We investigate twisted bilayer graphene near charge neutrality using a generalized Bistritzer-MacDonald continuum model, accounting for corrugation effects. The Fermi velocity vanishes for particular twist angles properly reproducing the physics of the celebrated magic angles. Using group representation theory, we identify all contact interaction potentials compatible with the symmetries of the model. This enables us to identify two classes of quartic interactions leading to either the opening of a gap or to nematic ordering. We then implement a renormalization group analysis to study the competition between these interactions for a twist angle approaching the first magic value. This combined group theory-renormalization study reveals that the proximity to the first magic angle favors the occurrence of a layer-polarized, gapped state with a spatial modulation of interlayer correlations, which we call nematic insulator.
Twisted bilayer graphene (TBG) provides a unique framework to elucidate the interplay between strong correlations and topological phenomena in two-dimensional systems. The existence of multiple electronic degrees of freedom -- charge, spin, and valley -- gives rise to a plethora of possible ordered states and instabilities. Identifying which of them are realized in the regime of strong correlations is fundamental to shed light on the nature of the superconducting and correlated insulating states observed in the TBG experiments. Here, we use unbiased, sign-problem-free quantum Monte Carlo simul…
We report on a fully self-consistent Hartree-Fock calculation of interaction effects on the Moiré flat bands of twisted bilayer graphene, assuming that valley U(1) symmetry is respected. We use realistic band structures and interactions and focus on the charge neutrality point, where experiments have variously reported either insulating or semimetallic behavior. Restricting the search to orders for which the valley U(1) symmetry remains unbroken, we find three types of self-consistent solutions with competitive ground state energy (i) insulators that break $C_2 {\mathcal T}$ symmetry, includin…
The spin$-1/2$ Heisenberg antiferromagnet on the honeycomb bilayer lattice is shown to display a rich variety of semiclassical and genuinely quantum phases, controlled by the interplay between intralayer frustration and interlayer exchange. Employing a complementary set of techniques, comprising spin rotationally invariant Schwinger boson mean field theory, bond operators, and series expansions we unveil the quantum phase diagram, analyzing low-energy excitations and order parameters. By virtue of Schwinger bosons we scan the complete range of exchange parameters, covering both long range orde…
It was suggested that the two consecutive metamagnetic transitions and the large residual resistivity discovered in Sr$_3$Ru$_2$O$_7$ can be understood via the nematic order and its domains in a single layer system. However, a recently reported anisotropy between two longitudinal resistivities induced by tilting the magnetic field away from the c-axis cannot be explained within the single layer nematic picture. To fill the gap in our understanding within the nematic order scenario, we investigate the effects of bilayer coupling and in-plane magnetic field on the electronic nematic phases in a …
We study frustrated spin-1/2 dimer systems in two dimensions with a bilayer structure, where spins are ferromagnetically coupled in dimers. Our model includes frustrated two-spin exchange interactions as well as four-spin interaction. We pay particular attention to the spin nematic phase, which does not exhibit any magnetic (spin-dipole) order but has a spin-quadrupolar long-range order. Employing a perturbation calculation, a mean-field approximation, and a numerical many-variable variational Monte Carlo method, we determine ground-state phase diagrams on various two-dimensional lattices. It …
Utilizing the Baym-Kadanoff formalism with the polarization function calculated in the random phase approximation, the dynamics of the $ν=0$ quantum Hall state in bilayer graphene is analyzed. Two phases with nonzero energy gap, the ferromagnetic and layer asymmetric ones, are found. The phase diagram in the plane $(\tildeΔ_0,B)$, where $\tildeΔ_0$ is a top-bottom gates voltage imbalance, is described. It is shown that the energy gap scales linearly, $ΔE\sim 14 B[T]K, with magnetic field.
Using the semiclassical quantum Boltzmann equation (QBE), we numerically calculate the DC transport properties of bilayer graphene near charge neutrality. We find, in contrast to prior discussions, that phonon scattering is crucial even at temperatures below 40K. Nonetheless, electron-electron scattering still dominates over phonon collisions allowing a hydrodynamic approach. We introduce a simple two-fluid hydrodynamic model of electrons and holes interacting via Coulomb drag and compare our results to the full QBE calculation. We show that the two-fluid model produces quantitatively accurate…
Moiré materials such as magic angle twisted bilayer graphene (MATBG) exhibit remarkable phenomenology, but present significant challenges for certain experimental methods, particularly scanning probes such as scanning tunneling microscopy (STM). Typical STM studies that can image tens of thousands of atomic unit cells can image roughly ten moiré cells, making data analysis statistically fraught. Here, we propose a method to mitigate this problem by aggregating STM conductance data from several bias voltages, and then using the unsupervised machine learning method of gaussian mixture model clus…
We study theoretically many-body properties of magic-angle twisted bilayer graphene for different doping levels. Our investigation is focused on the emergence, stability, and manifestations of nematicity of the ordered low-temperature electronic state. It is known that, at vanishing interactions, the low-energy spectrum of the system studied consists of four almost-flat almost-degenerate bands. Electron-electron repulsion lifts this degeneracy. To account for such an interaction effect, a numerical mean-field theory is used. Assuming that the ground state has spin-density-wave-like order, we i…
We explore several classes of quadrupolar ordering in a system of antiferromagnetically coupled quantum spin-1 dimers, which are stacked in the triangular lattice geometry forming a bilayer. Low-energy properties of this model is described by an $\mathcal{S}=1$ hard-core bosonic degrees of freedom defined on each dimer-bond, where the singlet and triplet states of the dimerized spins are interpreted as the vacuum and the occupancy of boson, respectively. The number of bosons per dimer and the magnetic and density fluctuations of bosons are controlled by the inter-dimer Heisenberg interactions.…
Nematic superconductors possess unconventional superconducting order parameters that spontaneously break rotational symmetry of the underlying crystal. In this work we propose a mechanism for nematic superconductivity stabilized by strong density wave fluctuations in two dimensions. While the weak-coupling theory finds the fully gapped chiral state to be energetically stable, we show that strong density wave fluctuations result in an additional contribution to the free energy of a superconductor with multicomponent order parameters, which generally favors nematic superconductivity. Our theory …
In the magic angle twisted bilayer graphene (MATBG), one of the most remarkable observations is the $C_3$-symmetry-breaking nematic state. We identify that the nematicity in MATBG is the $E$-symmetry ferro bond order, which is the modulation of correlated hopping integrals owing to the $E$-symmetry particle-hole pairing condensation. The nematicity in MATBG originates from prominent quantum interference among $SU(4)$ valley+spin composite fluctuations. This novel "valley + spin fluctuation interference mechanism" is revealed by the density wave equation analysis for realistic multiorbital Hubb…
Twisted bilayer graphene (TBG) develops large moiré patterns at small twist angles with flat energy bands hosting domes of superconductivity. The large system size and intricate band structure have however hampered investigations into the superconducting state. Here, using full-scale atomistic modelling with local electronic interactions, we find at and above experimentally relevant temperatures a highly inhomogeneous superconducting state with nematic ordering on both atomic and moiré length scales. The nematic state has a locally anisotropic real-valued d-wave pairing, with a nematic vector …
We show that unconventional nematic superconductors with multi-component order parameter in lattices with three-fold and six-fold rotational symmetries support a charge-$4e$ vestigial superconducting phase above $T_c$. The charge-$4e$ state, which is a condensate of four-electron bound states that preserve the rotational symmetry of the lattice, is nearly degenerate with a competing vestigial nematic state, which is non-superconducting and breaks the rotational symmetry. This robust result is the consequence of a hidden discrete symmetry in the Ginzburg-Landau theory, which permutes quantities…
We study the phase diagram of an effective model of competing nematic and antiferromagnetic orders of interacting electrons on the Bernal-stacked honeycomb bilayer, as relevant for bilayer graphene. In the noninteracting limit, the model features a semimetallic ground state with quadratic band touching points at the Fermi level. Taking the effects of short-range interactions into account, we demonstrate the existence of an extended region in the mean-field phase diagram characterized by coexisting nematic and antiferromagnetic orders. By means of a renormalization group approach, we reveal tha…
We analyze density-wave and Pomeranchuk orders in twisted bilayer graphene. This compliments our earlier analysis of the pairing instabilities. We assume that near half-filling of either conduction or valence band, the Fermi level is close to Van Hove points, where the density of states diverges, and study potential instabilities in the particle-hole channel within a patch model with two valley degrees of freedom. The hexagonal symmetry of twisted bilayer graphene allows for either six or twelve Van Hove points. We consider both cases and find the same two leading candidates for particle-hole …
Graphene-based moiré systems have attracted considerable interest in recent years as they display a remarkable variety of correlated phenomena. Besides insulating and superconducting phases in the vicinity of integer fillings of the moiré unit cell, there is growing evidence for electronic nematic order both in twisted bilayer graphene and twisted double-bilayer graphene (tDBG), as signaled by the spontaneous breaking of the threefold rotational symmetry of the moiré superlattices. Here, we combine symmetry-based analysis with a microscopic continuum model to investigate the structure of the n…
We use self-consistent Hartree-Fock calculations performed in the full $π$-band Hilbert space to assess the nature of the recently discovered correlated insulator states in magic-angle twisted bilayer graphene (TBG). We find that gaps between the flat conduction and valence bands open at neutrality over a wide range of twist angles, sometimes without breaking the system's valley projected ${\cal C}_{2}{\cal T}$ symmetry. Broken spin/valley flavor symmetries then enable gapped states to form not only at neutrality, but also at total moiré band filling $n = \pm p/4$ with integer $p = 1, 2, 3$, w…
In bilayer graphene, the phase diagram in the plane of a strain-induced bare nematic term, ${\cal N}_{0}$, and a top-bottom gates voltage imbalance, $U_{0}$, is obtained by solving the gap equation in the random-phase approximation. At nonzero ${\cal N}_0$ and $U_0$, the phase diagram consists of two hybrid spin-valley symmetry-broken phases with both nontrivial nematic and mass-type order parameters. The corresponding phases are separated by a critical line of first- and second-order phase transitions at small and large values of ${\cal N}_0$, respectively. The existence of a critical end poi…
Stacking two graphene layers twisted by the 'magic angle' $θ\approx 1.1^\circ$ generates flat energy bands, which in turn catalyzes various strongly correlated phenomena depending on filling and sample details. At charge neutrality, transport measurements reveal superficially mundane semimetallicity (as expected when correlations are weak) in some samples yet robust insulation in others. We propose that the interplay between interactions and disorder admits either behavior, even when the system is strongly correlated and locally gapped. Specifically, we argue that strong interactions supplemen…
We analyze the phase diagram of the Bilayer graphene (BLG) at zero temperature and doping. Assuming that at the high energies the electronic system of BLG can be described within a weak coupling theory (consistent with the experimental evidence), we systematically study the evolution of the couplings with going from high to low energies. The divergences of the couplings at some energies indicates the tendency towards certain symmetry breakings. Carrying out this program, we found that the phase diagram is determined by microscopic couplings defined on the short distances (initial conditions). …
We discuss twisted bilayer graphene (TBG) based on a theorem of flat band ferromagnetism put forward by Mielke and Tasaki. According to this theorem, ferromagnetism occurs if the single particle density matrix of the flat band states is irreducible and we argue that this result can be applied to the quasi-flat bands of TBG that emerge around the charge-neutrality point for twist angles around the magic angle $θ\sim1.05^\circ$. We show that the density matrix is irreducible in this case, thus predicting a ferromagnetic ground state for neutral TBG ($n=0$). We then show that the theorem can also…
In an externally applied magnetic field, ultra-pure crystals of the bilayer compound Sr$_3$Ru$_2$O$_7$ undergo a metamagnetic transition below a critical temperature, $T^*$, which varies as a function of the angle between the magnetic field $H$ and the Ru-O planes. Moreover, $T^*$ approaches zero when $H$ is perpendicular to the planes. This putative "metamagnetic quantum critical point", however, is preempted by a nematic fluid phase with order one resistive anisotropy in the {\it ab} plane. In a "realistic" bilayer model with moderate strength local Coulomb interactions, the existence of a s…
Triple point fermions are elusive electronic excitations that generalize Dirac and Weyl modes beyond the conventional high energy paradigm. Yet, finding real materials naturally hosting these excitations at the Fermi energy has remained challenging. Here we show that twisted bilayer graphene is a versatile platform to realize robust triple point fermions in two dimensions. In particular, we establish that the introduction of localized impurities lifts one of the two degenerate Dirac cones, yielding triple point fermions at charge neutrality. Furthermore, we show that the valley polarization is…
Using non-perturbative theoretical method, we address the problem of strong correlations in twisted bilayer-layer graphene at the magic angle. We concentrate on the solution without symmetry breaking, where conventional Mott insulating state is expected for all integer fillings. At Coulomb repulsion corresponding to dielectric constant $\varepsilon\approx 5$ and several integer fillings we find a Mott-semiconducting state, which simultaneously hosts the Mott state, and inside the Mott gap, a second much smaller semiconduting gap. The presence of these Mott-ingap states, which are located at th…
We present a framework for understanding the recently observed cascade transitions and the Landau level degeneracies at every integer filling of twisted bilayer graphene. The Coulomb interaction projected onto narrow bands causes the charged excitations at an integer filling to disperse, forming new bands. If the excitation moves the filling away from the charge neutrality point, then it has a band minimum at the moire Brillouin zone center with a small mass that compares well with the experiment; if towards the charge neutrality point, then it has a much larger mass and a higher degeneracy. A…
We propose an SU(4) spin-valley-fermion model to investigate the superconducting instabilities of twisted bilayer graphene (TBG). In this approach, bosonic fluctuations associated with an emergent SU(4) symmetry, corresponding to combined rotations in valley and spin spaces, couple to the low-energy fermions that comprise the flat bands. These fluctuations are peaked at zero wave-vector, reflecting the "ferromagnetic-like" SU(4) ground state recently found in strong-coupling solutions of microscopic models for TBG. Focusing on electronic states related to symmetry-imposed points of the Fermi s…
The emergence of controlled, two-dimensional moiré materials has uncovered a new platform for investigating topological physics. Twisted double bilayer graphene (TDBG) has been predicted to host a topologically non-trivial gapped phase with Chern number equal to two at charge neutrality, when half the flat bands are filled. However, it can be difficult to diagnose topological states using a single measurement because it is ideal to probe the bulk and edge properties at the same time. Here, we report a combination of chemical potential measurements, transport measurements, and theoretical calcu…
An extended Hubbard model on a honeycomb lattice with two orbitals per site at charge neutrality is investigated with unbiased large-scale quantum Monte Carlo simulations. The Fermi velocity of the Dirac fermions is renormalized as the cluster charge interaction increases, until a mass term emerges and a quantum phase transition from Dirac semi-metal to valence bond solid (VBS) insulator is established. The quantum critical point is discovered to belong to 3D $N=4$ Gross-Neveu chiral XY universality with the critical exponents obtained at high precision. Further enhancement of the interaction …
Employing the recently developed momentum-space quantum Monte Carlo scheme, we study the dynamic response of single-particle and collective excitations in realistic continuum models of twisted bilayer graphene. At charge neutrality, this unbiased numerical method reveals strong competition between different symmetry breaking channels with a leading instability towards the intervalley coherent state. Single-particle spectra indicate that repulsive interactions push the fermion spectral weight away from the Fermi energy and open up an insulating gap. The spectra of collective excitations suggest…
The nature of the insulating and superconducting states in twisted bilayer graphene systems is intensely debated. While many works seek for explanations in the few flat bands near the Fermi level, theory and a number of experiments suggest that nontwisted bilayer graphene systems do exhibit - or are at least close to - an ordered, insulating ground state related to antiferromagnetic ordering. Here we investigate in which ways this magnetic ordering scenario is affected by the slight twisting between the layers. We find that at charge neutrality the ordering tendencies of twisted systems interp…
An anisotropic metallic phase dubbed electronic nematic phase bounded by two consecutive metamagnetic transitions has been reported in the bilayer ruthenate Sr3Ru2O7. It has also been shown that the nematic and the accompanying metamagnetic transitions are driven by an effective momentum-dependent quadrupole-type interaction. Here, we study the microscopic origin of such an effective interaction. To elucidate the mechanism behind the spontaneous Fermi surface distortion associated with the nematic, we identify a simple tight binding model based on t2g orbitals, spin-orbit coupling and the rota…
Flat electronic bands can accommodate a plethora of interaction driven quantum phases, since kinetic energy is quenched therein and electronic interactions therefore prevail. Twisted bilayer graphene, near so-called the "magic angles", features \emph{slow} Dirac fermions close to the charge-neutrality point that persist up to high-energies. Starting from a continuum model of slow, but strongly interacting Dirac fermions, we show that with increasing chemical doping away from the charge-neutrality point, a time-reversal symmetry breaking, valley pseudo-spin-triplet, topological $p+ip$ supercond…
We perform a general group-theoretical study of the Kondo problem in monolayer and bilayer graphene around the charge neutrality point. Utilizing the group representation theory, we derive from symmetry considerations a family of the Kondo models for all symmetric placements with either 3- or 6-fold rotational axis of an impurity atom in an arbitrary orbital state. We find six possible classes of the partially anisotropic four-channel Kondo model. As the key result, we argue several possibilities to realize the regime of the dominant channel-symmetric two-channel Kondo effect, protected by the…
Current experiments on different samples of twisted bilayer graphene (TBG) have found different sets of insulating phases. Despite this diversity, many features of these insulating phases appear to be universal. They include the dispersion of Landau fans away from charge neutrality, a reduced Landau fan degeneracy from the expected value at charge neutrality, and the further reduction of this degeneracy when crossing an insulating phase with odd number of electrons in the superlattice unit cell. We point out that all these behaviors as well as the ferromagnetic behavior observed in some of the…
We study symmetry-broken phases in twisted bilayer graphene at small filling above charge neutrality and at Van Hove filling. We argue that the Landau functionals for the particle-hole order parameters at these fillings both have an approximate SU(4) symmetry, but differ in the sign of quartic terms. We determine the order parameter manifold of the ground state and analyze its excitations. For small fillings, we find a strong 1st-order transition to an SU(3)$\otimes$U(1) manifold of orders that break spin-valley symmetry and induce a 3-1 splitting of fermionic excitations. For Van Hove filling…
We propose a model of spin-polarized-current state for electrons in bilayer graphene. The model resolves the puzzles as revealed by experiments that (a) the energy gap $E_{\rm gap}$ of the insulating ground state at the charge neutrality point (CNP) can be closed by a perpendicular electric field of either polarity, (b) $E_{\rm gap}$ increases significantly with increasing the magnetic field $B$, (c) the particle-hole spectrum is asymmetric in the presence of $B$, (d) there is a peak structure in the electric conductivity at small $B$ at the CNP, and (e) there are quantum Hall states stemming …
We study the effects of heterostrain on moiré bands in twisted bilayer graphene and bilayer transition metal dichalcogenide (TMD) systems. For bilayer graphene with twist angle near $1^\circ$, we show that heterostrain significantly increases the energy separation between conduction and valence bands as well as the Dirac velocity at charge neutrality, which resolves several puzzles in scanning tunneling spectroscopy and quantum oscillation experiments at once. For bilayer TMD, we show that applying small heterostrain generally leads to flat moiré bands that are highly tunable.
In the present paper, we consider the excitonic effects on the single particle normal density of states (DOS) in the bilayer graphene (BLG). The local interlayer Coulomb interaction is considered between the particles on the non-equivalent sublattice sites in different layers of the BLG. We show the presence of the excitonic shift of the neutrality point, even for the noninteracting layers. Furthermore, for the interacting layers, a very large asymmetry in the DOS structure is shown between the particle and hole channels. At the large values of the interlayer hopping amplitude, a large number …
Twisted Bilayer graphene (TBG) is known to feature isolated and relatively flat bands near charge neutrality, when tuned to special magic angles. However, different criteria for the magic angle such as the vanishing of Dirac speed, minimal bandwidth or maximal band gap to higher bands typically give different results. Here we study a modified continuum model for TBG which has an infinite sequence of magic angles $θ$ at which, we simultaneously find that (i) the Dirac speed vanishes (ii) absolutely flat bands appear at neutrality and (iii) bandgaps to the excited bands are maximized. When param…
Low-energy electronic structure of (unbiased) bilayer graphene is made of two Fermi points with quadratic dispersions, if trigonal-warping and other high order contributions are ignored. We show that as a result of this qualitative difference from single-layer graphene, short-range (or screened Coulomb) interactions are marginally relevant. We use renormalization group to study their effects on low-energy properties of the system, and show that the two quadratic Fermi points spontaneously split into four Dirac points, at zero temperature. This results in a nematic state that spontaneously brea…
Correlated insulators and superconductivity have been observed in "magic-angle" twisted bilayer graphene, when the nearly flat bands close to neutrality are partially filled. While a momentum-space continuum model accurately describes these flat bands, interaction effects are more conveniently incorporated in tight-binding models. We have previously shown that no fully symmetric tight-binding model can be minimal, in the sense of capturing just the flat bands, so extended models are unavoidable. Here, we introduce a family of tight-binding models that capture the flat bands while simultaneousl…
The quantum Hall effect near the charge neutrality point in bilayer graphene is investigated in high magnetic fields of up to 35 T using electronic transport measurements. In the high field regime, the eight-fold degeneracy in the zero energy Landau level is completely lifted, exhibiting new quantum Hall states corresponding filling factors $ν=$0, 1, 2, & 3. Measurements of the activation energy gap in tilted magnetic fields suggest that the Landau level splitting at the newly formed $ν=$1, 2, & 3 filling factors are independent of spin, consistent with the formation of a quantum Hall ferromag…
Bilayer graphene (BLG) at the charge neutrality point (CNP) is strongly susceptible to electronic interactions, and expected to undergo a phase transition into a state with spontaneous broken symmetries. By systematically investigating a large number of singly- and doubly-gated bilayer graphene (BLG) devices, we show that an insulating state appears only in devices with high mobility and low extrinsic doping. This insulating state has an associated transition temperature Tc~5K and an energy gap of ~3 meV, thus strongly suggesting a gapped broken symmetry state that is destroyed by very weak di…
