Flowing granular materials segregate due to differences in particle size (driven by percolation) and density (driven by buoyancy). Modelling the segregation of mixtures of large/heavy particles and small/light particles is challenging due to the opposing effects of the two segregation mechanisms. Using discrete element method (DEM) simulations of combined size and density segregation we show that the segregation velocity is well described by a model that depends linearly on the local shear rate and quadratically on the species concentration. Concentration profiles predicted by incorporating this segregation velocity model into a continuum advection-diffusion-segregation transport model match DEM simulation results well for a wide range of particle size and density ratios. Most surprisingly, the DEM simulations and the segregation velocity model both show that the segregation direction for a range of size and density ratios depends on the local species concentration. This leads to a methodology to determine the combination of particle size ratio, density ratio, and particle concentration for which a bidisperse mixture will not segregate.
Individual constituent balance equations are often used to derive expressions for species-specific segregation velocities in flows of dense granular mixtures. We propose a semiempirical expression for the interspecies momentum exchange in density-bidisperse granular flows as an extension of ideas from kinetic theory and compare it to a previous viscous drag approach that is analogous to particles settling in a fluid. The proposed model expands the range of the granular kinetic theory from short-duration binary collisions to the multiple enduring contacts characteristic of dense shear flows and…
Reverse segregation and self-organization in inclined chute flows of bidisperse granular mixtures
Sandia National Laboratories（桑迪亚国家实验室）；Center for Computational Sciences and Engineering, Lawrence Berkeley National Laboratory（劳伦斯伯克利国家实验室计算科学与工程中心）；School of Math, Science, and Engineering, Central New Mexico Community College（新墨西哥中部社区学院数理工程学院）
Continuum modeling of size-segregation and flow in dense, bidisperse granular media: Accounting for segregation driven by both pressure gradients and shear-strain-rate gradients
Up to date, inertial migration of particles in microflows has demonstrated a great potential for a wide range of applications. In particular, this phenomenon is used to achieve particle separation or sorting in a suspension. Recent works reported that the focusing mode of particles can be modified in a polydisperse suspension. Nevertheless, the impact of the particle sizes in a mixture on their inertial migration has been rarely studied up to now. Thus, we have investigated in this work the influence of bidispersity on the lateral migration of the particles towards equilibrium positions and on…
While convective flows are implicated in many granular segregation processes, the associated particle-scale rearrangements are not well understood. A three-dimensional bidisperse mixture segregates under steady shear, but the cyclically driven system either remains mixed or segregates slowly. Individual grain motion shows no signs of particle-scale segregation dynamics that precede bulk segregation. Instead, we find that the transition from non-segregating to segregating flow is accompanied by significantly less reversible particle trajectories, and the emergence of a convective flow field.
Liquid foam flows in a Hele-Shaw cell were investigated. The plug flow obtained for a monodisperse foam is strongly perturbed in the presence of bubbles whose size is larger than the average bubble size by an order of magnitude at least. The large bubbles migrate faster than the mean flow above a velocity threshold which depends on its size. We evidence experimentally this new instability and, in case of a single large bubble, we compare the large bubble velocity with the prediction deduced from scaling arguments. In case of a bidisperse foam, an attractive interaction between large bubbles in…
We experimentally study particle scale dynamics during segregation of a bidisperse mixture under oscillatory shear. Large and small particles show an underlying asymmetry that is dependent on the local particle concentration, with small particles segregating faster in regions of many large particles and large particles segregating slower in regions of many small particles. We quantify the asymmetry on bulk and particle scales, and capture it theoretically. This gives new physical insight into segregation and reveals a similarity with sedimentation, traffic flow and particle diffusion.
Discrete element method simulations of confined bidisperse granular shear flows elucidate the balance between diffusion and segregation that can lead to either mixed or segregated states, depending on confining pressure. Results indicate that the collisional diffusion is essentially independent of overburden pressure. Because the rate of segregation diminishes with overburden pressure, the tendency for particles to segregate weakens relative to the re-mixing of particles due to collisional diffusion as the overburden pressure increases. Using a continuum approach that includes a pressure depen…
Using simulations and a virtual-spring-based approach, we measure the segregation force, Fseg, over a range of size-bidisperse mixture concentrations, particle size ratios, and shear rates to develop a model for Fseg that extends its applicability from the well-studied non-interacting intruders regime to finite-concentration mixtures where cooperative phenomena occur. The model predicts the concentration below which the single intruder assumption applies and provides an accurate description of the pressure partitioning between species.
The size-segregation of granular materials, a process colloquially known as the Brazil Nut Effect, has generally been thought to proceed faster the greater the size difference of the particles. We experimentally investigate sheared bidisperse granular materials as a function of the size ratio of the two species, and find that the mixing rate at low confining pressure behaves as expected from percolation-based arguments. However, we also observe an anomalous effect for the re-segregation rates, wherein particles of both dissimilar and similar sizes segregate more slowly than intermediate partic…
Using Brownian dynamics simulations we perform a systematic investigation of the shear-induced migration of colloidal particles subject to Poiseuille flow in both cylindrical and planar geometry. We find that adding an attractive component to the interparticle interaction enhances the migration effect, consistent with recent simulation studies of platelet suspensions. Monodisperse, bidisperse and polydisperse systems are studied over a range of shear rates, considering both steady states and the transient dynamics arising from the onset of flow. For bidisperse and polydisperse systems size seg…
We present a continuum approach to model segregation of size-bidisperse granular materials in unsteady bounded heap flow as a prototype for modeling segregation in other time varying flows. In experiments, a periodically modulated feed rate produces stratified segregation like that which occurs due to intermittent avalanching, except with greater layer-uniformity and higher average feed rates. Using an advection-diffusion-segregation equation and characterizing transient changes in deposition and erosion after a feed rate change, we model stratification for varying feed rates and periods. Feed…
Spatial segregation in the wall normal direction is investigated in suspensions containing a binary mixture of Neo-Hookean capsules subjected to pressure driven flow in a planar slit. The two components of the binary mixture have unequal membrane rigidities. The problem is studied numerically using an accelerated implementation of the boundary integral method. The effect of a variety of parameters was investigated, including the capillary number, rigidity ratio between the two species, volume fraction, confinement ratio, and the number fraction of the more floppy particle $X_f$ in the mixture.…
We present a method to estimate the segregation parameter, $S,$ a key input in a continuum transport model of particulate flows. $S$ is determined by minimizing the difference between measured and model-predicted concentration profiles. To validate the approach, we conduct discrete element method simulations of size-bidisperse mixtures in quasi-2D bounded heap flow; the resulting data show that $S$ calculated from concentration profiles is consistent with the directly measured value. The method's accuracy depends critically on the velocity profile during filling, but only weakly on the diffusi…
We use experiments and molecular dynamics simulations of vertically oscillated granular layers to study horizontal particle segregation induced by a kink (a boundary between domains oscillating out of phase). Counter-rotating convection rolls carry the larger particles in a bidisperse layer along the granular surface to a kink, where they become trapped. The convection originates from avalanches that occur inside the layer, along the interface between solidified and fluidized grains. The position of a kink can be controlled by modulation of the container frequency, making possible systematic h…
Using numerical simulations, we examine the dynamics of driven two-dimensional bidisperse disks flowing over quenched disorder. The system exhibits a series of distinct dynamical phases as a function of applied driving force and packing fraction including a phase separated state as well as a smectic state with liquid like or polycrystalline features. At low driving forces, we find a clogged phase with an isotropic density distribution, while at intermediate driving forces the disks separate into bands of high and low density with either liquid like or polycrystalline structure in the high dens…
We study the effect of fluids on the angle of repose and the segregation of granular matter poured into a silo. The experiments are conducted in two regimes where: (i) the volume fraction of the fluid is small and it forms liquid bridges between particles, and (ii) the particles are completely immersed in the fluid. The data is obtained by imaging the pile formed inside a quasi-two dimensional silo through the transparent glass side walls. In the first series of experiments, the angle of repose is observed to increase sharply with the volume fraction of the fluid and then saturates at a value …
We study a variable-coefficient Burgers equation arising in the modelling of segregation of dry bidisperse granular mixtures. The equation is subject to nonlinear boundary conditions for the particle flux. We construct a strongly implicit Crank--Nicolson type of numerical scheme for the latter equation. The scheme is benchmarked against a standard exact solution of kink type, showing second-order of accuracy and good discrete conservation properties. Two segregation problems considered in the literature are then solved and discussed. The first is the case of a linear kinetic stress profile, wh…
Size bidisperse granular materials in a spherical tumbler segregate into two different patterns of three bands with either small particles at the equator and large particles at the poles or vice versa, depending upon the fill level in the tumbler. Here we use discrete element method (DEM) simulations with supporting qualitative experiments to explore the effect of the tumbler wall roughness on the segregation pattern, modeling the tumbler walls as either a closely packed monolayer of fixed particles resulting in a rough wall, or as a geometrically smooth wall. Even though the tumbler wall is i…
Predicting segregation of granular materials composed of different-sized particles is a challenging problem. In this paper, we develop and implement a theoretical model that captures the interplay between advection, segregation, and diffusion in size bidisperse granular materials. The fluxes associated with these three driving factors depend on the underlying kinematics, whose characteristics play key roles in determining particle segregation configurations. Unlike previous models for segregation, our model uses parameters based on kinematic measures from discrete element method simulations in…
Segregation patterns of size-bidisperse particle mixtures in a fully-three-dimensional flow produced by alternately rotating a spherical tumbler about two perpendicular axes are studied over a range of particle sizes and volume ratios using both experiments and a continuum model. Pattern formation results from the interaction of size segregation with chaotic regions and non-mixing islands of the flow. Specifically, large particles in the flowing surface layer are preferentially deposited in non-mixing islands despite the effects of collisional diffusion and chaotic transport. The protocol-depe…
In bidisperse particle mixtures varying in size or density alone, large particles rise (driven by percolation) and heavy particles sink (driven by buoyancy). When the two particle species differ from each other in both size and density, the two segregation mechanisms either enhance (large/light and small/heavy) or oppose (large/heavy and small/light) each other. In the latter case, an equilibrium condition exists in which the two segregation mechanisms balance and the particles no longer segregate. This leads to a methodology to design non-segregating particle mixtures by specifying particle s…
It is well-known that granular mixtures that differ in size or shape segregate when sheared. In the past, two mechanisms have been proposed to describe this effect, and it is unclear if both exist. To settle this question, we consider a bidisperse mixture of spheroids of equal volume in a rotating drum, where the two mechanisms are predicted to act in opposite directions. We present the first evidence that there are two \emph{distinct} segregation mechanisms driven by relative \emph{over-stress}. Additionally, we showed that for non-spherical particles, these two mechanisms can act in differen…
Segregation and mixing of granular mixtures during heap formation have important consequences in industry and agriculture. This research investigates three different final particle configurations of bi-disperse granular mixtures -- stratified, segregated and mixed -- during filling of quasi-two dimensional silos. We consider a larger number and relatively wider range of control parameters than previous studies, including particle size ratio, flow rate, system size and heap rise velocity. The boundary between stratified and unstratified states is primarily controlled by the two-dimensional flow…
We simulate a model of self-propelled disks with soft repulsive interactions confined to a box in two dimensions. For small rotational diffusion rates, monodisperse disks spontaneously accumulate at the walls. At low densities, interaction forces between particles are strongly inhomogeneous, and a simple model predicts how these inhomogeneities alter the equation of state. At higher densities, collective effects become important. We observe signatures of a jamming transition at a packing fraction $ϕ\sim 0.88$, which is also the jamming point for non-active athermal monodisperse disks. At this …
Gravity-driven size segregation is important in mountain streams where a wide range of grain sizes are transported as bedload. More particularly, vertical size segregation is a multi-scale process that originates in interactions at the scale of particles with important morphological consequences on the reach scale. To address this issue, a volume-averaged multi-phase flow model for immersed bidisperse granular flows was developed based on an interparticle segregation force (Guillard et al. 2016) and a granular Stokesian drag force (Tripathi and Khakhar 2013). An advection-diffusion model was d…
We numerically examine clogging transitions for bidisperse disks flowing through a two dimensional periodic obstacle array. We show that clogging is a probabilistic event that occurs through a transition from a homogeneous flowing state to a heterogeneous or phase separated jammed state where the disks form dense connected clusters. The probability for clogging to occur during a fixed time increases with increasing particle packing and obstacle number. For driving at different angles with respect to the symmetry direction of the obstacle array, we show that certain directions have a higher clo…
Granular materials will segregate by particle size when subjected to shear, as occurs, for example, in avalanches. The evolution of a bidisperse mixture of particles can be modeled by a nonlinear first order partial differential equation, provided the shear (or velocity) is a known function of position. While avalanche-driven shear is approximately uniform in depth, boundary-driven shear typically creates a shear band with a nonlinear velocity profile. In this paper, we measure a velocity profile from experimental data and solve initial value problems that mimic the segregation observed in the…
Particle segregation is common in natural and industrial processes involving flowing granular materials. Complex, and seemingly contradictory, segregation phenomena have been observed for different boundary conditions and forcing. Using discrete element method simulations, we show that segregation of a single particle intruder can be described in a unified manner across different flow configurations. A scaling relation for the net segregation force is obtained by measuring forces on an intruder particle in controlled-velocity flows where gravity and flow kinematics are varied independently. Th…
In dense flowing bidisperse particle mixtures varying in size or density alone, smaller particles sink (driven by percolation) and lighter particles rise (driven by buoyancy). But when the particle species differ from each other in both size and density, percolation and buoyancy can either enhance (large/light and small/heavy) or oppose (large/heavy and small/light) each other. In the latter case, a local equilibrium condition can exist in which the two segregation mechanisms balance and particles remain mixed: this allows the design of minimally-segregating mixtures by specifying particle siz…
We present an experimental study of segregation of granular matter in a quasi-two dimensional silo emptying out of an orifice. Size separation is observed when multi-sized particles are used with the larger particles found in the center of the silo in the region of fastest flow. We use imaging to study the flow inside the silo and quantitatively measure the concentration profiles of bi-disperse beads as a function of position and time. The angle of the surface is given by the angle of repose of the particles, and the flow occurs in a few layers only near the top of this inclined surface. The f…
Dry granular material flowing on rough inclines can experience a self-induced Rayleigh-Taylor (RT) instability followed by the spontaneous emergence of convection cells. For this to happen, particles are different in size and density, the larger particles are the denser but still segregate toward the surface. When the flow is, as usual, initially made of two layers, dense particles above, a Rayleigh-Taylor instability develops during the flow. When the flow is initially made of one homogeneous layer mixture, the granular segregation leads to the formation of an unstable layer of large-dense pa…
Granular fronts are a common yet unexplained phenomenon emerging during the gravity driven free-surface flow of concentrated suspensions. They are usually believed to be the result of fluid convection in combination with particle size segregation. However, suspensions composed of uniformly sized particles also develop a granular front. Within a large rotating drum, a stationary recirculating avalanche is generated. The flowing material is a mixture of a visco-plastic fluid obtained from a kaolin-water dispersion, with spherical ceramic particles denser than the fluid. The goal is to mimic the …
Binary mixtures of dry grains avalanching down a slope are experimentally studied in order to determine the interaction among coarse and fine grains and their effect on the deposit morphology. The distance travelled by the massive front of the avalanche over the horizontal plane of deposition area is measured as a function of mass content of fine particles in the mixture, grain-size ratio, and flume tilt. A sudden transition of the runout is detected at a critical content of fine particles, with a dependence on the grain-size ratio and flume tilt. This transition is explained as two simultaneo…
