The onset of octupole deformation and its impact on related spectroscopic properties is studied in even-even neutron-rich lanthanide isotopes Xe, Ba, Ce, and Nd with neutron number $86\leqslant N\leqslant 94$. Microscopic input comes from the Hartree-Fock-Bogoliubov approximation with constrains on the axially symmetric quadrupole and octupole operators using the Gogny-D1M interaction. At the mean-field level, reflection asymmetric ground states are predicted for isotopes with neutron number around $N=88$. Spectroscopic properties are studied by diagonalizing the interacting boson model Hamiltonian, with the parameters obtained via the mapping of the mean-field potential energy surface onto the expectation value of the Hamiltonian in the $s$, $d$, and $f$ boson condensate state. The results obtained for low-energy positive- and negative-parity excitation spectra as well as the electric dipole, quadrupole, and octupole transition probabilities indicate the onset of pronounced octupolarity for $Z\approx 56$ and $N\approx 88$ nuclei.
Long-lived opposite-parity states and the onset of octupole collectivity in atomic nuclei
San Diego State University（圣地亚哥州立大学）；Ho Chi Minh City University of Education（胡志明市教育大学）；Institute for Basic Science（基础科学研究院）；Tel Aviv University（特拉维夫大学）
Enhanced octupole collectivity is expected in the neutron-deficient Ge, Se and Kr isotopes with neutron number $N \approx 40$ and has indeed been observed for $^{70,72}$Ge. Shape coexistence and configuration mixing are, however, a notorious challenge for theoretical models trying to reliably predict octupole collectivity in this mass region, which is known to feature rapid shape changes with changing nucleon number and spin of the system. To further investigate the microscopic configurations causing the prolate-oblate-triaxial shape transition at $A \approx 72$ and their influence on octupole…
Imprints of octupole collectivity in uranium-238 on relativistic heavy-ion flow observables
Key Laboratory of Nuclear Physics and Ion-beam Application (MOE), and Institute of Modern Physics, Fudan University（复旦大学现代物理研究所）；Shanghai Research Center for Theoretical Nuclear Physics, NSFC and Fudan University（复旦大学理论物理研究中心）；Department of Chemistry, Stony Brook University（石溪大学化学系）；Physics Department, Brookhaven National Laboratory（布鲁克海文国家实验室物理部）；Department of Physics and Astronomy, Wayne State University（韦恩州立大学物理与天文学系）；RIKEN BNL Research Center, Brookhaven National Laboratory（布鲁克海文国家实验室理研BNL研究中心）；Physics Department and Center for Particle Physics and Field Theory, Fudan University（复旦大学物理系及粒子物理与场论中心）
The evolution of quadrupole and octupole collectivity in neutron-deficient Xe, Ba, Ce, and Nd nuclei near the "octupole magic" neutron number $N=56$ is investigated within the mapped $sdf$-IBM framework. Microscopic input is obtained via quadrupole and octupole constrained Hartree-Fock-Bogoliubov calculations, based on the parametrization D1M of the Gogny energy density functional. Octupole-deformed mean-field ground states are predicted for Ba and Ce isotopes near $N=56$. Excitation energies of positive- and negative-parity states as well as electric transition rates are computed with wave fu…
We show that the collectivity of the particle-hole wave function of low-lying octupole 3^- states in doubly magic nuclei is mainly due to the neutron-proton interaction. Both the enhanced reduced transition probability to the ground state, B(E3;3-_1 -> 0+_1), and the coupling of the octupole excitation to a nucleon result from the coherent action of all the components of the collective state. The results obtained with a realistic shell-model interaction both for 208Pb and 209Pb agree with the geometric collective model of Bohr and Mottelson, where octupole excitations are associated with phono…
The lowest positive- and negative-parity bands of $^{20}$Ne and neutron-rich even-even Ne isotopes are investigated using a theoretical framework based on energy density functionals. Starting from a self-consistent relativistic Hartree-Bogoliubov calculation of axially-symmetric and reflection-asymmetric deformation energy surfaces, the collective symmetry-conserving states are built using projection techniques and the generator coordinate method. Overall a good agreement with the experimental excitation energies and transition rates is obtained. In particular, the model provides an accurate d…
We present a generator-coordinate calculation, based on a relativistic energy-density functional, of the low-lying spectra in the isotopes $^{150}$Nd and $^{150}$Sm and of the nuclear matrix element that governs the neutrinoless double-beta decay of the first isotope to the second. We carefully examine the impact of octupole correlations on both nuclear structure and the double-beta decay matrix element. Octupole correlations turn out to reduce quadrupole collectivity in both nuclei. Shape fluctuations, however, dilute the effects of octupole deformation on the double-beta decay matrix element…
The evolution of quadrupole and octupole collectivity and their coupling is investigated in a series of even-even isotopes of the actinide Ra, Th, U, Pu, Cm, and Cf with neutron number in the interval $130\leqslant N\leqslant 150$. The Hartree-Fock-Bogoliubov approximation, based on the parametrization D1M of the Gogny energy density functional, is employed to generate potential energy surfaces depending upon the axially-symmetric quadrupole and octupole shape degrees of freedom. The mean-field energy surface is then mapped onto the expectation value of the $sdf$ interacting-boson-model Hamilt…
Non-yrast, excited states in neutron-rich $^{186}$W were populated via inelastic-scattering reactions using beams of $^{136}$Xe nuclei accelerated to 725 and 800 MeV. Levels populated in the reactions were investigated via particle-$ γ$ coincidence techniques using the Gammasphere array of High-Purity Germanium detectors and the compact heavy-ion counter, CHICO2. The $ K^π = 2 ^{+} $ ($γ$), $ K^π = 0^{+}$ and $ K^π = 2^{-} $ (octupole) rotational side bands were extended to spins $ 14\hbar $, $ 12\hbar $, and $ 13\hbar $, respectively. A staggering pattern observed in the energies of levels in…
A systematic analysis of low-lying quadrupole and octupole collective states is presented, based on the microscopic energy density functional framework. By mapping the deformation constrained self-consistent axially symmetric mean-field energy surfaces onto the equivalent Hamiltonian of the $sdf$ interacting boson model (IBM), that is, onto the energy expectation value in the boson condensate state, the Hamiltonian parameters are determined. The study is based on the global relativistic energy density functional DD-PC1. The resulting IBM Hamiltonian is used to calculate excitation spectra and …
Continuum quasiparticle random-phase approximation for $(n,γ)$ reactions on neutron-rich nuclei: collectivity and resonances in low-energy cross section
There is sparse direct experimental evidence that atomic nuclei can exhibit stable pear shapes arising from strong octupole correlations. In order to investigate the nature of octupole collectivity in radium isotopes, electric octupole ($E3$) matrix elements have been determined for transitions in $^{222,228}$Ra nuclei using the method of sub-barrier, multi-step Coulomb excitation. Beams of the radioactive radium isotopes were provided by the HIE-ISOLDE facility at CERN. The observed pattern of $E$3 matrix elements for different nuclear transitions is explained by describing $^{222}$Ra as pear…
Quadrupole and octupole deformation energy surfaces, low-energy excitation spectra and transition rates in fourteen isotopic chains: Xe, Ba, Ce, Nd, Sm, Gd, Rn, Ra, Th, U, Pu, Cm, Cf, and Fm, are systematically analyzed using a theoretical framework based on a quadrupole-octupole collective Hamiltonian (QOCH), with parameters determined by constrained reflection-asymmetric and axially-symmetric relativistic mean-field calculations. The microscopic QOCH model based on the PC-PK1 energy density functional and $δ$-interaction pairing is shown to accurately describe the empirical trend of low-ener…
Mid-heavy nuclei offer unique opportunities to study the collective and single-particle aspects of nuclear structure. This mass regime is a dynamic area where protons and neutrons generally occupy different orbitals, giving rise to complex structures with a wide variety of shapes, shape evolution and shape coexistence. To that end, measurements of nuclear lifetimes and electromagnetic moments ($μ$,$Q$) can be invaluable. Recent experimental activities of the NuSTRAP group in Athens have focused on $γ$-spectroscopy studies employing the RoSPHERE array in Magurele, Romania. In recent studies [1,…
The phenomenon of reflection-asymmetric nuclear shapes is relevant to nuclear stability, nuclear spectroscopy, nuclear decays and fission, and the search for new physics beyond the standard model. Global surveys of ground-state octupole deformation, performed with a limited number of models, suggest that the number of pear-shaped isotopes is fairly limited across the nuclear landscape. We carry out global analysis of ground-state octupole deformations for particle-bound even-even nuclei with $Z \leq 110$ and $N \leq 210$ using nuclear density functional theory (DFT) with several non-relativist…
Low-frequency modes of excitation in deformed neutron-rich nuclei are studied by means of the quasiparticle random-phase approximation on the Skyrme-Hartree-Fock-Bogoliubov mean field. We investigate the microscopic structure of the soft $K^π=0^{+}$ modes systematically in neutron-rich Magnesium isotopes with $N=22, 24, 26$ and 28 close to the drip line, and it is found that the strong collectivity in $^{34}$Mg and $^{40}$Mg is acquired due to the coherent coupling between the $β$ vibration and the pairing vibration of neutrons. Microscopic structure of the $K^π=2^{+}$ modes changes gradually …
A characteristic feature of collective and particle-hole excitations in neutron-rich nuclei is that many of them couple to unbound neutron in continuum single-particle orbits. The continuum random phase approximation (cRPA) is a powerful many-body method that describes such excitations, and it provides a scheme to evaluate transition strengths from the ground state. In an attempt to apply cRPA to the radiative neutron capture reaction, we formulate in the present study an extended scheme of cRPA that describes gamma-transitions from the excited states under consideration, which decay to low-ly…
