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arXiv 2005.05233cond-mat.mtrl-sci
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同步辐射ARPES研究Sr $_{4}$ Ru PDMATHAAB O $_{10}$的费米面和扭结结构

Fermi surface and kink structures in Sr$_{4}$Ru$_{3}$O$_{10}$ revealed by synchrotron-based ARPES

Prosper Ngabonziza, Emanuela Carleschi, Volodymyr Zabolotnyy, Amina Taleb-Ibrahimi, François Bertran, Rosalba Fittipaldi, Veronica Granata, Mario Cuoco, Antonio… 展开作者

Prosper Ngabonziza, Emanuela Carleschi, Volodymyr Zabolotnyy, Amina Taleb-Ibrahimi, François Bertran, Rosalba Fittipaldi, Veronica Granata, Mario Cuoco, Antonio Vecchione, Bryan Patrick Doyle

摘要:

利用同步辐射角分辨光电子能谱首次研究了巡游超磁体Sr $_{4}$ Ru $_{3}$ O $_{10}$的低能电子结构,包括费米面拓扑.定义良好的准粒子带色散与矩阵元素依赖于光子能量或光子偏振。解决了四个带穿过费米能级,产生四个费米面片,并确定其完整的地形,有效质量以及它们的电子和空穴的性质。这些数据揭示了在近费米能级带色散的扭结结构的存在下,与能量范围从30毫电子伏到69毫电子伏。与以前报道的拉曼光谱和晶格动力学计算的研究,数据表明,这些扭结起源于强的电子-声子耦合存在于Sr $_{4}$ Ru $_{3}$ O $_{10}$。考虑到Sr $_{4}$ Ru $_{3}$ O $_{10}$的扭结结构与Ruddlesden Popper结构双烯酸盐的其他三个成员的扭结结构相似,提出了Sr $_{n+1}$ Ru $_{n}$ O $_{3n+1}$化合物中电子与氧相关声子强耦合的可能普遍性.

英文摘要:

The low-energy electronic structure, including the Fermi surface topology, of the itinerant metamagnet Sr$_{4}$Ru$_{3}$O$_{10}$ is investigated for the first time by synchrotron-based angle-resolved photoemission. Well-defined quasiparticle band dispersions with matrix element dependencies on photon energy or photon polarization are presented. Four bands crossing the Fermi-level, giving rise to four Fermi surface sheets are resolved; and their complete topography, effective mass as well as their electron and hole character are determined. These data reveal the presence of kink structures in the near-Fermi-level band dispersion, with energies ranging from 30 meV to 69 meV. Together with previously reported Raman spectroscopy and lattice dynamic calculation studies, the data suggest that these kinks originate from strong electron-phonon coupling present in Sr$_{4}$Ru$_{3}$O$_{10}$. Considering that the kink structures of Sr$_{4}$Ru$_{3}$O$_{10}$ are similar to those of the other three members of the Ruddlesden Popper structured ruthenates, the possible universality of strong coupling of electrons to oxygen-related phonons in Sr$_{n+1}$Ru$_{n}$O$_{3n+1}$ compounds is proposed.

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