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arXiv 2012.14499cond-mat.str-elcond-mat.mes-hall
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长程电子-电子相互作用对扭曲双层石墨烯磁性phase diagram的重要性

Importance of long-ranged electron-electron interactions for the magnetic phase diagram of twisted bilayer graphene

Lennart Klebl, Zachary A. H. Goodwin, Arash A. Mostofi, Dante M. Kennes, Johannes Lischner

摘要:

电子-电子相互作用本质上是长程的,但许多强相互作用电子的模型只考虑短程相互作用。在这里,我们提出的原子计算的结果,包括远程和短程电子-电子相互作用的扭曲双层石墨烯的磁相图,并表明,定性不同的结果时,远程相互作用被忽略。特别是,我们使用Hartree理论增强哈伯德相互作用和计算的相互作用自旋磁化率在一系列的掺杂水平和扭转角附近的魔角,以确定占主导地位的磁不稳定性。在魔角,主要是反铁磁秩序,而铁磁性占主导地位,在其他扭曲角。此外,长程相互作用显着增加的扭曲角窗口,其中强相关现象可以预期。这些发现与现有的实验数据吻合得很好。

英文摘要:

Electron-electron interactions are intrinsically long ranged, but many models of strongly interacting electrons only take short-ranged interactions into account. Here, we present results of atomistic calculations including both long-ranged and short-ranged electron-electron interactions for the magnetic phase diagram of twisted bilayer graphene and demonstrate that qualitatively different results are obtained when long-ranged interactions are neglected. In particular, we use Hartree theory augmented with Hubbard interactions and calculate the interacting spin susceptibility at a range of doping levels and twist angles near the magic angle to identify the dominant magnetic instabilities. At the magic angle, mostly anti-ferromagnetic order is found, while ferromagnetism dominates at other twist angles. Moreover, long-ranged interactions significantly increase the twist angle window in which strong correlation phenomena can be expected. These findings are in good agreement with available experimental data.

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