arXivDaily arXiv每日学术速递 周一至周五更新
arXiv 2003.11905cond-mat.mtrl-sci
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层状MoOCl2的费米液体行为和庞磁电阻

Fermi liquid behavior and colossal magnetoresistance in layered MoOCl2

Zhi Wang, Meng Huang, Jianzhou Zhao, Cong Chen, Haoliang Huang, Xiangqi Wang, Ping Liu, Jianlin Wang, Junxiang Xiang, Chao Feng, Zengming Zhang, Xudong Cui, Yal… 展开作者

Zhi Wang, Meng Huang, Jianzhou Zhao, Cong Chen, Haoliang Huang, Xiangqi Wang, Ping Liu, Jianlin Wang, Junxiang Xiang, Chao Feng, Zengming Zhang, Xudong Cui, Yalin Lu, Shengyuan A. Yang, Bin Xiang

摘要:

费米液体的一个特性是其电阻率与T^2的关系,有时也被称为巴伯定律。然而,对于大多数金属,这种行为仅限于非常低的温度,通常低于20 K。在这里,我们的实验表明,对于单晶范德瓦尔斯层状材料MoOCl 2,在很宽的温度范围内,高达~120 K的巴贝尔定律成立,这表明电子-电子散射在这种材料中起着主导作用。结合比热测量结果,我们发现该材料的修正Kadowaki-Woods比与许多其他强关联金属相一致。此外,在磁输运测量中,观察到庞磁阻,其在9 T下达到~350%,并且没有显示饱和的迹象。借助第一性原理计算,我们将这种行为归因于费米面上的开轨道。我们还建议,电子-电子散射的主导地位有关的初始电荷密度波状态的材料。我们的研究结果确立了MoOCl 2作为一种强关联金属,并揭示了潜在的物理机制,这可能为探索范德华层状结构中电子-电子相互作用的影响开辟了一条新的途径。

英文摘要:

A characteristic of a Fermi liquid is the T^2 dependence of its resistivity, sometimes referred to as the Baber law. However, for most metals, this behavior is only restricted to very low temperatures, usually below 20 K. Here, we experimentally demonstrate that for the single-crystal van der Waals layered material MoOCl2, the Baber law holds in a wide temperature range up to ~120 K, indicating that the electron-electron scattering plays a dominant role in this material. Combining with the specific heat measurement, we find that the modified Kadowaki-Woods ratio of the material agrees well with many other strongly correlated metals. Furthermore, in the magneto-transport measurement, a colossal magneto-resistance is observed, which reaches ~350% at 9 T and displays no sign of saturation. With the help of first-principles calculations, we attribute this behavior to the presence of open orbits on the Fermi surface. We also suggest that the dominance of electron-electron scattering is related to an incipient charge density wave state of the material. Our results establish MoOCl2 as a strongly correlated metal and shed light on the underlying physical mechanism, which may open a new path for exploring the effects of electron-electron interaction in van der Waals layered structures.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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