arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2011.14256cond-mat.str-elcond-mat.mtrl-sci
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CeRh $_6$ Ge $_4$中的电子结构

Pressure Dependent Electronic Structure in CeRh$_6$Ge$_4$

Chao Cao, Jian-Xin Zhu

摘要:

本文利用最新的动力学平均场论和密度泛函理论方法,对铁磁量子临界材料候选体CeRh $_6$ Ge $_4$的电子结构随温度和压力的变化进行了系统的研究。在-3.9 GPa和-8.3 GPa下,Ce-4 $f$占据变化、局域磁化率和低频电子自能行为表明Ce-4 $f$电子处于定域态;而在6.5 GPa和13.1 GPa下,这些量表明Ce-4 $f$电子处于巡游态。当释放外部压力时,与相干近藤屏蔽相关的特征温度逐渐被抑制到约0.8 GPa,指示局部量子临界点。有趣的是,动量分辨谱函数表明,即使在局域态侧,Ce-4 $f$和传导电子之间的高度各向异性的$\mathbf{k}$依赖的杂化仍然沿着$Γ$ -A存在,导致其间的杂化间隙。计算结果表明,在局域矩侧有8个费米面片,在近藤相干态有6个费米面片。最后,在0.8 GPa的自能可以很好地拟合的边缘费米液体形式,产生线性温度依赖的电阻率。

英文摘要:

Using the state-of-art dynamical mean-field theory combined with density functional theory method, we have performed systematic study on the temperature and pressure dependent electronic structure of ferromagnetic quantum critical material candidate CeRh$_6$Ge$_4$. At -3.9 GPa and -8.3 GPa, the Ce-4$f$ occupation variation, the local magnetic susceptibility, and the low-frequency electronic self-energy behaviors suggest the Ce-4$f$ electrons are in the localized state; whereas at 6.5 GPa and 13.1 GPa, these quantities indicate the Ce-4$f$ electrons are in the itinerant state. The characteristic temperatures associated with the coherent Kondo screening is gradually suppressed to 0 around 0.8 GPa upon releasing external pressure, indicative of a local quantum critical point. Interestingly, the momentum-resolved spectrum function shows that even at the localized state side, highly anisotropic $\mathbf{k}$-dependent hybridization between Ce-4$f$ and conduction electrons is still present along $Γ$-A, causing hybridization gap in between. The calculations predict 8 Fermi surface sheets at the local-moment side and 6 sheets at the Kondo coherent state. Finally, the self-energy at 0.8 GPa can be well fitted by marginal Fermi-liquid form, giving rise to a linearly temperature dependent resistivity.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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