Particle segregation is common in natural and industrial processes involving flowing granular materials. Complex, and seemingly contradictory, segregation phenomena have been observed for different boundary conditions and forcing. Using discrete element method simulations, we show that segregation of a single particle intruder can be described in a unified manner across different flow configurations. A scaling relation for the net segregation force is obtained by measuring forces on an intruder particle in controlled-velocity flows where gravity and flow kinematics are varied independently. The scaling law consists of two additive terms: a buoyancy-like gravity-induced pressure gradient term and a shear rate gradient term, both of which depend on the particle size ratio. The shear rate gradient term reflects a kinematics-driven mechanism whereby larger (smaller) intruders are pushed toward higher (lower) shear rate regions. The scaling is validated, without refitting, in wall-driven flows, inclined wall-driven flows, vertical silo flows, and free surface flows down inclines. Comparing the segregation force to the intruder weight results in predictions of the segregation direction that match experimental and computational results for various flow configurations.
We report on the scaling between the lift force and the velocity lag experienced by a single particle of different size in a monodisperse dense granular chute flow. The similarity of this scaling to the Saffman lift force in (micro) fluids, suggests an inertial origin for the lift force responsible for segregation of (isolated, large) intruders in dense granular flows. We also observe an anisotropic pressure/stress field surrounding the particle, which potentially lies at the origin of the velocity lag. These findings are relevant for modelling and theoretical predictions of particle-size segr…
Predicting segregation of granular materials composed of different-sized particles is a challenging problem. In this paper, we develop and implement a theoretical model that captures the interplay between advection, segregation, and diffusion in size bidisperse granular materials. The fluxes associated with these three driving factors depend on the underlying kinematics, whose characteristics play key roles in determining particle segregation configurations. Unlike previous models for segregation, our model uses parameters based on kinematic measures from discrete element method simulations in…
Discrete element method simulations of confined bidisperse granular shear flows elucidate the balance between diffusion and segregation that can lead to either mixed or segregated states, depending on confining pressure. Results indicate that the collisional diffusion is essentially independent of overburden pressure. Because the rate of segregation diminishes with overburden pressure, the tendency for particles to segregate weakens relative to the re-mixing of particles due to collisional diffusion as the overburden pressure increases. Using a continuum approach that includes a pressure depen…
Granular segregation is ubiquitous in industrial, geological or daily-life context, but there is still no unifying theoretical approach. In this review, we examine two examples of granular segregation -- shallow rapid flows and rotating drums -- which suggest that the dynamics of systems at intermediate and high density might be amenable to a statistical mechanics approach.
While convective flows are implicated in many granular segregation processes, the associated particle-scale rearrangements are not well understood. A three-dimensional bidisperse mixture segregates under steady shear, but the cyclically driven system either remains mixed or segregates slowly. Individual grain motion shows no signs of particle-scale segregation dynamics that precede bulk segregation. Instead, we find that the transition from non-segregating to segregating flow is accompanied by significantly less reversible particle trajectories, and the emergence of a convective flow field.
We study the granular segregation in a tapered rotating drum by means of simulations. In this geometry, both radial and axial segregation appear, the strength of which depends on the filling fraction. We study the effect of the drum's tapering angle on the segregation speed and show that, coherently with several recent studies, the axial segregation is due to the combined effect of the radial segregation and the shape of the drum. We show that the axial segregation behaves in a way analogous to the one found in chute flows, and corresponds to previous theories for shallow gravity driven surfac…
We present an X-ray tomography study of the segregation mechanisms of tracer particles in a three-dimensional cyclically sheared bi-disperse granular medium. Big tracers are dragged by convection to rise to the top surface and then remain trapped there due to the small downward convection cross-section, which leads to segregation. Additionally, we also find that the local structural up-down asymmetry due to arching effect around big tracers will induce the tracers to have a net upward displacement against its smaller neighbors, which is another mechanism for segregation.
Continuum modeling of size-segregation and flow in dense, bidisperse granular media: Accounting for segregation driven by both pressure gradients and shear-strain-rate gradients
Granular materials segregate by size under shear, and the ability to quantitatively predict the time required to achieve complete segregation is a key test of our understanding of the segregation process. In this paper, we apply the Gray-Thornton model of segregation (developed for linear shear profiles) to a granular flow with an exponential profile, and evaluate its ability to describe the observed segregation dynamics. Our experiment is conducted in an annular Couette cell with a moving lower boundary. The granular material is initially prepared in an unstable configuration with a layer of …
A two-dimensional, transient, multi-scale modeling approach is presented for predicting the magnitude and rate of percolation segregation for binary mixtures of granular material in a rotating drum and conical hopper. The model utilizes finite element method simulations to determine the bulk-level granular velocity field, which is then combined with particle-level diffusion and segregation correlations using the advection-diffusion-segregation equation. The utility of this modelling approach is demonstrated by predicting segregation patterns in a rotating drum and during the discharge of conic…
The size-segregation of granular materials, a process colloquially known as the Brazil Nut Effect, has generally been thought to proceed faster the greater the size difference of the particles. We experimentally investigate sheared bidisperse granular materials as a function of the size ratio of the two species, and find that the mixing rate at low confining pressure behaves as expected from percolation-based arguments. However, we also observe an anomalous effect for the re-segregation rates, wherein particles of both dissimilar and similar sizes segregate more slowly than intermediate partic…
Gravity-driven size segregation is important in mountain streams where a wide range of grain sizes are transported as bedload. More particularly, vertical size segregation is a multi-scale process that originates in interactions at the scale of particles with important morphological consequences on the reach scale. To address this issue, a volume-averaged multi-phase flow model for immersed bidisperse granular flows was developed based on an interparticle segregation force (Guillard et al. 2016) and a granular Stokesian drag force (Tripathi and Khakhar 2013). An advection-diffusion model was d…
Flowing granular materials segregate due to differences in particle size (driven by percolation) and density (driven by buoyancy). Modelling the segregation of mixtures of large/heavy particles and small/light particles is challenging due to the opposing effects of the two segregation mechanisms. Using discrete element method (DEM) simulations of combined size and density segregation we show that the segregation velocity is well described by a model that depends linearly on the local shear rate and quadratically on the species concentration. Concentration profiles predicted by incorporating th…
Granular segregation is an important mechanism for industrial processes aiming at mixing grains. Additionally, it plays a pivotal role in determining the kinematics of geophysical flows. Because of segregation, the grainsize distribution varies in space and time. Additional complications arise from the presence of comminution, where new particles are created, enhancing segregation. This has a feedback on the comminution process, as particles change their local neighbourhood. Simultaneously, particles are generally undergoing remixing, further complicating the segregation and comminution proces…
We present a continuum approach to model segregation of size-bidisperse granular materials in unsteady bounded heap flow as a prototype for modeling segregation in other time varying flows. In experiments, a periodically modulated feed rate produces stratified segregation like that which occurs due to intermittent avalanching, except with greater layer-uniformity and higher average feed rates. Using an advection-diffusion-segregation equation and characterizing transient changes in deposition and erosion after a feed rate change, we model stratification for varying feed rates and periods. Feed…
While granular segregation in partially filled containers has been studied extensively, granular dynamics in densely filled spheres is not fully understood. Here, surface band segregation and granular convection are reported in a rotating sphere of highly compacted glass beads. Distinct from Rayleigh-Benard convection, granular convection has a butterfly-shaped structure with vortexes of alternating layers of small/large beads, which is stable and independent of the sphere size. Two concentric interfaces at the zero tangential/norm flux are discovered, which divide the sphere into three layers…
In bidisperse particle mixtures varying in size or density alone, large particles rise (driven by percolation) and heavy particles sink (driven by buoyancy). When the two particle species differ from each other in both size and density, the two segregation mechanisms either enhance (large/light and small/heavy) or oppose (large/heavy and small/light) each other. In the latter case, an equilibrium condition exists in which the two segregation mechanisms balance and the particles no longer segregate. This leads to a methodology to design non-segregating particle mixtures by specifying particle s…
Individual constituent balance equations are often used to derive expressions for species-specific segregation velocities in flows of dense granular mixtures. We propose a semiempirical expression for the interspecies momentum exchange in density-bidisperse granular flows as an extension of ideas from kinetic theory and compare it to a previous viscous drag approach that is analogous to particles settling in a fluid. The proposed model expands the range of the granular kinetic theory from short-duration binary collisions to the multiple enduring contacts characteristic of dense shear flows and…
Segregation patterns of size-bidisperse particle mixtures in a fully-three-dimensional flow produced by alternately rotating a spherical tumbler about two perpendicular axes are studied over a range of particle sizes and volume ratios using both experiments and a continuum model. Pattern formation results from the interaction of size segregation with chaotic regions and non-mixing islands of the flow. Specifically, large particles in the flowing surface layer are preferentially deposited in non-mixing islands despite the effects of collisional diffusion and chaotic transport. The protocol-depe…
In this paper, granular segregation in a two-compartment cell in zero gravity is studied numerically by DEM simulation. In the simulation using a virtual window method we find a non-monotonic flux, a function which governs the segregation. A parameter is used to quantify the segregation. The effect of three parameters: the total number of particles N, the excitation strength Γ, and the position of the window coupling the two compartments, on the segregation ε and the waiting time τ are investigated. It is found that the segregation observed in zero gravity exists and does not depend on the exc…
Using simulations and a virtual-spring-based approach, we measure the segregation force, Fseg, over a range of size-bidisperse mixture concentrations, particle size ratios, and shear rates to develop a model for Fseg that extends its applicability from the well-studied non-interacting intruders regime to finite-concentration mixtures where cooperative phenomena occur. The model predicts the concentration below which the single intruder assumption applies and provides an accurate description of the pressure partitioning between species.
Gravel-river beds typically have an "armored" layer of coarse grains on the surface, which acts to protect finer particles underneath from erosion. River bed-load transport is a kind of dense granular flow, and such flows are known to vertically segregate grains. The contribution of granular physics to river-bed armoring, however, has not been investigated. Here we examine these connections in a laboratory river with bimodal sediment size, by tracking the motion of particles from the surface to deep inside the bed, and find that armor develops by two distinct mechanisms. Bed-load transport in …
We investigate axial segregation of binary mixtures in a laterally shaken horizontal channel formed by ratchet-like sidewalls that appear as concatenated trapeziums when not offset axially. Grain mixtures shaken in such a channel are observed to segregate in two stages: they first separate rapidly into two vertically arranged layers and, then, these layers move axially in opposite directions, segregating the two species. Here, we conduct experiments to study the influence on the segregation process of various parameters: the size ratio of grains, the shaking frequency and the channel's geometr…
When granular mixtures of different sizes are fluidized, each species spontaneously separates and condenses to form patterns. Although granular segregation has been extensively studied, the inability to directly observe the time evolution of the internal structure hinders the understanding of the mechanism of segregation dynamics driven by surface flow. In this study, we report rich band dynamics, including a self-replicating band, in a horizontally shaken granular mixture in a quasi-two-dimensional container where the granules formed steady surface waves. Direct observation of surface flow an…
Segregation induced by a thermal gradient of an impurity in a driven low-density granular gas is studied. The system is enclosed between two parallel walls from which we input thermal energy to the gas. We study here steady states occurring when the inelastic cooling is exactly balanced by some external energy input (stochastic force or viscous heating), resulting in a uniform heat flux. A segregation criterion based on Navier-Stokes granular hydrodynamics is written in terms of the tracer diffusion transport coefficients, whose dependence on the parameters of the system (masses, sizes and coe…
It has been recently reported that a granular mixture in which grains differ in their restitution coefficients presents segregation: the more inelastic particles sink to the bottom. When other segregation mechanisms as buoyancy and the Brazil nut effect are present, the inelasticity induced segregation can compete with them. First, a detailed analysis, based on numerical simulations of two dimensional systems, of the competition between buoyancy and the inelasticity induced segregation is presented, finding that there is a transition line in the parameter space that determines which mechanism …
