We use magneto-conductivity to study the magnetic proximity effect on surface states of doped topological insulators. Our bilayers consist of a layer of Fe$_7$Se$_8$, which is a metallic ferrimagnet and a layer of Bi$_{0.8}$Sb$_{1.2}$Te$_{3}$ which is a highly hole-doped topological insulator. Using transport measurements and a modified Hikami-Larkin-Nagaoka model, we show that the ferromagnet shortens significantly the effective coherence length of the surface states, suggesting that a gap is opened at the Dirac point. We show that the magnetically induced gap persists on surface states which are separated from the magnet by a topological insulator layer as thick as 170 [nm]. Furthermore, the size of the gap is found to be proportional to the magnetization that we extract from the anomalous Hall effect.
Our results give information on the ties between carrier density, induced magnetization and magnetically induced gap in topological insulator/ferromagnet bilayers. This information is important both for a theoretical understanding of magnetic interactions in topological insulators and for the practical fabrication of such bilayers, which are the basis of various suggested technologies, such as spintronic devices, far infra-red detectors etc.
Current-induced spin-orbit torques in Co$_2$FeAl/Pt ultrathin bilayers are studied using a magnetoresistive harmonic response technique, which distinguishes the dampinglike and fieldlike contributions. The presence of a temperature-dependent magnetic proximity effect is observed through the anomalous Hall and anisotropic magnetoresistances, which are enhanced at low temperatures for thin platinum thicknesses. The fieldlike torque efficiency decreases steadily as the temperature is lowered for all Pt thicknesses studied, which we propose is related to the influence of the magnetic proximity eff…
Room-temperature spin-lifetime anisotropy exceeding 60 in bilayer graphene spin valves proximity coupled to WSe$_2$
nd Institute of Physics and JARA-FIT, RWTH Aachen University（亚琛工业大学第二物理研究所和JARA-FIT）；Peter Grünberg Institute (PGI-9), Forschungszentrum Jülich（于利希研究中心彼得·格林贝格研究所（PGI-9））
Prediction of new superconducting bilayers heterostructures using quantum confinement and proximity effects
Politecnico di Torino（都灵理工大学）；National Research Nuclear University MEPhI (Moscow Engineering Physics Institute)（国立核研究大学莫斯科工程物理学院）；University of Milan（米兰大学）；University of Göttingen（哥廷根大学）
We identify and investigate thermal spin transport phenomena in sputter-deposited Pt/NiFe$_2$O$_{\textrm{4-x}}$ ($4\geq x \geq 0$) bilayers. We separate the voltage generated by the spin Seebeck effect from the anomalous Nernst effect contributions and even disentangle the intrinsic anomalous Nernst effect (ANE) in the ferromagnet (FM) from the ANE produced by the Pt that is spin polarized due to its proximity to the FM. Further, we probe the dependence of these effects on the electrical conductivity and the band gap energy of the FM film varying from nearly insulating NiFe$_2$O$_4$ to metalli…
Proximity orbital and spin-orbit effects of bilayer graphene on monolayer WSe$_2$ are investigated from first-principles. We find that the built-in electric field induces an orbital band gap of about 10 meV in bilayer graphene. Remarkably, the proximity spin-orbit splitting for holes is two orders of magnitude---the spin-orbit splitting of the valence band at K is about 2 meV---more than for electrons. Effectively, holes experience spin-valley locking due to the strong proximity of the lower graphene layer to WSe$_2$. However, applying an external transverse electric field of some 1 V/nm, coun…
Weak localization as probe of spin-orbit-induced spin-split bands in bilayer graphene proximity coupled to WSe$_2$
RWTH Aachen University（亚琛工业大学）；Forschungszentrum Jülich（于利希研究中心）；Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC and BIST（加泰罗尼亚纳米科学与技术研究所（ICN2，西班牙高等科研理事会与巴塞罗那自治大学联合））；National Institute for Materials Science（国立材料研究所）
The evolution of information technology has been driven by the discovery of new forms of large magnetoresistance (MR), such as giant magnetoresistance (GMR) and tunnelling magnetoresistance (TMR) in magnetic multilayers. Recently, new types of MR have been observed in much simpler bilayers consisting of ferromagnetic (FM)/nonmagnetic (NM) thin films; however, the magnitude of MR in these materials is very small (0.01 ~ 1%). Here, we demonstrate that NM/FM bilayers consisting of a NM InAs quantum well conductive channel and an insulating FM (Ga,Fe)Sb layer exhibit giant proximity magnetoresista…
We propose a novel heterostructure to achieve chiral topological superconductivity in 2D. A substrate with a large Rashba spin-orbit coupling energy is brought in proximity to a twisted bilayer of thin films exfoliated from a high-temperature cuprate superconductor. The combined system is then exposed to an out-of-plane magnetic field. The rare $d + id$ pairing symmetry expected to occur in such a system allows for nontrivial topology; specifically, in contrast to the case of the twisted bilayer in isolation, the substrate induces an odd Chern number. The resulting phase is characterized by th…
We investigate the effect of eddy currents on ferromagnetic resonance (FMR) in ferromagnet-normal metal (FM/NM) bilayer structures. Eddy-current effects are usually neglected for NM layer thicknesses below the microwave (MW) skin depth (approx. 800 nm for Au at 10 GHz). However, we show that in much thinner NM layers (10-100 nm of Au or Cu) they induce a phase shift in the FMR excitation when the MW driving field has a component perpendicular to the sample plane. This results in a strong asymmetry of the measured absorption lines. In contrast to typical eddy-current effects, the asymmetry is l…
We study the band structure of phases induced by depositing bilayer graphene on a transition metal dichalcogenide monolayer. Tight-binding and low-energy effective Hamiltonian calculations show that it is possible to induce topologically nontrivial phases that should exhibit spin Hall effect in these systems. We classify bulk insulating phases through calculation of the Z$_2$ invariant, which unequivocally identifies the topology of the structure. The study of these and similar hybrid systems under applied gate voltage opens the possibility for tunable topological structures in real experiment…
Ferromagnetic resonance (FMR) in exchange-coupled ferromagnet-antiferromagnet (FM/AFM) bilayers commonly shows a moderate increase in the resonance frequency owing to the induced unidirectional anisotropy. Here we report a large FMR frequency enhancement toward the sub-THz range observed in Py/FeMn with ultrathin AFM FeMn. The effect is connected with a sizable induced magnetic moment in FeMn caused by the magnetic proximity effect from the Py layer. The observed FMR properties are explained as due to the competing intrinsic antiferromagnetic order and the ferromagnetic proximity effect in nan…
Proximity Effects Between the Graphene Quasicrystal and Magic-Angle Twisted Bilayer Graphene
Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC and BIST（加泰罗尼亚纳米科学技术研究所（ICN2），西班牙国家研究委员会和巴塞罗那高等研究院）；Department of Physics, Campus UAB（巴塞罗那自治大学物理系）；Institute of Condensed Matter and Nanosciences, Université catholique de Louvain (UCLouvain)（天主教鲁汶大学凝聚态与纳米科学研究所）；ICREA–Institució Catalana de Recerca i Estudis Avançats（加泰罗尼亚研究与高级研究所（ICREA））
A ferromagnetic insulator attached to a superconductor is known to induce an exchange splitting of the Bardeen-Cooper-Schrieffer (BCS) singularity by a magnitude proportional to the magnetization, and penetrating into the superconductor to a depth comparable with the superconducting coherence length. We study this long-range magnetic proximity effect in EuS/Al bilayers and find that the exchange splitting of the BCS peaks is present already in the unpolarized state of the ferromagnetic insulator (EuS), and is being further enhanced when magnetizing the sample by a magnetic field. The measureme…
We study the proximity-induced superconducting state in a general bilayer -- conventional $s$-wave superconductor hybrid structure. For the bilayer we include a general parabolic dispersion, Rashba spin-orbit coupling, and finite layer tunneling as well as the possibility to apply a bias potential and a magnetic Zeeman field, in order to address experimentally relevant bilayer systems, ranging from topological insulator thin films to generic double quantum well systems. By extracting the proximity-induced anomalous Green's function in the bilayer we show on a very rich structure for the superc…
Compared to monolayer graphene, electrons in Bernal-stacked bilayer graphene (BLG) have an additional layer degree of freedom, offering a platform for developing {\it layered spintronics} with the help of proximity-induced magnetism. Based on an effective phenomenological model, we systematically study the effect of this magnetism on the spin-dependent band structure near the Fermi energy and identify the magnetic phases induced in BLG by proximity with magnets. We show that spin polarization can develop in BLG due to this proximity effect. This spin polarization depends strongly on the layer …
We discuss twisted bilayer graphene (TBG) based on a theorem of flat band ferromagnetism put forward by Mielke and Tasaki. According to this theorem, ferromagnetism occurs if the single particle density matrix of the flat band states is irreducible and we argue that this result can be applied to the quasi-flat bands of TBG that emerge around the charge-neutrality point for twist angles around the magic angle $θ\sim1.05^\circ$. We show that the density matrix is irreducible in this case, thus predicting a ferromagnetic ground state for neutral TBG ($n=0$). We then show that the theorem can also…
We report chirality-induced current-in-plane magnetoresistance (CIP-MR) in chiral molecule/ferromagnetic metal bilayer at room temperature. The previously reported chiralityinduced current-perpendicular-to-plane magnetoresistance (CPP-MR) originates from the chiral induced spin-selectivity (CISS) effect that needs charge-current passing through the molecule. In contrast, the observed CIP-MR in the present study requires no bias charge current through the molecule. The temperature dependence of CIP-MR suggests thermally induced spin-polarization in the chiral molecules is the key for the observ…
We propose an experimental scheme to determine the spin-transfer torque efficiency excited by the spin-orbit interaction in ferromagnetic bilayers from the measurement of the longitudinal magnetoresistace. Solving a diffusive spin-transport theory with appropriate boundary conditions gives an analytical formula of the longitudinal charge current density. The longitudinal charge current has a term that is proportional to the square of the spin-transfer torque efficiency and that also depends on the ratio of the film thickness to the spin diffusion length of the ferromagnet. Extracting this cont…
A theoretical formulation of magnetoresistance effect in a metallic ferromagnetic/nonmagnetic bilayer originated from the charge-spin conversion by the anomalous Hall effect is presented. Analytical expressions of the longitudinal and transverse resistivities in both nonmagnet and ferromagnet are obtained by solving the spin diffusion equation. The magnetoresistance generated from charge-spin conversion purely caused by the anomalous Hall effect in the ferromagnet is found to be proportional to the square of the spin polarizations in the ferromagnet and has fixed sign. We also find additional …
Depositing magnetic insulators on graphene has been a promising route to introduce magnetism via exchange proximity interaction in graphene for future spintronics applications. Molecule-based magnets may offer unique opportunities because of their synthesis versatility. Here, we investigated the magnetic proximity effect of epitaxial iron phthalocyanine (FePc) molecules on high-quality monolayer and bilayer graphene devices on hexagonal boron nitride substrate by probing the local and non-local transport. Although the FePc molecules introduce large hole doping effects combined with mobility de…
The spin polarization of Pt in Pt/NiFe2O4 and Pt/Fe bilayers is studied by interface-sensitive x-ray resonant magnetic reflectivity to investigate static magnetic proximity effects. The asymmetry ratio of the reflectivity was measured at the Pt L3 absorption edge using circular polarized x-rays for opposite directions of the magnetization at room temperature. The results of the 2% asymmetry ratio for Pt/Fe bilayers are independent of the Pt thickness between 1.8 and 20 nm. By comparison with ab initio calculations, the maximum magnetic moment per spin polarized Pt atom at the interface is dete…
The thickness dependence of spin-orbit torque and magnetoresistance in ferromagnet/heavy-metal bilayers is studied using the first-principles non-equilibrium Green's function formalism combined with the Anderson disorder model. A systematic expansion in orthogonal vector spherical harmonics is used for the angular dependence of the torque. The damping-like torque in Co/Pt and Co/Au bilayers can be described as a sum of the spin-Hall contribution, which increases with thickness in agreement with the spin-diffusion model, and a comparable interfacial contribution. The magnetoconductance in the p…
Two dimensional (2D) materials provide a unique platform to explore the full potential of magnetic proximity driven phenomena, which can be further used for applications in next generation spintronic devices. Of particular interest is to understand and control spin currents in graphene by the magnetic exchange field of a nearby ferromagnetic material in graphene/ferromagnetic-insulator (FMI) heterostructures. Here, we present the experimental study showing the strong modulation of spin currents in graphene layers by controlling the direction of the exchange field due to FMI magnetization. Owin…
We reveal a proximity effect between a topological band (Chern) insulator described by a Haldane model and spin-polarized Dirac particles of a graphene layer. Coupling weakly the two systems through a tunneling term in the bulk, the topological Chern insulator induces a gap and an opposite Chern number on the Dirac particles at half-filling resulting in a sign flip of the Berry curvature at one Dirac point. We study different aspects of the bulk-edge correspondence and present protocols to observe the evolution of the Berry curvature as well as two counter-propagating (protected) edge modes wi…
We investigate ferromagnetic resonance (FMR) modulation in $d$-wave superconductor (SC)/ferromagnetic insulator (FI) bilayer systems theoretically. The modulation of the Gilbert damping in these systems reflects the existence of nodes in the $d$-wave SC and shows power-law decay characteristics within the low-temperature and low-frequency limit. Our results indicate the effectiveness of use of spin pumping as a probe technique to determine the symmetry of unconventional SCs with high sensitivity for nanoscale thin films.
Bilayer Heisenberg ferromagnetic insulators hold degenerate terahertz Dirac magnon modes associated with two opposite valleys of the hexagonal Brillouin zone. We show that this energy degeneracy can be removed by breaking of the inversion symmetry (I), leading to a topological magnon valley current. We show furthermore that this current leads to valley Seebeck effect for magnons and is thereby detectable. We perform calculations in the specific example of bilayer CrBr3, where I can be broken by electrostatic doping.
Realizations of some topological phases in two-dimensional systems rely on the challenge of jointly incorporating spin-orbit and magnetic exchange interactions. Here, we predict the formation and control of a fully valley-polarized quantum anomalous Hall effect in bilayer graphene, by separately imprinting spin-orbit and magnetic proximity effects in different layers. This results in varying spin splittings for the conduction and valence bands, which gives rise to a topological gap at a single Dirac cone. The topological phase can be controlled by a gate voltage and switched between valleys by…
Gate-induced magnetic switching in bilayer CrI$_3$ has opened new ways for the design of novel low-power magnetic memories based on van der Waals heterostructures. The proposed switching mechanism seems to be fully dominated by electrostatic doping. Here we explain, by first-principle calculations, the ferromagnetic transition in doped bilayer CrI$_3$. For the case of a very small electron doping, our calculations predict the formation of magnetic polarons ("ferrons", "fluctuons") where the electron is self-locked in a ferromagnetic droplet in an antiferromagnetic insulating matrix. The self-t…
We explore the role of proximity-induced odd-frequency pairing in the thermoelectricity of a ferromagnet when coupled to a conventional $s$-wave spin-singlet superconductor through a spin-active interface. By varying both the polarization and its direction in the ferromagnet and the interfacial spin-orbit interaction strength, we analyze the behavior of all proximity-induced pair amplitudes in the ferromagnet and their contributions to the thermoelectric coefficients. Based on our results for the Seebeck coefficient, we predict that odd-frequency spin-triplet Cooper pairs are much efficient th…
Evidence of orbital Hall current induced correlation in second harmonic response of longitudinal and transverse voltage in light metal-ferromagnet bilayers
We demonstrate the anomalous Hall effect (AHE) in single-layer graphene exchange-coupled to an atomically flat yttrium iron garnet (YIG) ferromagnetic thin film. The anomalous Hall conductance has magnitude of ~0.09(2e2/h) at low temperatures and is measurable up to ~ 300 K. Our observations indicate not only proximity-induced ferromagnetism in graphene/YIG with large exchange interaction, but also enhanced spin-orbit coupling which is believed to be inherently weak in ideal graphene. The proximity-induced ferromagnetic order in graphene can lead to novel transport phenomena such as the quanti…
We report broadband spectroscopy and numerical analysis by which we explore propagating spin waves in a magnetic bilayer consisting of a 23 nm thick permalloy film deposited on 130 nm thick $Y_{3}Fe_{5}O_{12}$. In the bilayer, we observe a characteristic mode that exhibits a considerably larger group velocity at small in-plane magnetic field than both the magnetostatic and perpendicular standing spin waves. Using the finite element method, we confirm the observations by simulating the mode profiles and dispersion relations. They illustrate the hybridization of spin wave modes due to exchange c…
