Optically levitated micro- and nanoparticles offer an ideal playground for investigating photon-phonon interactions over macroscopic distances. Here we report the observation of long-range optical binding of multiple microparticles, mediated by intermodal scattering and interference inside the evacuated core of a hollow-core photonic crystal fibre (HC-PCF). Three polystyrene particles with 1 μm diameter are stably bound together with an inter-particle distance of ~40 μm, or 50 times longer than the wavelength of the trapping laser. The bound-particle array can be translated to-and-fro over centimetre distances along the fibre. When evacuated to 6 mbar gas pressure, the collective mechanical modes of the bound-particle array could be observed. The measured inter-particle distance at equilibrium and mechanical eigen-frequencies are supported by a novel analytical formalism modelling the dynamics of the binding process. The HC-PCF system offers a unique platform for investigating the rich optomechanical dynamics of arrays of levitated particles in a well-isolated and protected environment.
Flying particle sensors in hollow-core photonic crystal fibers require accurate localization of the optically trapped microparticles. We report position measurement to micrometer-resolution, using optical frequency domain reflectometry, of two 1.65-$μ$m-diameter polystyrene particles.
We present high-resolution spectroscopy of Iodine vapour that is loaded and trapped within the core of a hollow-core photonic crystal fibre (HC-PCF). We compare the observed spectroscopic features to those seen in a conventional iodine cell and show that the saturation characteristics differ significantly. Despite the confined geometry it was still possible to obtain sub-Doppler features with a spectral width of ~6 MHz with very high contrast. We provide a simple theory which closely reproduces all the key observations of the experiment.
We demonstrate a fibre-based approach that generates mid-infrared femtosecond pulses in the 3-4 μm spectral region with microjoule-level single pulse energy. This is realised in a piece of gas-filled antiresonant hollow-core fibre that is pumped by a two-micron light source. A rapid variation of the dispersion near a structural resonance of the fibre creates a phase-matching point in the mid-infrared, which mediates the frequency-down conversion. We generate femtosecond pulses centred at 3.16 μm wavelength with the pulse energy of more than 1 μJ, achieving the conversion efficiency as high as …
We investigate soliton self-compression and ultraviolet resonant dispersive wave emission in the higher-order modes of a gas-filled hollow capillary fibre. Our simple analytical scaling rules predict shorter required waveguides and different energy scales when moving from the fundamental to higher-order modes. Experimentally, we demonstrate soliton self-compression and ultraviolet dispersive wave emission in the double-lobe LP$_{11}$ mode of an argon-filled hollow capillary fibre, which we excite by coupling into the fibre at oblique incidence. We observe the generation of ultraviolet dispersi…
Optical soliton dynamics can cause the extreme alteration of the temporal and spectral shape of a propagating light pulse. They occur at up to kilowatt peak powers in glass-core optical fibres and the gigawatt level in gas-filled microstructured hollow-core fibres. Here we demonstrate optical soliton dynamics in large-core hollow capillary fibres. This enables scaling of soliton effects by several orders of magnitude to the multi-mJ energy and terawatt peak power level. We experimentally demonstrate two key soliton effects. First, we observe self-compression to sub-cycle pulses and infer the c…
Resonant dispersive wave (RDW) emission in gas-filled hollow waveguides is a powerful technique for the generation of bright few-femtosecond laser pulses from the vacuum ultraviolet to the near infrared. Here we investigate deep-ultraviolet RDW emission in a hollow capillary fibre filled with a longitudinal gas pressure gradient. We obtain broadly similar emission to the constant-pressure case by applying a surprisingly simple scaling rule for the gas pressure and study the energy-dependent dispersive-wave spectrum in detail using simulations. We further find that in addition to enabling dispe…
The possibility of performing time-resolved spectroscopic studies in the molecular fingerprinting region or extending the cut-off wavelength of high-harmonic generation has recently boosted the development of efficient mid-infrared ultrafast lasers. In particular, fibre lasers based on active media such as thulium or holmium are a very active area of research since they are robust, compact and can operate at high repetition rates. These systems, however, are still complex, are unable to deliver pulses shorter than 100 fs and are not yet as mature as their near-infrared counterparts. Here we re…
We present a new type of compact and all-glass based vapour cell integrating hollow-core photonic crystal fibres. The absence of metals, as in a traditional vacuum chamber and the much more compact geometry allows for fast and homogeneous heating. As a consequence we can fill the fibres on much faster timescales, ranging from minutes to hours. Additionally the all-glass design ensures optical access along the fibre. This allows live monitoring of the diffusion of rubidium atoms inside the hollow-core by measuring the frequency-dependent fluorescence from the atoms. The atomic density is numeri…
Gas-filled hollow-core fibres are a flexible platform for the manipulation of ultrafast laser pulses through a variety of nonlinear optical effects. Efficient high-fidelity coupling of the initial pulses is very important for system performance. Here we study the effect of self-focusing in gas-cell windows on the coupling of ultrafast laser pulses into hollow-core fibres using (2+1)-dimensional numerical simulations. As expected, we find that the coupling efficiency is degraded and the duration of the coupled pulses changed when the entrance window is too close to the fibre entrance. The inter…
Bright, coherent soft X-ray (SXR) radiation is essential to a variety of applications in fundamental research and life sciences. So far, high photon flux in this spectral region can only be delivered by synchrotrons, free electron lasers or high-order harmonic generation (HHG) sources, which are driven by kHz-class repetition rate lasers with very high peak powers. Here, we establish a novel route toward powerful and easy-to-use SXR sources by presenting a compact experiment, in which nonlinear pulse self-compression to the few-cycle regime is combined with phase-matched HHG in a single, heliu…
Preparation of an atomic ensemble in a particular Zeeman state is a critical step of many protocols for implementing quantum sensors and quantum memories. These devices can also benefit from optical fibre integration. In this work we describe experimental results supported by a theoretical model of single-beam optical pumping of $^{87}$Rb atoms within a hollow-core photonic crystal fibre. The observed 50% population increase in the pumped F=2, m$_F$=2 Zeeman substate along with the depopulation of remaining Zeeman substates enabled us to achieve a 3 times improvement in the relative population…
We use hollow-core fibre to preserve the spectrum and temporal profile of picosecond laser pulses in CBD to suppress 2.6 dB of amplitude noise at MHz noise frequencies, to within 0.01 dB of the shot-noise limit. We provide an enhanced version of the CBD scheme that concatenates circuits to suppress over multiple frequencies and over broad frequency ranges --- we perform a first demonstration that reduces total excess amplitude noise, between 2 - 6 MHz, by 85%. These demonstrations enable passive, broad-band, all-guided fibre laser technology operating at the shot-noise limit.
In hydrodynamics, vortex generation upon the transition from smooth laminar flows to turbulence is generally accompanied by increased dissipation. However, plane vortices can provide transport barriers and decrease losses, as it happens in numerous geophysical, astrophysical flows and in tokamaks. Photon interactions with matter can affectlight transportin waveguides in unexpected and somewhat counterintuitive ways resembling fluid dynamics. Here, we demonstrate dramatic impact of light vortex formation in micro-structured optical fibres on the energy dissipation. We show possibility of vortic…
We demonstrate, for the first time, the application of rare-gas filled hollow-core photonic crystal fibres (HC-PCFs) as tuneable ultraviolet light sources in femtosecond pump-probe spectroscopy. The time-resolved photoelectron imaging technique reveals non-adiabatic dynamical processes operating on three distinct timescales in the styrene molecule following excitation over the 242-258 nm region. These include ultrafast (<100 fs) internal conversion between the S2(pipi*) and S1(pipi*) electronic states and subsequent intramolecular vibrational energy redistribution within S1(pipi*). Compact, co…
The generation of large multiphoton quantum states - for applications in computing, metrology, and simulation - requires a network of high-efficiency quantum memories capable of storing broadband pulses. Integrating these memories into a fibre offers a number of advantages towards realising this goal: strong light-matter coupling at low powers, simplified alignment, and compatibility with existing photonic architectures. Here, we introduce a large-core kagome-structured hollow-core fibre as a suitable platform for an integrated fibre-based quantum memory with a warm atomic vapour. We demonstra…
Stimulated Brillouin scattering (SBS) offers among the highest nonlinear gains in solid materials and has demonstrated advanced photonics functionalities in waveguides. The large compressibility of gases suggests that SBS may gain in efficiency with respect to condensed materials. Here, by using a gas-filled hollow-core fibre at high pressure, we achieve a strong Brillouin amplification per unit length, exceeding by 6 times the gain observed in fibres with a solid silica core. This large amplification benefits from a higher molecular density and a lower acoustic attenuation at higher pressure,…
We numerically investigate the energy and arrival-time noise of ultrashort laser pulses produced via resonant dispersive wave emission in gas-filled hollow-core waveguides under the influence of pump-laser instability. We find that for low pump energy, fluctuations in the pump energy are strongly amplified. However, when the generation process is saturated, the energy of the resonant dispersive wave can be significantly less noisy than that of the pump pulse. This holds for a variety of generation conditions and while still producing few-femtosecond pulses. We further find that the arrival-tim…
The performances of optical fibre-based quantum information systems are limited by the intrinsic properties of silica glass materials, e.g. high latency, Rayleigh-scattering loss wavelength scaling law, and cross-coupling induced modal impurity. Hollow-core optical fibre (HCF) promises to unify air-borne light propagation and non-line-of-sight transmission, thus holding great potentials for versatile photonics-based quantum infor-mation applications. The early version of HCF based on photonic-bandgap guidance has not proven itself as a reliable quantum channel because of the poor modal purity …
Alkali-filled hollow-core fibres are a promising medium for investigating light-matter interactions, especially at the single-photon level, due to the tight confinement of light and high optical depths achievable by light-induced atomic desorption. However, until now these large optical depths could only be generated for seconds at most once per day, severely limiting the practicality of the technology. Here we report the generation of highest observed transient ($>10^5$ for up to a minute) and highest observed persistent ($>2000$ for hours) optical depths of alkali vapours in a light-guiding …
We propose and theoretically analyse a novel hollow-core photonic crystal fibre (PCF) that is engineered so as to strongly suppress higher order modes, i.e., to provide robust LP$_{01}$ single-mode guidance in all the wavelength ranges where the fibre guides with low loss. Encircling the core is a single ring of non-touching glass elements whose modes are tailored to ensure resonant phase-matched coupling to higher-order core modes, causing them to leak at a very high rate into the supporting solid glass sheath. Using a model based on coupled capillary waveguides, as well as full vectorial fin…
Efficient monitoring of airborne particulate matter (PM), especially particles with aerodynamic diameter less than 2.5 um (PM2.5), is crucial for improving public health. Reliable information on the concentration, size distribution and chemical characteristics of PMs is key to evaluating air pollution and identifying its sources. Standard methods for PM2.5 characterization require sample collection from the atmosphere and post-analysis using sophisticated equipment in a laboratory environment, and are normally very time-consuming. Although optical methods based on analysis of scattering of fre…
Whispering-gallery mode (WGM) resonators combine small optical mode volumes with narrow resonance linewidths, making them exciting platforms for a variety of applications. Here we report a flying WGM microlaser, realized by optically trapping a dye-doped microparticle within a liquid-filled hollow-core photonic crystal fiber (HC-PCF) using a CW laser and then pumping it with a pulsed excitation laser whose wavelength matches the absorption band of the dye. The laser emits into core-guided modes that can be detected at the endfaces of the HC-PCF. Using radiation forces, the microlaser can be fr…
We report on a highly-efficient experimental scheme for the generation of deep-ultraviolet ultrashort light pulses using four-wave mixing in gas-filled kagomé-style photonic crystal fiber. By pumping with ultrashort, few $μ$J, pulses centered at 400 nm, we generate an idler pulse at 266 nm, and amplify a seeded signal at 800 nm. We achieve remarkably high pump-to-idler energy conversion efficiencies of up to 38%. Although the pump and seed pulse durations are ~100 fs, the generated ultraviolet spectral bandwidths support sub-15 fs pulses. These can be further extended to support few-cycle puls…
Optical manipulation in the vicinity of optical micro- and nanofibres has shown potential across several fields in recent years, including microparticle control, and cold atom probing and trapping. To date, most work has focussed on propagation of the fundamental mode through the fibre. However, along the maximum mode intensity axis, higher order modes have a longer evanescent field extension and larger field amplitude at the fibre waist compared to the fundamental mode, opening up new possibilities for optical manipulation and particle trapping. In this work, we demonstrate a microfibre/optic…
The FAMU (Fisica degli Atomi Muonici) experiment at the RIKEN RAL pulsed muon facility will measure the proton Zemach radius with high precision, thus contributing to the solution of the so-called proton radius puzzle. The situation is now confused and new measurements will help reduce the discrepancy as measured with electrons or muons. To this aim, FAMU will make use of a high-intensity pulsed muon beam at RIKEN-RAL impinging on a cryogenic hydrogen target and a tunable Mid-infrared (MIR) laser emitting at around 6.78 um, to measure the hyperfine (HFS) splitting of the 1S state of muonic hyd…
In this Letter, we show theoretically that the nonlinear photoionisation process of a noble gas inside a hollow-core photonic crystal fibre can be exploited in obtaining broadband supercontinuum generation via pumping close to the mid-infrared regime. The interplay between the Kerr and photoionisation nonlinearities is strongly enhanced in this regime. Photoionisation continuously modifies the medium dispersion, in which the refractive index starts to significantly decrease and approach the epsilon-near-zero regime. Subsequently, the self-phase modulation induced by the Kerr effect is boosted …
