Resonant dispersive wave (RDW) emission in gas-filled hollow waveguides is a powerful technique for the generation of bright few-femtosecond laser pulses from the vacuum ultraviolet to the near infrared. Here we investigate deep-ultraviolet RDW emission in a hollow capillary fibre filled with a longitudinal gas pressure gradient. We obtain broadly similar emission to the constant-pressure case by applying a surprisingly simple scaling rule for the gas pressure and study the energy-dependent dispersive-wave spectrum in detail using simulations. We further find that in addition to enabling dispersion-free delivery to experimental targets, a decreasing gradient also reduces the pulse stretching within the waveguide itself, and that transform-limited pulses with 3 fs duration can be generated by using short waveguides. Our results illuminate the fundamental dynamics underlying this frequency conversion technique and will aid in fully exploiting it for applications in ultrafast science and beyond.
We demonstrate high-energy resonant dispersive-wave emission in the deep ultraviolet (218 to 375 nm) from optical solitons in short (15 to 34cm) hollow capillary fibres. This down-scaling in length compared to previous results in capillaries is achieved by using small core diameters (100 and 150 $μ$m) and pumping with 6.3 fs pulses at 800 nm. We generate pulses with energies of 4 to 6 $μ$J across the deep ultraviolet in a 100 $μ$m capillary and up to 11 $μ$J in a 150 $μ$m capillary. From comparisons to simulations we estimate the ultraviolet pulse to be 2 to 2.5 fs in duration. We also numeric…
We demonstrate an efficient scheme for the generation of broadband, high-energy, circularly polarized femtosecond laser pulses in the deep ultraviolet through seeded degenerate four-wave mixing in stretched gas-filled hollow capillary fibers. Pumping and seeding with circularly polarized 35 fs pulses centered at 400 nm and 800 nm, respectively, we generate idler pulses centered at 266 nm with more than 25 microjoule of energy and over 95% spectrally averaged ellipticity. Even higher idler energies and broad spectra (27 nm bandwidth) can be obtained at the cost of reduced ellipticity. Our syste…
We investigate soliton self-compression and ultraviolet resonant dispersive wave emission in the higher-order modes of a gas-filled hollow capillary fibre. Our simple analytical scaling rules predict shorter required waveguides and different energy scales when moving from the fundamental to higher-order modes. Experimentally, we demonstrate soliton self-compression and ultraviolet dispersive wave emission in the double-lobe LP$_{11}$ mode of an argon-filled hollow capillary fibre, which we excite by coupling into the fibre at oblique incidence. We observe the generation of ultraviolet dispersi…
We present high-resolution spectroscopy of Iodine vapour that is loaded and trapped within the core of a hollow-core photonic crystal fibre (HC-PCF). We compare the observed spectroscopic features to those seen in a conventional iodine cell and show that the saturation characteristics differ significantly. Despite the confined geometry it was still possible to obtain sub-Doppler features with a spectral width of ~6 MHz with very high contrast. We provide a simple theory which closely reproduces all the key observations of the experiment.
We demonstrate a fibre-based approach that generates mid-infrared femtosecond pulses in the 3-4 μm spectral region with microjoule-level single pulse energy. This is realised in a piece of gas-filled antiresonant hollow-core fibre that is pumped by a two-micron light source. A rapid variation of the dispersion near a structural resonance of the fibre creates a phase-matching point in the mid-infrared, which mediates the frequency-down conversion. We generate femtosecond pulses centred at 3.16 μm wavelength with the pulse energy of more than 1 μJ, achieving the conversion efficiency as high as …
Optical soliton dynamics can cause the extreme alteration of the temporal and spectral shape of a propagating light pulse. They occur at up to kilowatt peak powers in glass-core optical fibres and the gigawatt level in gas-filled microstructured hollow-core fibres. Here we demonstrate optical soliton dynamics in large-core hollow capillary fibres. This enables scaling of soliton effects by several orders of magnitude to the multi-mJ energy and terawatt peak power level. We experimentally demonstrate two key soliton effects. First, we observe self-compression to sub-cycle pulses and infer the c…
Optically levitated micro- and nanoparticles offer an ideal playground for investigating photon-phonon interactions over macroscopic distances. Here we report the observation of long-range optical binding of multiple microparticles, mediated by intermodal scattering and interference inside the evacuated core of a hollow-core photonic crystal fibre (HC-PCF). Three polystyrene particles with 1 μm diameter are stably bound together with an inter-particle distance of ~40 μm, or 50 times longer than the wavelength of the trapping laser. The bound-particle array can be translated to-and-fro over cen…
We present a new type of compact and all-glass based vapour cell integrating hollow-core photonic crystal fibres. The absence of metals, as in a traditional vacuum chamber and the much more compact geometry allows for fast and homogeneous heating. As a consequence we can fill the fibres on much faster timescales, ranging from minutes to hours. Additionally the all-glass design ensures optical access along the fibre. This allows live monitoring of the diffusion of rubidium atoms inside the hollow-core by measuring the frequency-dependent fluorescence from the atoms. The atomic density is numeri…
The possibility of performing time-resolved spectroscopic studies in the molecular fingerprinting region or extending the cut-off wavelength of high-harmonic generation has recently boosted the development of efficient mid-infrared ultrafast lasers. In particular, fibre lasers based on active media such as thulium or holmium are a very active area of research since they are robust, compact and can operate at high repetition rates. These systems, however, are still complex, are unable to deliver pulses shorter than 100 fs and are not yet as mature as their near-infrared counterparts. Here we re…
High-energy ultraviolet pulse generation in gas-filled hollow capillary fibers (HCFs) through dispersive-wave-emission process, has attracted considerable attentions in recent several years due to its great application potentials in ultraviolet spectroscopy and photochemistry. While the ability of this technique to deliver high-energy, ultrafast ultraviolet pulses is widely recognized, few-fs duration of μJ-level dispersive-wave (DW) pulses has, however, escaped direct measurements. In this letter, we demonstrate that using several chirped mirrors, few-fs ultraviolet DW pulses can be obtained …
Gas-filled hollow-core fibres are a flexible platform for the manipulation of ultrafast laser pulses through a variety of nonlinear optical effects. Efficient high-fidelity coupling of the initial pulses is very important for system performance. Here we study the effect of self-focusing in gas-cell windows on the coupling of ultrafast laser pulses into hollow-core fibres using (2+1)-dimensional numerical simulations. As expected, we find that the coupling efficiency is degraded and the duration of the coupled pulses changed when the entrance window is too close to the fibre entrance. The inter…
We report the direct observation of periodic intensity modulation of a laser pulse propagating in a hollow core waveguide. A series of equally spaced plasma sparks along the gas-filled capillary is produced. This effect can be explained by the beating of different fiber modes, which are excited by controlling the size of the focal spot at the capillary entrance. As compared to an artificial modulated waveguide structure, our presented approach represents an easier and more flexible quasi-phase-matching scheme for nonlinear-optical frequency conversion.
Bright, coherent soft X-ray (SXR) radiation is essential to a variety of applications in fundamental research and life sciences. So far, high photon flux in this spectral region can only be delivered by synchrotrons, free electron lasers or high-order harmonic generation (HHG) sources, which are driven by kHz-class repetition rate lasers with very high peak powers. Here, we establish a novel route toward powerful and easy-to-use SXR sources by presenting a compact experiment, in which nonlinear pulse self-compression to the few-cycle regime is combined with phase-matched HHG in a single, heliu…
Preparation of an atomic ensemble in a particular Zeeman state is a critical step of many protocols for implementing quantum sensors and quantum memories. These devices can also benefit from optical fibre integration. In this work we describe experimental results supported by a theoretical model of single-beam optical pumping of $^{87}$Rb atoms within a hollow-core photonic crystal fibre. The observed 50% population increase in the pumped F=2, m$_F$=2 Zeeman substate along with the depopulation of remaining Zeeman substates enabled us to achieve a 3 times improvement in the relative population…
We use hollow-core fibre to preserve the spectrum and temporal profile of picosecond laser pulses in CBD to suppress 2.6 dB of amplitude noise at MHz noise frequencies, to within 0.01 dB of the shot-noise limit. We provide an enhanced version of the CBD scheme that concatenates circuits to suppress over multiple frequencies and over broad frequency ranges --- we perform a first demonstration that reduces total excess amplitude noise, between 2 - 6 MHz, by 85%. These demonstrations enable passive, broad-band, all-guided fibre laser technology operating at the shot-noise limit.
We demonstrate, for the first time, the application of rare-gas filled hollow-core photonic crystal fibres (HC-PCFs) as tuneable ultraviolet light sources in femtosecond pump-probe spectroscopy. The time-resolved photoelectron imaging technique reveals non-adiabatic dynamical processes operating on three distinct timescales in the styrene molecule following excitation over the 242-258 nm region. These include ultrafast (<100 fs) internal conversion between the S2(pipi*) and S1(pipi*) electronic states and subsequent intramolecular vibrational energy redistribution within S1(pipi*). Compact, co…
In hydrodynamics, vortex generation upon the transition from smooth laminar flows to turbulence is generally accompanied by increased dissipation. However, plane vortices can provide transport barriers and decrease losses, as it happens in numerous geophysical, astrophysical flows and in tokamaks. Photon interactions with matter can affectlight transportin waveguides in unexpected and somewhat counterintuitive ways resembling fluid dynamics. Here, we demonstrate dramatic impact of light vortex formation in micro-structured optical fibres on the energy dissipation. We show possibility of vortic…
The generation of large multiphoton quantum states - for applications in computing, metrology, and simulation - requires a network of high-efficiency quantum memories capable of storing broadband pulses. Integrating these memories into a fibre offers a number of advantages towards realising this goal: strong light-matter coupling at low powers, simplified alignment, and compatibility with existing photonic architectures. Here, we introduce a large-core kagome-structured hollow-core fibre as a suitable platform for an integrated fibre-based quantum memory with a warm atomic vapour. We demonstra…
Stimulated Brillouin scattering (SBS) offers among the highest nonlinear gains in solid materials and has demonstrated advanced photonics functionalities in waveguides. The large compressibility of gases suggests that SBS may gain in efficiency with respect to condensed materials. Here, by using a gas-filled hollow-core fibre at high pressure, we achieve a strong Brillouin amplification per unit length, exceeding by 6 times the gain observed in fibres with a solid silica core. This large amplification benefits from a higher molecular density and a lower acoustic attenuation at higher pressure,…
Alkali-filled hollow-core fibres are a promising medium for investigating light-matter interactions, especially at the single-photon level, due to the tight confinement of light and high optical depths achievable by light-induced atomic desorption. However, until now these large optical depths could only be generated for seconds at most once per day, severely limiting the practicality of the technology. Here we report the generation of highest observed transient ($>10^5$ for up to a minute) and highest observed persistent ($>2000$ for hours) optical depths of alkali vapours in a light-guiding …
The performances of optical fibre-based quantum information systems are limited by the intrinsic properties of silica glass materials, e.g. high latency, Rayleigh-scattering loss wavelength scaling law, and cross-coupling induced modal impurity. Hollow-core optical fibre (HCF) promises to unify air-borne light propagation and non-line-of-sight transmission, thus holding great potentials for versatile photonics-based quantum infor-mation applications. The early version of HCF based on photonic-bandgap guidance has not proven itself as a reliable quantum channel because of the poor modal purity …
We numerically investigate the energy and arrival-time noise of ultrashort laser pulses produced via resonant dispersive wave emission in gas-filled hollow-core waveguides under the influence of pump-laser instability. We find that for low pump energy, fluctuations in the pump energy are strongly amplified. However, when the generation process is saturated, the energy of the resonant dispersive wave can be significantly less noisy than that of the pump pulse. This holds for a variety of generation conditions and while still producing few-femtosecond pulses. We further find that the arrival-tim…
We investigate various methods for extending the simple analytical capillary model to describe the dispersion and loss of anti-resonant hollow-core fibers without the need of detailed finite-element simulations across the desired wavelength range. This poor-man's model can with a single fitting parameter quite accurately mimic dispersion and loss resonances and anti-resonances from full finite-element simulations. Due to the analytical basis of the model it is easy to explore variations in core size and cladding wall thickness, and should therefore provide a valuable tool for numerical simulat…
Efficient monitoring of airborne particulate matter (PM), especially particles with aerodynamic diameter less than 2.5 um (PM2.5), is crucial for improving public health. Reliable information on the concentration, size distribution and chemical characteristics of PMs is key to evaluating air pollution and identifying its sources. Standard methods for PM2.5 characterization require sample collection from the atmosphere and post-analysis using sophisticated equipment in a laboratory environment, and are normally very time-consuming. Although optical methods based on analysis of scattering of fre…
We propose and theoretically analyse a novel hollow-core photonic crystal fibre (PCF) that is engineered so as to strongly suppress higher order modes, i.e., to provide robust LP$_{01}$ single-mode guidance in all the wavelength ranges where the fibre guides with low loss. Encircling the core is a single ring of non-touching glass elements whose modes are tailored to ensure resonant phase-matched coupling to higher-order core modes, causing them to leak at a very high rate into the supporting solid glass sheath. Using a model based on coupled capillary waveguides, as well as full vectorial fin…
We demonstrate efficient generation of coherent super-octave pulses via a single-stage spectral broadening of a Yb:KGW laser in a single, pressurized, Ne-filled, hollow-core fiber capillary. Emerging pulses spectrally spanning over more than $\sim$1 PHz (250 nm- 1600 nm) at a dynamic range of $\sim$60 dB, and an excellent beam quality open the door to combining Yb:KGW lasers with modern light field synthesis techniques. Compression of a fraction of the generated supercontinuum to intense (8 fs, $\sim$2.4 cycle, $\sim$650 $μ$J) pulses allows convenient use of these novel laser sources in strong…
Predictions and measurements of a multimode waveguide interferometer operating in a fibre coupled, ``dual-mode'' regime are reported. With a 1.32 micrometer source, a complete switching cycle of the output beam is produced by a 10.0 nanometer incremental change in the 8.0 micrometer width of the hollow planar mirror waveguide. This equates to a fringe spacing of $\simλ/130$. This is an order of magnitude smaller than previously reported results for this form of interferometer.
We report on a highly-efficient experimental scheme for the generation of deep-ultraviolet ultrashort light pulses using four-wave mixing in gas-filled kagomé-style photonic crystal fiber. By pumping with ultrashort, few $μ$J, pulses centered at 400 nm, we generate an idler pulse at 266 nm, and amplify a seeded signal at 800 nm. We achieve remarkably high pump-to-idler energy conversion efficiencies of up to 38%. Although the pump and seed pulse durations are ~100 fs, the generated ultraviolet spectral bandwidths support sub-15 fs pulses. These can be further extended to support few-cycle puls…
We report a silica glass nested capillary anti-resonant nodeless fiber with transmission and low bending sensitivity in the mid-infrared around 4000 nm. The fiber is characterized in terms of transmission over 1700-4200 nm wavelengths, revealing a mid-infrared 3500-4200 nm transmission window, clearly observable for a 12 m long fiber. Bending loss around 4000 nm is 0.5 dB/m measured over 3 full turns with 40 mm radius, going up to 5 dB/m for full turns with 15 mm radius. Our results provide experimental evidence of hollow-core silica fibers in which nested, anti-resonant capillaries provide hi…
Optical properties of hollow-core revolver fibers are numerically investigated depending on various parameters: the hollow-core diameter, the capillary wall thickness, the values of the minimum gap between the capillaries, the number of capillaries in the cladding and the type of glass (silica and chalcogenide). Preliminary, similar calculations are made for simple models of hollow-core fibers. Based on the obtained results, the optimal design of the revolver fiber for Raman laser frequency conversion (1560 nm to 4420 nm in H2) was determined. As a result, efficient ns-pulsed 4420 nm Raman las…
Low-threshold efficient N${_2^+}$ lasing driven by sub-cycle soliton dynamics in a hollow waveguide
State Key Laboratory of Ultra-intense Laser Science and Technology, Shanghai Institute of Optics and Fine Mechanics (SIOM), Chinese Academy of Sciences (CAS)（中国科学院上海光学精密机械研究所超强度激光科学与技术国家重点实验室）；Russell Centre for Advanced Lightwave Science, Shanghai Institute of Optics and Fine Mechanics (SIOM) and Hangzhou Institute of Optics and Fine Mechanics (HIOM)（上海光学精密机械研究所与杭州光学精密机械研究所先进光波科学中心）；Zhejiang Key Laboratory of Microstructured Specialty Optical Fiber, Hangzhou Institute of Optics and Fine Mechanics (HIOM)（杭州光学精密机械研究所微结构特种光纤浙江省重点实验室）；School of Optoelectronic Engineering, Xidian University（西安电子科技大学光电工程学院）；School of Optical-Electrical and Computer Engineering, University of Shanghai for Science and Technology（上海理工大学光电信息与计算机工程学院）；Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences（中国科学院大学杭州高等研究院）；Zhangjiang Laboratory（张江实验室）
In this Letter, we show theoretically that the nonlinear photoionisation process of a noble gas inside a hollow-core photonic crystal fibre can be exploited in obtaining broadband supercontinuum generation via pumping close to the mid-infrared regime. The interplay between the Kerr and photoionisation nonlinearities is strongly enhanced in this regime. Photoionisation continuously modifies the medium dispersion, in which the refractive index starts to significantly decrease and approach the epsilon-near-zero regime. Subsequently, the self-phase modulation induced by the Kerr effect is boosted …
We report a novel source of twin beams based on modulational instability in high-pressure argon-filled hollow-core kagomé-style photonic-crystal fibre. The source is Raman-free and manifests strong photon-number correlations for femtosecond pulses of squeezed vacuum with a record brightness of ~2500 photons per mode. The ultra-broadband (~50 THz) twin beams are frequency tunable and contain one spatial and less than 5 frequency modes.
