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arXiv 2103.07912cond-mat.str-el
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非磁性可果美金属KV $_3$ Sb $_5$中电荷密度波不稳定性的光学探测

Optical detection of charge-density-wave instability in the non-magnetic kagome metal KV$_3$Sb$_5$

E. Uykur, B. R. Ortiz, S. D. Wilson, M. Dressel, A. A. Tsirlin

摘要:

密度波和超导态的共存以及在没有局部磁性的情况下的大的反常霍尔效应仍然是AV $_3$ Sb $_5$可果美金属(A = K,Rb,Cs)的有趣和神秘的特征。在这里,我们表明,通过光学光谱和密度泛函计算,KV $_3$ Sb $_5$的低能量动力学的特点是非常规的本地化载流子,这是强烈的重整化的密度波过渡和电子相关性的指示。强烈的声子异常不仅在密度波跃迁下是突出的,而且在高温下也是突出的,这表明声子与底层电子结构之间存在复杂的相互作用。我们进一步提出了KV $_3$ Sb $_5$中密度波序的大卫星和三角形构型。这些配置是强烈地让人想起$p$波状态预期的哈伯德模型的kagome晶格在填充水平的范霍夫奇点。接近这一制度应该有有趣的和深远的影响KV $_3$锑$_5$和相关材料的物理。

英文摘要:

Coexisting density-wave and superconducting states along with the large anomalous Hall effect in the absence of local magnetism remain intriguing and enigmatic features of the AV$_3$Sb$_5$ kagome metals (A = K, Rb, Cs). Here, we demonstrate via optical spectroscopy and density-functional calculations that low-energy dynamics of KV$_3$Sb$_5$ is characterized by unconventional localized carriers, which are strongly renormalized across the density-wave transition and indicative of electronic correlations. Strong phonon anomalies are prominent not only below the density-wave transition, but also at high temperatures, suggesting an intricate interplay of phonons with the underlying electronic structure. We further propose the star-of-David and tri-hexagon (inverse star-of-David) configurations for the density-wave order in KV$_3$Sb$_5$. These configurations are strongly reminiscent of $p$-wave states expected in the Hubbard model on the kagome lattice at the filling level of the van Hove singularity. The proximity to this regime should have intriguing and far-reaching implications for the physics of KV$_3$Sb$_5$ and related materials.

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