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arXiv 2403.04590physics.optics
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多畴x切铌酸锂钽酸锂混晶中的近表面畴工程

Surface-near domain engineering in multi-domain x-cut lithium niobate tantalate mixed crystals

Laura Bollmers, Tobias Babai-Hemati, Boris Koppitz, Christof Eigner, Laura Padberg, Michael Ruesing, Lukas M. Eng, Christine Silberhorn

AI总结:

该研究通过电场极化和光刻结构化电极,在x切铌酸锂钽酸锂混晶中实现了近表面周期性极化,解决了畴反转受阻问题,为其非线性光学应用奠定基础。

摘要:

铌酸锂和钽酸锂是非线性集成光子学中最常用的材料。具有任意Nb-Ta比例的混晶为调节材料特性(如双折射)提供了新的自由度,同时结合了单一化合物的优势,例如将钽酸锂的热稳定性与铌酸锂更大的非线性或压电常数相结合。周期性极化是任何非线性光学应用的先决条件。对于混晶,由于缺乏均匀的单畴晶体,严重阻碍了畴生长和成核,迄今为止这仍是一个挑战。在这项工作中,我们证明了通过电场极化和光刻结构化电极,可以在x切铌酸锂钽酸锂混晶上实现近表面(深度<1 μm)的周期性极化。我们发现,生长态晶体中自然存在的头对头或尾对尾畴壁会阻碍更大尺度的畴反转。然而,如果极化电极之间的间隙尺寸与自然存在畴的平均尺寸处于相同数量级或更小,则周期性极化是可能的。这项工作为铌酸锂钽酸锂混晶的非线性光学应用奠定了基础。

英文摘要:

Lithium niobate and lithium tantalate are among the most widespread materials for nonlinear, integrated photonics. Mixed crystals with arbitrary Nb-Ta ratios provide a new degree of freedom to tune materials properties, such as the birefringence, but also leverage the advantages of the singular compounds, for example, by combining the thermal stability of lithium tantalate with the larger nonlinear or piezoelectric constants of lithium niobate. Periodic poling is the prerequisite for any nonlinear optical application. For mixed crystals this has been challenging so far due to the lack of homogeneous, mono-domain crystals, which severely inhibit domain growth and nucleation. In this work we demonstrate that surface-near ($< 1$~$μ$m depth) periodic poling on x-cut lithium niobate tantalate mixed crystals can be achieved via electric field poling and lithographically structured electrodes. We find that naturally occurring head-to-head or tail-to-tail domain walls in the as-grown crystal inhibit domain inversion at a larger scale. However, periodic poling is possible, if the gap size between the poling electrodes is of the same order of magnitude or smaller than the average size of naturally occurring domains. This work provides the basis for the nonlinear optical application of lithium niobate tantalate mixed crystals.

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