Broadband Tunable Photon-Pair Generation and Spectrum Measurement Based on Noncritical Lithium Niobate Crystals
University of Science and Technology of China（中国科学技术大学）；CAS Center for Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China（中国科学院量子信息与量子物理学前沿卓越创新中心）；Anhui Province Key Laboratory of Quantum Network, University of Science and Technology of China（安徽省量子通信重点实验室）；Anhui Kunteng Quantum Technology Co. Ltd.（安徽昆腾量子技术有限公司）
Photon pairs play a vital role in modern science, driving extensive research into their generation. Yet, the narrow phase-matching bandwidth of conventional crystals has largely confined studies to specific wavelengths, leaving research on broadband tunable sources underexplored. Here, we employ a non-critical phase-matched lithium niobate (LN) crystal to generate widely tunable photon pairs. The generated near-infrared (NIR) photon pairs exhibit a high coincidence-to-accidental ratio (CAR > 20 dB) and are tunable across the 800-1600 nm range. We further showcase the utility of NIR photon pairs in spectroscopy by detecting carbon monoxide (CO) gas absorption. This approach will facilitate the design of advanced LN-based photonic experiments.
Lithium niobate is a multi-functional material, which has been regarded as one of the most promising platform for the multi-purpose optical components and photonic circuits. Targeting at the miniature optical components and systems, lithium niobate microstructures with feature sizes of several to hundreds of micrometers have been demonstrated, such as waveguides, photonic crystals, micro-cavities, and modulators, et al. In this paper, we presented subwavelength nanograting metasurfaces fabricated in a crystalline lithium niobate film, which hold the possibilities towards further shrinking the …
We demonstrate second harmonic generation of blue light on an integrated thin-film lithium niobate waveguide and observe a conversion efficiency of $η_0= 33000\%/\text{W-cm}^2$, significantly exceeding previous demonstrations.
Lithium Niobate (LN or just niobate) thin-film micro-photonic resonators have promising prospects in many applications including high efficiency electro-optic modulators, optomechanics and nonlinear optics. This paper presents free-standing thin-film lithium niobate photonic resonators on a silicon platform using MEMS fabrication technology. We fabricated a 35um radius niobate disk resonator that exhibits high intrinsic optical quality factor (Q) of 484,000. Exploiting the optomechanical interaction from the released free-standing structure and high optical Q, we were able to demonstrate acous…
In this paper, we proposed and numerically demonstrated a giant enhancement up to 108 in both forward and backward propagation of the Second Harmonic Generation by combining the high-quality factor cavities of the Bound States in the Continuum and the excellent nonlinear optical crystal of lithium niobate. The enhancement factor is defined as the ratio of the second harmonic signal generated by the structure (lithium niobate membrane with Si grating) divided by the signal generated by lithium niobate membrane alone. Furthermore, a minimum interaction time of 350 ps is achieved despite the etch…
We demonstrate efficient multicycle terahertz pulse generation at 14.6 THz from large-area lithium niobate crystals by using high-energy (up to 2 J) femtosecond Ti:sapphire laser pulses. Such terahertz radiation is produced by phase-matched optical rectification in lithium niobate. Experimentally, we achieve maximal terahertz energy of 0.71 mJ with conversion efficiency of $\sim$0.04%. We also find that the effective interaction length for optimal terahertz conversion is fundamentally limited by terahertz absorption, laser pulse stretching by material dispersion, and terahertz-induced nonlinea…
Thin-film lithium niobate is an attractive integrated photonics platform due to its low optical loss and favorable optical nonlinear and electro-optic properties. However, in applications such as second harmonic generation, frequency comb generation, and microwave-to-optics conversion, the device performance is strongly impeded by the photorefractive effect inherent in thin-films. In this paper, we show that the dielectric cladding on lithium niobate microring resonator has a significant influence on the photorefractive effect. By removing the dielectric cladding layer, the photorefractive eff…
Lithium niobate on insulator (LNOI) waveguides, as an emerging technology, have proven to offer a promising platform for integrated optics, due to their strong optical confinement comparable to silicon on insulator (SOI) waveguides, while possessing the versatile properties of lithium niobate, such as high electro-optic coefficients. In this paper, we show that mode hybridization, a phenomenon widely found in vertically asymmetric waveguides, can be efficiently modulated in an LNOI ridge waveguide by electro-optic effect, leading to a polarization mode converter with 97% efficiency. Moreover, …
High quality lithium niobate thin film microresonators provide an ideal platform for on-chip nonlinear optics applications. However, the phase matching condition for efficient parametric process sets a high requirement for fabrication control. Here we demonstrate a photonic molecular structure composed of two strongly coupled lithium niobate microdisks of different diameters fabricated using femtosecond laser micromachining and focused ion beam milling. With a continuous wave excitation, rich nonlinear optical processes including cascaded four-wave mixing and stimulated Raman scattering were o…
In this paper, by cascading several bichromatic photonic crystals we demonstrate that the quality factor can be much larger compared with that in an isolated cavity without increasing the total size of the device. We take lithium niobate photonic crystal as an example to illustrate that the simulated quality factor of the cascaded cavity can attain 10^5 with a 70° slant angle, which is an order of magnitude larger than that in isolated cavity. The device can be fabricated easily by current etching technique for lithium niobate. We have fabricated the proposed device experimentally including ho…
Much progress, both experimentally and theoretically, has recently been made towards optical frequency comb generation from continuously pumped second-order nonlinear systems. Here, we present the first observations towards finding an integrated solution for such a system, using a titanium indiffused lithium niobate waveguide resonator. These results are compared to recently developed theory for equivalent systems. The system is seen to exhibit strong instabilities, which require further investigation in order to fully determine the suitability of this platform for stable optical frequency com…
We report intracavity Bragg scattering induced by photorefractive (PR) effect in high-Q lithium niobate (LN) ring resonators at cryogenic temperatures. We show that, when a cavity mode is strongly excited, the PR effect imprints a long-lived periodic space-charge field. This residual field in turn creates a refractive index modulation pattern that dramatically enhances the back scattering of an incoming probe light, and results in selective and reconfigurable mode splittings. This PR-induced Bragg scattering effect, despite being undesired for many applications, could be utilized to enable opt…
We demonstrate coherent supercontinuum generation (SCG) in a monolithically integrated lithium-niobate waveguide, under the presence of second- and third-order nonlinear effects. We achieve more than two octaves of optical bandwidth in a 0.5-cm-long waveguide with 100-picojoule-level pulses. Dispersion engineering of the waveguide allows for spectral overlap between the SCG and the second harmonic which enables direct detection of the carrier-envelope offset frequency fCEO using a single waveguide. We measure the fCEO of our femtosecond pump source with a 30-dB signal-to-noise ratio.
Monolithic integration of a high-quality factor lithium niobate microresonator with a free-standing membrane waveguide using femtosecond laser assisted ion beam writing (FLAIBW)
Tunable light sources are a key enabling technology for many applications such as ranging, spectroscopy, optical coherence tomography, digital imaging and interferometry. For miniaturized laser devices, whispering gallery resonator lasers are a well-suited platform, offering low thresholds and small linewidths, however, many realizations suffer from the lack of reliable tuning. Rare-earth ion-doped lithium niobate offers a way to solve this issue. Here we present a single-frequency laser based on a neodymium-doped lithium niobate whispering gallery mode resonator that is tuned via the linear e…
In this paper, we have investigated the interplay between the second and third-order nonlinearities in lithium-niobate waveguides with strong waveguide dispersion using uniform and linearly-chirped poling patterns at input powers in the pico-joule range. We have implemented the accurate unidirectional pulse propagation model to take into account all the possible nonlinear interactions inside these structures. In particular, the poling period has been designed to quasi-phase-match single and multiple sum- and difference-frequency generation processes. We have shown how the poling period can be …
Systematic Analysis of Ferroelectric Domain Dynamics in Periodically Poled Lithium Niobate Waveguides Using Two-Photon Microscopy and Digital Imaging Processing
Phase Sensitive Innovations Inc（Phase Sensitive Innovations 公司）；University of Delaware（特拉华大学）
Thin-film lithium niobate (TFLN) is an emerging platform for compact, low-power nonlinear-optical devices, and has been used extensively for near-infrared frequency conversion. Recent work has extended these devices to mid-infrared wavelengths, where broadly tunable sources may be used for chemical sensing. To this end, we demonstrate efficient and broadband difference frequency generation between a fixed 1-micron pump and a tunable telecom source in uniformly-poled TFLN-on-sapphire by harnessing the dispersion-engineering available in tightly-confining waveguides. We show a simultaneous 1-2 o…
Temporal cloaks have inspired the innovation of research on security and efficiency of quantum and fiber communications for concealing temporal events. The existing temporal cloaking approaches possessing ps ~ns cloaking windows employed the third-order nonlinearity mostly. Here we explore a temporal cloak for perpetually concealing pulse events using high efficiency second-order nonlinearity. A temporal pulse event was cloaked as a continuous wave with constant intensity and restored by polarization dependent sum frequency generation processes between the continuous wave and probe. The variet…
We report an on-chip single mode microlaser with low-threshold fabricated on Erbium doped lithium niobate on insulator (LNOI). The single mode laser emission at 1550.5 nm wavelength is generated in a coupled photonic molecule, which is facilitated by Vernier effect when pumping the photonic molecule at 970 nm. A threshold pump power as low as 200 uW is demonstrated thanks to the high quality factor above 10^6. Moreover, the linewidth of the microlaser reaches 4 kHz, which is the best result in LNOI microlasers. Such single mode micro-laser lithographically fabricated on chip is highly in deman…
The capability to modulate the intensity of an optical beam has scientific and practical significance. In this work, we demonstrate Y-Z cut lithium niobate acousto-optic modulators with record-high modulation efficiency, requiring only $1.5~\text{W}/\text{cm}^2$ for 100% modulation at 7 MHz. These modulators use a simple fabrication process; coating the top and bottom surfaces of a thin lithium niobate wafer with transparent electrodes. The fundamental shear acoustic mode of the wafer is excited through the transparent electrodes by applying voltage with frequency corresponding to the resonant…
Many applications of metasurfaces require an ability to dynamically change their properties in time domain. Electrical tuning techniques are of particular interest, since they pave a way to on-chip integration of metasurfaces with optoelectronic devices. In this work, we propose and experimentally demonstrate an electro-optic lithium niobate (EO-LN) metasurface that shows dynamic modulations to phase retardation of transmitted light. Quasi-bound states in the continuum (QBIC) are observed from our metasurface. And by applying external electric voltages, the refractive index of the LN is change…
Using an affordable ytterbium laser with sub-mJ of energy combined with a novel pulse compression technique, we demonstrate an extremely competitive state-of-the-art terahertz (THz) source with 53 mW of average power and 310 kV/cm at focus from the tilted-pulse front pumping scheme in lithium niobate at room temperature. Key points of this demonstration include the use of a pump pulse duration of 280 fs in combination with an echelon mirror. Our results present unmatched combined characteristics and are highly competitive with the existing THz sources pumped at the mJ range. This demonstration…
Thin-film lithium niobate on insulator (LNOI) has emerged as a superior integrated-photonics platform for linear, nonlinear, and electro-optics. Here we combine quasi-phase-matching, dispersion engineering, and tight mode confinement to realize nonlinear parametric processes with both high efficiency and wide wavelength tunability. On a millimeter-long, Z-cut LNOI waveguide, we demonstrate ultra-efficient ($1900\pm500 \% $W$^{-1}$cm$^{-2}$) and highly tunable (-1.71 nm/K) second-harmonic generation from 1530 to 1583 nm by type-0 quasi-phase-matching. Our technique is applicable to optical harm…
