Optical spectrometers are the central instruments for exploring the interaction between light and matter. The current pursuit of the field is to design a spectrometer without the need for wavelength multiplexing optics to effectively reduce the complexity and physical size of the hardware. Based on computational spectroscopic results and combining a broadband-responsive dynamic detector, we successfully demonstrate an optics-free single-detector spectrometer that maps the tunable quantum efficiency of a superconducting nanowire into an ill-conditioned matrix to build a solvable inverse mathematical equation. Such a spectrometer can realize a broadband spectral responsivity ranging from 660 to 1900 nm. The spectral resolution at the telecom is 6 nm, exceeding the energy resolving capacity of existing infrared single-photon detectors. Meanwhile, benefiting from the optics-free setup, precise time-of-flight measurements can be simultaneously achieved. We have demonstrated a spectral LiDAR with 8 spectral channels. This work provides a concise method for building multifunctional spectrometers and paves the way for applying superconducting nanowire detectors in spectroscopy.
Single-photon counters are single-pixel binary devices that click upon the absorption of a photon but obscure its spectral information, whereas resolving the colour of detected photons has been in critical demand for frontier astronomical observation, spectroscopic imaging and wavelength division multiplexed quantum communications. Current implementations of single-photon spectrometers either consist of bulky wavelength-scanning components or have limited detection channels, preventing parallel detection of broadband single photons with high spectral resolutions. Here, we present the first bro…
Recent advancements in silicon photonics are enabling the development of chip-scale photonics devices for sensing and signal processing applications, among which on-chip spectrometers are of particular interest for precision wavelength monitoring and related applications. Most chip-scale spectrometers suffer from a resolution-bandwidth trade-off, thus limiting the uses of the device. Here we report on a novel passive, chip-scale, hybrid speckle-enhanced Fourier transform device that exhibits a two order-of-magnitude improvement in finesse (bandwidth/resolution) over the state-of-the art chip-s…
A general-purpose all-fiber spectrometer is demonstrated to overcome the trade-off between spectral resolution and bandwidth. By integrating a wavelength division multiplexer with five multimode optical fibers, we have achieved 100 nm bandwidth with 0.03 nm resolution at wavelength 1500 nm. An efficient algorithm is developed to reconstruct the spectrum from the speckle pattern produced by interference of guided modes in the multimode fibers. Such algorithm enables a rapid, accurate reconstruction of both sparse and dense spectra in the presence of noise.
Optical cavities provide high sensitivity to dispersion since their resonance frequencies depend on the index of refraction. We present a direct, broadband, and accurate measurement of the modes of a high finesse cavity using an optical frequency comb and a mechanical Fourier transform spectrometer with a kHz-level resolution. We characterize 16000 cavity modes spanning 16 THz of bandwidth in terms of center frequency, linewidth, and amplitude. We retrieve the group delay dispersion of the cavity mirror coatings and pure N${_2}$ with 0.1 fs${^2}$ precision and 1 fs${^2}$ accuracy, as well as t…
We present a 100 kHz broadband vibrational sum-frequency generation (VSFG) spectrometer operating in the 5.5-10.5 $μ$m (950-1750 cm$^{-1}$) wavelength range. The mid-infrared beam of the system is obtained from a collinear, type-I LiGaS$_{2}$ crystal based optical parametric amplifier seeded by a supercontinuum and pumped directly by 180 fs, ~32 $μ$J, 1.03 $μ$m pulses from an Yb:KGd(WO$_{4}$)$_{2}$ laser system. Up to 0.5 $μ$J mid-infrared pulses with durations below 100 fs were obtained after dispersion compensation utilizing bulk materials. We demonstrate the utility of the spectrometer by r…
We propose the inverse design of ultracompact, broadband focusing spectrometers based on adaptive deep diffractive neural networks (a-D$^2$NNs). Specifically, we introduce and characterize two-layer diffractive devices with engineered angular dispersion that focus and steer broadband incident radiation along predefined focal trajectories with desired bandwidth and $5$ nm spectral resolution. Moreover, we systematically study the focusing efficiency of two-layer devices with side length $L=100~μ\mathrm{m}$ and focal length $f=300~\,μ\mathrm{m}$ across the visible spectrum and we demonstrate acc…
We present an asymmetric bifacial graphene metasurface to realize tunable and broadband coherent perfect absorption (CPA) at terahertz (THz) frequencies. The proposed design is composed of two dissimilar graphene square patch metasurfaces stacked over an ultrathin dielectric substrate. Nonlinear CPA performance without resorting to optical nonlinearities and amplification are demonstrated based on wave interference phenomena taking place along and inside this subwavelength structure. Broadband asymmetric reflection from opposite directions is obtained in the case of single wave illumination. T…
We propose the use of silicon graphene waveguides to implement a tunable broadband microwave photonics phase shifte based on integrated ring cavities. Numerical computation results show the feasibility for broadband operation over 40 GHz bandwidth and full 360 degree radiofrequency phase-shift with a modest voltage excursion of 0.12 volt.
A commercial single laser line Raman spectrometer is modified to accommodate multiline and tunable dye lasers, thus combining the high sensitivity of such single monochromator systems with broadband operation. Such instruments rely on high-throughput interference filters that perform both beam alignment and Rayleigh filtering. Our setup separates the dual task of the built-in monochromator into two independent elements: a beam splitter and a long pass filter. Filter rotation shifts the transmission passband, effectively expanding the range of operation. Rotation of the filters has a negligible…
We present and characterize a 2-D imaging spectrometer based on a virtually-imaged phased array (VIPA) disperser for rapid, high-resolution molecular detection using mid-infrared (MIR) frequency combs at 3.1 and 3.8 μm. We demonstrate detection of CH4 at 3.1 μm with >3750 resolution elements spanning >80 nm with ~600 MHz resolution in a <10 μs acquisition time. In addition to broadband detection, rapid, time-resolved single-image detection is demonstrated by capturing dynamic concentration changes of CH4 at a rate of ~375 frames per second. Changes in absorption above the noise floor of 5\time…
The development of optical fibers has revolutionized telecommunications by enabling long-distance broad-band transmission with minimal loss. In turn, the ubiquity of high-quality low-cost fibers enabled a number of additional applications, including fiber sensors, fiber lasers, and imaging fiber bundles. Recently, we showed that a mutlimode optical fiber can also function as a spectrometer by measuring the wavelength-dependent speckle pattern formed by interference between the guided modes. Here, we reach a record resolution of 1 pm at wavelength 1500 nm using a 100 meter long multimode fiber,…
We experimentally demonstrate a simple method to measure the biphoton joint spectrum by mapping the spectral information onto the temporal domain using a dispersive medium. Various top-hat spectral filters are used to limit the spectral (and hence, temporal) extent of the broadband downconversion photons measured. The sharp edges of the spectral filters are utilized as spectral markers for dispersion characterization of the dispersive medium. This method allows dispersion characterization and joint spectral measurement to be completed simultaneously. The joint spectrum (which extends beyond 10…
A simple scheme for a broadband polarization rotator with tunable rotation angle is proposed and verified experimentally. The rotator consists of only three wave-plates, one of which is a full-wave plate. The robust approach inspired by the composite pulses analogy allows to compensate the wave-plate dispersion in large extent.
We describe a tunable broadband mid-infrared laser source based on difference-frequency mixing of a 100 MHz femtosecond Yb:fiber laser oscillator and a Raman-shifted soliton generated with the same laser. The resulting light is tunable over 3.0 um to 4.4 um, with a FWHM bandwidth of 170 nm and maximum average output power up to 125 mW. The noise and coherence properties of this source are also investigated and described.
Dual-frequency comb spectroscopy has emerged as a disruptive technique for measuring wide-spanning spectra with high resolution, yielding a particularly powerful technique for sensitive multi-component gas analysis. We present a spectrometer system based on dual electro-optical combs with subsequent conversion to the mid-infrared via tunable difference frequency generation, operating in the range from 3 to 4.7 $μ$m. The simultaneously recorded bandwidth is up to 454(1) GHz and a signal-to-noise ratio of 7.3(2) x 10$^2$ Hz$^{-1/2}$ can be reached. The conversion preserves the coherence of the d…
Aligned, densely-packed carbon nanotube metamaterials prepared using vacuum filtration are an emerging infrared nanophotonic material. We report multiple hyperbolic plasmon resonances, together spanning the mid-infrared, in individual resonators made from aligned and densely-packed carbon nanotubes. In the first near-field scanning optical microscopy (NSOM) imaging study of nanotube metamaterial resonators, we observe distinct deeply-subwavelength field profiles at the fundamental and higher-order resonant frequencies. The wafer-scale area of the nanotube metamaterials allows us to combine thi…
The on-chip broadband optical spectrometers which cover the entire tissue transparency window (λ=650-1050 nm) with high resolution are highly demanded for the miniaturized bio-sensing and bio-imaging applications. Here, we propose a novel type of spatial heterodyne Fourier transform spectrometer (SHFTS) integrated with a sub-wavelength grating coupler (SWGC) for the dual-polarization bandpass sampling on the Si3N4 platform. Through tuning the coupling angles with different polarization, we experimentally demonstrated the unprecedented broadband spectrum retrieval results with the overall bandw…
We propose and design an ultra-compact and broadband tunable multimode interference (MMI) splitter in mid-infrared based on graphene plasmonic waveguides. The size of the device is only 0.56μm*1.2μm, which corresponds to device area of only about 0.014λ^2, where λ is the vacuum wavelength. And the center wavelength of the device can be tuned in a broad band from 7μm to 9μm with the Fermi level of graphene varied from 0.5eV to 1eV. Furthermore, the device is easy to be fabricated on chip.
Up-to-date network telemetry is the key enabler for resource optimization by capacity scaling, fault recovery, and network reconfiguration among other means. Reliable optical performance monitoring in general and, specifically, the monitoring of the spectral profile of WDM signals in fixed- and flex- grid architectures across the entire C-band, remains challenging. This article describes a two-stage spectrometer architecture amenable to integration on a single chip that can measure quantitatively the spectrum across the entire C-band with a resolution of 1 GHz approximately. The first stage co…
We have developed an angle-resolved photoemission spectrometer with tunable VUV laser as a photon source. The photon source is based on the fourth harmonic generation of a near IR beam from a Ti:sapphire laser pumped by a CW green laser and tunable between 5.3eV and 7eV. The most important part of the set-up is a compact, vacuum enclosed fourth harmonic generator based on KBBF crystals, grown hydrothermally in the US. This source can deliver a photon flux of over 10^14 photons/s. We demonstrate that this energy range is sufficient to measure the kz dispersion in an iron arsenic high temperatur…
Designing broadband enhanced chirality is of strong interest to the emerging fields of chiral chemistry and sensing, or to control the spin orbital momentum of photons in recently introduced nanophotonic chiral quantum and classical optical applications. However, chiral light-matter interactions have an extremely weak nature, are difficult to be controlled and enhanced, and cannot be made tunable or broadband. In addition, planar ultrathin nanophotonic structures to achieve strong, broadband, and tunable chirality at the technologically important visible to ultraviolet spectrum still remain el…
We demonstrate an RF photonic fractional Hilbert transformer based on an integrated Kerr micro-comb source featuring a record low free spectral range of 48.9 GHz, yielding 75 microcomb lines across the C-band. By programming and shaping the comb lines according to calculated tap weights, we demonstrate that the Hilbert transformer can achieve tunable bandwidths ranging from 1.2 to 15.3 GHz, switchable centre frequencies from baseband to 9.5 GHz, and arbitrary fractional orders. We experimentally characterize the RF amplitude and phase response of the tunable bandpass and lowpass Hilbert transf…
We report on a giant Faraday effect in an electron plasma in n-InSb probed via polarization-resolved terahertz (THz) time-domain spectroscopy. Polarization rotation angles and ellipticities reach as large as π/2 and 1, respectively, over a wide frequency range (0.3-2.5 THz) at magnetic fields of a few Tesla. The experimental results together with theoretical simulations show its promising ability to construct broadband and tunable THz polarization optics, such as a circular polarizer, half-wave plate, and polarization modulators.
The quest for extrasolar planets and their characterisation as well as studies of fundamental physics on cosmological scales rely on capabilities of high-resolution astronomical spectroscopy. A central requirement is a precise wavelength calibration of astronomical spectrographs allowing for extraction of subtle wavelength shifts from the spectra of stars and quasars. Here, we present an all-fibre, 400 nm wide near-infrared frequency comb based on electro-optic modulation with 14.5 GHz comb line spacing. Tests on the high-resolution, near-infrared spectrometer GIANO-B show a photon-noise limit…
By using the formal analogy between the evolution of the state vector in quantum mechanics and the Jones vector in polarization optics, we construct and demonstrate experimentally efficient broadband half-wave polarization retarders and tunable narrowband polarization filters. Both the broadband retarders and the filters are constructed by the same set of stacked standard multi-order optical wave plates rotated at different angles with respect to their fast polarization axes: for a certain set of angles this device behaves as a broadband polarization retarder while for another set of angles it…
Graphene is an ideal material for integrated nonlinear optics thanks to its strong light-matter interaction and large nonlinear optical susceptibility. Graphene has been used in optical modulators, saturable absorbers, nonlinear frequency converters, and broadband light emitters. For the latter application, a key requirement is the ability to control and engineer the emission wavelength and bandwidth, as well as the electronic temperature of graphene. Here, we demonstrate that the emission wavelength of graphene$'$ s broadband hot carrier photoluminescence can be tuned by integration on photon…
In this work, we report on the preparation of an ultra-broadband continuously-tunable, highly polarization-entangled photon-pair source covering the C+L telecom bands using a single type-II phase-matched bulk PPKTP crystal. Over 60 nm turning band of the down-converted photons is achieved experimentally. The broad tuning ability is due to operating near an extended phase match point in this crystal. The S parameter value of CHSH inequality is in the range between 2.60+/-0.04 (minimum) and 2.72+/-0.07 (maximum), which clearly demonstrates the high entanglement of the source over the whole tunab…
Black phosphorus (BP), a relative new plasmonic two-dimensional (2D) material, offers unique photonic and electronic properties. In this work, we propose a new tunable and broadband ultrathin coherent perfect absorber (CPA) device operating in the terahertz (THz) frequency range. It is based on a bifacial metasurface made of BP patch periodic arrays separated by a thin dielectric layer. Broadband CPA bandwidth is realized due to the ultrathin thickness of the proposed device and the extraordinary properties of BP. In addition, a substantial modulation between CPA and complete transparency is a…
Time-dependent nonlinear media, such as rapidly generated plasmas produced via laser ionization of gases, can increase the energy of individual laser photons and generate tunable high-order harmonic pulses. This phenomenon, known as photon acceleration, has traditionally required extreme-intensity laser pulses and macroscopic propagation lengths. Here, we report on a novel nonlinear material$-$an ultrathin semiconductor metasurface$-$that exhibits efficient photon acceleration at low intensities. We observe a signature nonlinear manifestation of photon acceleration: third-harmonic generation o…
We present optically tunable magnetic 3D metamaterials at terahertz (THz) frequencies which exhibit a tuning range of ~30% of the resonance frequency. This is accomplished by fabricating 3D array structures consisting of double-split-ring resonators (DSRRs) on silicon-on-sapphire, fabricated using multilayer electroplating. Photoexcitation of free carriers in the silicon within the capacitive region of the DSRR results in a red-shift of the resonant frequency from 1.74 THz to 1.16 THz. The observed frequency shift leads to a transition from a magnetic-to-bianisotropic response as verified thro…
Tunable metasurfaces provide a compact and efficient strategy for optical components that require active wavefront shaping. Varifocal metalens is one of the most important applications. However, the existing tunable metalens rarely serves broadband wavelengths restricting their applications in broadband imaging and color display due to chromatic aberration. Herein, we demonstrate an electrically tunable polarization-multiplexed varifocal achromatic dielectric metalens integrated with twisted nematic liquid crystals (TNLCs) in the visible region. The phase profiles at different wavelengths unde…
Dual comb spectroscopy (DCS) is a broadband technique offering high resolution and fast data acquisition. We describe a hybrid dual comb spectrometer comprising a broadband commercial fiber laser system offering a wide range of sample interrogation, and an actively mode locked semiconductor laser (MLL) having a widely tunable, relatively narrow spectrum. The mutual coherence over 100 seconds has been realized between the two combs. We employed the DCS system to characterize the absorption spectrum of rubidium atoms at 313 K with a high signal to noise ratio. The broadband laser is directly loc…
We integrate about 100 single Cadmium Selenide semiconductor nanowires in self-standing Silicon Nitride photonic crystal cavities in a single processing run. Room temperature measurements reveal a single narrow emission linewidth, corresponding to a Q-factor as large as 5000. By varying the structural parameters of the photonic crystal, the peak wavelength is tuned, thereby covering the entire emission spectral range of the active material. A very large spectral range could be covered by heterogeneous integration of different active materials.
The concept of `flat optics' is quickly conquering different fields of photonics, but its implementation in quantum optics is still at infancy. In particular, polarization entanglement, which is central to quantum photonics due to the simplicity of polarization qubit encoding and control, is so far not realized on flat platforms. Meanwhile, relaxed phase matching of flat nonlinear optical sources enables enormous freedom in tailoring their polarization properties. Here we use this freedom to generate photon pairs with tunable polarization entanglement via spontaneous parametric down-conversion…
East China Normal University（华东师范大学）；Chongqing Institute of East China Normal University（华东师范大学重庆研究院）；Shanxi University（山西大学）；Shanghai University（上海大学）
Flexible manipulation of terahertz-wave polarization during the generation process is very important for terahertz applications, especially for the next-generation on-chip functional terahertz sources. However, current terahertz emitters could not satisfy such demand, hence calling for new mechanism and conceptually new terahertz source. Here we demonstrate a magnetic-field-controlled, highly-efficient, cost-effective, and broadband terahertz source with flexible switch of terahertz polarization states in ferromagnetic heterostructures driven by femtosecond laser pulses. We verify that the chi…
A metamaterial composed of thin metallic strips as an efficient broadband absorber in the mid-infrared spectrum is investigated. Here the matching between dielectric and geometrical properties of the individual elements is critical to ensure high absorption. Detailed theoretical analysis based on the electric dipole approximation is performed to characterize the absorption and scattering properties of the individual elements of the unit cell and the results are used to design the metamaterial composed of such configurations. The absorption cross-section of a strip-shaped element can exceed its…
Calibration-Free Broadband Reconstructive Spectrometer based on Conical Phase Modulation
College of Advanced Interdisciplinary Studies, National University of Defense Technology（国防科技大学前沿交叉学院）；Nanhu Laser Laboratory, National University of Defense Technology（国防科技大学南湖激光实验室）；Hunan Provincial Key Laboratory of High Energy Laser Technology, National University of Defense Technology（国防科技大学湖南省高能激光技术重点实验室）
We experimentally demonstrate an efficient broadband second harmonic generation process with tunable mode-locked Ti: sapphire oscillator. We have achieved a robust broadband and efficient flat conversion of more than 35nm wavelength, by designing an adiabatic aperiodically poled potassium titanyl phosphate (KTP) crystal. Moreover, we have shown that with such efficient flat conversion, we can shape and control broadband second harmonic pulses. More specifically, we assign spectral-phase of abs-value and π-step, which allows wavelength tunable intense pump-probe and amplitude modulation of the …
Broadband THz spectroscopy system beyond 25 THz using BNA crystals and a tunable single-ring-fiber compressor
University of Ottawa（渥太华大学）；Max Planck Institute for the Science of Light（马克斯·普朗克光科学研究所）；University of Erlangen-Nürnberg（埃尔朗根-纽伦堡大学）；National Research Council Canada（加拿大国家研究委员会）
Non-Hermitian exceptional points (EPs) represent a special type of degeneracy where not only the eigenvalues coalesce, but also the eigenstates tend to collapse on each other. Recent studies have shown that in the presence of an EP, light-matter interactions are profoundly modified, leading to a host of novel optical phenomena ranging from enhanced sensitivity to chiral light transport. As of now, however, in order to stabilize a system at the vicinity of an exceptional point, its related parameters must be carefully tuned and/or continuously controlled. To overcome this limitation, here we in…
Broadband tunable microwave photonic radar for simultaneous detection of human respiration, heartbeat, and speech with deep learning-based speech recognition
