to 1200 nm. The transfer of the vortex phase profile results from the inhibition of multiple filamentation and the preservation of vortex ring with relatively uniform intensity distribution by means of the thin-plate scheme, where the supercontinuum is mainly generated from the self-phase modulation and self-steepening effects. Our scheme works for vortex beams with different topological charges, which provides a simple and effective method to generate supercontinuum vortices with high power.
We propose and optimize theoretically a supercontinuum (SC) laser source in the mid-IR based on using As-Se-Te/As-S core/clad step-index fibers and a femtosecond all-fiber laser system at 2 μm. Numerically simulated spectra extending from ~1 μm to more than 8 μm are demonstrated for pump energy of order 100 pJ in a fiber with a core diameter of 2 μm. To the best of our knowledge, the possibility of such long-wavelength spectral conversion of pump pulses at the wavelength of 2 μm in optical fibers is demonstrated for the first time. The theoretical calculations are performed on the base of real…
Nonlinear propagation of intense femtosecond laser pulses in bulk transparent media leads to a specific propagation regime, termed femtosecond filamentation, which in turn produces dramatic spectral broadening, or superbroadening, termed supercontinuum generation. Femtosecond supercontinuum generation in transparent solids represents a compact, efficient and alignment-insensitive technique for generation of coherent broadband radiation at various parts of the optical spectrum, which finds numerous applications in diverse fields of modern ultrafast science. During recent years, this research fi…
Supercontinuum (SC) generation via femtosecond (fs) pumping in all-normal-dispersion (ANDi) fiber is predicted to offer completely coherent broadening mechanisms, potentially allowing for substantially reduced noise levels in comparison to those obtained when operating in the anomalous dispersion regime. However, previous studies of SC noise typically treat only the quantum noise, typically in the form of one-photon-per-mode noise, and do not consider other technical noise contributions, such as the stability of the pump laser, which become important when the broadening mechanism itself is coh…
Frequency combs with mode spacing in the range of 10 to 20 gigahertz (GHz) are critical for increasingly important applications such as astronomical spectrograph calibration, high-speed dual-comb spectroscopy, and low-noise microwave generation. While electro-optic modulators and microresonators can provide narrowband comb sources at this repetition rate, a significant remaining challenge is a means to produce pulses with sufficient peak power to initiate nonlinear supercontinuum generation spanning hundreds of terahertz (THz) as required for self-referencing in these applications. Here, we pr…
We demonstrate a novel approach to producing coherent, directional supercontinuum via cascaded dispersive wave generation. By pumping in the normal group-velocity dispersion regime, pulse compression of the first dispersive wave results in the generation of a second dispersive wave, resulting in an octave-spanning supercontinuum generated primarily to one side of the pump spectrum. We theoretically investigate the dynamics and show that the generated spectrum is highly coherent. We experimentally confirm this dynamical behavior and the coherence properties in silicon nitride waveguides by perf…
Oscillator-driven broadband femtosecond transient microspectroscopy with supercontinuum probes generated in a photonic crystal fiber
Osaka Metropolitan University（大阪公立大学）；Institute for Molecular Science, National Institutes of Natural Sciences（国立自然科学研究所分子科学研究所）；Instituto de Ciencia de Materiales de Madrid (ICMM-CSIC)（马德里材料科学研究所）
Tunable supercontinuum in multimode fiber via bending-induced dispersion modification
Massachusetts Institute of Technology（麻省理工学院）；Research Laboratory of Electronics, Massachusetts Institute of Technology（麻省理工学院电子研究实验室）；Department of Biology, Massachusetts Institute of Technology（麻省理工学院生物学系）；Beth Israel Deaconess Medical Center, Harvard Medical School（哈佛医学院贝斯以色列女执事医疗中心）
Bright and broadband coherent mid-IR radiation is important for exciting and probing molecular vibrations. Using cascaded nonlinearities in conventional quadratic nonlinear crystal like lithium niobate, self-defocusing near-IR solitons have been demonstrated that led to very broadband supercontinuum generation in the visible, near-IR and short-wavelength mid-IR. Here we conduct an experiment where a mid-IR crystal pumped in the mid-IR gives multiple-octave spanning supercontinua. The crystal is cut for noncritical interaction, so the three-wave mixing of a single mid-IR femtosecond pump source…
We demonstrate theoretically that few-cycle vortex beam with subterawatt peak power can be generated by self-compression of mid-infrared femtosecond vortex beam using the thin-plate scheme. The 3 μm femtosecond vortex beam with input duration of 90 fs is compressed to 15.1 fs with the vortex characteristics preserved. The conversion efficiency is as high as 91.5% and the peak power reaches 0.18 TW. The generation of the high-peak-power few-cycle vortex beam is owing to the proper spatiotemporal match by this novel scheme, where the spectrum is broadened enough, the negative group velocity disp…
Fast fabrication of micro-optical elements for generation of optical vortex beams based on the q-plate design is demonstrated by femtosecond (fs) laser ablation of gold film on glass. Q-plates with diameter of ~0.5 mm were made in ~1 min using galvanometric scanners with writing speed of 5 mm/s. Period of gratings of 0.8 micrometers and groove width of 250 nm were achieved using fs-laser ablation at 343 nm wavelength. Phase and intensity analysis of optical vortex generators was carried out at 633 nm wavelength and confirmed the designed performance. Efficiency of spin-orbital conversion of th…
The propagation of high-power femtosecond laser pulses in air under conditions of superposed spatial phase modulation is considered theoretically. The numerical simulations are carried out on the basis of the reduced form of nonlinear Schrodinger equation (NLSE) for time-averaged electric field envelope. Initial spatial modulations are applied to pulse wavefront profiling by a staggered (TEM33) phase plate which is simulated numerically. The dynamics of laser pulse self-focusing, filamentation, and post-filamentation self-channeling after the phase plates with variable phase jumps is studied. …
The use of femtosecond lasers to introduce controlled stress states has recently been demonstrated in silica glass. We use this technique, in combination with chemical etching, to generate and control stress-induced birefringence over a well-defined region of interest, demonstrating direct-write wave plates with precisely tailored retardance levels. This tailoring enables the fabrication of laser-written polarization optics that can be tuned to any wavelength for which silica is transparent and with a clear aperture free of any laser modifications. Using this approach, we achieve sufficient re…
Laser pulses with a duration of one femtosecond or shorter can be generated both in the IR-VIS and in the extreme UV, but the deep UV is a spectral region where such extremely short pulses have not yet been demonstrated. Here, a method for the synthesis of ultrashort pulses in the deep UV is demonstrated, which utilizes the temporal and spatial harmonics that are generated by two noncollinear IR-VIS pulses in a thin MgF2 plate. By controlling the groove-envelope phase of the IR-VIS pulses, spatial harmonics are concatenated to form deep UV waveforms with a duration of 1.5 fs.
Femtosecond Engineering of PolyMethylPentene(PMP) Nonlinearity via NA, Spin/orbital angular momentum (OAM), and In-Situ SC Diagnostics
Hong Kong Polytechnic University（香港理工大学）；Chongqing University of Arts and Sciences（重庆文理学院）；University of Liverpool（利物浦大学）；John Moores University（约翰摩尔斯大学）；TPM3D Direct Manufacturing Co., Ltd.（TPM3D直接制造有限公司）
We report generation of a femtosecond supercontinuum extending from the ultraviolet to the near-infrared and detection of its carrier-envelope phase variation by f-to-2f interferometry. The spectrum is generated in a gas-filled hollow-core photonic crystal fiber where soliton dynamics allows CEP-stable self-compression of OPCPA pump pulses at 800 nm to a duration of 1.7 optical cycles, followed by dispersive wave emission. The source provides up to 1 μJ of pulse energy at 800 kHz repetition rate resulting in 0.8 W of average power, and can be extremely useful for example in strong-field physic…
Multiple filamentation in air of high-power ultrashort laser radiation with transverse intensity profile resembling a "corona" composed by incoherent combining of several annularly distributed independent top-hat sub-beams is theoretically studied. Through the numerical solution of time-averaged nonlinear Schrodinger equation, we study the spatio-angular dynamics of synthesized near-infrared "corona-beam" (CB) along the optical path by varying the number and power of the beamlets (corona-spikes). For the first time to our knowledge, the evident advances in the multiple filamentation region man…
We demonstrate the electromagnetic performance of waveguides for femtosecond electron beam bunch manipulation and compression with strong-field terahertz (THz) pulses. The compressor structure is a dispersion-free exponentially-tapered parallel-plate waveguide (PPWG) that can focus single-cycle THz pulses along one dimension. We show test results of the tapered PPWG structure using electro-optic sampling (EOS) at the interaction region with peak fields of at least 300 kV/cm given 0.9 uJ of incoming THz energy. We also present a modified shorted design of the tapered PPWG for better beam manipu…
Historically, infinity was long considered a vague concept - boundless, endless, larger than the largest - without any quantifiable mathematical foundation. This view changed in the 1800s through the pioneering work of Georg Cantor showing that infinite sets follow their own seemingly paradoxical mathematical rules. In 1924, David Hilbert highlighted the strangeness of infinity through a thought experiment now referred to as the Hilbert Hotel paradox, or simply Hilbert's Hotel. The paradox describes an "fully" occupied imaginary hotel having infinite number of single-occupancy rooms, the manag…
We put forward a co-axial pump(optical)-probe(X-rays) experimental concept and show performance of the optical component. A Bessel beam generator with a central 100 micrometers-diameter hole (on the optical axis) was fabricated using femtosecond (fs) laser structuring inside a silica plate. This flat-axicon optical element produces a needle-like axial intensity distribution which can be used for the optical pump pulse. The fs-X-ray free electron laser (X-FEL) beam of sub-1 micrometer diameter can be introduced through the central hole along the optical axis onto a target as a probe. Different …
We report on generation and control of tunable, broad orbital angular momentum (OAM) spectrum of a vortex beam. Using two spiral phase plates (SPPs), we have converted the Gaussian beam of Yb-fiber femtosecond laser at 1064 nm into optical vortices of orders, l=1-6, with conversion efficiency >95%. By adjusting the transverse shift of the SPPs with respect to the incident Gaussian beam axis, we have transformed the symmetric (intensity distribution) optical vortex of order, l, into an asymmetric vortex beam of broad OAM spectrum of orders, l, l-1, l-2,..,0. While the position of the SPPs deter…
