Spin noise spectroscopy is emerging as a powerful technique for studying the dynamics of various spin systems also beyond their thermal equilibrium and linear response. Here, we study spin fluctuations of room-temperature neutral atoms in a Bell-Bloom type magnetometer. Driven by indirect pumping and undergoing a parametric excitation, this system is known to produce noise-squeezing. Our measurements not only reveal a strong asymmetry in the noise distribution of the atomic signal quadratures at the magnetic resonance, but also provide insight into the mechanism behind its generation and evolution. In particular, a structure in the spectrum is identified which allows to investigate the main dependencies and the characteristic timescales of the noise process. The results obtained are compatible with parametrically induced noise squeezing. Notably, the noise spectrum provides information on the spin dynamics even in regimes where the macroscopic atomic coherence is lost, effectively enhancing the sensitivity of the measurements. Our work promotes spin noise spectroscopy as a versatile technique for the study of noise squeezing in a wide range of spin based magnetic sensors.
With our all-atomic squeezing and filtering setup, we demonstrate control over the noise amplitudes and manipulation of the frequency-dependent squeezing angle of a squeezed vacuum quantum state by passing it through an atomic medium with electromagnetically induced transparency (EIT). We generate low sideband frequency squeezed vacuum using the polarization self-rotation effect in a hot Rb vapor cell, and input it into a second atomic vapor subject to EIT conditions. We use the frequency-dependent absorption of the EIT window to demonstrate an example of squeeze amplitude attenuation and sque…
Squeezed states of light have received renewed attention due to their applicability to quantum-enhanced sensing. To take full advantage of their reduced noise properties to enhance atomic-based sensors, it is necessary to generate narrowband near or on atomic resonance single-mode squeezed states of light. We have previously generated bright two-mode squeezed states of light, or twin beams, that can be tuned to resonance with the D1 line of $^{87}$Rb with a non-degenerate four-wave mixing (FWM) process in a double-lambda configuration in a $^{85}$Rb vapor cell. Here we report on the use of fee…
We measured the spin noise spectroscopy (SNS) of rubidium atomic ensemble with two different atomic vapor cells (filled with the buffer gases or coated with paraffin film on the inner wall), and demonstrated the enhancement of signal to noise ratio (SNR) by using of the polarization squeezed state (PSS) of 795 nm light field with Stokes operator S2 squeezed. PSS is prepared by locking the relative phase between the squeezed vacuum state of light obtained by a sub-threshold optical parametric oscillator and the orthogonal polarized local oscillator beam by means of the quantum noise lock. Under…
We investigate the prospects of using two-mode intensity squeezed twin-beams, generated in Rb vapor, to improve the sensitivity of spectroscopic measurements by engaging two-photon Raman transitions. As a proof of principle demonstration, we demonstrated the quantum-enhanced measurements of the Rb $5D_{3/2}$ hyperfine structure with reduced requirements for the Raman pump laser power and Rb vapor number density.
We report quantum enhancement of Faraday rotation spin noise spectroscopy by polarization squeezing of the probe beam. Using natural abundance Rb in 100 Torr of N_2 buffer gas, and squeezed light from a sub-threshold optical parametric oscillator stabilized 20 GHz to the blue of the D_1 resonance, we observe that an input squeezing of 3.0 dB improves the signal-to-noise ratio by 1.5 dB to 2.6 dB over the combined (power)$\otimes$(number density) ranges (0.5 mW to 4.0 mW )$\otimes$(1.5 x 10^{12} cm^{-3} to 1.3 x 10^{13} cm^{-3}), covering the ranges used in optimized spin noise spectroscopy exp…
With the help of Stokes operator S2 squeezed state (also called polarization squeezed state (PSS)) of 795-nm light, rubidium-87 (87Rb) atomic magnetometer based on Faraday rotation has been implemented and characterized.The PSS of Stokes operator S2 of 795-nm light has been prepared by means of coherently combining the polarization coherent state (PCS) of a linearly p-polarized bright 795-nm light beam and a linearly s-polarized squeezed vacuum state (SVS) generated by a 397.5-nm ultraviolet laser pumped sub-threshold optical parametric oscillator (OPO) with a PPKTP bulk crystal inside the OPO…
We investigate the prospect of enhancing the phase sensitivity of atom interferometers in the Mach-Zehnder configuration with squeezed light. Ultimately, this enhancement is achieved by transferring the quantum state of squeezed light to one or more of the atomic input beams, thereby allowing operation below the standard quantum limit. We analyze in detail three specific schemes that utilize (1) single-mode squeezed optical vacuum (i.e. low frequency squeezing), (2) two-mode squeezed optical vacuum (i.e. high frequency squeezing) transferred to both atomic inputs, and (3) two-mode squeezed opt…
The dynamics of the Jaynes-Cummings interaction of a two-level atom interacting with a single mode of the radiation field is investigated, as the state of the field is gradually changed from a coherent state to a squeezed coherent state. The effect of mild squeezing on the coherent light is shown to be striking: the photon number distribution gets localized and it peaks maximally for a particular value of squeezing. The atomic inversion retains its structure for a longer time. The mean linear entropy shows that the atom has a tendency to get disentangled from field within the collapse region a…
Quantum fluctuations of the electromagnetic vacuum are responsible for physical effects such as the Casimir force and the radiative decay of atoms, and set fundamental limits on the sensitivity of measurements. Entanglement between photons can produce correlations that result in a reduction of these fluctuations below the vacuum level allowing measurements that surpass the standard quantum limit in sensitivity. Here we demonstrate that the radiative decay rate of an atom that is coupled to quadrature squeezed electromagnetic vacuum can be reduced below its natural linewidth. We observe a two-f…
We investigated the propagation of a squeezed optical field, generated via the polarization self-rotation (PSR) effect, with a sinusoidally-modulated degree of squeezing through an atomic medium with anomalous dispersion. We observed the advancement of the signal propagating through a resonant Rb vapor compared to the reference signal, propagating in air. The measured advancement time grew linearly with atomic density, reaching a maximum of $11 \pm 1~μ$s, which corresponded to a negative group velocity of $v_g\approx - 7,000~$m/s. We also confirmed that the increasing advancement was accompani…
Building scalable quantum systems that demonstrate genuine performance enhancement based on entanglement is a major scientific goal for fields including computing, networking, simulations, and metrology. The tremendous challenge arises from the fragility of entanglement in increasingly larger sized quantum systems. Optical atomic clocks utilizing a large number of atoms have pushed the frontier of measurement science, building on precise engineering of quantum states and control of atomic interactions. However, today's state-of-the-art optical atomic clocks are limited by the quantum projectio…
We study a squeezed vacuum field generated in hot Rb vapor via the polarization self-rotation effect. Our previous experiments showed that the amount of observed squeezing may be limited by the contamination of the squeezed vacuum output with higher-order spatial modes, also generated inside the cell. Here, we demonstrate that the squeezing can be improved by making the light interact several times with a less dense atomic ensemble. With optimization of some parameters we can achieve up to -2.6 dB of squeezing in the multi-pass case, which is 0.6 dB improvement compared to the single-pass expe…
We have investigated the benefits of spin squeezed states for clocks operated with typical Brownian frequency noise-limited laser sources. Based on an analytic model of the closed servo-loop of an optical atomic clock, we can give quantitative predictions on the optimal clock stability for a given dead time and laser noise. Our analytic predictions are in very good agreement with numerical simulations of the closed servo-loop. We find that for usual cyclic Ramsey interrogation of single atomic ensembles with dead time, even with the current most stable lasers spin squeezing can only improve th…
As an "input" state of a linear (Mach-Zehnder or Ramsey) interferometer, the phase-squeezed state proposed by Berry and Wiseman exhibits the best sensitivity approaching to the Heisenberg limit [Phys. Rev. Lett. 85, 5098 (2000)]. In this paper, we find that it can be generated dynamically with atomic Bose-Einstein condensates confined in a symmetric double well. Similar with the Berry and Wiseman's state, the prepared states show the squeezing along spin operator S_y and the anti-squeezing along S_z, leading to a sub-shot-noise of the phase sensitivity.
The erbium atomic system is a promising candidate for an atomic Bose-Einstein condensate of atoms with a non-vanishing orbital angular momentum ($L \neq 0$) of the electronic ground state. In this paper we report on the frequency stabilization of a blue external cavity diode laser system on the 400.91 $nm$ laser cooling transition of atomic erbium. Doppler-free saturation spectroscopy is applied within a hollow cathode discharge tube to the corresponding electronic transition of several of the erbium isotopes. Using the technique of frequency modulation spectroscopy, a zero-crossing error sign…
We investigated the Autler-Townes splitting produced by microwave transitions between atomic Rydberg states explored by optical spectroscopy from the ground electronic state. The laser-atom Hamiltonian describing the double irradiation of such a multilevel system is analysed on the basis of the Morris-Shore transformation. The application of this transformation to the microwave-dressed atomic system allows the identification of bright, dark, and spectator states associated with different configurations of atomic states and microwave polarisation. We derived synthetic spectra that show the main…
A new approach to precise determination of atomic matrix elements is described whereby measurement of spectral locations of zeros in the Rayleigh scattering cross-section allows frequency-domain extraction of matrix elements in terms of a fiducial quantity. Illustrations are made for scattering off the ground state in Li and Cs.
The dynamics of spontaneous emission of an atomic system is studied in the framework of an open quantum system. The resulting quantum master equation for the atomic system is non hermitian. The generator $\mathcal{L}$ can possess non-hermitian degeneracies, i.e. exceptional points ($EP$), for specific values of the external laser driving amplitude and detuning from the atomic lines. We suggest to employ the special properties of these $EP$s for accurate parameter estimation. The method is demonstrated for the atomic spectrum of $S \rightarrow P$ transitions of $~^{85}$Rb and $~^{40}$Ca$~^+$.
Using squeezed states it is possible to surpass the standard quantum limit of measurement uncertainty by reducing the measurement uncertainty of one property at the expense of another complementary property. Squeezed states were first demonstrated in optical fields and later with ensembles of pseudo spin-1/2 atoms using non-linear atom-light interactions. Recently, collisional interactions in ultracold atomic gases have been used to generate a large degree of quadrature spin squeezing in two-component Bose condensates. For pseudo spin-1/2 systems, the complementary properties are the different…
We present a technique for simultaneous laser frequency stabilization on transitions of multiple atomic species with a single optical setup. The method is based on modulation transfer spectroscopy and the signals are separated by modulating at different frequencies and electronically filtered. As a proof of concept, we demonstrate simultaneous spectroscopy of the potassium D$_1$, D$_2$ and rubidium D$_2$ transitions. The technique can easily be extended to other atomic species and allows the development of versatile and compact frequency reference modules.
When the atoms of a dimer remain most of the time very far apart, in so-called long-range molecular states, their mutual interaction is ruled by plain atomic properties. The high-resolution spectroscopic study of some molecular excited states populated by photoassociation of cold atoms (photoassociative spectroscopy) gives a good illustration of this property. It provides accurate determinations of atomic radiative lifetimes, which are known to be sensitive tests for atomic calculations. A number of such analyses has been performed up to now, for all stable alkali atoms and for some other atom…
This article presents a review of the most recent theoretical and experimental results in hydrogen. We particularly emphasize the methods used to deduce the Rydberg constant $R_\infty$ and we consider the prospects for future improvements in the precision of $R_\infty$.
We present a method for recovery of narrow homogeneous spectral features out of broad inhomogeneous overlapped profile based on second-derivative processing of the absorption spectra of alkali metal atomic vapor nanocells. The method is shown to preserve the frequency positions and amplitudes of spectral transitions, thus being applicable for quantitative spectroscopy. The proposed technique was successfully applied and tested for: measurements of hyperfine splitting and atomic transition probabilities; development of an atomic frequency reference; determination of isotopic abundance; study of…
Frequency comb based multidimensional coherent spectroscopy is a novel optical method that enables high resolution measurement in a short acquisition time. The method's resolution makes multidimensional coherent spectroscopy relevant for atomic systems that have narrow resonances. We use double-quantum multidimensional coherent spectroscopy to reveal collective hyperfine resonances in rubidium vapor at 100 C induced by dipole-dipole interactions. We observe tilted lineshapes in the double-quantum 2D spectra, which has never been reported for Doppler-broadened systems. The tilted lineshapes sug…
We develop a method for extracting the physical parameters of interest for a dipole trapped cold atomic ensemble. This technique uses the spatially dependent ac-Stark shift of the trap itself to project the atomic distribution onto a light-shift broadened transmission spectrum. We develop a model that connects the atomic distribution with the expected transmission spectrum. We then demonstrate the utility of the technique by deriving the temperature, trap depth, lifetime, and trapped atom number from data that was taken in a single shot experimental measurement.
Direct frequency-comb spectroscopy is used to probe the absolute frequencies of $6S_{1/2}$-$8S_{1/2}$ two-photon transitions of atomic cesium in hot vapor environment. By utilizing the coherent control method of temporally splitting the laser spectrum above and below the two-photon resonance frequency, Doppler-free absorption is built in two spatially distinct locations and imaged for high-precision spectroscopy. Theoretical analysis finds that these transition lines are measured with uncertainty below $5\times10^{-10}$, mainly contributed from laser-induced AC Stark shift.
The atomic recoil effect leads to large (25 %) asymmetries in simple spectroscopic investigations of Ca atoms that have been laser-cooled to 10 microkelvin. Starting with spectra from the more familiar Doppler-broadened domain, we show how the fundamental asymmetry between absorption and stimulated emission of light manifests itself when shorter spectroscopic pulses lead to the Fourier transform regime. These effects occur on frequency scales much larger than the size of the recoil shift itself, and have not been observed before in saturation spectroscopy. These results are relevant to state-o…
The prospects of studying nonminimal operators for Lorentz violation using spectroscopy experiments with light atoms and muon spin-precession experiments are presented. Possible improvements on bounds on minimal and nonminimal operators for Lorentz violation are discussed.
Active Stark Atomic Spectroscopy (ASAS) method can be used to determine a high electric field in the diode of an ion or electron accelerator as a function of position and time, including the positions of anode and cathode plasma emission surfaces (in order to obtain the effective accelerating gap). As possible probe beams, we suggest the use of lithium and sodium atoms. The diagnostic provides a means to measure diode quantities spectroscopically with excellent spatial resolution.
We describe the operation of two GaN-based diode lasers for the laser spectroscopy of gallium at 403 nm and 417 nm. Their use in an external cavity configuration enabled the investigation of absorption spectroscopy in a gallium hollow cathode. We have analyzed the Doppler broadened profiles accounting for hyperfine and isotope structure and extracting both the temperature and densities of the neutral atomic sample produced in the glow discharge. We have also built a setup to produce a thermal atomic beam of gallium. Using the GaN-based diode lasers we have studied the laser induced fluorescenc…
Spectra of spin-forbidden and spin-allowed transitions in the mixed b$^3Π_u$ ~ A$^1Σ_u^+$ state of Na$_2$ are measured separately by two-photon excitation using a single tunable dye laser. The two-photon excitation produces Na*(3p) by photodissociation, which is easily and sensitively detected by atomic fluorescence. At low laser power, only the A$^1Σ_u^+$ state is excited, completely free of triplet excitation. At high laser power, photodissociation via the b$^3Π_u$ triplet state intermediate becomes much more likely, effectively "switching" the observations from singlet spectroscopy to tripl…
This paper addresses the three following questions. (i) How the structures of group and of chain of groups enter nuclear, atomic and molecular spectroscopy? (ii) How these structures can be exploited, in a quantum- mechanical framework, in the problems of state labelling and (external) symmetry breaking? (iii) How it is possible to associate a Wigner-Racah algebra to a group or a chain of groups for making easier the calculation of quantum-mechanical matrix elements? Numerous examples illustrate the philosophy of qualitative and quantitative applications to spectroscopy.
We explore the applications of spin noise spectroscopy (SNS) for detection of the spin properties of atomic ensembles in and out of equilibrium. In SNS, a linearly polarized far-detuned probe beam on passing through an ensemble of atomic spins acquires the information of the spin correlations of the system which is extracted using its time-resolved Faraday-rotation noise. We measure various atomic, magnetic and sub-atomic properties as well as perform precision magnetometry using SNS in rubidium atomic vapor in thermal equilibrium. Thereafter, we manipulate the relative spin populations betwee…
We describe an inexpensive instructional experiment that demonstrates the rotational energy levels of diatomic nitrogen, using the emission band spectrum of molecular nitrogen ionized by various processes in a commercial AC capillary discharge tube. The simple setup and analytical procedure is introduced as part of a sequence of educational experiments employed by a course of advanced atomic and molecular spectroscopy, where the study of rotational spectra is combined with the analysis of vibrational characteristics for a multifaceted picture of the quantum states of diatomic molecules.
