For two decades now, the importance of microstructure in the mechanical behaviour of a large collection of grains has been a topic of intense research. Many approaches have been developed to study the microstructure in granular materials, based on local or mesoscopic measures or using ideas from diverse fields like percolation theory, complex networks and persistent homology. However, we do not fully understand the role of microstructure in the mechanical behaviour of simple and commonplace packings like a pile of sand or box of grains. Here, by characterizing the spatial variation of local microstructure, we uncover intriguing large-scale spatial patterns in particle packings deposited under the influence of gravity. We detail the emergence of these patterns, and provide a unified fundamental explanation of classic and puzzling mechanical behaviours of granular materials like central stress minimum and Janssen effect. Further, we show the striking dependence of spatial structure on the history of preparation, size distribution of particles and boundary conditions. Our study reveals the existence of global spatial structure in a locally disordered media, and elucidates its significance in the mechanical behaviour of granular materials.
The confining pressure $P$ is perhaps the most important parameter controlling the properties of granular matter. Strongly compressed granular media are, in many respects, simple solids in which elastic perturbations travel as ordinary phonons. However, the speed of sound in granular aggregates continuously decreases as the confining pressure decreases, completely vanishing at the jamming-unjamming transition. This anomalous behavior suggests that the transport of energy at low pressures should not be dominated by phonons. In this work we use simulations and theory to show how the response of …
Recent diffraction experiments on metallic glasses have unveiled an unexpected non-cubic scaling law between density and average interatomic distance, which lead to the speculations on the presence of fractal glass order. Using X-ray tomography we identify here a similar non-cubic scaling law in disordered granular packing of spherical particles. We find that the scaling law is directly related to the contact neighbors within first nearest neighbor shell, and therefore is closely connected to the phenomenon of jamming. The seemingly universal scaling exponent around 2.5 arises due to the isost…
Stress in dense granular materials and other athermal particle aggregates is transmitted through a visually striking subnetwork of interparticle contacts, the filamentary segments of which are referred to as force chains. The emergence of such preferred subnetwork in structurally disordered media with constituents interacting primarily by physical contact is not fully understood. In this work, we study locally correlated transport in Random Geometric Graphs (RGGs), and show the spontaneous emergence of preferred subnetwork. Our findings reveal that, despite structural disorder, system spanning…
Dense granular materials and other particle aggregates transmit stress in a manner that belies their microstructural disorder. A subset of the particle contact network is strikingly coherent, wherein contacts are aligned nearly linearly and transmit large forces. Important material properties are associated with these force chains, but their origin has remained a puzzle. We classify subnetworks by their linear connectivity, and show the emergence of a percolation transition at a critical linearity at which the network is sparse, coherent, and contains the force chains. The subnetwork at critic…
We have found a way to analyze Edwards' density of states for static granular packings in the special case of round, rigid, frictionless grains assuming constant coordination number. It obtains the most entropic density of single grain states, which predicts several observables including the distribution of contact forces. We compare these results against empirical data obtained in dynamic simulations of granular packings. The agreement is quite good, helping validate the use of statistical mechanics methods in granular physics. The differences between theory and empirics are mainly related to…
We report a transition from a disordered state to an ordered state in the flow of nearly mono-disperse granular matter flowing in an inclined channel with a bumpy base, in discrete element method simulations. For low particle-sidewall friction coefficients, the particles are disordered and the Bagnold velocity profile is obtained. However, for high sidewall friction, an ordered state is obtained, characterized by a layering of the particles and hexagonal packing of the particles in each layer. The extent of ordering, quantified by the local bond-orientational order parameter, varies in the cro…
The transmission of forces through a disordered granular system is studied by means of a geometrical-topological approach that reduces the granular packing into a set of layers. This layered structure constitutes the skeleton through which the force chains set up. Given the granular packing, and the region where the force is applied, such a skeleton is uniquely defined. Within this framework, we write an equation for the transmission of the vertical forces that can be solved recursively layer by layer. We find that a special class of analytical solutions for this equation are Lévi-stable distr…
We measure experimentally the rearrangements due to a small localized cyclic displacement applied to a packing of rigid grains under gravity in a 2D geometry. We analyze the evolution of the response to this perturbation by considering the individual particle displacement and the coarse grained displacement field, as well as the mean packing fraction and coordination number. We find that the displacement response is rather long ranged, and evolves considerably with the number of cycles. We show that a small difference in the preparation method (induced by tapping the container) leads to a sign…
Despite extensive theoretical \cite{GanterPRL1998, ElliotPRL2001,SchirmacherPRL2007, TanakaNatureM2008, MonacoPNAS2009, MarruzzoSCIRP2013} and experimental studies \cite{ChumakovPRL2011, ChumakovPRL2014, KayaScience2010,KChenPRL2010, LXuPRL2012, BonnPreprint2014}, a longstanding puzzle in condensed matter physics remains regarding the origin and nature of "Boson peak" (BP), where the vibrational density of states (DOS) in glasses possesses an excess of states compared with the crystalline counterpart. Here we show that BP is successfully observed in 2D hexagonal granular packing, where the dis…
Contrary to the theoretical predictions that all waves in two-dimensional disordered materials are localized, Anderson localization is observed only for sufficiently high frequencies in an isotropically jammed two-dimensional disordered granular packing of photoelastic disks. More specifically, we have performed an experiment in analyzing the level statistics of normal mode vibrations. We observe delocalized modes in the low-frequency boson-peak regime and localized modes in the high frequency regime with the crossover frequency just below the Debye frequency. We find that the level-distance d…
In a granular solid, mechanical equilibrium requires a delicate balance of forces at the disordered grain scale. To understand how macroscopic rigidity can emerge in this amorphous solid, it is crucial that we understand how Newton's laws pass from the disordered grain scale to the laboratory scale. In this work, we introduce an exact discrete calculus, in which Newton's laws appear as differential relations at the scale of a single grain. Using this calculus, we introduce gauge variables which describe identically force- and torque-balanced configurations. In a first, intrinsic formulation, w…
We employ numerical simulations to understand the evolution of elastic standing waves in disordered frictional disk systems, where the dispersion relations of rotational sound modes are analyzed in detail. As in the case of frictional particles on a lattice, the rotational modes exhibit an "optical-like" dispersion relation in the high frequency regime, representing a shoulder of the vibrational density of states and fast oscillations of the autocorrelations of rotational velocities. A lattice-based model describes the dispersion relations of the rotational modes for small wave numbers. The ro…
Upon mechanical loading, granular materials yield and undergo plastic deformation. The nature of plastic deformation is essential for the development of the macroscopic constitutive models and the understanding of shear band formation. However, we still do not fully understand the microscopic nature of plastic deformation in disordered granular materials. Here we used synchrotron X-ray tomography technique to track the structural evolutions of three-dimensional granular materials under shear. We establish that highly distorted coplanar tetrahedra are the structural defects responsible for micr…
We describe an experimental and computational investigation of the ordered and disordered phases of a vibrating thin, dense granular layer composed of identical metal spheres. We compare the results from spheres with different amounts of inelasticity and show that inelasticity has a strong effect on the phase diagram. We also report the melting of an ordered phase to a homogeneous disordered liquid phase at high vibration amplitude or at large inelasticities. Our results show that dissipation has a strong effect on ordering and that in this system ordered phases are absent entirely in highly i…
We study the order-disorder transition of horizontally swirled dry and wet granular disks by means of computer simulations. Our systematic investigation of the local order formation as a function of amplitude and period of the external driving force shows that a large cluster of hexagonally ordered particles forms for both dry and wet granular particles at intermediate driving energies. Disordered states are found at small and large driving energies. Wet granular particles reach a higher degree of local hexagonal order, with respect to the dry case. For both cases we report a qualitative phase…
An understanding of homogeneous nucleation of crystalline structure from a disordered medium such as a liquid remains an important unsolved problem in condensed matter physics. Guided by the results from a number of experiments on granular and colloidal systems in the past two decades, including in particular observations of homogeneous nucleation in colloidal and granular systems, we suggest an alternative to the statistical mechanics approach to static granular matter initiated by Edwards and Oakeshott in 1989.
The mechanical properties of a disordered heterogeneous medium depend, in general, on a complex interplay between multiple length scales. Connecting local interactions to macroscopic observables, such as stiffness or fracture, is thus challenging in this type of material. Here, we study the properties of a cohesive granular material composed of glass beads held together by soft polymer bridges. We characterise the mechanical response of single bridges under traction and shear, using a setup based on the deflection of flexible micropipettes. These measurements, along with information from X-ray…
The frictional properties of disordered systems are affected by external perturbations. These perturbations usually weaken the system by reducing the macroscopic friction coefficient. This friction reduction is of particular interest in the case of disordered systems composed of granular particles confined between two plates, as this is a simple model of seismic fault. Indeed, in the geophysical context frictional weakening could explain the unexpected weakness of some faults, as well as earthquake remote triggering. In this manuscript we review recent results concerning the response of confin…
Stress transmission in planar open-cell cellular solids is analysed using a recent theory developed for marginally rigid granular assemblies. This is made possible by constructing a one-to-one mapping between the two systems. General trivalent networks are mapped onto assemblies of rough grains, while networks where Plateau rules are observed, are mapped onto assemblies of smooth grains. The constitutive part of the stress transmission equations couples the stress directly to the local rotational disorder of the cellular structure via a new fabric tensor. An intriguing consequence of the analy…
We propose an explanation for the onset of oscillations seen in numerical simulations of dense, inclined flows of inelastic, frictional spheres. It is based on a phase transition between disordered and ordered collisional states that may be interrupted by the formation of force chains. Low frequency oscillations between ordered and disordered states take place over weakly bumpy bases; higher-frequency oscillations over strongly bumpy bases involve the formation of particle chains that extend to the base and interrupt the phase change. The predicted frequency and amplitude of the oscillations i…
We investigate the mechanical properties of a static dense granular assembly in response to a local forcing. To this end, a small cyclic displacement is applied on a grain in the bulk of a 2D disordered packing under gravity and the displacement fields are monitored. We evidence a dominant long range radial response in the upper half part above the sollicitation and after a large number of cycles the response is `quasi-reversible' with a remanent dissipation field exhibiting long range streams and vortex-like symmetry.
A two-dimensional system of photoelastic disks subject to vertical tapping against gravity was experimentally monitored from ordered to disordered configurations by varying bidispersity. The packing fraction $ϕ$, coordination number $Z$, and an appropriately defined force chain orientational order parameter $S$, all exhibit similar sharp transition with small increase in disorder. A measurable change in $S$, but not $ϕ~\&~Z$, was detected under tapping. We find disorder-induced metastability does not show configurational relaxation, but can be detected via force chain reorientations.
We study experimentally the fracture mechanisms of a model cohesive granular medium consisting of glass beads held together by solidified polymer bridges. The elastic response of this material can be controlled by changing the cross-linking of the polymer phase, for example. Here we show that its fracture toughness can be tuned over an order of magnitude by adjusting the stiffness and size of the polymer bridges. We extract a well-defined fracture energy from fracture testing under a range of material preparations. This energy is found to scale linearly with the cross-sectional area of the bri…
We investigate the spatial structure of cohesive granular matter with spheres floating at an air-liquid interface that form disordered close packings with pores in between. The interface is slowly lowered in a conical container to uniformly compress and study the system as a function of area fraction $ϕ$. We find that the free area distributions associated with Voronoi cells show significant exponential tails indicating greater heterogeneity compared with random distributions at low $ϕ$ with a crossover towards a $Γ$-distribution as $ϕ$ is increased. Further, we find significant short range or…
The series of equilibrium states reached by disordered packings of rigid, frictionless discs in two dimensions, under gradually varying stress, are studied by numerical simulations. Statistical properties of trajectories in configuration space are found to be independent of specific assumptions ruling granular dynamics, and determined by geometry only. A monotonic increase in some macroscopic loading parameter causes a discrete sequence of rearrangements. For a biaxial compression, we show that, due to the statistical importance of such events of large magnitudes, the dependence of the resulti…
In glasses and other disordered materials, measurements of the vibrational density of states reveal that an excess number of long-wavelength (low-frequency) modes, as compared to the Debye scaling seen in crystalline materials, is associated with a loss of mechanical rigidity. In this paper, we present a novel technique for measuring the density of modes (DOM) in a real granular material, in which we mimic thermal excitations using white noise acoustic waves. The resulting vibrations are detected with piezoelectric sensors embedded inside a subset of the particles, from which we are able to co…
The topological structure resulting from the network of contacts between grains (contact network) is studied for very large samples of disorderly-packed monosized spheres with densities ranging from 0.58 to 0.64. The hierarchical organization of such a structure is studied by means of a topological map which starts from a given sphere and moves outwards in concentric shells through the contact network. We find that the topological density of disordered sphere packing is larger than the topological density of equivalent lattice sphere packings.
The fluid flow through porous media is described by Darcy's law, while the fluid/wall interactions can be neglected. In nanopores, where adsorption dominates, Darcy's extension has been made, but approaches able to describe flows in mesopores are still lacking. We show here that molecular flows through nano-constrictions is well described by Berverloo's law, predicting the mass flow rate of granular material through macro-apertures. This molecular and granular analogy, allows to derive a relationship providing a theoretical framework for the molecular flow in disordered mesoporous systems.
We use machine learning methods on local structure to identify flow defects - or regions susceptible to rearrangement - in jammed and glassy systems. We apply this method successfully to two disparate systems: a two dimensional experimental realization of a granular pillar under compression, and a Lennard-Jones glass in both two and three dimensions above and below its glass transition temperature. We also identify characteristics of flow defects that differentiate them from the rest of the sample. Our results show it is possible to discern subtle structural features responsible for heterogene…
While memory effects have been reported for dense enough disordered systems such as glasses, we show here by a combination of analytical and simulation techniques that they are also intrinsic to the dynamics of dilute granular gases. By means of a certain driving protocol, we prepare the gas in a state where the granular temperature $T$ coincides with its long time limit. However, $T$ does not subsequently remain constant, but exhibits a non-monotonic evolution before reaching its non-equilibrium steady value. The corresponding so-called Kovacs hump displays a normal behavior for weak dissipat…
We use an analogy with the statistical mechanics of gas to build the statistical mechanics of granular media. The case of an isotropic disordered packing of equal spheres submitted to an isotropic stress is considered. We use the assumption of a maximal disorder and the method of the Lagrange multipliers to demonstrate that the distribution of the force moduli decreases exponentially and obeys an exponential-decay statistics. This distribution results from the above hypotheses and from the existence of a mean stress, which acts as a constraint. This distribution is confirmed by experiments and…
Our understanding of the elasticity and rheology of disordered materials, such as granular piles, foams, emulsions or dense suspensions relies on improving experimental tools to characterize their behaviour at the particle scale. While 2D observations are now routinely carried out in laboratories, 3D measurements remain a challenge. In this paper, we use a simple model system, a packing of soft elastic spheres, to illustrate the capability of X-ray microtomography to characterise the internal structure and local behaviour of granular systems. Image analysis techniques can resolve grain positio…
Granular materials such as sand, powders, foams etc. are ubiquitous in our daily life, as well as in industrial and geotechnical applications. Although these disordered systems form stable structures if unperturbed, in practice they do relax because of the presence of unavoidable external influences such as tapping or shear. Often it is tacitly assumed that for granular systems this relaxation dynamics is similar to the one of thermal glass-formers, but in fact experimental difficulties have so far prevented to determine the dynamic properties of three dimensional granular systems on the parti…
Time reversal (TR) focusing of ultrasound in granular packings is experimentally investigated. Pulsed elastic waves transmitted from a compressional or shear transducer source are measured by a TR mirror, reversed in time and back-propagated. We find that TR of ballistic coherent waves onto the source position is very robust regardless driving amplitude but provides poor spatial resolution. By contrast, the multiply scattered coda waves offer a finer TR focusing at small amplitude by a lens effect. However, at large amplitude, these TR focusing signals decrease significantly due to the vibrati…
If you walk on sand, it supports your weight. How do the disordered forces between particles in sand organize, to keep you from sinking? This simple question is surprisingly difficult to answer experimentally: measuring forces in three dimensions, between deeply buried grains, is challenging. We describe here experiments in which we have succeeded in measuring forces inside a granular packing subject to controlled deformations. We connect the measured micro-scale forces to the macro-scale packing force response with an averaging, mean field calculation. This calculation explains how the combin…
We report on experiments to measure the temporal and spatial evolution of packing arrangements of anisotropic, cylindrical granular material, using high-resolution capacitive monitoring. In these experiments, the particle configurations start from an initially disordered, low-packing-fraction state and under vertical vibrations evolve to a dense, highly ordered, nematic state in which the long particle axes align with the vertical tube walls. We find that the orientational ordering process is reflected in a characteristic, steep rise in the local packing fraction. At any given height inside th…
The stress profile and reorientation of grains, in response to a point force applied to a preloaded two dimensional granular system, are calculated in the context of a continuum theory that incorporates the texture of the packing. When high friction prevents slip at the inter-grain contacts, an anisotropic packing propagates stress along two peaks which amalgamate into a single peak as the packing is disordered into a less anisotropic structure; this single peak may be wider or narrower than in the isotropic case, depending on the preparation of the packing. At lower frictions, an effective tr…
Discrete element method is conducted to investigate the bidisperse dense granular flow having big and small grains in a two dimensional hopper. A half-circular dynamical force arch is observed above the outlet and Beverloo's law is verified to describe the relationship between flow rate and outlet size. The bidisperse flow can reach the maximum flow rate when a small fraction of big grains is added into the monodisperse flow with only small grains. The distributions of contact force, packing fraction and grain velocity indicate that the flow properties in the hopper are closely related to the …
Force networks form the skeleton of static granular matter. They are the key ingredient to mechanical properties, such as stability, elasticity and sound transmission, which are of utmost importance for civil engineering and industrial processing. Previous studies have focused on the global structure of external forces (the boundary condition), and on the probability distribution of individual contact forces. The disordered spatial structure of the force network, however, has remained elusive so far. Here we report evidence for scale invariance of clusters of particles that interact via relati…
Forecasting fracture locations in a progressively failing disordered structure is of paramount importance when considering structural materials. We explore this issue for gradual deterioration via beam breakage of two-dimensional disordered lattices, which we represent as networks, for various values of mean degree. We study experimental samples with geometric structures that we construct based on observed contact networks in 2D granular media. We calculate geodesic edge betweenness centrality, which helps quantify which edges are on many shortest paths in a network, to forecast the failure lo…
We numerically study the distribution P(f) of contact forces in frictionless bead packs, by averaging over the ensemble of all possible force network configurations. We resort to umbrella sampling to resolve the asymptotic decay of P(f) for large f, and determine P(f) down to values of order 10^{-45} for ordered and disordered systems in two and three dimensions. Our findings unambiguously show that, in the ensemble approach, the force distributions decay much faster than exponentially: P(f) ~ exp(-f^α), with alpha \approx 2.0 for 2D systems, and alpha \approx 1.7 for 3D systems.
We probe the effects of particle shape on the global and local behavior of a two-dimensional granular pillar, acting as a proxy for a disordered solid, under uniaxial compression. This geometry allows for direct measurement of global material response, as well as tracking of all individual particle trajectories. In general, drawing connections between local structure and local dynamics can be challenging in amorphous materials due to lower precision of atomic positions, so this study aims to elucidate such connections. We vary local interactions by using three different particle shapes: discre…
Rigid particles pack into structures, such as sand dunes on the beach, whose overall stability is determined by the average number of contacts between particles. However, when packing spatially extended objects with flexible shapes, additional concepts must be invoked to understand the stability of the resulting structure. Here we study the disordered packing of chains constructed out of flexibly-connected hard spheres. Using X-ray tomography, we find long chains pack into a low-density structure whose mechanical rigidity is mainly provided by the backbone. On compaction, randomly-oriented, se…
