We explore the role of proximity-induced odd-frequency pairing in the thermoelectricity of a ferromagnet when coupled to a conventional $s$-wave spin-singlet superconductor through a spin-active interface. By varying both the polarization and its direction in the ferromagnet and the interfacial spin-orbit interaction strength, we analyze the behavior of all proximity-induced pair amplitudes in the ferromagnet and their contributions to the thermoelectric coefficients. Based on our results for the Seebeck coefficient, we predict that odd-frequency spin-triplet Cooper pairs are much efficient than the conventional spin-singlet even-frequency pairs in enhancing thermoelectricity of the junction, especially mixed-spin triplet pairing is favorable. Our results on the thermoelectric figure of merit show that ferromagnet/superconductor junctions are very good thermoelectric systems when superconductivity is dominated by odd-frequency pairing.
UCoGe exhibits superconductivity in the presence of ferromagnetism. When a field is applied along the b axis (perpendicular to the easy axis), ferromagnetism is weakened and superconductivity is enhanced. This enhancement has been attributed to an increase in coupling as observed in the enhanced effective mass produced by the critical fluctuations as the ferromagnetic transition is strongly suppressed. However it is also important to know if and how the Fermi surface changes near the critical point. Here we report measurements of the thermoelectricity of UCoGe which reveal a low carrier densit…
We study the effects of spin-splitting and spin-flip scattering in a superconductor (S) on the thermoelectric properties of a tunneling contact to a metallic ferromagnet (F) using the Green's function method. A giant thermopower has been theoretically predicted and experimentally observed in such structures. This is attributed to the spin-dependent particle-hole asymmetry in the tunneling density of states in the S/F heterostructure. Here, we evaluate the S density of states and thermopower for a range of temperatures, Zeeman-splitting, and spin-flip scattering. In contrast to the naive expect…
A ferromagnetic insulator (FI) attached to a conventional superconductor (S) changes drastically the properties of the latter. Specifically, the exchange field at the FI/S interface leads to a splitting of the superconducting density of states. If S is a superconducting film, thinner than the superconducting coherence length, the modification of the density of states occurs over the whole sample. The co-existence of the exchange splitting and superconducting correlations in S/FI structures leads to striking transport phenomena that are of interest for applications in thermoelectricity, superco…
We show that quantum spin fluctuations in inhomogeneous ferromagnets drastically affect the Andreev reflection of electrons and holes at a ferromagnet-superconductor interface. As a result a strong long-range proximity effect appears, associated with electron-hole spin triplet correlations and persisting on a lenght scale typical for non-magnetic materials, but anomalously large for ferromagnets.
We have measured the electrical transport of submicron ferromagnets (Ni) in contact with a mesoscopic superconductor (Al) for a range of interface resistances. In the geometry measured, the interface and the ferromagnet are measured separately. The ferromagnet itself shows no appreciable superconducting proximity effect, but the ferromagnet/superconductor interface exhibits strong temperature, field and current bias dependences. These effects are dependent on the local magnetic field distribution near the interface arising from the ferromagnet. We find that the temperature dependences may be f…
The theory of the I-V characteristics in diffusive superconductor/weak ferromagnet/superconductor (SFS) junction is developed. We show that the exchange field $h$ of the ferromagnet manifests itself as an additional conductance peak at $eV \sim Δ+h$ in the phase-coherent regime, when the Thouless energy is of the order of superconducting order parameter. The excess current exhibits non-monotonous dependence on the exchange field and non-trivial temperature behavior, which is strongly influenced by the temperature dependence of the exchange field.
We consider a bi-layer consisting of a $d-$wave layerd superconductor and diffusive ferromagnet with a domain wall (DW). The $c-$axis in the superconductor and DW in the ferromagnet are assumed to be perpendicular to the interface. We demonstrate that in such a heterostructure the inhomogeneous exchange field enhances the proximity effect. It is shown that, whereas in the absence of the exchange field the $d-$wave condensate decays in the normal metal on the mean free path $l$, the superconductivity penetrates the ferromagnet along the DW over much larger distances. This happens because the pr…
We have measured the evolution of the tunneling density of states (DOS) in superconductor/ferromagnet (S/F) bilayers with increasing F-layer thickness, where F in our experiment is the strong ferromagnet Ni. As a function of increasing Ni thickness, we detect multiple oscillations in the DOS at the Fermi energy from differential conductance measurements. The features in the DOS associated with the proximity effect change from normal to inverted twice as the Ni thickness increases from 1 to 5 nm.
We study the electronic density of states in a mesoscopic superconductor near a transparent interface with a ferromagnetic metal. In our tunnel spectroscopy experiment, a substantial density of states is observed at sub-gap energies close to a ferromagnet. We compare our data with detailed calculations based on the Usadel equation, where the effect of the ferromagnet is treated as an effective boundary condition. We achieve an excellent agreement with theory when non-ideal quality of the interface is taken into account.
The very special characteristic of the proximity effect in superconductor-ferromagnet systems is the damped oscillatory behavior of the Cooper pair wave function in a ferromagnet. In some sense, this is analogous to the inhomogeneous superconductivity, predicted long time ago by Larkin and Ovchinnikov (1964), and Fulde and Ferrell (1964), and constantly searched since that. After the qualitative analysis of the peculiarities of the proximity effect in the presence of the exchange field, the author provides a unified description of the properties of the superconductor-ferromagnet heterostructur…
We reconsider the problem of the superconducting proximity effect in a diffusive ferromagnet bounded by tunneling interfaces, using spin-dependent boundary conditions. This introduces for each interface a phase-shifting conductance Gphi which results from the spin dependence of the phase shifts acquired by the electrons upon scattering on the interface. We show that Gphi strongly affects the density of states and supercurrents predicted for superconducting/ferromagnetic hybrid circuits. We show the relevance of this effect by identifying clear signatures of Gphi in the data of T. Kontos et al …
We discuss the Josephson effect in strongly spin-polarized ferromagnets where triplet correlations are induced by means of spin-active interface scattering, extending our earlier work [Phys. Rev. Lett. 102, 227005 (2009)] by including impurity scattering in the ferromagnetic bulk and the inverse proximity effect in a fully self-consistent way. Our quasiclassical approach accounts for the differences of Fermi momenta and Fermi velocities between the two spin bands of the ferromagnet, and thereby overcomes an important short-coming of previous work within the framework of Usadel theory. We show …
We review the present status of the experimental and theoretical research on the proximity effect in heterostructures composed of superconducting (S) and ferromagnetic (F) thin films. First, we discuss traditional effects originating from the oscillatory behavior of the superconducting pair wave function in the F-layer. Then, we concentrate on recent theoretical predictions for S/F layer systems. These are a) generation of odd triplet superconductivity in the F-layer and b) ferromagnetism induced in the S-layer below the superconducting transition temperature $T_{c}$ (inverse proximity effect)…
We have previously shown that a ferromagnet-superconductor heterostructure may possess a spontaneous current circulation parallel to the interface. This current is caused by Andreev bound states in the thin ferromagnetic layer, and can be fully spin-polarized. Here we investigate the total energy of the system in cases where the current either does or does not flow. We show that the current is a true quantum ground state effect, and examine the effect of the current on the different contributions to the total energy.
We theoretically investigate an opportunity to implement a source of highly spin-polarized ac current on the basis of superconductor/weak ferromagnet/superconductor (SFS) voltage-biased junction in the regime of essential proximity effect and calculate the current flowing through the probe electrode tunnel coupled to the ferromagnetic interlayer region. It is shown that while the polarization of the dc current component is generally small in case of weak exchange field of the ferromagnet, there is an ac component of the current in the system. This ac current is highly spin-polarized and entire…
We discuss some properties of the ferromagnet-superconductor proximity system. In particular, the emphasis is put on the physics of the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) like state. In addition to Andreev reflections it features a number of unusual thermodynamic and transport properties, like: oscillatory behavior of the pairing amplitude, density of states and superconducting transition temperature as a function of the ferromagnet thickness. Surprisingly, under certain conditions spontaneous spin polarized current is generated in the ground state of such a system. We provide some inform…
We study the ground state properties of a ferromagnet-superconductor heterostructure on the basis of a quasiclassical theory. We have solved the Eilenberger equations together with Maxwell's equation fully self-consistently and found that due to the proximity effect a Fulde-Ferrel-Larkin-Ovchinnikov (FFLO) like state is realized in such system. Moreover this state has oscillations of the pairing amplitude in either one or two directions, depending on the exchange splitting and thickness of the ferromagnet. In particular, using semiclassical arguments (Bohr-Sommerfeld quantization rule) we show…
The magnetization in a superconductor induced due to the inverse proximity effect is investigated in hybrid bilayers containing a superconductor and a ferromagnetic insulator or a strongly spin-polarized ferromagnetic metal. The study is performed within a quasiclassical Green function framework, wherein Usadel equations are solved with boundary conditions appropriate for strongly spin-polarized ferromagnetic materials. A comparison with recent experimental data is presented. The singlet to triplet conversion of the superconducting correlations as a result of the proximity effect with a ferrom…
We study thermal and charge transport in a three-terminal setup consisting of one superconducting and two ferromagnetic contacts. We predict that the simultaneous presence of spin filtering and of spin- dependent scattering phase shifts at each of the two interfaces will lead to very large nonlocal thermo- electric effects both in clean and in disordered systems. The symmetries of thermal and electric transport coefficients are related to fundamental thermodynamic principles by the Onsager reciprocity. Our results show that a nonlocal version of the Onsager relations for thermoelectric current…
We consider the proximity effects in hybrid superconductor (S) - ferromagnet (F) structures drawing attention to the induced ferromagnetism of the S metal. The analysis is based on a quasiclassical theory of proximity effect for metals in the dirty limit conditions. It is shown that, below the superconducting critical temperature, ferromagnetic correlations extend a distance of order of the superconducting coherence length ξ_{S} into the superconductor, being dependent on the S/F interface parameters. We argue that the properties of mesoscopic SF hybrids may drastically depend upon the magneti…
Superconductor/ferromagnet proximity effect has been studied for Pb/Co$_2$Cr$_{1-x}$Fe$_x$Al bilayers. Different substrate temperatures allowed us to prepare the Heusler alloy Co$_2$Cr$_{1-x}$Fe$_x$Al films with different degree of spin polarization of conduction band of the Heusler layer. We obtain a strong correlation between the dependence of the superconducting transition temperature on the Pb-layer thickness at fixed thickness of the Heusler layer and the degree of spin polarization in the ferromagnetic layer.
Scanning tunneling spectroscopy measurements conducted on epitaxially grown bilayers of half-metallic ferromagnetic La2/3Ca1/3MnO3 (LCMO) on superconducting (SC) (100)YBa2Cu3O7-delta (YBCO) reveal long-range penetration of superconducting order into the LCMO. This anomalous proximity effect manifests itself in the tunneling spectra measured on the LCMO layer as gaps and zero bias conductance peaks. Remarkably, these proximity-induced spectral features were observed for bilayers with LCMO thickness of up to 30 nm, an order of magnitude larger than the expected ferromagnetic coherence length in …
Magnetization noncollinearity in ferromagnet-superconductor (F/S) heterostructures is expected to enhance the superconducting transition temperature (Tc) according to the domain-wall superconductivity theory, or to suppress Tc when spin-triplet Cooper pairs are explicitly considered. We study the proximity effect in F/S structures where the F layer is a Sm-Co/Py exchange-spring bilayer and the S layer is Nb. The exchange-spring contains a single, controllable and quantifiable domain wall in the Py layer. We observe an enhancement of superconductivity that is nonmonotonic as the Py domain wall …
We theoretically study the magnetism induced by the proximity effect in the normal metal of ferromagnetic Josephson junction composed of two $s$-wave superconductors separated by ferromagnetic metal/normal metal/ferromagnetic metal junction (${S}/{F}/{N}/{F}/{S}$ junction). We calculate the magnetization in the $N$ by solving the Eilenberger equation. We show that the magnetization arises in the ${N}$ when the product of anomalous Green's functions of the spin-triplet even-frequency odd-parity Cooper pair and spin-singlet odd-frequency odd-parity Cooper pair in the ${N}$ has a finite value. Th…
Resonant proximity effect in the normal metal / insulator / diffusive ferromagnet / insulator / $s$- and d-wave superconductor (N/I/DF/I/S) junctions is studied for various regimes by solving the Usadel equation with the generalized boundary conditions. It is shown that the resonant proximity effect originating from the exchange field in DF layer strongly modifies the tunneling conductance and density of states.
The long-range proximity effect in superconductor/ferromagnet (S/F) hybrid nano-structures is observed if singlet Cooper pairs from the superconductor are converted into triplet pairs which can diffuse into the fer- romagnet over large distances. It is commonly believed that this happens only in the presence of magnetic inhomogeneities. We show that there are other sources of the long-range triplet component (LRTC) of the con- densate and establish general conditions for their occurrence. As a prototypical example we consider first a system where the exchange field and spin-orbit coupling can …
We study peculiarities of proximity effect in clean superconductor -- ferromagnet structures caused by either spatial or momentum dependence of the exchange field. Even a small modulation of the exchange field along the quasiparticle trajectories is shown to provide a long range contribution to the supercurrent due to the specific interference of particle- and hole- like wave functions. The momentum dependence of the exchange field caused by the spin -- orbit interaction results in the long -- range superconducting correlations even in the absence of ferromagnetic domain structure and can expl…
We find that the dependence on temperature and magnetic field of the electrical resistance of diffusive ferromagnetic nano-wires measured with superconducting electrodes changes drastically with the distance, $L$, between the ferromagnet/superconductor contacts, however is remarkably similar for the wires with the same $L$ ranging from 300 nm to 1000 nm, prepared under identical conditions. The result gives an evidence for the long-range superconductor-induced changes in transport properties of ferromagnetic nano-wires.
This work is devoted to experimental study of influence of superconductivity (S) on ferromagnetism (FM) (inverse proximity effects) with the help of Polarized Neutron Reflectivity. Combining meausurements of specular and diffuse intensities it is possible to obtain full picture of magnetization change in S/FM layered systems like magnetization rotation, domain state formation, inducing of magnetization in S layer, etc. To increase weak magnetic signal we propose to use enhanced neutron standing wave regime (e.g. waveguides). In previous work we have made calculation to increase enhcanced facto…
Measurements of the polar Kerr effect using a zero-area-loop Sagnac magnetometer on Pb/Ni and Al/(Co-Pd) proximity-effect bilayers show unambiguous evidence for the "inverse proximity effect," in which the ferromagnet (F) induces a finite magnetization in the superconducting (S) layer. To avoid probing the magnetic effects in the ferromagnet, the superconducting layer was prepared much thicker than the light's optical penetration depth. The sign and size of the effect, as well as its temperature dependence agree with recent predictions by Bergeret et al..
The ferromagnetic resonance of thin sputtered Ni80Fe20 films grown on Nb is measured. By varying the temperature and thickness of the Nb the role of the superconductivity on the whole ferromagnetic layer in these heterostructures is explored. The change in the spin transport properties below the superconducting transition of the Nb is found to manifest itself in the Ni80Fe20 layer by a sharpening in the resonance of the ferromagnet, or a decrease in the effective Gilbert damping co-efficient. This dynamic proximity effect is in contrast to low frequency studies in these systems, where the effe…
We investigate the effect of an inhomogeneous exchange field on the proximity effect in superconductor-ferromagnet hybrid structures within the quasi-classical theory of superconductivity. As an example we study the proximity effect in a superconductor-ferromagnet bilayer with an in-plane spiral magnetic order in the ferromagnet. This model simulates a multiple magnetic domain structure where the domain walls of the Néel type are of equal size as the domains. Triplet correlations are induced in the bilayer by the superconducting proximity effect, which are sensitive to the local quantization a…
We study theoretically the influence of ferromagnetic metals on a superconducting film in the clean limit. Using a self-consistent solution of the Bogoliubov--de Gennes equation for a ferromagnet-superconductor-ferromagnet double junction we calculate the pair potential and conductance spectra as a function of the superconducting layer thickness $d$ for different strengths of ferromagnets and interface transparencies. We find that the pair potential and the critical temperature are weakly perturbed by the exchange interaction and do not drop to zero for any finite $d$. On the other hand, for t…
We study proximity effects at ferromagnet superconductor interfaces by self-consistent numerical solution of the Bogoliubov-de Gennes equations for the continuum, without any approximations. Our procedures allow us to study systems with long superconducting coherence lengths. We obtain results for the pair potential, the pair amplitude, and the local density of states. We use these results to extract the relevant proximity lengths. We find that the superconducting correlations in the ferromagnet exhibit a damped oscillatory behavior that is reflected in both the pair amplitude and the local de…
The injection of pure spin current into superconductors by the dynamics of a ferromagnetic contact is studied theoretically. Taking into account suppression of the order parameter at the interfaces (inverse proximity effect) and the energy-dependence of spin-flip scattering, we determine the temperature-dependent ferromagnetic resonance linewidth broadening. Our results agree with recent experiments in Nb|permalloy bilayers [C. Bell et al., arXiv:cond-mat/0702461].
Considerable evidence for proximity-induced triplet superconductivity on the ferromagnetic side of a superconductor-ferromagnet (S-F) interface now exists; however, the corresponding effect on the superconductor side has hardly been addressed. We have performed scanning tunneling spectroscopy measurements on NbN superconducting thin films proximity coupled to the half-metallic ferromagnet La2/3Ca1/3MnO3 (LCMO) as a function of magnetic field. We have found that at zero and low applied magnetic fields the tunneling spectra on NbN typically show an anomalous gap structure with suppressed coheren…
The spread of the Cooper pairs into the ferromagnet in proximity coupled superconductor - ferromagnet (SF) structures is shown to cause a strong inverse electromagnetic phenomenon, namely, the long-range transfer of the magnetic field from the ferromagnet to the superconductor. Contrary to the previously investigated inverse proximity effect resulting from the spin polarization of superconducting surface layer, the characteristic length of the above inverse electrodynamic effect is of the order of the London penetration depth, which usually much larger than the superconducting coherence length…
The usually negligibly small thermoelectric effects in superconducting heterostructures can be boosted dramatically due to the simultaneous effect of spin splitting and spin filtering. Building on an idea of our earlier work [Phys. Rev. Lett. $\textbf{110}$, 047002 (2013)], we propose realistic mesoscopic setups to observe thermoelectric effects in superconductor heterostructures with ferromagnetic interfaces or terminals. We focus on the Seebeck effect being a direct measure of the local thermoelectric response and find that a thermopower of the order of $\sim200$ $μV/K$ can be achieved in a …
We examined the proximity effect in granular films made of Pb, a superconductor, and Ni, a ferromagnet, with various compositions. Slow decay of the critical temperature as a function of the relative volume concentration of Ni per sample was demonstrated by our measurements, followed by a saturation of T$_c$. Using an approximate theoretical description of our granular system in terms of a layered one, we show that our data can only be reasonably fitted by a multilayer model. This indicates the importance of the interplay between different ferromagnetic grains; when non-collinearly magnetized …
We study the perpendicular transport characteristics of small superconductor/ferromagnetic insulator/superconductor (YBa$_2$Cu$_3$O$_{7-x}$/LaMnO$_{3+δ}$/YBa$_2$Cu$_3$O$_{7-x}$) tunnel junctions. At a large bias voltage $V\sim 1$ V we observe a step-like onset of excess current that occurs below the superconducting transition temperature $T<T_c$ and is easily suppressed by a magnetic field. The phenomenon is attributed to a novel type of the superconducting proximity effect of non-equilibrium electrons injected into the conduction band of the ferromagnetic insulator via a Fowler-Nordheim tunne…
We consider superconductivity nucleation in multiply connected mesoscopic samples such as thin-walled cylinders or rings placed in electrical contact with a ferromagnet. The superconducting critical temperature and order parameter structure are studied on the basis of linearized Usadel equations. We suggest a mechanism of switching between the superconducting states with different vorticities caused by the exchange field and associated with the oscillatory behavior of the Cooper pair wave function in a ferromagnet.
When a ferromagnet is placed in contact with a superconductor, owing to incompatible spin order, the Cooper pairs from the superconductor cannot survive more than one or two nanometers inside the ferromagnet. This is confirmed in the measurements of ferromagnetic nickel (Ni) nanowires contacted by superconducting niobium (Nb) leads. However, when a 3 nm thick copper oxide (CuO) buffer layer made by exposing an evaporated or a sputtered 3 nm Cu film to air, is inserted between the Nb electrodes and the Ni wire, the spatial extent of the superconducting proximity range is dramatically increased …
We investigate inverse proximity effects in a spin-triplet superconductor (TSC) interfaced with a ferromagnet (FM), assuming different types of magnetic profiles and chiral or helical pairings. The region of the coexistence of spin-triplet superconductivity and magnetism is significantly influenced by the orientation and spatial extension of the magnetization with respect to the spin configuration of the Cooper pairs, resulting into clearcut anisotropy signatures. A characteristic mark of the inverse proximity effect arises in the induced spin-polarization at the TSC interface. This is unexpec…
We show that in superlattices with alternating superconducting (S) and ferromagnetic (F) layers the spontaneous magnetic field induced in the superconducting layers due to the electromagnetic proximity effect becomes dramatically enhanced compared to the previously studied S/F bilayers. The effect reveals itself for the in-plane orientation of the magnetic moments both for ferromagnetic and anti-ferromagnetic ordering of the moments in the F layers. In the finite size samples the magnetic field decays from the sample surface towards the bulk of the structure, and the decay length strongly depe…
Heterostructures made of itinerant ferromagnets and superconductors are studied. In contrast to most previous models, ferromagnetism is not enforced as an external Zeeman field but induced in a correlated single-band model (CSBM) that displays itinerant ferromagnetism as a mean-field ground state. This allows us to investigate the influence of an adjacent superconducting layer on the properties of the ferromagnet in a self-consistent Bogoliubov-de Gennes approach. The CSBM displays a variety features not present in the Zeeman exchange model that influence the behavior of order parameters close…
At the interface between a superconductor and a ferromagnetic metal spin-singlet Cooper pairs can penetrate into the ferromagnetic part of the heterostructure with an oscillating and decaying spin-singlet Cooper pair density. However, if the interface allows for a spin-mixing effect, equal-spin spin-triplet Cooper pairs can be generated that can penetrate much further into the ferromagnetic part of the heterostructure, known as the long-range proximity effect. Here, we present results of spin-mixing based on self-consistent solutions of the microscopic Bogoliubov-de Gennes equations incorporat…
We study the proximity effect in SF'(AF)F'S and SF'(F)F'S planar junctions, where S is a clean conventional (s-wave) superconductor, while F' and middle layers are clean or moderately diffusive ferromagnets. Middle layers consist of two equal ferromagnets with antiparallel (AF) or parallel (F) magnetizations that are not collinear with magnetizations in the neighboring F' layers. We use fully self-consistent numerical solutions of the Eilenberger equations to calculate the superconducting pair amplitudes and the Josephson current for arbitrary thickness of ferromagnetic layers and the angle be…
We present a microscopic theory of proximity effect in the ferromagnet/superconductor/ferromagnet (F/S/F) nanostructures where S is s-wave low-T_c superconductor and F's are layers of 3d transition ferromagnetic metal. Our approach is based on the solution of Gor'kov equations for the normal and anomalous Green's functions together with a self-consistent evaluation of the superconducting order parameter. We take into account the elastic spin-conserving scattering of the electrons assuming s-wave scattering in the S layer and s-d scattering in the F layers. In accordance with the previous quasi…
The proximity effect, quasiparticle transport, and local magnetic moment in ferromagnet--d-wave superconductor junctions with {110}-oriented interface are studied by solving self-consistently the Bogoliubov-de Gennes equations within an extended Hubbard model. It is found that the proximity induced order parameter oscillates in the ferromagnetic region. The modulation period is shortened with the increased exchange field while the oscillation amplitude is depressed by the interfacial scattering. With the determined superconducting energy gap, a transfer matrix method is proposed to compute the…
We have studied the proximity-induced superconducting triplet pairing in CoO$_x$/Py1/Cu/Py2/Cu/Pb spin-valve structure (where Py = Ni$_{0.81}$Fe$_{0.19}$). By optimizing the parameters of this structure we found a triplet channel assisted full switching between the normal and superconducting states. To observe an "isolated" triplet spin-valve effect we exploited the oscillatory feature of the magnitude of the ordinary spin-valve effect $ΔT_c$ in the dependence of the Py2-layer thickness $d_{Py2}$. We determined the value of $d_{Py2}$ at which $ΔT_c$ caused by the ordinary spin-valve effect (th…
We study theoretically the proximity effect in a ferromagnetic semiconductor with Rashba spin-orbit interaction. The exchange potential generates opposite-spin-triplet Cooper pairs which are transformed into equal-spin-triplet pairs by the spin-orbit interaction. In the limit of strong spin-orbit interaction, symmetry of the dominant Cooper pair depends on the degree of disorder in a ferromagnet. In the clean limit, spin-singlet $s$-wave Cooper pairs are the most dominant because the spin-momentum locking stabilizes a Cooper pair consisting of a time-reversal partner. In the dirty limit, on th…
We study Superconductor/Ferromagnet/Superconductor junctions with CuNi, PtNi, or Ni interlayers. Remarkably, we observe that supercurrents through Ni can be significantly larger than through diluted alloys. The phenomenon is attributed to the dirtiness of disordered alloys leading to a short coherence length despite a small exchange energy. To the contrary, pure Ni is clean resulting in a coherence length as long as in a normal metal. Analysis of temperature dependencies of critical currents reveals a crossover from short (dirty) to long (clean) range proximity effects in Pt1-xNix with increas…